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Bose-Einstein-Condensate Interferometer with Macroscopic Arm Separation Ofir Garcia-Salazar San José, Costa Rica B.S., Eckerd College, 2000 M.A., University of Virginia, 2004 A Dissertation presented to the Graduate Faculty of the University of Virginia in Candidacy for the Degree of Doctor of Philosophy Department of Physics University of Virginia January, 2007 Abstract The basis of our study was to implement an atom interferometer using 87 Rb Bose Einstein condensates which has advantages in sensitivity over current interferometers that use cold atoms and light. Interferometers are devices which can accurately measure phase differences between waves that interfere and originate from a coherent source (or sources). We developed a weakly confining waveguide having ωx ≈ 3 Hz, ωz ≈ 3 Hz, ωy ≈ 1 Hz as characteristic oscillation frequencies. Weak confinement, specially along the “y” direction, means the condensate can displace along this axis and interaction energies of the atoms in the condensate are reduced [1]. We have been able to successfully demonstrate condensate interference in our waveguide using a Mach Zehnder configuration. Coherence times of up to 40 ms have been observed, and the maximum center to center separation of the condensates recorded was of 240 µm. At this separation length, the two clouds corresponding to each of the interferometer’s arms are completely separated. To our knowledge, this is the first time a picture has been taken of two groups of atoms separated by a macroscopic distance while in a quantum superposition of being in either cloud. The coherence time and length measurements presented in our work have been among the longest ones achieved so far for interferometry using condensed atoms. Interference visibility of 60% was observed up to 40 ms. We believe technical limitations in the techniques used to manipulate the atoms are responsible for the sudden drop in visibility at 44 ms. For example, unwanted laser reflections and interference patterns in our chamber affect the tecniques used to split and reflect the atoms. However, we see coherence up to 80 ms from shot to shot, suggesting we could dramatically improve coherence times. Becasue of the weak confinement of our trap, we expect to improve coherence times up to an order of magnitude before running into phase diffusion effects [2]. It is our hope to use our condensate interferometer for future studies in calculating the electric polarizability of 87 Rb. The macroscopic time and length scale presented are novel in experimental quantum mechanics and of valuable pedagogical insight. ii Acknowledgments I would like to make an important note of appreciation to all of those who joined me during these seven years in grad school. In reality many people have been involved in my life as a student so far. They have, in my opinion, influenced who I am, and continue to influence me in many ways. The list is very extensive and it would not be possible to mention every one here, however, I salute and thank all of you (you know who you are). I would like to start by expressing my infinite gratitude to my amazing wife! Karina, I feel you truly deserve much of the credit for the achievements presented in this work. Thank you for all the tenderness, love, and hard work. They have provided all the support to fulfill this mission. All my love goes out to you. My parents, Andres Garcia and Gloria Salazar, there are almost no words to express how much your influence and guidance have helped me through life. Thank you for always listening to me under every circumstances and giving me the confidence that I can indefinitely trust you. To my sister Varinia, having you so close during my graduate studies has been incredible! You have provided me that sense of family, just like when we were little ones. Thank you for giving me the notion of remembering where I came from and of the immense value of our immediate family. You are a huge example to me and I am very proud of you. Cass Sackett, you have been the best academic mentor and life adviser. It is my impression that I could have not possibly made a better choice in order to carry out my graduate studies. I wanted to express to you how meaningful your patience and efforts towards teaching me physics has been. My aspiration is that I will be able to pass on that knowledge to many more. Thank you for giving me the motivation and inspiration to understand things the best I can. Also, thank you for always giving me confidence in my abilities. To my lab colleagues (Ben, Jeramy, Jessica, Ken, Au, John), all of you have been great peers and a true joy to work with. I thank you all for putting up with my unusual personality. Given that, I do feel all of you got to know me, appreciated and understood me for who I am! Ben Deissler, I felt impelled to write out your full name! Thank you for answering all my questions and always considering my point of view. As many of you know, In addition to all the experimental work, I have endured some of the most difficult emotional and psychological times of my life while in iii iv grad school. I would like to thank Jessica Reeves for helping me identify the root cause of my problem (Obsessive Compulsive Disorder). This can be a very crippling condition, but thanks to the incredible support network mentioned above, I have been able to successfully manage it. Bethany Teachman, thank you for giving me the tools to overcome this condition and allowing me to re-learn how to ignore thoughts that are not important. I truly hope your efforts in figuring out techniques in order to help people suffering from OCD continue to flourish. I would like to thank my professors Harry Ellis, Anne Cox, Stephen Weppner and Jerry Junevichus at my undergraduate institution Eckerd College, for giving me the foundations to pursue this work. Thank you for preparing very well to attend graduate school. All my life friends like Kifah Sasa, Carlos Luis Salas, Guillermo Gomez, John Akl, Amadeo Martinez and many more, thank you for being there constantly even after many many years of unconditional friendship. Finally, I would like to end my acknowledgements by expressing my deepest hopes that the work presented here will have a positive effect on humanity. I have faith that the more we understand this remarkably complicated universe, the better we can understand each other and learn how appreciate life for what it is. Contents Abstract ii Acknowledgments iii 1 Introduction 1.1 The Nature of BEC . . . . . . 1.2 Interference . . . . . . . . . . 1.3 What is an Interferometer . . 1.4 Coherence . . . . . . . . . . . 1.5 BEC, a Coherent Matter-wave 1.6 Outline of Thesis . . . . . . . 1.7 Experimental conventions . . . . . . . . . 1 3 7 9 11 15 17 18 . . . . . . . . . . . . . . 21 21 22 25 36 36 37 38 39 39 40 43 48 53 55 3 Magnetic Waveguide 3.1 Loading a Wave Guide . . . . . . . . . . . . . . . . . . . . . . . . . . 3.2 Magnetic Trap . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 3.2.1 Conventions and Set Up . . . . . . . . . . . . . . . . . . . . . 59 60 60 60 . . . . . . . . . . . . . . . . Source . . . . . . . . . . . . . . . . . . . . . . 2 Making BEC 2.1 Rubidium Atoms . . . . . . . . . . . . . 2.1.1 External magnetic fields . . . . . 2.2 Creating a MOT . . . . . . . . . . . . . 2.2.1 Supplying 87 Rb . . . . . . . . . . 2.3 Increasing the number density . . . . . . 2.4 Loading a Magnetic Trap . . . . . . . . . 2.4.1 Compressed MOT . . . . . . . . 2.4.2 Optical pumping . . . . . . . . . 2.4.3 Switching The Magnetic Trap On 2.5 Transferring Atoms . . . . . . . . . . . . 2.6 Loading a TOP trap . . . . . . . . . . . 2.7 Evaporative Cooling . . . . . . . . . . . 2.8 Imaging . . . . . . . . . . . . . . . . . . 2.9 Calculating NA . . . . . . . . . . . . . . v . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . vi CONTENTS 3.3 3.4 3.5 3.2.2 Superimposing Magnetic Fields . Generating the Time Averaged Potential 3.3.1 Total Field Approximation . . . . 3.3.2 Calculating the Time Average . . Design Limitations . . . . . . . . . . . . 3.4.1 Curvature Along “y” . . . . . . . 3.4.2 Trap Characterization . . . . . . 3.4.3 Trap Oscillations . . . . . . . . . Measuring the Magnetic Field . . . . . . 3.5.1 Connections and Field Directions 3.5.2 Field Gradient & Magnitude . . . 3.5.3 End cap coils . . . . . . . . . . . 3.5.4 Preparing for Interferometry . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 62 65 65 68 69 69 70 70 72 72 73 75 76 4 Interferometry Techniques 4.1 Interferometer Operation . . . . . 4.2 Splitting the Matter Wave . . . . 4.2.1 Two-Level Approximation 4.2.2 The Two Level Solution . 4.2.3 The Light Shift . . . . . . 4.2.4 The Bloch Picture . . . . 4.2.5 Splitting Operation . . . . 4.2.6 Experimental Verification 4.3 Reflecting the Matter Wave . . . 4.3.1 Three Level System . . . . 4.3.2 Experimental Verification 4.4 Recombination . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 78 81 86 86 90 94 94 95 105 106 106 108 109 5 Experimental Results 5.1 Expected Output State . . . . 5.2 Measurements . . . . . . . . . 5.3 Output Fit Function . . . . . 5.4 Visibility . . . . . . . . . . . . 5.5 Results . . . . . . . . . . . . . 5.6 Decohering Effects . . . . . . 5.7 Intrinsic Limits of the Output 5.8 Number Fluctuation . . . . . 5.9 Atomic Interactions . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 113 114 114 116 119 120 121 123 124 125 . . . . . . . . . . . . . . . . . . 6 Conclusion 128 6.1 Achieved Interference . . . . . . . . . . . . . . . . . . . . . . . . . . . 128 6.2 Long Arm Separation . . . . . . . . . . . . . . . . . . . . . . . . . . . 130 6.3 Future Adaptations . . . . . . . . . . . . . . . . . . . . . . . . . . . . 130 CONTENTS vii A Temperature Interlock 132 B Control Panel 134 C Sequences 138 D Image Analysis Program 141 D.1 Fit Function . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 141 D.2 Operation . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 142 E Experiment Setup 145 F Mathematical Calculations 149 F.1 Two Level Solution . . . . . . . . . . . . . . . . . . . . . . . . . . . . 149 F.2 Matrix Elements of Ĥs . . . . . . . . . . . . . . . . . . . . . . . . . . 152 List of Figures 1.1 1.2 1.3 1.4 1.5 1.6 Interfering waves . . . . . . . Mach-Zehnder interferometer Double slit experiment . . . . Coherence examples . . . . . . Condensate interfering . . . . Coordinate system . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 8 10 13 13 16 19 2.1 2.2 2.3 2.4 2.5 2.6 2.7 2.8 2.9 2.10 2.11 2.12 Hyperfine structure . . . . . . . Doppler force . . . . . . . . . . MOT field configuration . . . . MOT . . . . . . . . . . . . . . . MOT 3-D . . . . . . . . . . . . Atom transfer . . . . . . . . . . Majorana losses . . . . . . . . . Circle of death . . . . . . . . . Evaporative cooling . . . . . . . Maxwell Boltzmann distribution Imaging system . . . . . . . . . Bose-Einstein condensate . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 23 30 33 34 35 42 44 46 49 50 57 58 3.1 3.2 3.3 3.4 3.5 3.6 3.7 3.8 Coordinates 2 . . . Trap structure . . . Trap scale drawing Trap circuits . . . . Quadrupole field . Bias fields . . . . . Magnetic ramps . . Pin connections . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 61 62 63 64 66 67 71 73 4.1 4.2 4.3 4.4 Small arm separation interferometer Chamber, trap, Bragg beam . . . . Chamber, trap, Bragg beam 2 . . . Interferometer configuration . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 79 82 82 83 . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . viii LIST OF FIGURES ix 4.5 4.6 4.7 4.8 Michelson interferometer Interferometer path . . . Bloch picture . . . . . . 10 ms after split . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 84 85 104 105 5.1 5.2 5.3 5.4 5.5 Interferometer output . . . Expected output . . . . . 10-20-10 interferometer . . Visibility . . . . . . . . . . Maximum arm separation . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 115 116 117 118 122 A.1 Temperature interlock circuit . . . . . . . . . . . . . . . . . . . . . . 133 B.1 Real time control set up . . . . . . . . . . . . . . . . . . . . . . . . . 135 B.2 De-bouncing circuit . . . . . . . . . . . . . . . . . . . . . . . . . . . . 136 D.1 Screen shot of AI 3 . . . . . . . . . . . . . . . . . . . . . . . . . . . . 144 E.1 Experiment map 1 . . . . . . . . . . . . . . . . . . . . . . . . . . . . 146 E.2 Experiment map 2 . . . . . . . . . . . . . . . . . . . . . . . . . . . . 147 E.3 Experiment map 3 . . . . . . . . . . . . . . . . . . . . . . . . . . . . 148 List of Tables 1.1 List of variables . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 20 2.1 2.2 2.3 Trapped stages . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 41 Summary . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 48 Evaporation sequence . . . . . . . . . . . . . . . . . . . . . . . . . . . 53 3.1 3.2 3.3 Trap field formulas . . . . . . . . . . . . . . . . . . . . . . . . . . . . 74 Pin polarities . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 74 Measured trap fields . . . . . . . . . . . . . . . . . . . . . . . . . . . 75 B.1 Control panel channel key . . . . . . . . . . . . . . . . . . . . . . . . 137 C.1 C.2 C.3 C.4 C.5 C.6 Loadcmot sequence . . . Movetrap sequence . . . Probesplit sequence . . . Splitpulse sequence . . . Reflectpulse sequence . . Interferometer sequence . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . x . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 138 139 139 139 139 140 Chapter 1 Introduction Early in the history of great civilizations, humans developed an inherent desire to further understand natural phenomena. Cultures like those of the Mayans, Aztecs, Chinese, Arabs, Babylonians and Greeks have all explored the understanding of nature through applied mathematics and observation based on the scientific method. In today’s world, developments in the field of experimental physics seek to add contributions to our broad understanding of modern science. They fulfill our society’s desire for understanding nature, following the essence of the theoretical and experimental methods pioneered by these cultures. The advent of modern physics in the early 1900’s led to the foundations of quantum mechanics and in particular the understanding of black body radiation emission. Consolidating this new understanding, in 1916 [3] Einstein established the theory for stimulated absorption and emission for a material interacting with electromagnetic radiation [4]. Half a century later, it became the basis for the development of the laser. As a consequence, techniques like the cooling of atoms using the coherent nature of laser light emerged, an achievement recognized by the Nobel prize in 1997 (S. Chu, C. Cohen-Tannoudji and William D. Phillips). The ability to laser cool atoms at low densities enabled researchers to further study low temperature quantum mechanical systems. One example is the theoretical work based on statistical arguments set forth by Bose and Einstein back in 1924, [5]. It proposed the existence of a quantum mechanical phase transition known as BoseEinstein condensation. To introduce phase transitions, we can think of examples that surround us in everyday life. For instance, water has three commonly known states, liquid, solid and gaseous. These physical states occur at differing atmospheric (pressure) and temperature conditions for water. When enjoying an icy cold drink in a hot summer day, we are all familiar when small water droplets start forming around the outside of the container. This happens because the invisible water vapour in the air condenses as it comes in contact with the container. Specifically, we can assume the exterior walls of our container are close to 0◦ C. 1 2 CHAPTER 1. INTRODUCTION Air has a small percentage of water vapour in it. Normally air at sea level will hold a maximum of ∼ 2.5% of water vapour at 30◦ C. As a result, water vapour molecules come in contact with the walls of the container, and thermally equilibrate with the walls. This lowers their temperature well below the dew point of water, causing the state of the molecule to change from gaseous to liquid. Hence, we see the droplets forming on our container. This change of physical state is a phase transition. Here, the physical properties of the system have changed dramatically given a small change in temperature. Just as there are phase transitions between the gaseous, liquid and solid states of matter, there are unique phase transitions for systems described by quantum statistics. In quantum statistics there are three different types of particles which determine how states are counted. There are distinguishable particles, fermions and bosons. For the latter, Bose and Einstein developed a theoretical prediction in which the particles at a given density will abruptly accumulate in the ground state of the system if the temperature is lowered below a critical value. This is analogous to the condensation of vapor to liquid in water. In such a state all the particles would have the same wave function and exhibit unique wave like properties not seen in classical systems. A more precise description of Bose and Einstein’s predicted phase transition [6] can be derived by thinking of an ensemble of N particles at fixed temperature T . For this system, the maximum number of particles allowed in the excited states Ne , is limited. If the total number of particles N > Ne then the additional particles are forced to populate the ground state. From another perspective, for an ensemble with fixed number of particles, there is a critical temperature Tc . If the temperature of the system drops such that T < Tc , then a fraction of the particles will become forced to populate the ground state of the system. The particles which populate the same single quantum ground state are said to be in a Bose-Einstein condensate and the discontinuity in the population growth of the ground state is known as Bose-Einstein condensation. Because all the particles are in the same quantum state, this new state of matter was predicted to be coherent (discussed in Sec. 1.4), analogous to photons in a laser. In 1995, experiments by C. Wieman and E.A. Cornell et al. at the University of Colorado [7], Hulet et al. at Rice University [8] and W. Ketterle et al. at MIT [9], verified the quantum mechanical phase transition for bosons. The result’s importance in physics earned it the recognition of the Nobel prize in 2001. Up to date many experimental groups around the world have successfully achieved BEC. Currently there are various standard procedures in developing a BEC machine. Most of the experimental techniques used in making BEC are readily understood by the scientific community and have been documented in detail [10]. The most common elements to use for BEC experiments have been 87 Rb and 23 Na. For other elements, BEC can be hard to achieve or even unstable. For example, experiments [11] have demonstrated that due to lack of ionization suppression, 1.1. THE NATURE OF BEC 3 BEC formation of Ne is not practically possible. In the case of our experiment, we have opted to use 87 Rb to make our Bose-Einstein condensate. Our main objective is to create an interferometer with long arm separation using a Bose-Einstein condensate. Interferometers are devices which measure phase shifts in the interference pattern obtained by combining waves. On many occasions, interferometers use a single source of waves which is split and later recombined, in order to measure the interference between them, (see Sec. 1.3). Similarly, we want to take a wave function and split it, recombine it, and finally measure the output state which should resemble that of interfering wave functions (a superposition of wave functions). In light of this, the separation distance of the two waves at any instant is said to be the arm separation. To this day, current efforts in implementing BEC interferometers have been successful [12], but not much progress has been done in extending the arm separation. We pursue a design which will provide large arm separation, allowing for interferometry experiments which require individual access to each arm. A more detailed account of interferometry and how condensates are suited for them will be given in the following sections. It turns out that due to their low velocities, a condensate’s motion is easily manipulated. Granted that, although condensates consist of particles and thus are expected to behave classically, their unique quantum configuration enables them to exhibit wave-like properties. For this reason, a condensate is said to behave like a matter-wave. Moreover, we seek to take advantage of certain key characteristics of our 87 Rb condensate in order to generate large arm separation. Development of BEC research marked a starting point for experiments like the one introduced in this thesis which rely on the low velocity of the atoms which make up a condensate. As will be presented in the following chapters, a low velocity condensate allows for simple manipulation of the motion of the atoms. In our experiment, we want to achieve a large arm separation condensate interferometer, and low velocity atoms enable us to easily achieve this. As a result, we hope the efforts set forth in the experimental work explained in this thesis adds a contribution in the applicability of condensates for interferometry. More generally, we try to provide some pedagogical insight in the behaviour of macroscopic quantum systems. 1.1 The Nature of BEC Bose-Einstein condensates will play an essential role in the implementation of our interferometer. For this reason, we will introduce their physical meaning and then proceed to outline the key steps needed to create one in the laboratory setting. Because Bose-Einstein condensation is a state of matter occurring to systems of many particles, we use statistical mechanics to understand this phase transition. Furthermore, it is important to comprehend why we must use quantum statistics in 4 CHAPTER 1. INTRODUCTION order for this unique transition to become evident. Generally, when studying a dilute system of many particles like that of a monoatomic gas, the Maxwell-Boltzmann distribution of velocities yields the appropriate thermodynamical properties which describe the system. However, this is a purely classical approach which does not include any quantum effects. Quantum mechanics asserts that for a particle of mass m and velocity v, the associated wavelength for any particle is given by the de Broglie relation using Planck’s constant h, [13]. λd = h mv (1.1) Similarly, the thermodynamical equivalent of this relationship is the thermal de Broglie wavelength. It can be thought of as the average de Broglie wavelength for atoms in a gas at some temperature T : λt = h (2πmkb T )1/2 (1.2) where kb is the Boltzmann constant. By substituting 13 mhv 2 i for kb T , we obtain: λt = q λt h 2πm2 13 hv 2 i Ãr ! 3 h = 2π mvrms (1.3) (1.4) which recovers the De Broglie wavelength up to a constant, demonstrating the similarities between λt and λd . The quantity (1.2), in conjunction with the mean inter-particle spacing (V /N )1/3 , can be used to determine whether or not quantum effects will become important when modeling the system. For a gas whose atoms have an inter-particle spacing much greater than their thermal de Broglie wavelength, the quantum properties of each atom play a negligible role in he macroscopic behavior of the gas. In this situation the gas is said to be classical. However, if the particle spacing is comparable to or smaller than λt , quantum effects become important. This condition can be expressed as: h ≥ (V /N )1/3 (2πmkb T )1/2 nh3 ≥ 1 (2πmkb T )3/2 (1.5) (1.6) where the number density n = N/V has been used. One can visualize that each atom’s associated wavelength is comparable to (or greater than) to the distance of its nearest neighbour. This means that the atoms’ wave-functions are overlapping 1.1. THE NATURE OF BEC 5 and thus the quantum mechanical effects on the macroscopic system are going to become important. Because Bose-Einstein condensation in experiments like ours occurs with n ≈ 1012 cm−3 and temperatures in the order of 35 × 10−9 K, the condition expressed in Eq. (1.6) is expected to be satisfied. In this way we know that a Bose-condensed gas will exhibit unique quantum wave like properties that ordinary gases do not have. Additionally, the condensate’s velocity will be very low, and this will prove to be an advantage for our interferometer. The process of Bose-Einstein condensation (as the name suggests) is particular to bosons and can be fundamentally explained by quantum statistics. Typically, to derive the condition for the onset of BEC, one must first obtain the formula for the occupation number as a function of the energy for indistinguishable particles of integer spin (bosons). This derivation is lengthy and is extensively found in many books like [14], which is why it will not be covered here. Nevertheless, with a simple system as an example, we can illustrate why introducing quantum statistical effects to a classical statistical mechanical treatment changes considerably the macroscopic properties of the system. In fact, one major characteristic which separates classical systems from quantum ones is indistinguishability of particles. In principle, for a classical system one could pinpoint every particle and determine their position and momenta. This means that one is allowed to label and follow all the dynamics of the system, essentially being able to distinguish each particle. But according to quantum mechanics, because we cannot measure something without disturbing it, there is always an uncertainty which limits the ability to pinpoint every position and momenta. Consequently, it is not possible to keep track of which particle is which. For indistinguishable particles, the fundamental difference between fermions and bosons is their total value of spin angular momentum. Bosons possess an integer spin value, where as fermions have a half integer spin value. Another characteristic which separates the two families of particles is that only one fermion can occupy a single state, this is known as the Pauli exclusion principle. In contrast, bosons do not have such a restriction. To place into context our example, it is important to highlight that Bose-Einstein condensation is a phenomenon which only occurs (as the name suggests) to particles of integer spin, thus excluding fermions. Moreover, as established by the Pauli exclusion principle [15], the following example will not permit a multiple particle system1 , making the example inapplicable to fermions. This means that the following illustration need only focus on differentiating between distinguishable bosons and indistinguishable bosons. With the following example, one can obtain some basic intuition as to why quantum statistics differ from classical statistics by considering the differences arising in the counting of states between indistinguishable and distinguishable particles. 1 Given the Pauli condition, no more than one ↓ atom can be in the the system, thus N > 2. 6 CHAPTER 1. INTRODUCTION Similarly, this difference illustrates why condensation to the ground state requires quantum statistics. Consider a case of 10 distinguishable blocks labeled 1 through 10. Each block has the possibility of being oriented up or down as labeled by an arrow ↑ or ↓. For instance, let’s give special consideration to the configuration where all the blocks are pointing downwards like ↓↓↓↓ . . . , and give this state the label N↓ . Our aim is to figure out what the likelihood to find the system in the configuration N↓ is if the blocks were to be randomly oriented. In order to obtain the probability of the state N↓ we must find the total number of states available in our system. Because each particle only has two possible states, it is not hard to identify that the total number of states is 2 · 2 · 2 . . . 2 = 210 , which yields a total number of states Ωs = 1024. Accordingly, the probability to find the system of distinguishable blocks in state N↓ is given by: PD (N↓ ) = 1/1024 ∼ 10−3 (1.7) On the other hand let’s consider the same system, but this time the blocks are not enumerated making them indistinguishable. Additionally, they are considered as quantum blocks obeying the symetrization postulate. With this in mind, it is clear that for any fixed number of ↑ blocks, there is only one arrangement. For example, there is only one way to get all the blocks like ↓↓↓ . . . ↓, ↑↓↓ . . . ↓ or ↑↑↓ . . . ↓, because for a given configuration, a change in the choice of ↑ blocks can just be rearranged to give back the same state. For this case the total number possible states in the system is just 11. Hence the probability to find the system of indistinguishable blocks in state N↓ is given by: PI (N↓ ) = 1/11 ∼ 10−1 (1.8) If we compare PD (N↓ ) and PI (N↓ ), it is clear that PD (N↓ ) < PI (N↓ ), making the N↓ state for the indistinguishable system much more likely than its distinguishable counterpart. Extending this example to a larger number of blocks, means the difference in the likelihood for the N↓ state for these systems would just grow further. On the whole, this example helps illustrate how introducing indistinguishability into the statistics of blocks makes the N↓ state 2 orders of magnitude more likely in this particular case. Therefore extending this idea in general we can say that indistinguishable bosons are more likely to be in the same state. In fact, in a realistic physical model of bosons, we find that for low enough temperatures a macroscopic fraction of particles in the system will collect in the ground state due to the statistics shown in the above example. The example with blocks demonstrates how indistinguishable particles make condensation to the ground state a likely outcome and why quantum statistics are necessary for this process to occur. Specifically, for a system of particles with number density n, the physical condition for Bose-Einstein condensation to take place is [14]: nλ3t ≤ 2.612 (1.9) 1.2. INTERFERENCE 7 Equation 1.9 means that for excited states in a dilute ensemble of integer spin particles, nλ3t is limited to 2.612. When this number is exceeded, by an increase in the number of particles or a decrease in the temperature, particles exceeding Ne are forced to populate the ground state and the quantum mechanical phase transition known as BEC occurs. The work presented in this thesis will not focus on BEC creation, but rather, its application in atomic interferometry. To further motivate this study, it is important to understand what an interferometer consists of and the underlying principles that explain its functionality. These principles will provide useful insight to the wave nature of BEC given interferometry requires waves interacting. Similarly, understanding the quantum nature of BEC will explain why they are well suited for interferometry. 1.2 Interference In general waves are disturbances in fields which can travel and can transmit information from one point to another. Waves have the fundamental property of constructively adding or destructively canceling when interacting. The resulting pattern of the field when the waves add or cancel each other is called an interference pattern. The interference pattern is observed by measuring the intensity of the resulting waves. It should be noted that the intensity of the wave is the physical attribute of the field which can be experimentally measured. In the casep of a elec2 tromagnetic field E, the intensity is defined as I = |E| /2ξ, where ξ = ²0 /µ0 is the impedance of free space. A simple example describing this phenomena is seen in Fig. 1.1. In this picture, two circular waves representing fluctuation in the surface of water create a familiar criss-cross pattern of ripples. The crests are where the waves have added up (maxima) and the troughs are where they have cancelled each other (minima). At any rate, interference requires at least two waves interacting in such a way that the amplitudes of the fields superimpose, resulting in a pattern that can be observed or measured. It is important to note that there are many physical examples of waves which can interfere. In the case of light and the probability density in quantum mechanics, the observable quantity is the modulus squared of the amplitudes of each field. The corresponding amplitudes are the electric field and the wave function. In fact, it is crucial to note that the interference pattern which can be observed is the square of the sum of the amplitudes and not the sum of the squares. This means that upon squaring, there will be “cross terms” which will either add or detract from the measurable result. Equally important to the understanding of interference is the concept of the wave’s phase. For example, we can think of a two dimensional field like the one presented in Fig. 1.1 having two point sources (A and B), which oscillate in the 8 CHAPTER 1. INTRODUCTION Figure 1.1: Mathematical model of two disturbances in a field (e.g. water) lying in the x, y plane (not labeled), generating concentric waves. The height of the function represents the amplitude of the wave (along z not labeled). Depending on the type of field, the amplitude may or may not be a physical observable. For water, it is. At the points where the waves meet, an interference pattern is created 1.3. WHAT IS AN INTERFEROMETER 9 vertical direction to generate waves. If the two sources began to oscillate with constant frequency ω0 at the same time and started at the same position, then the waves created are said to have the same phase. In other words, at some point (x0 , y0 ) equidistant from the two sources, the amplitude of each field will be identical for all time. When a particular crest is emitted from A and B, it will arrive at exactly the same time to (x0 , y0 ). The same dynamic would happen for the troughs emitted from A and B. Hence, at a given time, the fields always add constructively doubling the amplitude of the total field. However, if the sources were not synchronized, that is to say, A started to oscillate before B, then the waves created would have a different phase. Thinking of a snap shot in time for each wave, if we were to look at a point lying on the axis defined by the two sources, the phase difference between the waves would be proportional to the distance between the crests (or troughs) of the waves coming from each source. Another illustration would include taking pictures of a single wave at time intervals equal to the period of the wave. The resulting images would yield an intensity pattern that would not vary from shot to shot. If the phase were to change from one shot to the next, then there would be a forwards or backwards shift in the crests (or troughs) compared to their original position. If we take a cross-section somewhere where the two waves overlap and measure the total field, the resulting field would be the superposition of both waves in this region. Equivalently, this would be the resulting interference pattern between the two waves. In the interference pattern itself we would see nodes where the field remains leveled and sections where the total field oscillates up and down. If we were to look at the nodes of the interference pattern when the waves from A and B are in phase, their position would remain fixed over time. However, if we were to introduce a phase difference between the waves, the nodes of the interference pattern would shift a distance proportional to the new distance between the crests. For this reason introducing a relative phase between interfering waves causes a shift in the interference pattern. 1.3 What is an Interferometer The word interferometer already conveys substantial meaning. As the word suggests, it is a “meter” or instrument that measures interference. In general, interferometers are devices that can accurately measure changes in the interference pattern of waves. To create an interferometer we must intersect at least two waves. Usually this is done by interfering two wave sources with constant phase relation. An illustrative example is the Mach Zehnder interferometer shown in Fig. 1.2. An incoming laser is split using an optical beam splitter. The two resulting beams are redirected with mirrors in such a way that an area is enclosed between the arms of the interferometer. Finally the two beams are redirected to a second beam splitter 10 CHAPTER 1. INTRODUCTION Figure 1.2: Mach-Zehnder Interferometer. (a)Input Beam. (b)Beam splitter. (c)Mirrors.(d)Beam splitter for recombination. (e)Intensity detector. where they are recombined and a photo detector is used to measure the intensity variation. Often, interferometers will split the wave emitted by the source and recombine its parts at a later time to produce an output. The output is the resulting interference pattern of the waves’ intensity. When the arms of the interferometer are recombined on output, their resulting destructive or constructive interference is seen as an increase or cancelling of the intensity signal. When one arm of the interferometer experiences a change in its environment, the wave travelling through this channel will experience a positive or negative retardation. The retardation in one of the waves will change the relative phase between the two waves of each arm in the interferometer. A change in phase between the two arms will be reflected in a change of the interference pattern on the output which will cause a change in the measured intensity. Consequently, if the shift in the interference pattern is quantified with accuracy, it can be used to measure with precision some physical parameter related to the cause of the shift. So far, there has been no attempt to limit the implementation of interferometers to any specific kind of wave, but rather to give a general notion of how interferometers operate. Although the example presented above makes use of interfering light waves, interferometry is not limited to light. In principle, any kind of travelling wave could be utilized to perform an analogous experiment. For this reason, it becomes evident that quantum mechanical wave functions can be used to perform interferometry experiments. Although the wave function itself is non-observable (i.e a complex quantity), its modulus square corresponds to the probability of finding a certain state, which is measurable. In this regard, different wave functions can overlap, meaning that the resulting intensity pattern is just the resulting probability to find a system in a particular state after the individual wave functions have interfered. Atoms can interact with external forces much more so than photons. Usually, the 1.4. COHERENCE 11 interaction between photons and fundamental forces is only observed at extremely high energies and it is extremely weak [16]. On the other hand, atoms readily interact with gravity and electromagnetic fields. For this reason, atoms make better sensory devices to perform experiments with precision measurements involving most forces. This is one important motivation for the research presented in this thesis. Because a Bose-Einstein condensate exhibits wave like properties, we are motivated to use its wave function to carry out an interferometer. Although there are other advantages we will explore when using BEC for interferometry, a condensate also has the added advantage described of increased sensitivity. This makes it competitive with other types of atom interferometers. As we will explore in Sec. 1.5, matter can behave like a wave, implying that potentially atoms could be used for interferometry in a similar way to light. Using atoms for interferometry does not seem intuitive, but the progress in atomic cooling, trapping and motion control have made such an experiment accessible. 1.4 Coherence In many situations on varying applications, waves consist of superpositions of several different waves. A demonstration of this situation can be explained through Fourier analysis [17]. By Fourier analyzing any generic wave or pulse, we will decompose it into its various frequency components. For this reason, the waves we are seeking to use in an interferometer could consist of many different waves with multiple frequencies and phases. The visibility of interference patterns depends on the range of frequencies and direction of the wave-vectors present in the waves interacting. In the case of light, the observable is the intensity, proportional to the square of the electric field. When the range of frequencies present in light is broad, the superposition of the various components makes it harder to detect the interference pattern. Additionally, if the wave-vectors of the light are randomly pointing in different directions, the interference pattern can become blurred, making it undetectable [3]. Sunlight is a good example of a wave source that contains multiple frequencies with randomly pointing wave-vectors. For this reason, observing an interference pattern with sunlight was not possible for many years. Creating two wave sources with a stable enough phase relation (see Fig. 1.1) and single-directional wave-vector, was not experimentally realisable. However, this changed when the wave nature of light was understood. For example although there are multiple frequencies present in white light, today we know that in a set up like Fig. 1.2 with a collimated input of white light, if the path length for each arm is equal, an interference pattern will be observed. This happens because, even though there are multiple frequencies present, there are points where the maxima for the different waves always line up. One of the first experiments to demonstrate that light interfered like water waves 12 CHAPTER 1. INTRODUCTION do, was performed by Thomas Young in 1805 [3]. He set up a dark room with a pinhole which let sunlight in. After the first hole, there were two additional holes. Light emanating out of these two holes was then allowed to overlap over some distance inside and later imaged at a wall in the back of the closed room. See Fig. 1.3. It was expected to see interference if light was a wave. Traditionally, similar experiments were carried out (without the first pinhole), but no interference would be observed at the back of the room because the light contained randomly pointing wave-vectors. However the ingenuity in Young’s experiment was the first pinhole which created a single point source at normal incidence to the subsequent holes. In this way, the wavefronts emanating from the first hole are be evenly distributed as a function of the angle θy Fig. 1.3. This meant that there was one set of wave-vectors coming from a point source on the subsequent holes and not several sets of vectors from unrelated random point sources. Additionally, it created a single source of white light, meaning that the wave fronts (of each frequency) arriving at the the subsequent holes would have the same phase relation. Or in other words, the crests (or troughs) would arrive at each hole at exactly the same time. Hence each hole would see the same field variation for all time. In this way, the holes would act as two independent wave sources with a constant phase relation between them, just like the example in Fig. 1.1. Also see Fig. 1.4 [3]. As a result, the two sources emitted light which interfered, creating a pattern which was imaged at the back of the room. The pattern resulted in a series of dark and white fringes indicating the minima and maxima of the interference pattern, see Fig. 1.3 [3]. This experiment demonstrated the wave nature of light and thus its ability to interfere. It also provided a useful technique for obtaining wave sources with a constant phase relation in time and well-defined (non-random) wave-fronts. Stable interference patterns require the waves interacting to have a well defined phase relation between them as much as possible. The clarity and thus ability to measure an interference pattern is best described by the degree of coherence of the waves superimposing. There are two distinct types of coherence in waves. There is spatial coherence, pertaining to the extent the phase of the wave remains constant over some distance. An example illustrating spatial coherence is seen in Fig. 1.4 where a point source emits a circular wave, and the wavefronts are depicted by black circles. Here, points A and B are said to be spatially coherent because the wave will vary identically in each case. Equally important, there is temporal coherence between waves. The temporal coherence is often associated with the coherence length. The degree of temporal coherence between waves involves how large you can make the arrival time of different wave fronts in a particular region before the interference pattern averages out to zero, making it undetectable. This is also known as the coherence time of the waves. 1.4. COHERENCE 13 Figure 1.3: Set up for Young’s double slit experiment. 1 A non coherent source of light is incident on a pinhole. 2. The pinhole outputs spatially coherent light which in turn is incident on two other pinholes. 3. Because the light is spatially coherent, the output of the two pinholes acts as two spatially coherent sources generating the light and dark fringes in 4. Figure 1.4: Two different types of point sources emitting circular waves. The dark lines represent maxima and the faint lines minima, 1. Points A and B will experience the same variation over time, they are said to be completely correlated, the source is spatially coherent. 2. Having a monochromatic source means that knowing the wave at C completely determines the wavefront seen at at D, the source is temporally coherent. 14 CHAPTER 1. INTRODUCTION An example of the coherence time for waves can be seen in Fig. 1.3. By extending the distance between the two sources and the imaging screen, the time over which the waves propagate is increased. In this context, the longer the propagation time is while still producing the interference pattern shown, the longer the coherence time. Generally, as long as the waves have a sufficiently constant phase relationship between them over time and the wave fronts are not random, the interference pattern will remain stable and clear. If the phase between the waves changes in time, so will the position of the minima and maxima. This means that the phase between them can change, but if it happens too quickly (faster than the detector’s sampling rate), then the interference pattern will become blurred. For this reason, waves whose phase relation varies slowly over time yield a stable interference pattern. The constant phase relation will play an important role in many of the interference examples presented next and most importantly in the creation of our interferometer. The temporal and spatial coherence mentioned above are relevant to the performance of our interferometer regarding a single run of the experiment. Nevertheless, it is very important for us to obtain coherence from shot to shot of the experiment. Initially, we want to to obtain an interference pattern where we have complete control of the relative phase introduced between the arms of the interferometer. To achieve the desired control in the phase of the output state, it is important that we eliminate unwanted phase fluctuations which cause decoherence in each run of the experiment. Unwanted phase shifts from shot to shot will also decrease the contrast of our interferometer, limiting its sensitivity. Currently, lasers have tremendously facilitated the study of interference. A version of Young’s double slit experiment can be performed using laser light instead of white light and the two slits are substituted by a diffraction grating. In a similar way to the two slits, the diffraction grating will cause an interference pattern that when imaged reveals a series of light and dark fringes. Nevertheless, contrary to white light, the imaging plane can be extended for hundreds of meters. A laser with a 1 MHz line width will maintain its constant phase over a distance of 300 m (compared to mm for a discharge lamp). For these reasons, laser interferometers have become the popular choice when performing interferometry experiments. Furthermore, lasers provide a continuous source of monochromatic spatially coherent light, which dramatically improves the visibility of the interference. Having a collimated beam means the wave fronts are not randomly distributed. Also a single frequency means no other mode will blur the interference pattern when averaged over time. In short, the coherence of waves is an important factor when trying to implement an interferometer. In order to obtain a functional interference signal, we must make sure that the type of wave used has long enough coherence times and lengths for the specific purpose in mind. The next section will motivate why Bose Einstein condensates which have small energies and small velocity spreads, are well suited for interferometry. It will also show how these characteristics benefit our aim of 1.5. BEC, A COHERENT MATTER-WAVE SOURCE 15 building an interferometer with individually accessible arms. 1.5 BEC, a Coherent Matter-wave Source Young’s double slit experiment [3] demonstrated that when light passed through two slits, its intensity pattern was not consistent with typical particle behavior but rather established that light exhibited wave characteristics. Further experiments performed a century and a half later by Jönsson [18] established that fundamental particles such as electrons yielded results identical in nature to those observed by Young’s famous experiment. The experiment consisted of passing the electron through a multiple slit configuration like that in Fig. 1.3. This experiment corroborated the understanding that the electron was not localized and had gone through multiple slits simultaneously yielding an interference pattern just like the one obtained for light. To complicate interpretations further, a variation of the electron experiment was performed by Tonomura [19]. In this situation a detector was positioned right after one of the slits to corroborate which path was taken by the electron. This version of the experiment demonstrated that indeed the electron was localized like a particle and had gone through one of the slits. Today, the wavelike behaviour of the electron observed by Jönsson et al. is attributed to the fundamental particle-wave duality of matter. Depending on the experiment, a particle can exhibit wavelike or particle like behaviour as shown above. Conversely, modern experiments using weak lasers like [20] have shown that if a single photon is allowed to pass through the two slits, the detector will correspondingly show a pattern of a single photon going through. Moreover, if you allow more photons to continuously pass through the slits, the wavelike interference pattern will be reconstructed over time as more photons hit the detector. This corroborates that in the limit of many particles, wave behaviour can be recovered from particles. Our current understanding of quantum mechanics has demonstrated that at a fundamental level, matter exhibits wave-like propperties. It is well understood that when position and momentum variations approach the quantum limit as described by Eq. (1.5) and set by the value of h = 6.63 × 10−34 Js, matter is best described using the dynamics of the Schrödinger wave equation. In this limit, matter can constructively and destructively interfere. In our experiment, 87 Rb will transition into BEC at an approximate temperature of 200 nK. At this temperature, the average kinetic energy of the system is 4.14 × 10−30 J implying the average velocity of the atoms is approximately 7.6 mm/s. In this situation, the thermal de Broglie relation (1.2) states that the associated wavelength of the particles is 0.42 µm [21]. This is much larger than the average inter-atomic spacing of 87 Rb which is ra = 0.37 µm (at n = 2 × 1013 cm−3 ). For this reason the physics describing BEC atoms is best described by quantum mechanics, 16 CHAPTER 1. INTRODUCTION Figure 1.5: Two Bose Einstein condensates, released from a magnetic trap, free falling and overlapping while expanding. Because a condensate exhibits properties of a matter wave, as they expand they interfere. The fringes of the interference pattern are clearly resolved [22]. meaning the wavelike properties of matter will become more prominent. In this sense BEC makes a good source of atoms that will exhibit wave like properties. Having a condensate means that all the atoms have the same wave function. Similarly, because all the atoms are in the same state and time evolve the same, it is expected for every atom to remain in phase and thus be quantum coherent across the whole condensate. In 1997, an atomic wave version of Young’s double slit experiment was conducted by Andrews et al., at MIT [22]. Two condensates were separated and released from their magnetic trap and allowed to ballistically expand. As the condensates expanded, the clouds crossed paths and interfered as matter waves, see Fig. 1.5. This result proved that the condensed atoms were coherent on the time scale of the experiment, which imaged the interference pattern after 40 ms of free fall. Because the condensates are in a minimal energy state (lowest state of the trapping potential ignoring atomic interactions), their kinetic energy is extremely low. Hence, manipulating the motion of the condensates proves simple and an attractive proposition for further applications. Our hope is to perform an experiment which exploits the wave-like behavior of condensates in a controlled way. Instead of using ballistic expansion we aim to use a waveguide for the atoms. Currently, interferometry using cold atoms has proven successful [23, 24, 25]. However the condensate atoms have special characteristics which allow them long temporal and spatial coherence. This gives them some important advantages as 1.6. OUTLINE OF THESIS 17 wave sources for interferometry. The condensates have long temporal coherence because all the atoms are in the same state. This means that all the atoms start off at the same velocity and because each atom’s quantum phase evolves steadily in the same way, their phase relation does not change over a long period. The result is a condensate that can evolve for long times without losing coherence. In our case, this means that we could potentially split the condensate and allow it to travel for long time intervals before recombining it, and still be able to observe interference. All the atoms in the condensate are in the same state and each atom’s quantum phase is identical. Hence the phase relation for each atom is constant, meaning the condensate is spatially coherent across the whole ensemble. When the condensate is sitting still in the magnetic trap, all the atoms are in phase. At any instant in time, the wave function at different points in the condensate is correlated, meaning the wave function at one point of the condensate can be determined from another point at any moment. In the end, long temporal coherence means the frequency variation in the wave will be small (i.e monochromatic), therefore the energy variation for the wave functions will be minimal such that ~∆ω ∼ ∆E ∼ ∆K.E. for small clouds of atoms. Additionally, due to spatial coherence, the phase variation across the condensate is small. Hence the variation in the wavelength of the wave functions will be small too. For both reasons, it means the spread of velocities ∆v across the condensate is small too, which is one of the most important characteristics about condensates we exploit in our experiment. Having a small ∆v at low temperatures will dramatically improve our ability to control the motion of the atoms, which is what we need to obtain large arm separation. We hope to take advantage of the increased coherence length provided by a condensate to maximize the distance over which we can separate the arms of the interferometer. In turn this would yield longer propagation times and result in large coherence times. 1.6 Outline of Thesis The purpose of this thesis is to concisely describe the steps involved in implementing a BEC interferometer using a special weak magnetic trap designed to allow long coherence times and large arm separation. Chapter 2 gives an introduction to the 87 Rb atom and explains how we produce BEC. It summarizes the properties of 87 Rb atoms, and explains how we use laser cooling techniques to obtain an ultra-cold sample of atoms. The atoms are then loaded into a magnetic trap and evaporatively cooled until BEC is reached. Finally there is a section on how imaging of the condensate is performed. Chapter 3 focuses on our novel waveguide design. It starts with an explanation 18 CHAPTER 1. INTRODUCTION of how the magnetic waveguide is loaded. It continues explaining how the magnetic fields it uses are achieved. It explains how the trap is used for the evaporative cooling phase and gives a detailed discussion on the role each circuit has in making up the wave guide. At the end of this section, the total B field is presented, illustrating what the overall potential the atoms experience is. The measured B field distribution is found to agree well with the observed trap parameters. Finally the chapter documents in detail the appropriate settings and connections used for the guide. The main focus of this thesis is to present the implementation of a working one dimensional analog of the Michelson interferometer in Fig. 4.5. Chapter 4 provides an in depth explanation of the main experimental techniques that were used to achieve long coherence times and arm separation. Our implementation requires operations to both split the condensate into two moving packets, and to reflect the motion of the packets. These operations are explained and analyzed and the dependence of the output state on the interferometer phase is determined. We developed an interferometer scheme which (in sequential order) consisted of four main operations: a splitting stage, two reflections and a final recombination stage. In Chapter 5 we study the interference results in detail and obtain the expected results for the output state of the interferometer. We also discuss these results. The value of the output state was observed to be consistent with our predicted sinusoidal function for experiments of up to 44 ms in duration. We were able to identify that although our interferometer lost visibility after ∼40 ms, coherence was still observed for longer times up to ∼80 ms from shot to shot. We believe vibrations in our trap and unwanted fluctuations in laser intensities affecting interferometer operations (Ch. 4) could be responsible for decoherence effects so we have tried to improve upon this. Finally, we attribute the long coherence times to the weak confinement provided by the trap. We provide some theoretical background explaining the intrinsic quantum limit of the phase contrast. Following this calculation, we analyze the effects atomic interactions have on the phase contrast observed. In Chapter 6, the conclusion, we summarize our results and stress their importance as a stepping stone in the applicability of BEC in interferometry. We value the importance of this experiment as a demonstration of quantum mechanical effects in a macroscopic scale having important pedagogical value. Future applications of the trap and adaptations of the current design are discussed. 1.7 Experimental conventions Through out this thesis there will be several terms that are abbreviated with acronyms, shorter words or even symbols with the intent of preventing interruptions to the flow of the topic at hand. Table 1.1 contains the symbol or abbreviation being used along with a more detailed description of it. Readers can use this table as a quick reference 1.7. EXPERIMENTAL CONVENTIONS 19 Figure 1.6: Two glass chambers are connected via a thin tube 1 cm in diameter and 28.75 cm in length. The cylindrical chamber on the left is used to create a MOT and load a quadrupole magnetic trap generated with the two anti-Helmholtz coils shown on the outside. Atoms are transfered to the second chamber (science cell) on the right where the interferometer wave guide is located. The center of the coordinate system used to describe the magnetic fields is located at the center of the trap structure labeled (0,0,0). The x direction is along the direction of the mechanical translation of the atoms, z is the vertical direction and y is along the axis of the waveguide. For chapter 2, the magnetic fields used for the MOT are referenced to an origin where the x coordinate is offset by D as shown above but is ~ fields. not reflected in the mathematical expressions of the B when the context of a particular abbreviation is not sufficient. 20 CHAPTER 1. INTRODUCTION Symbol or acronym description BEC Bose-Einstein condensate MOT Magneto optical trap TOP Time-orbiting potential r.m.s. root mean squared σ+ Sigma plus polarized light σ− Sigma minus polarized light ~ Planck’s constant / 2π kB Boltzmann constant λt Thermal de Broglie wavelength i, j, k Unit vectors Table 1.1: List of variables and acronym Chapter 2 Making BEC 2.1 Rubidium Atoms Rubidium is an element which is very well suited to make BEC because it has physical properties that make its cooling and trapping relatively simple. Denoted in the periodic table by the symbol Rb, rubidium is a metal having a vapor pressure at 25◦ C of 3.0 × 10−10 Torr. It is found in group 1 of the periodic table of elements, also known as the alkali metals. Alkali metals all contain a single valence electron. By containing a single electron in the outer most electron shell, alkali atoms have the ability to readily ionize, making them highly reactive. Rubidium has atomic number 37; its most common natural occurrence is 85 Rb making up ∼ 72.2% of the known isotopes. The second most common ocurrence is that of 87 Rb with ∼ 27.8% [26]. Currently, this isotope is used extensively in experiments involving laser cooling which takes advantage of its cycling transition between hyperfine states, a characteristic shared with all the other alkalis. The transitions of 87 Rb relevant to laser cooling can be derived from extending the simple hydrogen electronic shell structure. To an approximation, the quantum model of the electronic configuration in 87 Rb can be thought of as equivalent to hydrogen, but with different nuclear mass, higher number of electrons and spin. Light atoms like hydrogen with low number of electrons demonstrate experimentally a very fine division in their spectral lines, e.g. 4.5 × 10−5 eV [27] for the H-alpha line (2P1/2 → 2P3/2 ). It is known as the fine structure of the atomic energy levels. This small effect is due to the interaction between the total orbital angular momentum of the atom and the electron’s spin. It can be thought of as the interaction between the electron’s magnetic spin and the magnetic field emanating from the current loop set up by the rotating electron. The energy shift is analogous to that experienced by a magnet with moment µ surrounded by a loop of current producing a field B, where ∆E = −µ · B. Accordingly, the interaction is known as the spin-orbit coupling and depends on the operator L · S. For atoms that have many electrons and a heavier nucleus (i.e. more neutrons 21 22 CHAPTER 2. MAKING BEC and protons like 87 Rb), it is important to keep in mind the spin-orbit coupling. For example, the total angular momentum of an electron Ji = Li + Si can couple to the total angular momentum of other electrons Jj = Lj + Sj , which means the total momenta interact with each other (this effect is known as the j-j coupling). It can be thought of as a repulsive interaction the one active electron feels from the others. However, a larger effect in the case of 87 Rb is the coulomb interaction between the nucleus and the electrons. Due to this, different orbitals that would normally be degenerate are now energetically split. For the case of 87 Rb, the degenerate energy eigenstates 52 S1/2 , 52 P become split. The resulting split gives rise to transitions from the 52 S1/2 state to the 52 P states. In turn the 52 P states are split due to the L · S coupling, wich yields a break in the degeneracy of the 52 P3/2 and 52 P1/2 states. For this reason, the coulomb interaction mentioned between the 52 S and 52 P states and the L · S (also known as spin orbit coupling) interaction, give rise to transitions between the 52 S1/2 and 52 P1/2 states and the 52 S1/2 to 52 P3/2 states. They are known as the D1 and D2 lines respectively. Furthermore in 87 Rb, introducing the interaction between the nuclear spin I and the total angular momentum of the electron J creates another subgroup of split energy levels known as the hyperfine structure of the atom. The total angular momentum of the atom is denoted by F which follows the usual rules for addition of angular momenta: F=I+J (2.1) where the minimum and maximum values for the magnitude of F are given by |J − I| ≤ F ≤ J + I . (2.2) The ground state for 87 Rb is the 52 S1/2 state where L = 0, J = 1/2 and I = 3/2. This means that the hyperfine structure for this state will consist of two sub-levels where F = 1 or F = 2. The exited states occur for L = 1, using the addition rules for angular momenta we obtain that J = 3/2 or J = 1/2 giving us the previously mentioned excited states. Due to the hyperfine interaction, additional sub levels appear for each of these excited states. Using equation (2.2), the hyperfine structure revealed for the two exited states is such that F can take the values of 1 or 2 for the P1/2 state and 0, 1, 2 or 3 for the P3/2 state. The diagram on Fig. 2.1 represents the energy levels and splitting due to hyperfine interactions for the ground and exited states of 87 Rb. 2.1.1 External magnetic fields For each individual hyperfine state labeled F, there is subset of 2F + 1 states corresponding to a particular projection of the the angular momentum state along the quantization axis labeled mf . Normally all these states share the same energy, but in the presence of an external magnetic field their energies are shifted according to 2.1. RUBIDIUM ATOMS 23 Figure 2.1: The atomic states of 87 Rb are split due to the hyperfine interaction. Our experiment uses the cycling transition found in the D2 line. The magneto-optical trap uses the transition from F = 2 to F 0 = 3 at 780.246 nm as the main trapping frequency. A second laser tuned to 780.232 nm drives the F = 1 to F = 2 transition. The values for the Landé g-factors gf are given for every different F level. 24 CHAPTER 2. MAKING BEC the Landé g-factor specific to each type of angular momenta S, L, I and the electron magnetic moment µB . The energy shift due to the external magnetic field for each mf projection is called the Zeeman effect. Specifically the Hamiltonian describing this interaction can be expressed as explained in [13, 28]: HBext = µB (gS S + gL L + gI I) · B ~ (2.3) By choosing the quantization axis to be along the the direction of a magnetic field in the z direction we obtain HBext = µB (gS Sz + gL Lz + gI Iz ) Bz ~ (2.4) Moreover, when the energy shift due to the external field is smaller than the hyperfine shift itself, Eq. (2.4) can be approximated yielding the following energy shift [26]. µB ∆EBext = gF mf Bz (2.5) ~ where mF is the z projection of the total F angular momentum and gf is the Landé g-factor for each angular momentum configuration. A derivation of the expression for the Landé g-factor can be found in many texts [29]. Figure 2.1 includes values for the Landé g-factors in the various | F i sub-levels for the 5S1/2 , 5P1/2 and 5P3/2 states. If the atom makes a transition from a ground F state to an excited F’ state, the transition selection rules [28] establish that ∆mF = ±1 or 0. A photon inducing a transition can carry different values of angular momentum depending on its polarization. If the polarization is linear then ∆mF = 0, and if it is circular then ∆mF = ±1. For circularly polarized light we use two conventions depending on the helicity of the photon at hand. If the k vector of the light is aligned with its angular momentum L, it labeled left hand circularly polarized. For the case of an anti-aligned k and L, it is labeled right hand circularly polarized. The different cases of circular polarization are abbreviated as LHC and RHC respectively. Adittionally, for σ + polarized light (L parallel to an external B), the change in angular momentum after the transition is ∆mF = 1, on the other hand, σ − light (L anti-parallel to an external B) induces a ∆mF = −1 change1 . In this way, the change of angular momentum the atom experiences after a transition will depend on the angular momenta carried by the photon that caused it. If resonant light incident on the atom is polarized such that ∆mF = 1, then after successive transitions, the atom could find itself in the highest | F 0 , mF 0 i state. At this point it is incapable of transitioning to higher mF 0 states. Its only option is to decay to the highest | F, mF i state from where it can only go back to up to the 1 more about circular polarization and external B fields is discussed in Sec. 2.2 2.2. CREATING A MOT 25 highest | F 0 , mF 0 i state. Consequently the transition it remains locked to is called a cycling transition. Rubidium has two cycling transitions according to its frequency which are useful in optical cooling and magnetic trapping. In particular, as will be discussed later, cycling transitions are used in order to pump trapped atoms into the desired hyperfine state. In order to achieve the desired phase space densities of 87 Rb to obtain BEC, we use laser cooling as a first step in lowering the the temperature from Tr = 300 K (room temperature) to approximately T = 100 µK. Understanding the hyperfine structure of rubidium reveals why this element as well as all the other alkalis, are suited for laser cooling. As described on Fig. 2.1, the characteristic frequencies that couple the ground with excited states are found in the near infrared spectrum, this means we can take advantage of the wide range of commercial diode and Ti:sapphire continuous wave lasers available in this frequency range to perform laser cooling. 2.2 Creating a MOT Conceptually, utilizing the force induced by the scattering of laser photons to slow down the velocity of thermal atoms, was introduced by Letokhov et al. , Wineland et al. and Hänsch et al. [30, 31, 32, 33] in the mid to late 70’s. Their efforts culminated 15 years later when S. Chu et al. was awarded the Nobel prize for experimentally demonstrating laser cooling techniques [34]. A detailed description of laser cooling can be found in many texts [35]. We give a condensed treatment here. Our first step in creating a BEC involves confining atoms which start out as a dilute gas at room temperature of T = 300 K. This is experimentally achieved by setting up a magneto-optical trap. It combines viscous forces provided by laser light tuned to the resonance of the atoms with confining forces resulting from introducing a magnetic field. Laser cooling uses light-induced forces to reduce the momentum of thermally distributed atoms. As the name suggests, the aim is to use resonant light to cool, or equivalently slow, the atoms, thereby reducing the average kinetic energy of the sample. Temperature is just a macroscopic thermodynamic property of the system proportional to the average velocity of a sample of atoms. This can be demonstrated by the well known statistical result hEi = 3/2kb T , where hEi is the average energy of a 3 dimensional ideal gas. If one can reduce the average r.m.s velocity of the atoms in a sample, then the temperature of the system can be reduced. 3 1 mhv 2 i = kb T (2.6) 2 2 To understand the mechanisms we can use to slow down the atoms, we must introduce the dynamics of the absorption of photons in a simple two level quantum system and how the effects of spontaneous emission enter into the two level problem. K.E. = 26 CHAPTER 2. MAKING BEC We can include spontaneous emission into the two level problem by using the density matrix formalism in quantum mechanics. In general, in addition to the wave function expressed as: X | Ψi = ci | ii, (2.7) i information about what state the system is in, is given by the density operator in conjunction with the complete set of basis vectors for that system. The density operator is given by ρ = | Ψih Ψ| (2.8) such that the matrix elements of the density operator are obtained by ρij = hi|ΨihΨ|ji = ci cj∗ (2.9) where i and j denote the indexes for two distinct basis vectors in a given space. Using the example of a simple two level system, the complex coefficients cg (t) and ce (t) are the time dependent coefficients for the ground and excited states of the system respectively. For this system, the total wave function can be written as: | Ψi = cg | gi + ce | ei (2.10) Following Eq. (2.9) such a system’s density matrix can be explicitly written as: · ¸ · ¸ ce c∗e ce c∗g ρee ρeg ρ= = (2.11) ρge ρgg cg c∗e cg c∗g Although the two level system will be covered with more detail in Sec. 4, we can use the results obtained in Metcalf and van der Straten’s Laser Cooling and Trapping [35] for the purpose of this discussion. It calculates time dependent coefficients cg and ce regarding a two level system denoted by a ground and an excited state initially coupled via the Hamiltonian H(t) = −eE(r, t) · r. In this case E is set up as a plane wave polarized in the z direction. The resulting coefficients are: ¶ µ Ω0 t i∆t/2 Ω0 t ∆ cg (t) = cos − i 0 sin e (2.12) 2 Ω 2 Ω0 t −i∆t/2 Ω e (2.13) ce (t) = −i 0 sin Ω 2 using Ω0 = √ Ω 2 + ∆2 (2.14) 0 The parameter Ω ≡ −eE h e|r| gi is known as the Rabi frequency where E0 is the ~ amplitude of the electric field E and ∆ = ωl − ωa is the detuning of the incident radiation field from the transition frequency between the two levels. The next step is to find out the time evolution of the matrix elements ρij . For this purpose, we 2.2. CREATING A MOT 27 take the time derivative of each matrix element ρij as defined by their respective ci c∗j . Then we substitute in the explicit time dependence of the coefficients ce ,cg and finally re-write the equations back in terms of the matrix elements ρij . Using the example of ρgg we obtain: dc∗g dρgg dcg ∗ Ω∗ Ω = cg + cg = i ρeg ei∆t − i ρge e−i∆t dt dt dt 2 2 (2.15) Additionally we must include in the time evolution of ρij the effects caused by spontaneous emission. The derivation of how spontaneous emission is obtained will not be covered here but is discussed in many quantum mechanics texts like [13, 36]. Specifically, it is found that in a system comprised of a two level atom and a photon field, the state | ei describing the excited atom is short lived. This means the atom decays to the ground level. The time evolution of the amplitude for this state is given by the coefficient ce in: dce (t) Γ = − ce (t) dt 2 (2.16) which means the excited state amplitude has an exponential spontaneous decay factor of Γ/2. For 87 Rb the excited state 52 P3/2 will have Γ = 2π × 6.07 MHz. Consequently the decay rate of the probability is Γ and the lifetime of the excited state is τ = 1/Γ. We now apply this result to the simple two level problem. If the excited state probability ρee decays at a rate Γ then the ground state probability ρgg will grow at a rate Γ. For this reason we introduce this growth factor into Eq. (2.15). ¢ dρgg i¡ ∗ = Γρee + Ω ρeg ei∆t − Ωρge e−i∆t dt 2 (2.17) The same procedure described above can be performed to the remaining density matrix elements ρeg , ρge and ρee . This would result in four equations for the time derivatives of each element of ρ known as the optical Bloch equations. They will not be presented here, but the result can be found in [35]. Still, we can use two restrictions imposed by the two level density matrix which allow us to find the steady state solutions to these matrix elements. We know that in the two level system, the sum of the population in the two states must be conserved as ρee + ρgg = 1. Furthermore, the matrix elements ρij are hermitian as demonstrated by Eq. (2.9). Applying these conditions to the optical Bloch equations can yield the following: µ ¶ Γ iΩ(ρgg − ρee ) dρeg = − − i∆ ρeg + (2.18) dt 2 2 ¢ ¡ d(ρgg − ρee ) (2.19) = −Γ(ρgg − ρee ) − i Ωρ∗eg − Ω∗ ρeg + Γ dt 28 CHAPTER 2. MAKING BEC To obtain the steady state solution for the ρij coefficients shown above we can set the time derivatives to zero and obtain: ρgg − ρee = ρeg = 1 1+s (2.20) iΩ 2(Γ/2 − i∆)(1 + s) (2.21) where we have defined the saturation parameter s = |Ω|2 /2(∆2 + Γ2 /4). Careful observation reveals that by introducing the value of Γ given in Eq. (2.16), the intensity I = c²0 E02 /2 appears in s. Accordingly we define Is = πhc/3λ3 τ as the saturation intensity where λ is the wavelength of the radiation field and τ is the life time defined in Eq. (2.16). s≡ |Ω|2 /2 I/Isat = ∆2 + Γ2 /4 1 + (2∆/Γ)2 (2.22) For the D2 line in 87 Rb λ = 780.24 nm and τ = 26.24 ns, meaning the saturation intensity Isat = 2.5 mW/cm2 . If the incident light beam is below saturation intensity then s ¿ 1, meaning ρgg − ρee ≈ 1 and the system is mainly in the ground state. Otherwise, when s À 1, ρgg − ρee ≈ 0 and the populations for the excited and ground state are equal. Using the same method utilized to get Eqns. Eq. (2.20) and Eq. (2.21) we can obtain an expression for ρee : ρee = s I/2Isat = 2(1 + s) 1 + I/Isat + (2∆/Γ)2 (2.23) The above expression shows how the probability for the system to be in the excited state approaches 1/2 as I À Isat . The model depicted above is for a generic two level system interacting with a an electromagnetic plane wave. Hence, we can apply it to a real atom like 87 Rb interacting with a laser, in which the D1 or D2 lines act as a two level system for the valence electron. Thinking about Eq. (2.23) in the context of an atom in a laser field means that every time the electron decays to the ground state of the system, there will be a photon emitted. This allows us to multiply the probability to be in the excited state ρee by the the decay rate of the excited state (1 photon emission/decay) to obtain the photon scattering rate Rs as: µ ¶ I/Isat Γ . (2.24) Rs = Γρee = 2 1 + I/Isat + (2∆/Γ)2 Now that we have uncovered the mechanism by which a simple two level atom scatters photons from a laser beam, we can shift towards discussing how to reduce the thermal energy in a large sample of atoms. Slowing down fast moving atoms requires an overall momentum exchange. By absorbing a photon that drives the 2.2. CREATING A MOT 29 atom to the excited state, the atom gains an overall momentum of ~k. Here ~ is related to Plancks constant by ~ = h/2π and k is the wave-vector for the photon. The atom will eventually decay to the ground state through spontaneous emission. It will emit a photon in a random direction meaning that on average, over several emissions, the overall net momentum change due to emission is zero. After the absorption and emission process, the atom would have an overall momentum change in the direction of the absorbed photon which results in a “kick” along the direction of the propagating beam. One can express the net force experienced by the atoms due to absorption and spontaneous emission as Fae = ~k Γ ρee . (2.25) By writing the force in terms of ρee , it can incorporate the saturation effects that limit absorption at high intensity light fields. Substituting for ρee in terms of the detuning ∆ and the ratio of intensity to saturation intensity I/Is of Eq. (2.23), yields the expression for the force due to absorption and emission. µ ¶ ~kIΓ 1 Fae = (2.26) 2Is 1 + I/Is + (2∆/Γ)2 The maximum value ρee can take due to saturation effects is 1/2, meaning that Fae saturates to a value of ~kΓ/2. From the expression above it is clear that a laser beam tuned near the atomic resonance can effectively be used to impart a force that would push the atoms in the direction of k, the wave vector of the light. If the atoms have a component of the velocity v opposite to k then this force can be used to slow down this particular component of the velocity. One can extend this idea to a pair of counter propagating beams. The sum of the forces due to both beams results in a configuration that will slow down atoms from two directions in one dimension. More generally the Doppler shift ωD = −k · v of the light field experienced by 87 Rb atoms at room temperature is not negligible. As indicated by the dot product, any component of k which is perpendicular to v will not contribute to the Doppler shift. In turn, any component of k parallel to v will add or subtract to the Doppler shift. For example, consider the one dimensional case of an atom whose velocity v is opposite in direction to the propagation of the light k. The effective field “seen” by the atom is Doppler shifted to the blue by an amount ωD = kv. This means that the Doppler-shifted light seen by the atoms can be used advantageously. For laser light slightly tuned red of resonance, an atom moving with some component of its motion towards the incident beam will experience a light field closer to resonance. Consequently, it will scatter more photons from that beam and experience a greater force. In the one dimensional case of a pair of counter propagating beams, an atom will preferentially absorb and thus feel a greater force from the beam that has a k pointing opposite to the velocity of the atom. On the whole the force can be written as follows: 30 CHAPTER 2. MAKING BEC Figure 2.2: The two grey curves represent the velocity dependent forces for two counter propagating laser beams with the same frequency and intensity . The top curve corresponds to the force field obtained for a beam with k, the bottom curve represents that of a beam with −k. The black line is the sum of both curves. The total field is non conservative but damps the motion of the atoms µ F= ~s0 Γk 2 ¶· 1 1 − 2 1 + s0 + [2(∆ − ωD )/Γ] 1 + s0 + [2(∆ + ωD )/Γ]2 ¸ (2.27) The above equation represents an atom moving with velocity v in a one dimensional force field. There are two main components to the equation. The first term is due to the force experienced by the atom from the light beam whose wave vector is pointing in the positive direction, and in the negative direction for the second term. Both add up to give a total force that is velocity dependent and is illustrated by the plot shown in Fig. 2.2. The resultant force field in equation (2.27) can be extended to slow atoms in three dimensions by adding two additional pairs of counter propagating beams such that all three pairs are perpendicular to each other. Similar to the one dimensional case, in the region where the beams overlap a moving atom will always preferentially absorb a photon from the beams having k vectors anti-parallel to its velocity v. For atoms moving too fast, ωD is very large and the interaction with any light beam is negligible. But for slower atoms the net result is a volume where atoms experience a non-conservative viscous damping force, slowing down their velocity 2.2. CREATING A MOT 31 considerably and consequently their temperature. This configuration of red-detuned laser beams has the name of optical molasses which describes the dissipative nature of the force. A limitation of optical molasses is the lack of confinement provided by the damping forces. As a result atoms are not truly trapped but rather slowed. Typically, an experimental set up of 87 Rb optical molasses can slow down any one atom to µK temperatures, in a ms time scale. Optical molasses are relatively easy technique to set up in the laboratory but their confinement effect is non-existent. As discussed previously, the net momentum change per atom due to the absorption and emission process is ~k. Additionally, due to the discrete nature of photons, the recoil momentum ~k is the minimum obtainable momentum when using a molasses configuration. This intrinsically prevents Fae from slowing the atoms completely. The recoil limit can be expressed as: k b Tr = ~2 k 2 MRb (2.28) Furthermore, because there are no restoring forces that bring atoms back to the center of the molasses region, atoms moving in the order of the recoil limit will normally be lost. Although optical molasses can cool atoms down to low temperatures (∼ µK), they can only do so for very dilute samples because of the lack of confinement forces. We utilize a magneto-optical trap (MOT) in order to provide the necessary confinement for neutral atoms. This technique was first developed by Raab et al. [37]. It is a very effective way to add a restoring component to the optical molasses viscous forces by using a magnetic field gradient. The beam configuration is the same to that of optical molasses, however the polarization of each beam must be chosen carefully as will be demonstrated later. Additionally, it requires a pair of magnetic coils to achieve zero field at the center and a linear magnetic gradient in all directions of the volume where the beams overlap. Introducing a magnetic field causes an energy shift in the atomic states. As a result, an additional shift in the frequency experienced by the atom (in a light field), is introduced. For this reason the total detuning experienced by the atoms is now given by: ∆ = ∆0 − k · v + µeg B(r)/~ (2.29) where ∆0 is now the laser detuning from resonance for a zero velocity atom, −kv is the Doppler shift, and B(r) is the magnitude of the external magnetic field. Additionally, µeg = µbe − µbg , where µbe and µbg are the the effective moments for the excited and ground states, meaning µeg is the difference between magnetic moments of different states (which depend on gF ). Adding a magnetic field means that the degenerate states are Zeeman shifted proportionally to the magnitude of the magnetic field as (for the z direction) ∆E = gF µb mF Bz . (2.30) 32 CHAPTER 2. MAKING BEC More detail of how magnetic fields are used to trap 87 Rb atoms will be addressed in the next section, but it is important to note that the Zeeman energy shifts are also dependent on the spin quantum number mF and the Landé g-factor gF discussed in Sec. 2.1.1 given in Fig. 2.1. Depending on the sign of mF , the hyperfine state will either increase or decrease in energy as the magnitude of the field increases away from the center. A key component to creating a MOT is choosing the correct right and left hand circular polarization of light in order to drive the cycling transitions in 87 Rb. To figure this out, it is useful to define a convention of polarization relative to the magnetic field. Circularly polarized photons carrying an angular momentum L aligned to the magnetic field B, are said to be “sigma plus” or σ + polarized. For the case of circularly polarized photons carrying an L anti-aligned to the magnetic field, the light is said to be “sigma minus” polarized or σ − . Equally important, we must relate the helicity of the light to the σ − , σ + basis. To do this we use the convention discussed in Sec. 2.1.1 where we define left and right hand circularly polarized light in terms of angular momentum L carried by the photon, and its wave vector k. LHC ⇔ k k L RHC ⇔ k ¼¹ L (2.31) (2.32) For Zeeman shifted states in 87 Rb, the cycling transitions optimum for laser cooling occur for σ + and σ − light between the 52 S1/2 , F = 2 and 52 P3/2 , F 0 = 3 transition. To create a MOT we need to use these transitions. Consequently, we require a magnetic field whose geometry in combination with three pairs of counterpropagating beams will yield these transitions at the right location. See Fig. 2.3. Consider an atom with the | F, mF i to | F 0 , m0F i transition in a one dimensional magneto-optical trap. Figure 2.4 shows a schematic for the case of a one dimensional MOT along the z direction. Atoms positioned away from the center in the +z direction will experience a higher magnetic field than those in the center. The further away from the center, the greater the Zeeman energy shift. If the laser is red detuned the right amount (∼ 15 MHz) from the desired cycling transition, the Zeeman shift is enough to bring the atom’s energy levels close to resonance with the light. For example in the case of a | 0, 0i to | 10 , −10 i transition, the shifts lower the mF = −1 state’s energy enough for a σ − beam to drive the cycling transition. Similarly, for an atom positioned away from the center in the −z direction, the mF = 1 state will be shifted such that the σ + transition comes into resonance. For the case of a one dimensional field, if the magnetic field points away from the origin along the z axis we get a MOT. Also, the two beams along the axis have their respective k pointing towards the origin. This means that in order to get a σ − beam on the +z axis and a σ + beam on the −z axis, the light must be left hand circularly (LHC) polarized on the beam coming from the +z direction and right hand circularly polarized (RHC) on the beam coming from the −z direction. In 2.2. CREATING A MOT 33 Figure 2.3: 3 pairs of counter-propagating beams aligned perpendicular to each other to create a MOT. Each beam should have the right helicity of circular polarization in order to provide LHC or RHC as shown above. In the x and y axes, to obtain σ − light, given the direction of B, k will always be anti-parallel to the angular momentum of the light L. This means the light should be RHC polarized. The reverse is true in order to obtain σ − light for the z axis. The plane x = 0 shows a cross section of the quadrupole field relative to the incident beams required to have a MOT. 34 CHAPTER 2. MAKING BEC both cases the atoms will be pushed back towards the center of the magnetic field providing a restoring confinement force which traps the atoms. In order to extend this restoring mechanism to 3 dimensions, we must keep track of which transition (whether σ + or σ − ) needs to be driven on each side of every axis in order for the atoms to receive a momentum transfer towards the center (i.e k is towards the center). Then, compare this to the direction for the quadrupole field in that region and establish if LHC or RHC is required. Figure 2.3 illustrates the required polarizations to obtain a MOT given a particular field. We use a laser tuned to 780.246 nm to drive the F = 2 → F 0 = 3 transition required by the six MOT beams. However, there is a small probability for this light to excite atoms to the F 0 = 2 state. This can become a problem when implementing a MOT because according to selection rules, atoms in this state can spontaneously decay to the F = 1 state. The F = 1 ground state is 6.8 GHz detuned from the F = 2 becoming a dark state to the laser light and disabling the MOT beams from interacting with the atoms. In order to resolve this problem, we use a re-pump laser beam tuned to 780.232 nm that drives the F = 1 → F 0 = 2 which gives the atoms an opportunity to decay back to the F = 2 ground state where they will interact with the MOT beams (see Fig. 2.1). A MOT can achieve low temperatures with the added advantage of the confinement forces that trap neutral atoms which is not present in an optical molasses set up. However, optical molasses can cool further than a MOT configuration. Optical molasses can reach lower temperatures, but as mentioned earlier their limitation arises from the single photon recoil momentum present in the absorption emission process. Generally MOTs can achieve temperatures in the order of tens to hundreds of µK. In our experiment we have measured temperatures of ∼ 800 µK for a number density of 0.8×1010 atoms/cm−3 using ballistic expansion methods (see Sec. 2.8). Compared to the temperatures and densities required to obtain BEC, which is usually hundreds of nK at n = 1013 atoms/cm−3 , a MOT does not achieve low enough temperatures at the given density to achieve the desired phase transition. Along with the limitations of cooling with lasers addressed briefly in Eq. (2.28), there are others which prevent us from obtaining the densities required for BEC. In a MOT, the atoms that are at the core will experience a type of “light shielding” since atoms near the outer edge will absorb most of the light. This is why atoms near the core will not get cooled as effectively and high enough densities will not be achieved. To solve this problem, we perform evaporative cooling. This technique requires very low background pressures (three orders of magnitude less) in order to be effective, more details will be explained in section 2.7. 2.2. CREATING A MOT 35 Figure 2.4: The laser frequency ωl , tuned 15 MHz red of the atomic resonance of Rb, drives the F = 2 → F 0 = 3 transition for atoms whose velocities provide the adequate Doppler shift. The presence of a magnetic field creates a Zeeman shift in the hyperfine states, tuning the m = −1 closer to resonance. The chosen polarization of the beams causes atoms which are positioned away from the center of the trap to preferentially absorb the light propagating opposite to them, pushing the atoms back towards the center of the trap. The lower portion of the diagram shows the magnitude and orientation of the field along z direction for x = 0, y = 0. 87 36 CHAPTER 2. MAKING BEC Figure 2.5: A 3-D representation of the MOT beams, the coils that make the anti Helmholtz magnetic field and the glass cell that contains 87 Rb at room temperature. Typically, a MOT can load 109 atoms in 3 s and achieve a temp of 100 µK. The small tube extruding from the chamber leads into the UHV region where evaporative cooling is performed 2.2.1 Supplying 87 Rb In addition to the light shielding effects mentioned above, the way we supply 87 Rb atoms to the MOT limits our ability to achieve the necessary phase space densities to achieve BEC. We have installed inside the first chamber two pairs of 87 Rb getters that release Rb vapour. Hence, the first chamber is flooded with 87 Rb vapour in order to readily capture the atoms using a MOT. 87 In the MOT chamber, a current of approximately 2.2 A is run across the dispensers. This activates a chemical reaction causing the rubidium dispenser to release hot rubidium gas flooding the chamber with both 87 Rb and 85 Rb. In this chamber the MOT is created and subsequently a purely magnetic trap is loaded using a pair of trapping coils which lie outside the cylindrical shaped chamber. When the getters are on, the recorded pressure is usually P = 7 × 10−10 Torr. For these kinds of pressures the MOT will suffer a loss rate caused by collisions with the background gas. With this in mind, background collisions not only limit the MOT densities, but they also greatly limit the ability to confine atoms in a purely magnetic trap. We will explore how to solve this problem in Sec. 2.5. 2.3. INCREASING THE NUMBER DENSITY 2.3 37 Increasing the number density Challenged with the problem of limited phase space density available in a MOT, we seek to find an alternate method to increase the phase space density of the trapped 87 Rb. One way to achieve this increase in phase space density is to dramatically lower the temperature of the system. A standard technique used to decrease the temperature of dilute samples like 87 Rb to produce BEC is evaporative cooling. Evaporative cooling is an equivalent process as that involved in cooling a cup of coffee. In coffee, the fastest molecules are the hottest molecules which are already in a gaseous state. When air is blown over a hot cup of coffee, the fastest molecules are forced away from the thermal ensemble. The fastest molecules are the most energetic molecules in the sample, so by removing them, the average energy is decreased and the system is no longer in thermal equilibrium. After a while, the coffee’s thermal distribution equilibrates but at a lower average temperature. If we keep blowing on the cup, this process repeats itself until the coffee is in thermal equilibrium with the surroundings and in the end we have managed to substantially reduce its temperature. An important aspect of evaporative cooling is the ability to hold on to the atoms while performing the evaporation. For this reason it is important to first load a purely magnetic trap or “cup” in which to perform evaporation. During the evaporative cooling of 87 Rb atoms, we use special techniques that remove the most energetic atoms from our magnetic trap. The average energy of the remaining atoms is lower, causing the temperature to drop. If we do this enough times, we can reach the critical temperature, causing the atoms to form a condensate. All of this assumes that BEC is achieved before the number of atoms in the trap runs out. As we can see, one of the downfalls of the evaporation is the inherent loss of atoms. In light of the loss of atoms, we aim to initially load a purely magnetic trap with as many atoms as possible. That way we will not run out of atoms before reaching the critical temperature. Because the atoms loaded into the magnetic trap are in turn loaded from an initial MOT, we seek to have a MOT with large number of atoms NA . The higher the number of atoms, the higher the initial density right before evaporating. Above all, since evaporating will always require a loss of atoms, a MOT with high NA will mean a condensate with a large number of atoms. Although a MOT configuration will not yield the appropriate phase space density (see Eq. (1.9)) to achieve BEC, it is a very useful mechanism by which to slow the atoms enough to load them into a purely magnetic trap. Once loaded into a magnetic “bowl” evaporative cooling can take place, see Fig. 2.9. The next section describes the experimental steps taken to load the magnetic trap and how and why we transfer the atoms to he UHV region to perform evaporative cooling. 38 2.4 CHAPTER 2. MAKING BEC Loading a Magnetic Trap Evaporative cooling is an essential step in the process of making BEC because it allows us to reach the necessary phase space densities to reach condensation. In turn, the cooling technique requires a mechanism which will allow us to hold on to the atoms while we perform evaporation. Normally trying to hold on to neutral atoms is non-trivial. Because they are not charged (like e.g. ions) it is not possible to use electric fields and their forces to suspend them. Another possibility is using laser forces. Nevertheless, as mentioned in the previous section, there are heating factors which are not trivially overcome. A solution to this problem can be obtained by suspending neutral atoms via their spin magnetic moment in a purely magnetic trap. This is our motivation to load a purely magnetic trap of 87 Rb atoms and physically transfer it to a region where the pressure is low enough to perform the evaporation. With this in mind, it becomes important to recall the basic interaction between the magnetic field B and the atom’s total magnetic moment µm due to the total angular momentum of the atom. See Sec. 2.1.1. To motivate how to obtain the energy due to this interaction we can think of having a magnetic field in the z direction which selects the z component of the angular momentum operators in equation (2.3). If the energy shift due to the field is small compared to the hyperfine splitting, then mF becomes a good quantum number. Also, in many occasions the atomic spin will follow the external magnetic field, and we choose the quantization axis to be along the direction of the field so that Bz is in fact just the overall magnitude of the field B(r). Deriving the final expression for the energy requires subtleties not be addressed here (due to its length), although a full derivation can be found in [13]. In this way the energy due to an external magnetic field can be written as: Umag = µB gF mF B(~r) ~ (2.33) It should be noted that for a potential like this, the normally degenerate mF states within a particular F manifold will become split. The splitting will occur according to the Landé g factors for each F level. This splitting has already been discussed with Eq. (2.5) in Sec. 2.1.1 and Eq. (2.30) in Sec. 2.2. In order to obtain the force that an external B field exerts on the atoms we take the gradient of the potential using F = −∇U (r) so that Fmag = − µB gF mF ∇B(r). ~ (2.34) Equation (2.34) shows that an external magnetic field can be used to trap atoms if an appropriate B(r) configuration is found. In our experiment we start with a simple spherical quadrupole field configuration which was initially suggested by 2.4. LOADING A MAGNETIC TRAP 39 Wolfgang Paul [38]. His contributions were later applied to ion traps and successfully used in 1985 to trap neutral atoms [39] using magnetic fields. The design of such a configuration can be motivated as follows: for a magnetic field which is symmetric in x and y, the derivatives along these two directions should be the same. Above all, the field should also satisfy Maxwell’s equation ∇ · B = 0. Applying these two constraints we get: ∂B ∂B 1 ∂B ·i= ·j=− ·k ∂x ∂y 2 ∂z (2.35) In order to satisfy Maxwell’s condition, the derivative of Bz must be twice the value and opposite in sign to those of x and y. In this regard, it is not hard to see why the equation below yields the appropriate symmetry configuration for a spherical quadrupole field when approximated for small |r|. A cross-section in the x = 0 plane for the field expressed below can be seen in Fig. 2.3. x y B(r) = B 0 (zk − i − j ) 2 2 2.4.1 (2.36) Compressed MOT We use a quadrupole field like the one shown in Eq. (2.36) to trap atoms from a MOT. In order to do so without loosing a lot of phase density we must carry out an extra step, creating a compressed MOT or CMOT. The aim of this step is to increase the density of the atoms before they are captured by the purely magnetic trap. For this purpose the CMOT stage includes, an increased red detuning for the main trapping beams and decreased power of the re-pump beams. A higher magnetic field gradient means that the confining forces occur at smaller radius from the center of the MOT, compressing the atoms more, achieving higher densities. Higher detuning from resonance decreases the scattering rate, reducing the optical density of the outer atoms, allowing the trapping light to penetrate deeper into the core of the MOT, cooling more effectively. Reducing the power of the re-pump means more atoms will remain in the 52 S1/2 F = 1 ground state making less atoms sensitive to the trapping light, further increasing the ability of atoms at the core of the MOT to be compressed by the light. The disadvantage of using a CMOT stage is its decreased loading rate, so we do not have it on for very long. 2.4.2 Optical pumping The third stage in creating a BEC is to optically pump the 87 Rb atoms into the appropriate hyperfine state for loading the magnetic trap. In our case, we use the atoms in the F = 2 manifold of the ground state 52 S1/2 . Specifically, we want to have a magnetic trap that is populated by atoms in the | F = 2, mF = 2i hyperfine 40 CHAPTER 2. MAKING BEC state. Using a decreased power in re-pump frequency during the CMOT stage leaves most atoms in the dark | F = 1i ground state. In order to get atoms out of this state we apply a short (∼ 1) ms pulse of re-pump light in addition to circularly polarized “pumping” light. The re-pump light is to provide a mechanism for atoms in the | F = 1i state to end up in the | F = 2i ground state (Section 2.2). The circularly polarized light is tuned to the F = 2 → F 0 = 2 transition. In addition, we have an appropriately chosen magnetic field which makes the circularly polarized light σ + . This light not only drives transitions from the | F = 2i state to the | F 0 = 2i, but changes the m0F value by +1 upon absorption of the photon to the excited state. When spontaneous emission causes the atom to decay to the | F = 2i ground state, the atom can change its mF state such that ∆mF = 0, ±1. If ∆mF = 1 upon decay, then the next time it absorbs a σ + photon it will also change its m0F value by one. Over many cycles, the atoms will end up in the | F = 2, mF = 2i state, corresponding to the state with maximum mF . The atom’s final state is such that it cannot absorb any more σ + photons. In other words, the atom is trapped in a “dark state”, becoming insensitive to the light and unable to transition into any other state. The final result consists of atoms populating the desired state. 2.4.3 Switching The Magnetic Trap On In order to finally transfer the atoms into a purely magnetic trap without losing much phase space density it is important to set the correct trap strength so that atoms neither expand nor compress non-adiabatically after the optical pumping stage. To capture the atoms we set the correct initial trap strength by choosing the appropriate B field gradient. After the atoms are caught, we adiabatically ramp the field gradient to the desired final strength. By catching the atoms at the correct B field gradient, sloshing of the atoms in their new trap due to the non-adiabatic jump in the potential can be avoided. Finding the correct gradient is done by matching the average cloud size after the optical pumping stage to the cloud size of the initial magnetic trap. Additionally, we use the temperature during the optical pumping stage, which is measured to be 200 µK. The B field near the center of the trap (which is lined up with the center of the MOT) can be approximated as linearly dependant on the coordinates, such that Umag (r) = µB 0 r. Hence the radius of the atom cloud in the magnetic trap can be found by equating the thermal energy of the atoms ∼ kb T , to their potential energy in the magnetic trap and solving for the radius at this energy. Consequently, the gradient of the field is set by matching the radius of the atoms in the magnetic trap to the atoms in the optical pumping stage. In our case we have found B 0 = 124 G/cm. Finally, after the magnetic trap has been loaded, the gradient of the field is ramped up adiabatically to its maximum value of 387 G/cm. This will give us the necessary densities for evaporative cooling. See Table 2.1 for a list of B field 2.5. TRANSFERRING ATOMS Stage 41 Detuning [Mhz] MOT CMOT Optical pumping Load magnetic trap Magnetic trap ramp -15 -28 Magnetic Gradient Bz0 [G/cm] Time 10 13.5 0 124 100 → 387 1 × 104 30 1 50 500 [ms] Table 2.1: Summary of stages leading up to the pureley manetic trap. settings at different loading stages. Additionally, we measure the 87 Rb atoms in the compressed magnetic trap to have a temperature of T = 800 µK. In order to create the quadrupole field shown in Eq. (2.36), two coils made out of copper tubing were placed outside the glass vacuum chamber. The coils were aligned on their azimuthal axis as shown on Fig. 2.5. We applied dc currents of opposite direction through each coil, and an anti-Helmholtz configuration was achieved. The field gradient used in order to hold the atoms and perform evaporative cooling, was of 387 G/cm. Each coil was built out of 1/4 inch outer diameter copper and had a total of 16 turns. The outer radius of the coil structure measured 122 mm and the inner radius was 45 mm, making the average radius 83.5 mm. To obtain the maximum field strength desired, the coils had to endure a current of 750 A at a resistance of 17 mΩ. At these currents the pair of coils dissipated approximately 12 KW of power. In order to dissipate the generated heat, a supply of chilled water flowed through the copper tubing at a rate of 1.25 l/min [21]. Additionally a water flow and temperature interlock were set up (appendix A) to prevent water vapour build up in the coils which could cause hazardous situations involving overheating explosions. 2.5 Transferring Atoms When the getters which provide 87 Rb are on, the measured pressure inside the chamber is Pmot = 3 × 10−10 Torr. At these pressures, the background particles will be constantly colliding with MOT atoms, ejecting them out of the MOT. Although atoms trapped in the MOT are lost to background collisions, the MOT can coexist in the previously mentioned pressures because the lasers continuously refill it with newly cooled atoms. However, atoms lost due to background collisions in a pureley magnetc trap will not be replenished, thus greatly reducing the lifetime 42 CHAPTER 2. MAKING BEC Figure 2.6: (a) The quadrupole coils start at the MOT side of the chamber where the magnetic trap is loaded. (b) Trapped atoms are moved across a thin tube 1cm in diameter for a distance of 54.3 cm. (c) The trapped atoms arrive at the science cell and are positioned on the center of the waveguide structure. We use the waveguide structure in conjunction with the quadrupole coils to generate the TOP. of the trapped atoms. The measured life time for the magnetically trapped atoms in the MOT chamber is τmot = 4 s. Unfortunately, the lifetime of the magnetically trapped atoms we obtain is not long enough to perform evaporative cooling. The evaporative cooling technique relies on atomic collisions which redistribute the energy of the trapped atoms, see Sec. 2.2. This process of re-thermalization can take several seconds, e.g 10-15 s. If the evaporation is carried out faster than the atoms’ ability to re-thermalize, then we would lose all the atoms before ever reaching the desired critical temperature Tc . For this reason, we first load the magnetic trap from a MOT in the chamber containing 87 Rb vapour. Afterwards, we transfer the magnetically trapped atoms to a second ultra high vacuum chamber. In this chamber the pressure is Psci = 4×10−11 Torr, meaning background collisions are much lower and the lifetime of the magnetic trap is considerably extended. We denote this second chamber as the science cell, and measure the lifetime of the atoms in the magnetic trap to be τsci = 80 s. As a result, we can hold on to the atoms long enough to perform evaporative cooling. Specifically, the chamber used in our experiment consists of two separate glass 2.6. LOADING A TOP TRAP 43 cells joined via a thin tube, see Fig. 1.6. The first cell, where the MOT is created, is cylindrically shaped, with a diameter of 63.85 mm and a length of 260 mm. The thin tube connected to one of the ends of the MOT chamber is approximately 1 cm in diameter and 35 cm in length. It separates the chambers enough to allow for a large pressure differential between the two chambers. Equally important is the second cell known as the “science cell”. It is box shaped with a length, width and height of 330 mm, 81.2 mm and 52.2 mm respectively. Following the scheme by Lewandowski et al. [10], we use a programmable translation stage which supports the coils for the magnetic trap loaded in the first chamber. After ramping the magnetic trap’s field to its maximum value, we proceed to move the coils towards the second chamber, moving the atoms via the thin tube into the UHV region, see Fig. 1.6. The translation stage has a track allowing a total displacement for the quadcoils of 600 mm. The total distance the atoms must be translated is 543 mm. In particular, the stage is programed to follow a motion with three stages. First is a stage accelerating the atoms from rest. Second is a constant velocity period, and finally a deceleration stage brings the atoms to their final position in the science cell. More details of how the programmable moving station is operated can be found in Jessica Reeves’ thesis [21]. Because our ultimate goal is to create a condensate interferometer, we require a magnetic trap in which we can manipulate the motion of the atoms. For this purpose, we have created a specially designed magnetic waveguide which traps the atoms but allows them to easily move in one dimension. This trap is analogous to a optical fiber, which confines light in all but one direction. The technical details and operation of the guide will be discussed in the following sections and chapter 3. Because of this requirement, another important function for the science cell is housing the magnetic waveguide. We translate the quadrupole coils until the atoms are located in the center of the guide structure. By performing the evaporation in the center of the guide structure we take advantage of the bias fields that can be generated from it (see Fig. 3.1) to create a TOP trap as described in Sec. 2.6. 2.6 Loading a TOP trap Although evaporative cooling is a very effective technique in reducing the temperature of the trapped atoms and increasing the density, it causes a large loss of atoms (as will be explained in the next section). Losses also occurr due to stray light and RF fields which pump the atoms into untrapped states. We can limit the amount of unwanted stray RF fields and laser light causing loses by shielding the science cell. Moreover, the quadrupole field configuration described in Eq. (2.36) suffers from a loss of atoms at the zero of the field. 44 CHAPTER 2. MAKING BEC When a magnetically trapped atom with velocity ~v finds itself near the zero of the field, its interaction with the magnetic field is lost momentarily. As the atom traverses this region, the atom could undergo a non adiabatic transition where its mF value changes sign, emerging at the non zero region of the field with an opposite anti-trapping force. This is called a Majorana transition [40, 41]. A change in sign of the mF quantum number is equivalent to an inversion of the magnetic spin, causing the atom to be ejected from the trap. The lifetime of the atoms in the magnetic trap due to Majorana losses is given by [42]: 1 τm = ασF2 W HM 4 (2.37) in which α = 3.7 × 104 s/cm2 is determined experimentally [42] and σF W HM is the full width half max of the atom cloud in the trap. We can model the cloud of atoms as having a Gaussian density distribution of the form: µ ¶ x2 y2 z2 n(r) = n0 exp − − − (2.38) wx wy wz where n0 is the peak number density, and wx = wy = 2wz = w0 is the width of the symmetric Gaussian distribution. We can relate the width of the Gaussian function to its full width half max using σF2 W HM = 4w02 ln 2. Therefore, the expression Eq. (2.37) can be rewritten in terms of w = 1.8w0 , the width of the actual cloud (which is not non-Gaussian) if modeled by a Gaussian density distribution. This yields the following expression for the Majorana lifetime: ³ w ´2 = w2 × 80 s/mm2 (2.39) τm = α ln 2 1.8 Loss of atoms via Majorana spin flips can be greatly reduced by applying a technique known as the time orbiting potential or TOP [43, 44, 42]. In summary the technique consists of shifting the zero of the field from the center of the trap and then rotating it. As a result, the time dependent zero creates a path where the atoms leave the trap known as the ellipse of death. Specifically, we can describe the functioning of the TOP trap by calculating the time dependent field and then averaging it over time. Mathematically the ellipse of death can be derived as follows. First introduce a bias field at origin (Fig. 1.6) where the center of the spherical quadrupole is located after the mechanical translation stage. We denote the oscillation frequency as Ω, B0 = B0 [cos(Ωt)i + sin(Ωt)k] . (2.40) This can be combined with a quadrupole field Bq of the form given in Sec. 2.4 to yield the following total field: Bq + B0 = B0 (cos(Ωt)i + sin(Ωt)k) + B 0 (2zk − xi − yj ) BT OP = (B0 cos(Ωt) −B 0 x)i +(B0 sin(Ωt) +2B 0 z)k −(B 0 y)j (2.41) 2.6. LOADING A TOP TRAP 45 Figure 2.7: Diagram A shows an atom in the mF = 1 state approaching the center of the field corresponding to a trapping potential given by U (r) = µB gF mF B(~r)/~. In diagram B the atom goes through the zero, loses its spin information and transitions to a mF = −1 state where it experiences an anti-trapping potential U (r) = −µB gF mF B(~r)/~. Undergoing the Majorana transition, the atom is ejected from the trap. By using Eq. (2.41) one can obtain expressions for the path where the field is zero, substituting xe , ye , ze into BT OP and setting it to zero, one can solve for the coordinates where the atoms can escape the magnetic trap via Majorana spin flips. Using the form of Eq. (2.41) it is simple to obtain independent expressions for x, y and z. For the y direction the result reveals ye = 0 and the circle or in this case ellipse of death lies in the x, z plane. For the x and z direction we obtain: xe = B0 cos(Ωt) B0 ze = B0 sin(Ωt) 2B 0 (2.42) The set of equations (2.42) describe a point which moves in time along a parametrized ellipse. If the frequency of rotation is faster than the atom’s ability to follow the zero adiabatically (the oscillation frequency of the atoms in TOP, ωx = 2π × 78 Hz, ωy = 2π × 110 Hz and ωz = 2π × 156 Hz) they experience a time averaged potential rather than an instantaneous potential. It is important not to oscillate the field faster than the Larmor frequency of the atoms ωl = µb B0 /~ = 14 MHz, which determines how fast their spin precesses around the magnetic field. Doing so would mean the atom’s spin cannot follow the field’s direction adiabatically. Extending the size of the ellipse of death larger than the atom cloud by controlling the currents which yield B 0 and B0 , minimizes the loss rate from Majorana flips. 46 CHAPTER 2. MAKING BEC Figure 2.8: Cross section in the z, x plane of the region around the origin defined in Fig. 1.6. Using superposition, the vector fields of Bq and B0 are added, offsetting the original position of the zero in Bq denoted by the black arrow. By time varying the currents in the trap structure that generate B0 , the position of the zero is rotated, following the ellipse shown above parametrized by the equations for xe and ze 2.6. LOADING A TOP TRAP 47 The actual time averaged field the atoms experience can be calculated by integrating the magnitude of the total field over one full cycle and dividing by the oscillation period of the field. Denoting θ = Ωt, the time average becomes a function of θ: Z 2π 1 h|B|it = |B(θ)|dθ (2.43) 2π 0 By squaring each component we can obtain the magnitude of the total TOP field as: |BT OP | = [B02 +B 02 (x2 + y 2 + 4z 2 ) − 2B0 B 0 x cos(Ωt) + 4B0 B 0 z sin(Ωt)]1/2 Expanding the square root of the equation above the time average gives: µ B 02 1 2 h|Btop |it = B0 + x + B0 4 (2.44) to second order and calculating 1 2 y + z2 2 ¶ (2.45) which yields a quadratic dependence in the magnitude of BT OP . Plugging in ~ T OP |. Eq. (2.45) into Eq. (2.33) one can obtain an expression for U in terms of |B Ignoring any constants that introduce offsets to the energy, the atoms are trapped on average by a harmonic potential of the form 1 UT OP = m(ωx2 x2 + ωy2 y 2 + ωz2 z 2 ) 2 (2.46) This allows us to extract by comparison the values for the trap’s oscillation frequencies, 1 µB 02 µB 02 µB 02 ωx2 = ωy2 = ωz2 = 2 (2.47) 2 mB0 mB0 mB0 As shown in this section, a magnetic trap consisting of a spherical quadrupole field and an appropriately chosen bias field can be used to trap atoms minimizing the Majorana loses. In the experiment we turn on the TOP trap when the evaporative cooling process has removed enough atoms that the size of the atomic cloud has shrunk to the point where it lies inside the ellipse of death. At this stage, T = 85 µK and the density at the center of the trap is high enough that the Majorana losses are no longer a negligible loss in the evaporation process. As previously explained (Sec. 2.7), evaporative cooling relies on the slow re-thermalization of the atoms in the trap, which in turn relies on the density of the atoms. Minimizing the loss of atoms in the trap during evaporation is a crucial requisite to achieve BEC. To help with the focus of this discussion, I summarize the key steps in the process of loading a condensate into a magnetic waveguide. First we make a MOT where the measured temperature is at T = 800 µK and NA = 4 × 109 . Second we make a compressed MOT, reducing the temperature to T = 400 µK and keeping the 48 CHAPTER 2. MAKING BEC Stage T [µK] NA MOT CMOT Optical Pumping Quadrupole Quadrupole Transfer Quad in Science cell Evaporation BEC 800 400 400 800 900 0.2 4 × 109 4 × 109 2 × 109 2 × 109 1.5 × 109 2 × 104 Note Atoms end in | 2, 2i state catch at 124 G/cm ramp 124 V → 387 V From MOT to Science cell TOP on TOP on Table 2.2: Summary of major steps towards achieving BEC. The voltages shown reflect the setting on the power supply driving the spherical quadrupole coils. same number of atoms. Third, we introduce an optical pumping stage where the atoms appear in the | 2, 2i state. Fourth, the pure magnetic trap is turned on at the appropriate level to catch NA = 2 × 109 atoms. The coils are then ramped to provide the maximum gradient and achieve densities necessary for evaporative cooling giving T = 800 µK. Fifth, the atoms are transferred using the translation stage to the science cell and positioned inside the waveguide structure. At this stage there are NA = 1.5 × 109 atoms at T = 900 µK. Sixth, we commence evaporative cooling. Additionally, during the evaporation, we turn on the TOP field in order to reduce Majorana losses. We reach critical temperature at Tc = 200 nK and produce a condensate with NA = 2 × 104 . 2.7 Evaporative Cooling Evaporative cooling was briefly introduced at the end of Sec. 2.3 but a more detailed explanation behind the cooling mechanism will be discussed in this section. Evaporative cooling, as its name suggests, works by evaporating away (thus removing) hot atoms from the sample you are trying to cool. The principle behind this technique is analogous to the way a coffee cup is cooled when a current of air blows over the surface of the coffee. Because temperature is just a measure of the average energy of the particles, repeatedly removing the most energetic atoms reduces the temperature of the coffee substantially. See Sec. 2.3. The same technique can be applied to atoms in a magnetic trap which is analogous to the coffee cup and can be thought of as a “magnetic bowl”. After optically selecting the Rubidium atoms in the | 2, 2i ground state, loading them into the mag- 2.7. EVAPORATIVE COOLING 49 netic trap and transferring them to the evaporation region, we apply an RF field on to the atoms using an antenna. The RF is tuned to a range of frequencies that drive the mF → mF − 1 transition for atoms trapped in the magnetic potential. Depending on the exact energy of the photons in the RF field, atoms that posses the appropriate potential energy will absorb a photon. If the atoms absorb a RF photon, then they transition into a untrapped state and no longer form part of the original ensemble. In this context, the appropriate energy corresponds to the atoms that have a potential Umag which tunes the atom to the transition with frequency difference ∆ν = ∆mF µB gF |B|/~, where ∆mF = 1 (see Fig. 2.9). The RF radiation field can be tuned so only the atoms with sufficient potential energy are resonant with the mF → mF − 1 transition. Because the magnetic field is spatially dependent, it makes the transition spatially dependent as well. If this is the case, then only the atoms which are the furthest away from the center of the trap will undergo the transition. This is because the more energetic an atom is, the further it can reach out in the magnetic potential. Therefore, atoms which are distributed spatially on the outer surface of the cloud will be ejected. If the RF frequency only removes the outermost atoms from the atomic cloud, then it acts like the “lip” of a bowl where only the atoms which are at the top can escape. In fact, the technique involves lowering the “lip” in order to progressively remove the hottest atoms until Tc is obtained. For an effective cooling technique the evaporation needs to be done at an appropriate rate. The speed of evaporation will be limited by the the ability of the sample to equilibrate thermally. Ultimately this depends on how energy is transferred within the atoms by their collisions/interactions [45, 46]. For this reason, high collision rates between atoms improve energy transfer between them and thus improve possible evaporation rates. Sweeping down the RF field is analogous to lowering the lip of the magnetic trap, allowing only the hottest atoms to escape. It is some times called an“RF knife” which “chops” off the high velocity atoms from the Maxwell-Boltzmann thermal distribution. For this process to be effective, the atoms that are left in the trap must collide with each other and redistribute their kinetic energy among other atoms, returning close to thermal equilibrium. During the process we do not wait for the atoms to fully equilibrate as this would take too much time. Instead, we continuously ramp down the frequency removing at each instant the hottest atoms. In doing so, the atoms reduce their average velocity and consequently lower their temperature, see Fig. 2.10. The time it takes for the sample to stay close to thermal equilibrium limits how fast evaporative cooling can be performed and sets the time scale for the process. An important parameter required to perform evaporative cooling is the minimum energy of the magnetic trapping potential given by gF µB0 . Knowing the minimum 50 CHAPTER 2. MAKING BEC Figure 2.9: An RF field is incident upon the atoms in the magnetic trap driving the | 2, 2i → | 2, 1i → | 2, −1i → | 2, −2i transitions which are equivalent to a spin flip where mF → m0F = −mF . The frequency of the radiation is ramped down exponentially according to Eq. (2.48), at a rate slower than the re-thermalization rate, but faster than the loss rate due to background collisions and 3 body loses. 2.7. EVAPORATIVE COOLING 51 Figure 2.10: (a) Maxwell Boltzmann probability distribution for thermal atoms in terms of the velocity v where hv 2 i ∼ T . The dotted line represents the RF knife, removing the highest energy atoms down to those having Umag = hν where ν is the RF frequency. (b) As the distribution approaches thermal equilibrium, T decreases, and the RF knife is swept lower. (c) The distribution tries to approach equilibrium once again but the RF knife is lowered more. The result is a substantial drop in the temperature of the sample. 52 CHAPTER 2. MAKING BEC energy of the trap will let us know the lowest energy RF field we can apply to the atoms in order to drive a transition. It is also a parameter used to program the ramp into our experimental apparatus, in this case, the pulse sequence regarding evaporation, see appendix C. To calculate the bottom frequency of the magnetic trap, we simply equate the energy of the incoming photon to the energy corresponding to the minimum value of the magnetic field B0 . Hence ν0 = gF µB B0 /~2 . The RF sweep is described by the following exponential ramp model which is used in the evaporation sequence. The final frequency as a function of time is given in terms of the bottom frequency ν0 , the initial ramp frequency νi and the time constant τe as: νf (τ ) = (νi − ν0 )e−t/τe + ν0 . (2.48) In order to carefully control the ramp down for the frequency of the RF field incident on the atoms, we lower the the frequency ν in a series of sub-steps Table 2.3. Each sub-step consists of smaller frequency changes, covering a particular frequency range. For our experiment 4 different ramps covered the entire range of the frequency sweep needed. Also, the sub-steps are useful because we can determine the loss rate due to evaporation by measuring the number of atoms before and after a sweep sub-step. A typical sequence of evaporation steps towards BEC in our experiment is described in Table 2.3. For example, the second line starts the ramp at 30 MHz and ends it at 10 MHz, uses a time constant of τ = 4 s, a power of -15 dBm and the bottom frequency of the ramp is set to 2.55 MHz. See Eq. (2.48) for the functional form of the ramp. Starting with magnetically trapped atoms at T = 800 µK, we begin the evaporation ramp with ν = 60 MHz and perform several evaporation ramps like those in Table 2.3. BEC is achieved at νf = 0.18 MHz, using various time constants for each evaporation sub-step. Unfortunately, there are atom losses through the zero of the magnetic trap which complicate the evaporation sequence. Inspecting Eq. (2.36) it is evident that the quadrupole magnetic field in which the atoms are trapped has a zero. This is a problem for magnetically trapped atoms because when they cross the B = 0 point, the spin of the atom is unable to follow the change in B. Consequently the atom may find itself anti-aligned and thus ejected from the trap because the magnetic force is reversed, Eq. (2.34). As a result, the trap has an effective leak of atoms which we need to plug. To solve this problem we turn on a time varying field resulting in a TOP trap (Time Orbiting Potential) as explained in Sec. 2.6. Briefly, the TOP trap consists of a rotating zero for the field, which the atoms cannot catch up to. The path of the rotating zero is labeled “the circle of death”. This special technique helps out by 2 For the spherical quadrupole field in Eq. (2.36) the minimum is 0. However, this will not be the case when we use the TOP trap to eliminate Majorana loses, see Sec. 2.6 2.7. EVAPORATIVE COOLING 53 νi [MHz] νf [MHz] τ [s] p [dBm] ν0 [MHz] 50 30 30 15 12 6 -13 -13 0 0 Table 2.3: A typical evaporation instruction set sent to the RF generator from the real time controller. For this instruction there are two ramps. See appendix C for the complete set of evaporation instructions used in the experiment. The power set here goes to a 50 dBm amplifier before reaching the RF antenna. effectively plugging the undesired leak, uncompromising the number of atoms left to make BEC. The starting size of the atomic cloud in the magnetic trap is larger than the maximum size for the circle of death. Because of this, the TOP trap is turned on in the sequence when the size of the cloud drops below that of the circle of death, Fig. 2.8. Because the circle of death expels atoms from the trap, we can take advantage of this effect and use it as another “lip” to expel atoms. For this reason we start RF evaporating from 50 to 15 MHz, and then stop. Next, we turn the TOP trap on and gradually reduce its radius, expelling some hot atoms and reducing the temperature. Finally we resume the RF evaporation from 1.85 MHz to 0.18 Mhz but using the TOP field as an aid to prevent a loss of density in the trap. Another complication when performing evaporation is that it cannot be done too slowly. The upper time limit or slowest rate at which the evaporation can be done is set by maintaining an adequate balance between the number of atoms lost due to evaporation and those lost via background collisions and three body collisions. Three body collisions cause atoms to form molecules which are no longer held by the trapping potential. Similarly, ejection of atoms from the trap due to stray RF fields and light are counted as part of the background loses. The total loss rate not including evaporation is given by: RL = Rbackg + R3body (2.49) where Rbackg ∼ 1/80 s−1 , R3body = G3 n2 depends on the number density n and we use the measured value of G3 = 1.8 × 10−29 cm6 /s [47]. In the end, using the evaporative cooling technique, we have successfully achieved BEC’s having Na = 1 × 104 atoms starting with a magnetic trap containing Na = 1 × 109 atoms. The drop in atoms from initial loading of the magnetic trap to the creation of BEC is quite dramatic but it is the price paid to obtain the critical density required for condensates. Figure 2.12 shows 3-D absorption images3 in false 3 imaging system will be explained in Sec. 2.8 54 CHAPTER 2. MAKING BEC color taken after the final RF ramp down for different values of stop frequency νf . The first image is before critical temperature is achieved, the second at critical temperature and the final image shows a full BEC. 2.8 Imaging In general, a large portion of the measurements leading up to and including the interferometer experiment involve imaging the atoms. Usually the imaging is used to find out the number of atoms NA and the temperature T , allowing us to derive from these other physical properties of our trapped atom clouds (e.g. the collision rate). For example, in the stages prior to the implementation of the BEC interferometer, measuring T and nλ3t are crucial components to ensure the production of condensed atoms. These physical properties are calculated from the raw data obtained in the images of the atom cloud. The successful operation of the BEC interferometer requires measuring the number of atoms after all its operations are finalized. For this reason, the explanation presented in this section will focus on the atom clouds obtained after the interferometer operation. However, a detailed discussion of the methods used to obtain NA , T and the physical properties derived from these prior to the measurement of interferometer’s output state is given in [21]. It is important to note that all imaging done in the harmonic trap (in the science cell) is performed the in the same way. We need to be able to image Bose-Einstein condensates. In our experiment, the size of these clouds are on the order of tens of microns. For this reason we need an imaging system that magnifies these small objects and has high resolution, allowing us to mathematically analyze the signal captured in the image. Additionally in the condensate, approximately 104 atoms will scatter light from a few 100’s of µW at 780 nm. We use a technique called absorption imaging to create a picture of the atoms. This technique consists of shining a near-resonant probe beam in the region where the atoms are contained. The probe beam should pass through the atoms and possess a beam waist which is larger than the atom cloud. In our case the waist of the probe beam needs to cover an area several mm2 in order to probe non-condensed clouds. After the light exits the region of the atoms, it is redirected into a camera. Because the light is near the resonant frequency of the atoms, the light is absorbed by the atoms, leaving a shadow against a bright background. Mirrors and lenses are then used to direct and image this light onto the camera. The atoms appear as dark regions within the area of the probe beam. To perform temperature measurements we use ballistic expansion. This technique consists of letting the atomic cloud free fall from the magetic trap and taking pictures of its expansion at several time intervals. We then plot the widths as func- 2.8. IMAGING 55 tions of time and fit the expansion to a quadratic form. Then we extrapolate the temperature from the fit parameters obtained. Before flashing the probe beam, the atoms are released from the magnetic potential holding them in place. This means that the atoms drop up to 2 mm before the image is captured by the camera. Consequently, the imaging system includes a lens mounted on a micrometer to adjust the focusing if the image plane of the atoms changes. The magnification of the system is controlled using a 2× or 5× microscope objective. The camera we use is an Apogee, model AP47 CCD. Also, the binning of the pixels in the CCD was varied between a 3 × 3 pixel block and a 1 × 1 pixel block. The 1 × 1 binning permitted a higher resolution but increased the download time of the images for data acquisition. The download time of the images varied from 3 s to 26 s (depending on the binning and array size). When taking pictures of condensates, we mainly used the 5× objective and the 1 × 1 binning, producing images like those in Fig. 4.8. The absorption image is derived by processing three distinct raw images. The first image is denoted as the “atom image”, hence it is taken with the probe laser beam going through the atoms creating the shadow effect described. The second is a picture without any atoms present or probe light coming into the camera. This image captures the background light coming into the camera and is therefore labeled the “background image”. Finally, we take a picture labeled the “no atoms image” which captures the light with the probe beam going through without any atoms present. The idea is to simulate the lighting when the probe is on, to later normalize the atoms image. The resulting processed image is obtained as follows: S(x, y) = atoms image − background image no atoms image − background image (2.50) Each image consists of a 2-dimensional array of values representing the intensity of each pixel on the CCD. We assume the transmission of light through the region of the atoms is given by e−α (beer’s Law), where α(x, y) is the 2-dimensional absorption profile of the atom cloud. Using the 3 images described above we write an expression which relates the processed image to the absorption profile of the atoms: S(x, y) = e−α(x,y) (2.51) In turn the absorption profile α(x, y) is assumed to take form of a Gaussian function such that: h 2 2 − x−xa − y−ya α(x, y) = A + B exp ( wx ) ( wx ) i (2.52) where A is an offset allowing for power variation in the probe, B is the peak absorption coefficient, wx , wy are the widths, and xa , ya are the center of the absorption profile. The image is fit using a special program developed in Matlab discussed in App[?] called AI 3. 56 CHAPTER 2. MAKING BEC It is important to mention that due to the expansion, the density of the atoms is decreased, lowering the absorption coefficient B. In many instances the processed image is over-saturated, meaning that the absorption signal by the atoms is very high because the probe is too close to resonance. This means that the true absorption profile of the image will be hidden, yielding inaccurate widths. Consequently, the temperature measurement is incorrect. For this reason, we normally allowed the cloud to expand until the image did not look saturated having a typical absorption coefficient B between 0.2 and 0.5. Aditionally, oversaturation has the effect of flattening the shape of the absorption profile, hiding the true density profile of the atoms. 2.9 Calculating NA To calculate the number of atoms in the wave packets of the output state, we can use the absorption profile α(x, y) and the number density function n(x, y, z) of atoms in the trapping potential in which they are found. A full calculation of how NA is obtained for the condensate atoms is given in [21]. However an outline of how to get NA assuming a Gaussian distribution for the number density will be given here. We start with the expression which gives the the absorption α(x, y) in terms of the number density of the atoms in the waveguide n(x, y, z). Z α(x, y) = σ n(x, y, z) dz (2.53) where σ is the scattering cross section for the atoms. The integral over z indicates summing the absorption over the thickness of the cloud. In our case z represents the vertical direction. For illustrative purposes we assume that the number density n(x) has the form of a three dimensional Gaussian. · ¸ x2 y2 z2 n(x) = n0 exp − 2 − 2 − 2 (2.54) wx wy wz R If the n(x) is normalized such that NA = n d3 r, then we can carry out the integration and solve for n0 to obtain the peak density for n(x) n0 = NA x wy wz (2.55) π 3/2 w Carrying out the integral of n(x) with respect to the coordinate z we obtain an expression which can be used to get α. Z − NA exp n dz = πwx wy y2 x2 2 + w2 wx y (2.56) 2.9. CALCULATING NA 57 However, we need an expression for σ. We will not derive σ, nevertheless we will use the result obtained in [21] σ0 ΓΓ0 σ = 02 Γ + 4∆2 (2.57) to get an expression for α. Finally we combine σ with Eq. (2.56) to obtain: NA σ0 ΓΓ0 α0 = α(xa , yb ) = 02 Γ + 4∆2 πwx wy (2.58) We have chosen the point (xa , ya ) which yields the maximum absorption α0 . The variable α0 is precisely the fit parameter B in Eq. (2.52), which allows us to introduce a measured parameter into the result for NA . Finally we solve Eq. (2.58) for NA . In the end we obtain an expression for NA in terms of the experimental observable α0 NA = 4π 2 × α0 (Γ02 + ∆2 )wx wy 2.8λ2 ΓΓ0 (2.59) where Γ0 is the observed broadened linewidth, see [21]. In the specific case of the condensate modeled using the Thomas-Fermi aproximation, from [45, 21] we obtain the following expression for NA using the method described above. NA (condensate) = 2πα0 wx wy 5σ (2.60) Inspecting the above equation, we use α0 = B, wx , wy and σ to obtain N . Hence we use the program AI 3 to obtain these fit parameters to get the final result. The image processing before carrying out the fit was done with a script program written to obtain Eq. (2.50). In order to facilitate the image processing, we took one background image per day which was repeatedly used by the script. It is important that we kept the exposure time of the atoms and no atoms image the same in order for the processed image to normalize correctly. We used short 30 µs probe flashes at an intensity of a few µW’s to take the images. As a result, we obtained an imaging system which performed effectively. The imaging system is illustrated in Fig. 2.11. 58 CHAPTER 2. MAKING BEC Figure 2.11: Diagram representing the optics used to create the imaging system to perform absorption imaging. The microscope objective could be swapped, allowing us to choose between the 5× and 2× objective. Additionally, to account for any changes in the image plane of the atoms (hence a change in the z position of the atoms), we have a lens mounted on a micrometer to re-adjust the focus of the image back onto the plane of the CCD. 2.9. CALCULATING NA 59 Figure 2.12: Three different absorption images of the atoms in the TOP trap in false color. The vertical direction denotes higher absorption thus higher density of atoms, the remaining axes are the x and y position in the trap. Each picture has a corresponding stopping frequency denoting the lowest RF frequency reached during evaporation. From left to right, stopping evaporation at 2.95 MHz shows a cold atom cloud on the verge of condensing, atoms start condensing at a stopping frequency of 2.90 MHz with some atoms still un-condensed, finally stopping at 2.77 MHz most atoms are Bose-condensed in the lowest state possible of the magnetic trap. Chapter 3 Magnetic Waveguide To begin this chapter, it is worth mentioning that much of the motivation, design considerations and characterization of the interferometer trap for the waveguide are provided in the thesis project presented by Jessica Reeves in [21]. Our goal is to create a one dimensional BEC interferometer where we can control the relative phase of the arms to control the output state. Keeping in sight this objective, we need to figure out how to effectively control the motion of the condensate and perform splitting and recombination operations common to most interferometers. Moreover, we must optimize the potential in order to reduce the introduction of unwanted phase shifts and support the atoms against gravity. For these purposes we have designed a magnetic trap which provides the necessary confinement in the x and z directions (see Fig. 1.6) but permits motion along the y, allowing us to implement the interferometer. Given that we must reduce unwanted phase shifts, it is important to understand the main mechanisms which cause them. One of them is the interactions between atoms confined in the waveguide. In brief, the interactions between atoms will cause the arms of the interferometer to develop an extra phase which will modulate the overall interference pattern of the output state. This modulation will result in a decrease in contrast of the interference pattern proportional to the number density of atoms in the trap and the propagation time of the waves. Chapter 5 will explain this effect in more detail. In this regard, a potential with stronger confinement will compress the atoms more, resulting in higher number densities. Therefore reducing the confinement strength of the potential will greatly increase the contrast and maximum propagation time of our device. Additionally, it is important to avoid any asymmetries in the trapping potential. In general, if one arm of the interferometer experiences a different trapping potential, hence a different potential energy, a relative phase shift will develop between the arms. We seek to have no development of a relative phase shift as a direct result of the propagation of the waves. One way to achieve this is to perform the experiment in a trap that is perfectly symmetric, but this proves unrealistic. Usually there 60 3.1. LOADING A WAVE GUIDE 61 are fringe effects and imperfections in the shapes and materials making up a trap, limiting their symmetry. For this reason, we can set up an interferometer sequence where both arms will acquire the same phase shift after all the motion is completed. In a one dimensional case, this can be done by allowing each wave to travel both arms of the interferometer, see Ch. 4. As a result, our magnetic trap design should include minimal confinement along the x and z directions, along with as little confinement in y as possible. This will allow for one dimensional propagation of the atoms. These characteristics point to a very weak trap in general. However, the atoms must be suspended against gravity. For this reason, we must carefully balance the gravitational potential with the magnetic potential along the z direction. This ensures the atoms do not fall out of the trap. This will be addressed in Sec. 3.3.2. A more detailed account of the experimental procedure utilized to produce and load the condensate into the waveguide can be found in Reeves et al. [48]. Details of the Adwin sequences used to make BEC and load the waveguide are given in appendix C. 3.1 Loading a Wave Guide We use a 4-rod copper structure located in the science cell (Fig. 1.6) to generate the rotating bias field for the TOP trap that is used during evaporative cooling. Additionally, the copper structure is used to generate the magnetic fields used in the atomic wave guide. A detailed description of how these fields are created using the trap structure will be discussed in the following sections. In summary, concentric to the 4 rods are tube-like insulators containing another 4 rods which are used to generate a linear quadrupole field for the atom waveguide. To load the guide, we adiabatically ramp down the TOP trap’s quadrupole field (the field provided by the coils described in Sec. 2.4.3) while the waveguide field is turned on, allowing the condensate to adiabatically position itself into the atomic wave guide. After the quadrupole coils are off, the guide remains on. 3.2 3.2.1 Magnetic Trap Conventions and Set Up The origin of the coordinate system used to describe the magnetic fields generated by the trap structure is located at the center of the trap structure. Figure 1.6 shows the location of the trap relative to the two glass chambers, while Fig. 3.1 zooms into the science cell providing a more detailed perspective of the trap structure, its components and the coordinate system used. The trap structure is mounted onto a set of 33 cm long copper block leads that conduct current to each individual circuit 62 CHAPTER 3. MAGNETIC WAVEGUIDE Figure 3.1: A different view of the science cell, with the trap structure visible through the glass chamber. The thin tube connects to the MOT chamber. The center of trap structure is aligned to the thin tube, which allows the mechanically transferred atoms to arrive as close as possible to the minimum of the waveguide trap. The coordinate system used to describe the waveguide fields is centered on the trap as shown. in the trap. In turn, these leads are connected to a 4 − 3/4” con-flat feed-through with 8 pins, which correspond to the 4 independent circuits available in the trap structure. One end of the science cell uses several cylindrical sections made of different types of glass in order to gradually transition into a glass-metal seal. The additional glass required to make the seal adds an extra 20 cm of length to the chamber. The chosen length of the trap is set by the necessity to accommodate for the glass metal transition. A top and side view of the trap in conjunction with the leads is shown in Fig. 3.2. A pair of y-coils whose axes are aligned to the waveguide axis are also visible. These are to provide optional confinement along the y direction if necessary. The geometry of the trap consists of 4 visible rods forming a 5×1.5×1.5 cm3 box region. When viewed from the side, each rod is centered on and lies perpendicular to the corner of a 1.5 × 1.5 cm2 square, see Fig. 3.3. The trap structure consists of four 5-cm copper rods (Fig. 3.3). Each rod is actually a compound structure consisting of an outer copper tube (5 mm in diameter, 1 mm thick wall) containing an alumina insulating tube, itself containing a copper wire. The alumina tube has 2.4 mm outer diameter with a 0.8 mm wall making room for a 1.6 mm inner wire. The outermost tube is made out of oxygen-free, highconductivity copper to minimize its electrical resistance. As shown in Fig. 3.4, the 3.2. MAGNETIC TRAP 63 Figure 3.2: Top image is a side view of the magnetic trap structure including leads that provide current to generate the fields for the waveguide. Bottom image is a top view of the structure. Eight copper pins (of which five are visible) are connected to the leads via a custom made feed through mounted on a 43/4” con-flat flange. The pins connect to the copper leads corresponding to four independent circuits. At the right end of the structure, the “y” coils which provide confinement along the “y” direction are visible. conductors are connected in three independent circuits. A fourth circuit consisting of a pair of coils is located perpendicular to and on each side of the rods. One circuit consists of the four outer copper tubes that create a linear quadrupole field. Two other circuits are made up of oppositely paired inner rods that generate the bias field. Finally, the fourth circuit connects the two y-coils visible on Fig. 3.2 in an anti-Helmholtz configuration for confinement along y, but it is omitted for clarity in the figures. This circuit was not used in the work presented here. Having a total of four independent circuits means there are eight total connections to be made. These connections correspond to eight pins. Five pins are visible in Fig. 3.2, extruding from the vacuum chamber through the con-flat feed through. The assignment of circuits to each pin is summarised in Table 3.2. 3.2.2 Superimposing Magnetic Fields A motivation for the main considerations of the waveguide design used for our interferometer were discussed at the beginning of this chapter. Two key factors to take into account are the need for a weakly confining waveguide in order to decrease the effects of interactions, and the need for a field strong enough to suspend the atoms against gravity. A weak field provides weak confinement, but if it its too weak, the atoms will fall. In light of these contradicting requirements, we developed 64 CHAPTER 3. MAGNETIC WAVEGUIDE Figure 3.3: Mechanical model of the trap drawn to scale. Four horizontal copper tubes 50 mm in length and 5 mm in outer diameter with a 1 mm wall provide the quadrupole field. Inside each tube are alumina insulator tubes which surround an inner conductor consisting of 1.6 mm diameter copper wire which provide the bias fields. The tubes, insulator and wire are supported on a pair of boron nitride blocks which in turn support the copper leads which supply the current to the rods and wire. The right block is depicted transparently to show the connections. 3.2. MAGNETIC TRAP 65 Figure 3.4: Three of the circuits included in Fig. 3.3 have been separated to demonstrate their spatial configuration and current flow. On each diagram the wires extending in/out of the page represent the leads which supply the current. Diagrams (a) and (b) represent the thin wires inside the insulators with their respective currents which provide the bias fields according to Fig. 3.6. Diagram (c) represents the outer conductor and the corresponding current flow which provides the linear quadrupole field shown in Fig. 3.5. The loops in the ends help cancel any residual axial fields. 66 CHAPTER 3. MAGNETIC WAVEGUIDE a novel solution. A good candidate for the choice of field to make a waveguide is a quadrupole field similar to that explained in Sec. 2.4 which possessed symmetry about the axis in which we seek to guide the atoms (y). This can be achieved by using a linear quadrupole field having a cross-sectional form just like the one depicted in Fig. 2.3. However, instead of having cylindrical symmetry about the z axis (like Eq. (2.36)), it has linear symmetry along y. In other words a (x, z) cross-section of the field at any point in y looks identical to the field depicted in Fig. 2.3. Once again we are faced with the loss of condensate atoms via Majorana spin flips at the zero of the field. But we can implement a rotating bias field to make a TOP similar to that described in Sec. 2.6. In fact, we use a linear quadrupole field as described above in conjunction with a bias field that can offset the zero of the field. We implement a technique similar to the TOP trap but with a modification to suit our interferometer. In addition to rotating the bias field, like the case of our TOP to perform evaporative cooling, we vary the linear quadrupole in time. The currents in all the circuits oscillate with a specific phase relationship (see Eq. (3.4)). This causes the zero of the field to oscillate in a plane above the atoms. Therefore, they are constantly attracted to the zero overhead, allowing us to lower the confinement further than that allowed by a conventional TOP set up. We use the basic principle of vector superposition to construct a mathematical model which describes the magnetic waveguide used in the interferometry experiments. 3.3 3.3.1 Generating the Time Averaged Potential Total Field Approximation The operation of our trap can be mathematically described by starting with the expression for an oscillating linear quadrupole field. As can be seen from the expression below, there is no y dependence in the equation. Hence the x, z cross-section of Bq at every y does not change, a characteristic important in obtaining a waveguide axis along that direction. Bq = Bq0 (xi − zk) cos(Ωt) (3.1) To create the above field, we use circuit (c) seen in Fig. 3.4, which controls the current through the four copper tubes of the trap structure generating the field in Fig. 3.5. Because the tubes which generate the quadrupole are finite in length (i.e. 5 cm), there are fringe effects which introduce y dependence to the field. These effects, although small, are addressed in Sec. 3.4.1. In order to offset the zero of the field, we use a bias field similar to that described in section 2.6. Achieving a bias field at the location of the atoms along the waveguide 3.3. GENERATING THE TIME AVERAGED POTENTIAL 67 Figure 3.5: A cross section looking from the right side of the trap centered on the waveguide axis, shows the quadrupole field generated from the four copper tubes. The four copper tubes are shown and highlighted to denote current through them. The direction of the current flow is shown in Fig. 3.4 (c). axis requires that we use two of the circuits available in the trap structure. We use circuit (a) in conjunction with circuit (b) (Fig. 3.4) to generate a field with fixed magnitude pointing in the −i direction. Looking from a side perspective (down the y direction from the right in Fig. 3.4) on circuit (a) and (b), we obtain a view for two pairs of diagonally opposed rods as seen in Fig. 3.6. We can use the well known result for a concentric magnetic field produced around a current conducting wire to construct the total bias field [49]. In Cartesian coordinates, the field due to a single wire carrying current Isw is: · ¸ µ0 Iw −(z − z0 ) (x − x0 ) Bsw = i+ k (3.2) 2π (x − x0 )2 + (z − z0 )2 (x − x0 )2 + (z − z0 )2 where z0 and x0 establish the position of the wire in the z, x plane and Isw is the current carried by a single wire and µ0 is the permeability of free space. We can superpose four fields, each represented by Eq. (3.2), having their respective centers located at the position of the wires seen in Fig. 3.6. Accordingly, is not hard to see how the resultant bias field near the origin is produced for circuits (a) and (b). Using the configuration in Fig. 3.6 for equal magnitude currents through the wires of circuits (a) and (b), we obtain two perpendicular bias fields. One points in the k − i direction for circuit (a) and another in the −k − i direction for circuit (b). By sinusoidally oscillating the current for each bias field and having a π/2 phase shift between them, the direction of the total bias field will rotate in time causing the zero of Bq to rotate as depicted on Fig. 2.8. 68 CHAPTER 3. MAGNETIC WAVEGUIDE Figure 3.6: A cross section looking from the right side of the trap centered on the waveguide axis, shows the two bias fields generated from the copper wires. For each field, the corresponding pairs of wires carrying currents are highlighted. The direction of the current flow is shown in Fig. 3.4 a, b. In general, with a particular choice of currents, adding the two fields produced by circuits (a) and (b), yields the bias field1 : B0 = B0 [sin(Ωt)i + cos(Ωt)k] (3.3) As discussed in Sec. 2.6, the rate at which we oscillate the fields must be faster than the atomic motional frequency (10 Hz) but slower than the Larmor frequency of the atoms ωl = µb B/~ ∼ 10 MHz. This is to prevent the atoms from catching up to the field’s zero (avoiding Majorana flips), but still have their spins adiabatically follow the orientation of the field. It should be noted that noise oscillations much faster or slower than the rate of rotation of the field tend to cancel out. For these reasons the 1-100 kHz range is adequate. Furthermore, as explained in Reeves’ thesis work [21], a noise spectrum of the laboratory was analyzed in order to choose the most appropriate frequency of oscillation. The noise data revealed that within the 1 − 100 kHz range, the lowest average noise was around 10 kHz. Taking into account the avoidance of noise peaks observed in the data, we choose the rotation frequency of the field to be Ω = 11.88 kHz, see [21]. Next, we calculate the total magnitude of the waveguide field Bw = Bq + B0 and 1 In practice the equation for B0 does not correspond to the correct field obtained at t = 0 having both bias circuits on with the same current. However Fig. 3.6 shows the correct configuration obtained at t = 0. Choosing B0 in this way makes the calculation of the average potential of the waveguide simpler. 3.3. GENERATING THE TIME AVERAGED POTENTIAL 69 obtain: |Bw | = {B02 + Bq02 (x2 + z 2 ) cos2 (Ωt) + Bq0 B0 [cos(Ωt) sin(Ωt) − cos2 (Ωt)]}1/2 Bq0 2 = B0 {1 + (x + z 2 ) cos2 (Ωt) B0 Bq0 + [cos(Ωt) sin(Ωt) − cos2 (Ωt)]}1/2 (3.4) B0 square root of the above expression using the expansion √ Approximating the 1 + ² ≈ 1 + ²/2 − ²2 /8 and preserving up to second order terms, we obtain: Bq02 2 |Bw | = B0 + (x + z 2 ) cos2 (Ωt) − Bq0 z cos2 (Ωt) 2B0 ¤ 1 Bq02 £ 2 − x cos2 (Ωt) sin2 (Ωt) + z 2 cos4 (Ωt) 8 B0 3.3.2 (3.5) Calculating the Time Average To calculate the time average as defined by Eq. (2.43) it is useful to know the following quantities given below. Note that we have used the same definition θ = Ωt: hcos2 θiθ = hsin2 θiθ = 1/2 hcos4 θiθ = hsin4 θiθ = 3/8 hsin2 θ cos2 θiθ = 1/8 (3.6) (3.7) (3.8) Using the results presented above, we finally obtain an expression for the timeaveraged magnitude for the field used as the interferometer’s waveguide: Bq02 1 h|Bw |it = B0 − Bq0 z + (3x2 + z 2 ) 2 16B0 (3.9) The potential energy including gravity for the atoms in the waveguide becomes Uw = µb h|Bw |i + M gz ³ µb Bq02 µb ´ (3x2 + z 2 ) = µb B0 + M g − Bq0 z + 2 16 B0 (3.10) (3.11) where M is the atomic mass, g is the acceleration due to gravity and µb is the magnetic moment for 87 Rb in a particular hyperfine state. We want to counteract the effect gravity has on the potential. By setting Bq0 = 2M g/µb we can cancel out the second term in the above equation and obtain the following 2-D harmonic potential 1 (3.12) Uw = µb B0 + M (ωx2 x2 + ωz2 z 2 ) 2 70 CHAPTER 3. MAGNETIC WAVEGUIDE where we identify the trapping frequencies as µ ¶1 3M g 2 2 ωx ωx = (3.13) and ωz = √ . 2µb B0 3 Using a bias field with a magnitude of 20 G for 87 Rb atoms trapped in the | 2, 2i state, the waveguide exhibits trapping frequencies ωx = 2π × 5.3 Hz and ωz = 2π × 3.0 Hz. Because the linear quadrupole and bias fields are independent of the y direction, the potential calculated does not have any y dependence. This is a limitation in the model describing the waveguide because there are imperfections in the trap structure that yield non-zero contributions in the y direction for Bw . However, the model presented above gives a clear and intuitive picture of a potential which confines the atoms weakly in the x and z directions. At the same time, the potential preferentially allows the atoms to move along the y direction, achieving the function of a channel or guide for the atoms in this direction, hence the name waveguide. 3.4 Design Limitations 3.4.1 Curvature Along “y” Because the rods and tubes of the trap structure are finite in length and they are connected on their side to conducting leads which supply current, the waveguide field suffers from variations from the mathematical model calculated in section 3.3. Taking into account every possible correction would be a daunting task, but we improved our basic model with one that incorporates some variations in the quadrupole and bias fields. For the quadrupole field, there can be an extra term that takes into account any gradient field in the j direction as follows Bq = (axi + cyj − bzk) cos(Ωt) (3.14) where c = b − a in order for Bq to satisfy Maxwell’s equation ∇ · Bq = 0. Including also variations in the bias field parametrized by coefficients α, β and γ, one can approximate the total field by using the procedure described earlier for calculating the time average and obtain [21]: µ ¶ 1 3 2 h|Bq |it = B0 − bz + a + αB0 x2 2 16B0 µ ¶ µ ¶ 1 2 1 2 2 + c + γB0 y + b + βB0 z 2 (3.15) 4B0 16B0 The associated oscillation frequencies for the corrected trapping potential are recognized by comparing them to a harmonic potential form as ¶¸ 21 · µ 2 2µb 3a + αB0 ωx = M 16B0 3.4. DESIGN LIMITATIONS 71 · ωy = · ωz = 2µb M 2µb M µ µ c2 + γB0 4B0 ¶¸ 21 b2 + βB0 16B0 ¶¸ 21 To this end, we made a numerical calculation of the total field using the BiotSavart law. It calculated the field at every point taking into account the leads of the trap structure and its finite size. We later fit this model to the form expressed in Eq. (3.15) and obtained values for the parameters a, b, c, α, β and γ. The values from the fitted model for each parameter (in terms of the respective currents) are given in [21]. 3.4.2 Trap Characterization After the production of the condensate in the science cell we load it into the magnetic waveguide. The loading consists of a series of steps which ramp down the quadrupole magnetic field which makes up the TOP trap in conjunction with steps which ramp up the fields which make up the waveguide. In general, transferring the condensate involves reducing the strength of the external quadrupole field, which reduces the oscillation frequencies of the TOP mentioned in Sec. 2.6. Before the confinement of the TOP field is totally lost, the linear quadrupole field of the waveguide is turned up to obtain the weak trapping frequencies in Eq. (3.13). A detailed description of the the ramps involved in the loading can be seen in Fig. 3.7. In order to minimize residual oscillations after the loading (which are detrimental to the interferometer operation (Sec. 5.6)) we try to make the ramps slow so that the condensate follows the changing magnetic fields adiabatically. To characterize the waveguide, we measured its frequencies of oscillation along x y and z. In the x and z directions we observed and measured the oscillation for the center of mass of the condensate. We used absorption imaging to track the position of the cloud, and then plotted it in time. In the y direction we observed and measured oscillations of the semi-major axis of the condensate. In other words we measured the breathing mode of the condensate. Again, we used absorption imaging to track the size of the cloud along y as a function of time. We later made a plot of the position y vs. time. For all cases x, y and z, we fit the data to a damped sine function and extracted the oscillation frequencies. More details and the results obtained for the frequencies are given in [21]. 3.4.3 Trap Oscillations We initially recorded oscillations of up to 200 µm in amplitude of the condensate upon loading it to the magnetic waveguide. We noted oscillations in the x, y and z 72 CHAPTER 3. MAGNETIC WAVEGUIDE Figure 3.7: Ramps for different magnetic fields during the loading of the waveguide. The vertical axis indicates the control voltage for the labeled magnetic field, see appendix C. (a) B0 the bias field. (b) Bqw the waveguide quadrupole. (c) Bq the external spherical quadrupole. (d) Initial ramp is not to scale, actual time is 10 s. The last evaporation occurs after this ramp. Evaporation takes 9 ms and is not shown. (e) Exponential ramp is not to scale. Ramp takes an approximate of 4s to complete with an exponential decay constant of 800 ms. 3.5. MEASURING THE MAGNETIC FIELD 73 directions. Initially we thought these were a product of vibrations of the mechanical trap structure described in Fig. 3.4. To investigate this possibility we watched the structure with a camera and monitored its motion with an optical interferometer which used a mirror that was mounted on the structure. The oscillation amounted to less than 1 µm in amplitude (∼ 10× smaller than the condensate itself), thus we determined that motion from the trap structure was not responsible for the condensate oscillation in the waveguide. In the end we fixed the oscillation problem by optimizing the loading sequence (Fig. 3.7). It is important to note that we initially also observed a large displacement of the condensate along the y direction upon its loading to the waveguide [21]. The condensate moved approximately 2 mm in the process of ramping down the quadrupole coils. This was caused by a misalignment in the minima of the TOP trap and the waveguide. However we re-adjusted the position of the quadrupole coils at their final position in the science cell, and realigned the minima. This solved the problem of the condensate displacement during loading. Additionally, we observed (by taking pictures of the condensate at rest in the waveguide) that the minimum of the waveguide varied after some time. Initially we thought that the shift was due to thermal effects in the waveguide structure. However we tracked down this effect and concluded it was a shift in the tilt of the optical table which shifted the rest position of the condensate. We realized the pneumatic system responsible for floating the table was under-pressured, allowing random shifts in position. We solved this problem by increasing the system’s pressure. It is very important to consider any motion of the condensate when loading it to the waveguide. Before beginning the interferometer operations, it is beneficial for the condensate to be at rest. Having a condensate with v = 0 m/s means the subsequent splitting reflection and recombining operations explained in Chapter 4, will work more effectively, making interference measurements possible. 3.5 3.5.1 Measuring the Magnetic Field Connections and Field Directions To properly implement the circuits available in the magnetic trap structure shown in Fig. 3.3, it is important to know which current to apply and how to make the necessary connections. As shown in Fig. 3.2, the trap structure is supported by copper leads which in turn are connected to a series of pins. These pins extrude to the outside of the evacuated chamber using a con-flat feedthrough. The pins are grouped in four pairs corresponding to each circuit available to the trap structure. This section documents in detail how the trap structure circuits are configured to each pin and what fields are obtained given a particular choice of currents. Figure 3.8 maps out the pins to their respective trap circuit. Table 3.1 briefly describes the direction of characteristic features that each individual field exhibits. Additionally, 74 CHAPTER 3. MAGNETIC WAVEGUIDE Figure 3.8: A bakeable feed-through is mounted on a 4 − 3/4” con-flat flange connecting eight copper pins to the trap leads. See Table 3.2 to match up corresponding circuits. The arrow indicates the upright direction for the trap structure. The trap is mounted with one of the leads (which is neutral) shown in Fig. 3.2 facing up. to properly connect the magnetic trap and obtain the desired waveguide fields, the polarity of the pin connectors and the corresponding field direction are summarized in Table 3.2. 3.5.2 Field Gradient & Magnitude It is important to document in detail the calibration of the waveguide’s various magnetic field strengths to the current applied on each of the trap’s four circuits. This will enable us to properly configure the control voltages, function generators and amplifiers used to drive current through the connector pins in Fig. 3.8. To summarize the operation of the trap in dc mode (using dc currents), we describe key parameters of the magnetic fields that are obtained using the settings described in Table 3.2. We describe in table Table 3.3, the calibration of the gradients and magnitude of the fields with respect to the current applied. It is important to mention that this calibration was done by running the trap’s circuits at 25 A dc. A small probe was used to measure the three different directions x, y and z for four different fields. It was adapted correctly in conjunction with a 3-dimensional translator to properly measure the magnetic fields. While the trap structure was not under vacuum, it was held in a fixed position using an aluminum stand which in turn was bolted to an optics table. The tip of the 3.5. MEASURING THE MAGNETIC FIELD 75 Type of field Formula Quadrupole Field ~ q = B10 [−xi + zk] B ~1 = B Bias Field 1 ~2 = B Bias Field 2 End caps Field B1 √ [k 2 B2 √ [−i 2 − i] − k] ~ endc = α(z)k + β(x)i + (α + β)yj B Table 3.1: The trap structure contains four independent circuits which provide four fields described above. This table describes the name of the fields available and their corresponding mathematical formula pin 1 8 2 4 6 5 7 3 polarity + + + + - description k−i Field Bias 1 −k − i Bias 2 −xi + zk Quadrupole i+k Endcap Coils at y = 0 plane Table 3.2: Each circuit available in the waveguide has a corresponding pair of pins. The table above shows the characteristic feature of the field obtained for each circuit given the polarity applied to each corresponding pair of pins . 76 CHAPTER 3. MAGNETIC WAVEGUIDE formula ~q = B Bi0 (x − x0q )i + Bii0 (z − z0q )k ~ 1 = B1i i + B1ii k B ~ 2 = B2i i + B2ii k B ~ endc = α(z − z0 )k + β(x − x0 )i + (α + β)(y − y0 )j B parameter measured value Bi0 Bii0 x0q z0q B1i B1ii B2i B2ii α β x0 y0 z0 -1.82 G/mm 1.79 G/mm -2.78 mm 2.14 mm -6.84 G 7.07 G -7.08 G -7.62 G 0.19 G/mm 0.29 G/mm 3.60 mm 2.64 mm 5.55 mm Table 3.3: The equation for each field available on the trap structure is given corresponding to the polarities in Table 3.2. Additionally, experimentally measured field parameters are provided. All measurements were taken by applying a 25 A dc current. The coordinate system used to describe fields is noted in Fig. 3.1. probe was positioned in the center of the waveguide structure denoting the origin, see Fig. 3.1. Its starting location (the origin of the coordinate system used to measure the fields), was carefully recorded by positioning the point of a needle right next to the tip of the probe. Initially, the probe’s Hall sensor was positioned horizontal to the table to measure the z component of each field. Then, using the translator, the probe was scanned throughout the volume enclosed by the rods of the trap. Data points were taken at 1 mm intervals with the aid of a computer for recording the data. After this was done, the probe was rotated and re-centered, enabling it to measure another component of the field. This was done for the remaining i and j components. 3.5.3 End cap coils At the moment we do not make use of the end cap coils found on either side of the waveguide rods which provide axial confinement along the y axis. Originally, we planned to use them to provide the force required to turn around the condensate atoms during interferometry, but we have opted to not use a magnetic field to turn around the condensates. Instead, we use off-resonant Bragg scattering in a series of pulses to control the 3.5. MEASURING THE MAGNETIC FIELD 77 motion of the condensate in the wave guide. Using the off-resonant beam has proven to be successful in implementing the interferometer. In the future the end-cap coils could be used to perform experiments where the atoms turn around due to the curvature along the guide axis as an alternative to the reflection pulse described in Sec. 4.3. As shown in the previous sections, the waveguide potential does posses curvature along y due to the finite size of the trap’s copper rods. This curvature could be asymmetric in the region where the atoms travel during the interferometer sequence. Therefore, it can add unwanted relative phases between the arms of the interferometer. Hypothetically, a set of external coils could be used to create an opposing field which cancels out unwanted fields. Moreover, if you have independent control of the coils, there would be flexibility in the type of cancelling field you could generate. Applying different currents to different coils would yield different strength fields on each side of the waveguide. 3.5.4 Preparing for Interferometry At this point it is important to remember that one needs to consider the alignment between the minimum of the TOP trap provided by the spherical quadrupole (which determines the atoms’ position after evaporation), and the potential minimum of the waveguide. A misalignment can cause unwanted oscillations for the condensate after loading the waveguide. Having curvature along the y axis means that there could be a misalignment between the minimum in the TOP and the minimum along y of the waveguide. We cannot do much about this problem, however we move the final y position in the science cell of the spherical quadrupole field in order to align minima. Similarly, there could be a mismatch in the minimum of the TOP and waveguide along the x direction. But we can move the atoms further (or less) down the track along x until the minima are matched along x. Finally, there could be a mismatch in the minima along z. However to our advantage we can control the minimum of the waveguide along the z by varying the strength of B0q . In this way, we can try to better match the minima along z and reduce unwanted oscillations. In addition to the techniques mentioned above, we developed a slow set of ramps (including a final exponential ramp) to“ease” the condensate into the waveguide, reducing oscillations in the waveguide after the loading process (Fig. 3.7). We will analyze in detail the interferometer operations and their experimental verification in Ch. 4. But at this stage it is important to mention that loading the condensate into the waveguide proves to be a crucial step in our experiment. The effectiveness of subsequent steps like the splitting, reflection and recombination of the condensate heavily depend on any residual motion after the loading of 78 CHAPTER 3. MAGNETIC WAVEGUIDE the waveguide. We found out that as we relaxed the TOP trap by reducing the gradient of the spherical quadrupole field, its trapping frequency crossed the 60 Hz value. There are many sources of stray noise at this particular frequency in the laboratory, hence they induced the condensate to oscillate after we crossed this frequency. To solve this problem, we finished the evaporation sequence such that the bias field for the TOP trap ended at a higher value. Because ωi2 ∼ Bi02 /B0 (the i denotes the different spatial coordinates) for the TOP, we chose a final B0 that would make ω lower than 60 Hz. In his way after we performed the final ramp down of the TOP quadrupole gradient during the loading, the atoms would never experience a potential with a frequency of 60 Hz. Consequently the atoms’ motion would not resonate with the background noise at ∼ 60 Hz. By performing the evaporation as described above, we aim to achieve as little residual motion as possible after the atoms are first loaded into the waveguide. Chapter 4 Interferometry Techniques Atom interferometers are amazingly sensitive devices. In general, atoms have stronger interactions with forces available in the laboratory setting when compared to photons. For example, atoms readily interact with electromagnetic and gravitational fields, whereas light does not. For this reason, interferometers using atoms as a wave source have the potential to substantially outperform those using light. In particular, atom interferometers used for precision measurements would have a much improved sensitivity. For example, interferometers can be configured to perform gyroscopic measurements. Using a Sagnac configuration which encloses an area A and rotates with angular velocity Ω, the change in phase is given by: 4π A· Ω (4.1) λv in which λ is the wavelength of the photon or atom and v the velocity of the particle being used. For an atom travelling at velocity v the wavelength is given by the de-Broglie relation λa = h/mv. In the case of photons travelling at c = 3 × 108 m/s, the wavelength is given by λl = 2πc/ω. By substituting the corresponding values of wavelength for visible light, mass for a 87 Rb atom and the velocity for atoms and light into Eq. (4.1), the ratio of sensitivities in each case yields: ∆φ = ∆φa mc2 = ≈ 1011 . ∆φl ~ω (4.2) At best, this would represent the largest theoretical gain in sensitivity for an atom based interferometer. In practice, achieving such an increased gain in sensitivity will be a difficult task. Among the best examples of experiments which use the increased sensitivity of atoms is the Sagnac atom interferometer developed by T.L. Gustavson et al. [50]. It has achieved rotation sensitivities of 2 × 10−8 (rad/s)/Hz, equivalent to those obtained by the best laser gyroscopes. Therefore improving sensitivities in atom interferometers promises significant enhancements in these sensory devices. Other examples of interferometry using thermal atoms are [25, 24, 23]. 79 80 CHAPTER 4. INTERFEROMETRY TECHNIQUES Figure 4.1: Atom beam interferometers cannot achieve large deflection angles due to the high velocity of the beam, typically atoms move at 290 m/s. This diagram depicts the small arm separation a = 54 µm obtained. Our design can improve this limitation increasing a to a = 250 µm. Nevertheless, interferometers using light do pose certain key advantages over their atomic counterparts. In general the experimental manipulation of photons is more simple than that of atoms. For example the deflection and positioning of light beams is easily achieved by using simple optics, typically mirrors and lenses. In fact, the use of optics permits light interferometers to achieve arbitrary deflection angles which permit the enclosure of large areas and thus become useful in cases like that of Eq. (4.1). Similarly, large deflection angles can allow large arm separation, which can then allow individual access to the arms. In contrast the interferometer implemented by Gustavson et al. uses an atom beam with a velocity of 290 m/s. Due to the high velocity of the beam, it becomes hard to control the direction and overall motion of the atoms, which makes it hard to achieve large deflection angles. This limits the area that can be enclosed, hindering the application of a Sagnac sensing interferometer. Arm separations up to 54 µm (with 17 µm width beams) have been demonstrated in [51]. Up to date, the largest packet separations have been achieved in experiments like [52, 53], obtaining up to 13 µm using optical traps and magnetic traps in [54]. Equally important, interferometers using light have a supply of photons which is orders of magnitude larger than most atomic sources. Hence the rate at which you can produce an output signal is much higher. This significantly improves the signal to noise ratio which then increases accuracy in the measurements of the phase shift. In our experiment we chose to use Bose-Einstein condensates as a coherent source because it resolved some limitations inherent to atomic beam interferometers, but still provided the advantage of using highly sensitive atoms. In light of this, it is important to highlight some of the main advantages BEC interferometers have over interferometers using thermal atoms. In the laboratory, condensates are usually produced at temperatures close to absolute zero. As a result, condensates can be thought of as stationary when com- 81 pared to thermal atoms having velocities in the order of 100 m/s. For this reason, manipulating the motion of the condensate requires very small forces. Similarly, this allows for large deflection angles which are useful as mentioned earlier. This is not the case for thermal beams. Another key advantage is that condensates are sources of highly coherent matter waves. As discussed in chapter 1, condensates are spatially coherent across their entire length, meaning typical coherence lengths are ∼ 100 µm. When performing an interferometer measurement, an interference pattern will only be seen if the difference in path length is equal or less than the coherence length of the condensate. On the contrary the coherence length for a beam of atoms is given by the de Broglie wavelength. For a beam of Cesium atoms travelling at 290 m/s the de Broglie wavelength is tens of pm which is much smaller than the coherence length of condensates. For this reason, the difference in path lengths allowing measurable interference will be greater for condensed atoms. From another perspective, all the atoms in a condensate are in the same state of the potential trapping them. This makes them analogous to a laser whose photons are all all in the same state. In contrast, a high velocity beam of atoms has a wide velocity spread, meaning that the atoms are in multiple translational states, making them analogous to a beam of white light. Consequently, condensates will experience longer coherence lengths in comparison to atomic beams, much like the longer coherence lengths of lasers compared to those of white light. Furthermore, interferometers using thermal beams of atoms obtain their arm separation by inducing transitions to the internal states of the atom. Usually when measuring the output state, the populations of different internal states are recorded. In turn, these depend on the relative phase of the arms. For this type of splitting, the relative phase of the arms is sensitive to the phase of the laser. This will introduce decohering effects to the output state if there is any noise in the laser. Considering our particular experiment, the low velocities of a condensate greatly facilitate the implementation of the Michelson type configuration we use. Additionally, low velocities can be exploited to obtain large wave packet separation and hence a larger area to enclose. The larger area advantage should further motivate the study of BEC in its application to interferometry. Other examples of BEC in interferometry are given in [22, 55, 44, 56, 53, 52, 57, 12]. Starting with a condensate at rest enables us to easily split it in two and obtain clouds moving apart in one dimension. Moreover, we have been able to fully separate the wave packets from each other such that each can be observed as a separate entity. With this in mind, we will refer to the distance which separates the center of each individual atom cloud as the arm separation. In this way the arm separation is directly related to the actual wave-packet separation. It should be noted that in most atomic beam experiments the arm separation is attributed to the separation of the center line of each beam (therefore, the arm separation can be smaller than the resulting beam widths). However in many cases, the matter waves(beams) never 82 CHAPTER 4. INTERFEROMETRY TECHNIQUES fully separate from each other; therefore the packets do not fully separate. As a result of these advantages, we have been able to obtain macroscopic arm separations which have great potential in many applications where access to a single arm of the interferometer is essential. Current atom interferometers have limited individual arm accessibility, hindering experiments where large arm separations are necessary, see Fig. 4.1. With this purpose in mind, we seek to implement an interferometer that has atomic sensitivity with a motion control that permits large arm separation. 4.1 Interferometer Operation Our main objective is to create a one dimensional interferometer where the condensate moves along the axis of the waveguide described in Sec. 3.3. The magnetic wave guide is an analog of an optical fiber confining photons in two dimension. The operation of the interferometer is described as follows. First, after the condensate is loaded into the waveguide at y = 0, we apply an off-resonant standing light field with vector k to split the atoms into two clouds, giving them an initial symmetric momentum kick in the y or −y direction of the waveguide. This puts the condensate in a quantum superposition of two translational states corresponding to the momenta ±2~k. The atoms propagate for some time, each covering a maximum spatial amplitude y = ±d. We then apply a second off-resonant standing wave to reverse the motion of each wave packet. We let the packets propagate crossing each other at y = 0. When they reach the maximum separation distance y = 2d, the off resonant pulse is applied a third time to reverse the motion once more. Finally, when the wave packets overlap for the second time at y = 0, the off resonant standing wave is used to bring the atoms back to rest. See Fig. 4.4 and 4.6 for illustrations of these operations. The physics of how all these processes take place is explained in Sec. 4.2 and Sec. 4.3. To create the off-resonant standing wave we use a second diode laser beam, that we refer to as the Bragg beam. The Bragg beam is detuned −7.8 GHz from resonance and enters the science cell from the −y direction through the magnetic waveguide structure along the waveguide axis (the y-axis). After the Bragg beam exits the waveguide and science cell, a mirror retro-reflects it to yield a pair of counter-propagating beams which generate the standing wave used for splitting and reflecting the condensate. Figure (4.2) shows a close up side perspective of the magnetic trap as viewed from the outside of the science cell. This figure includes the Bragg beam’s orientation and position relative to the science cell and waveguide structure. The mirror used to generate the standing wave is also seen. In particular, Fig. E.3 in appendix E, shows in detail how the Bragg beam is routed on the optics table to finally reach the configuration shown in Figure 4.2. 4.1. INTERFEROMETER OPERATION 83 Figure 4.2: Side perspective of the waveguide structure as viewed from the outside of the science cell. (a) The Bragg beam enters the chamber from the y direction centered on the waveguide axis. (b) The beam traverses the entire waveguide region and exits the science cell. (c) The Bragg beam is retro-reflected by a mirror outside the chamber. By having a pair of counter-propagating beams, a standing wave is created which is used to split and reflect the condensate during the interferometry experiment. Figure 4.3: Zoom into the science cell, looking head on to the waveguide region or “interaction region”. The Bragg beam can be seen traversing along the waveguide axis (y-axis) setting up a standing wave. The two arrows illustrate the direction of the Bragg beam and the red sphere represents the condensate atoms suspended against gravity in the center of the waveguide. 84 CHAPTER 4. INTERFEROMETRY TECHNIQUES Figure 4.4: Diagram illustrating the wave-packet trajectory along the y-axis. The solid ovals represent the condensate before the split and reflect operation. The dashed ovals represent the condensate some time after each of these operations. The different letters correspond to different times (a) Two red arrows represent the standing wave used to split the atoms, analogous to an optical beam splitter. A box at 1 has been drawn to represent the location of the corresponding beam splitter. (b) The reflection pulse represented by the outermost arrows at 2, is analogous to mirrors in an optical interferometer. (c) The recombination pulse is identical to the split. Accordingly, this configuration is a one-dimensional equivalent of the Michelson interferometer where both packets travel the same path in Fig. 4.5. Imaging camera at 3 takes pictures of the output, analogous to the photo-detector. 4.1. INTERFEROMETER OPERATION 85 Figure 4.5: Michelson Interferometer. (a) Input beam is divided with beam-splitter 1. (b) First arm of the interferometer is directed to mirror 2 and reflected back to splitter 1. (c) second arm of the interferometer is directed to mirror 3 and back to splitter 1. (d) The two arms are recombined at splitter 1 and the output redirected to the detector 4. As shown in Fig. 4.4, we implement a one-dimensional interferometer in which the wave packets travel the same path twice, hence a version of the Michelson configuration. This particular set up suits the one dimensional magnetic waveguide obtained from the trap structure and is relatively simple to implement in comparison to multidimensional configurations. Granted that, having only one dimension means we are not able to enclose an area with the arms, which makes it impossible for us to make gyroscopic measurements like [50]. But our first aim is to test the coherence of our wave packets and achieve an output state which demonstrates that the condensate is interfering. To this end we will ensure no phase difference is acquired by the packets during their propagation. However, we will change the position of the light field when recombining the wave-packets in order to change the output phase. Additionally we seek to obtain a fully separated pair of wave-packets at their point of maximum travel (from the center) in the waveguide. Also, the double reflection technique causes the packets to traverse identical paths therefore both packets will experience the same potential cancelling any relative phase shift between them. This means our configuration is insensitive to the gravitational potential, so we cannot make precision measurements of this type. However, in the future, extending the current trap structure along its axis to form a loop would yield a 2-D waveguide suitable for Sagnac experiments. The waveguide potential was initially designed with this conceptual extension in mind. 86 CHAPTER 4. INTERFEROMETRY TECHNIQUES Figure 4.6: Position vs. time graph summarising path and pulse sequence of the interferometer. The left black oval represents the condensate starting position and the black lines its trajectory . First pair of red arrows represents splitting pulse applied at t = 0, the middle two arrow pairs represent reflection pulses at t = T /4 and t = 3T /4 respectively. A final recombination pulse at t = T is used to produce the output state. Output states can be: atoms brought to rest, atoms moving at ±2~k or a linear combination of atoms at rest and moving. The latter state is illustrated by the three black ovals at the end of the condensate trajectory. 4.2. SPLITTING THE MATTER WAVE 4.2 87 Splitting the Matter Wave The first step in the implementation of the interferometer sequence is splitting the condensate atoms at rest into two wave packets travelling away from each other. Next we reflect twice and at the end of the interferometer sequence, the splitting pulse is used to recombine the atoms and generate the output state. The following sections will cover the physics required to understand and model the origin of the splitting, reflection and the dynamics of the wave packets during the interferometer sequence. 4.2.1 Two-Level Approximation Applying a pair of counter-propagating beams along the y−axis through the waveguide results in the condensate atoms experiencing a standing wave pattern that sets up a periodic potential as will be explained below. Because the condensate is coherent, we treat it as a quantum wave packet that follows the Schrödinger equation in the presence of an electric field E(t). In this system, the Hamiltonian consists of two parts, the time independent part Ĥ0 and the time dependent component Ĥ 0 such that Ĥ = Ĥ0 + Ĥ 0 . The time evolution of this problem can be obtained by relating the translational states of the condensate to a two-level system. First, it is essential to understand how the laser light interacts with the internal states of the atom. Understanding this interaction will allow us to find out how the laser light shifts the energy levels of the atoms. We can then use the generic form of the two level exact solution to model the translational states of the condensate in the standing wave. We begin by considering the internal states of the atoms. In this context, we demonstrate why it is appropriate to use the two level approach of a ground and excited state only. Initially we consider a laser beam modeled by using the potential of a travelling electromagnetic plane wave, and assign it to H 0 . We start by writing the Schrödinger equation for the valence electron to obtain a general solution. i~ ∂| ψ(t)i = Ĥ| ψ(t)i ∂t (4.3) The wave function can be expanded in terms of the eigen-state vectors with their corresponding time dependent coefficients and energy phases. In this situation it will be convenient to explicitly include the energy phases in the expansion of the wave function. The eigen-states are represented by their respective quantum number n denoting the energy state | ψ(t)i = X n cn (t) e−i ωn t | ni (4.4) 88 CHAPTER 4. INTERFEROMETRY TECHNIQUES here hr|ni = ψn (r) and coordinate r denotes the electron position. Plugging in the above equation into (4.3) and multiplying both sides by another wave vector h j|, we obtain the following expression: X X ∂ X i~ cn hj|nie−i ωn t = cn hj|Ĥ0 |nie−i ωn t + cn hj|Ĥ 0 |nie−i ωn t (4.5) ∂t n n n In order to simplify the calculation we assume that we know the stationary states of the system such that Ĥ0 | ni = En | ni. Using the ortho-normality relationship hj|ni = δjn , we can collapse the sums of the first two terms such that: i~ X ∂ 0 cj e−i ωj t = Ej cj e−i ωj t + Hjn cn e−i ωn t ∂t n (4.6) 0 ≡ hj|Ĥ 0 |ni. We carry out the time derivative on the left hand side Where Hjn using the product rule. A factor of ωj will be pulled down in one of the resulting terms, which when multiplied by ~, yields the energy Ej . The term containing Ej , then cancels with the first term on the right hand side to give: X ∂ 0 i~ cj = Hjn cn ei(ωj −ωn )t (4.7) ∂t n We now define the meaning of the subscript n to consider the internal states of an atom. Normally Eq. (4.7) would yield an infinite set of coupled differential equations for the cn ’s, but using an approximation studied by Rabi [58], only two internal energy levels of the atom are considered (n = 1, 2), truncating the infinite set. This is done because the probability to populate subsequently higher or lower energy states is small. Consequently, we only consider the ground and a particular excited state of the atom coupled via a laser whose frequency ω0 is tuned near the transition energy between them. In order to justify this approach, we can consider the rate of driving a transition between the ground state and states separated by energies much greater or less than ~ω0 . Specifically, we can consider the coupling during the splitting and reflecting pulses. We will use a laser frequency detuned 7.8 GHz from the transition between the 5S1/2 ground, and the 5P3/2 excited state. The closest available transition for a laser tuned to the D2 line is the D1 line, which we will show has a low transition rate. To calculate the transition rate for the D1 line, we can use time dependent perturbation theory on the exact result of Eq. (4.7). The time dependent perturbation will be given by the following interaction [35, 59, 60]: H 0 = −eE · r (4.8) The above result is not trivial to obtain but can be thought of by considering the electric potential V (r), such that UE = eV (r). To obtain the potential energy UE , 4.2. SPLITTING THE MATTER WAVE 89 the electric field E generating the potential must satisfy −∇V (r) = E(r). Noting that ∇(E · r) = E (for dipole interaction), then we can obtain Eq. (4.8) as our interaction potential. Here we assume a simple travelling plane wave form for the electric field and write it in complex notation as E = k E0 ei(ky−ωl t) . Here, the wavelength of the light used in the experiment is much larger than that of the wavefunction of the electron in use. For this reason we can neglect the spatial and directional variation of the E field relative to the coordinate of the atom (E → k E0 e−iωl t ). This is called the dipole approximation. As a result, the matrix elements of the time dependent perturbation can be written as: 0 Hjn = −~ eE0 hj|z|nie−iωl t ~ (4.9) We define Ωjn ≡ eE~ 0 hj|z|ni to be the Rabi frequency. Figuring out the integrals in the Rabi frequency can be a difficult task in many instances, but there are alternate methods to obtain this number. Once we obtain the final expression for the transition rate, we will plug in values for this important parameter. 0 For now we will focus on the time dependent aspect of Hjn and relabel it as 0 0 −iωl t 0 Hjn → Hjn e where Hjn /~ is just the Rabi frequency for the transition between j and n. This allows us to more clearly obtain the equation for the transition rate. Equation (4.7) can be expressed in terms of matrix operators and vectors. In it, 0 we include the new labeling of Hjn which has the oscillation frequency of the laser ωl and introduce ωjn ≡ ωj − ωn . 0 −iωl t 0 i(ω12 −ωl )t c1 H11 e H12 e . c1 ∂ 0 i(ω21 −ωl )t 0 −iωl t (4.10) i~ c2 = H21 e H22 e . c2 ∂t . . . . . In principle we would have to solve an infinite set of equations, but a perturbative approach can be taken. First we use the initial state of the system where c1 = 1, cj6=1 = 0 at t = 0 and we assume the vector 1 0 (4.11) . to be the zero order solution to the system. Making this assumption means that we plug in this vector into the right hand side of Eq. (4.10) and solve all the resulting equations for cj6=1 by integrating. Since j can be any integer up to infinity, and can be considered the final state where the atoms end up, we can label it by the index “f” to denote any generic final state. In general we obtain: Z −i t 0 i(ωf 1 −ωl )t0 0 dt H e cf = ~ 0 f1 90 CHAPTER 4. INTERFEROMETRY TECHNIQUES −i Hf0 1 i(ωf 1 −ωl )t (e − 1) ~ iωf 1 µ ¶ −i i(ωf 1 −ωl )t/2 Hf0 1 sin (t(ωf 1 − ωl )/2) = e ~ (ωf 1 − ωl )/2 = (4.12) Above, we have rewritten the exponential in terms of a sine function. To obtain second and higher order corrections, Eq. (4.12) in conjunction with c1 = 1 is plugged into the right hand side of Eq. (4.10) to generate another infinite set of equations that can later be integrated. The first order transition probability is found by taking the magnitude of cf : 1 sin (t(ωf 1 − ωl )/2)2 0 2 |cf | = 2 |Hf 1 | ~ ((ωf 1 − ωl )/2)2 2 (4.13) For long times t → ∞, the average rate can be calculated by dividing the transition probability by the time such that: |cf |2 t→∞ t R1→f = lim (4.14) At this point, we can use a mathematical identity which is an alternate definition of the delta function sin [t(ωf 1 − ωl )/2]2 = πδ((ωf 1 − ωl )/2) t→∞ t[(ωf 1 − ωl )/2]2 lim (4.15) and replace it into Eq. (4.14). In the limit where t → ∞, we obtain Fermi’s Golden rule for the transition rates between states. π R1→f = 2 δ [(ωf 1 − ωl )/2] |hf |Ĥ 0 |1i|2 (4.16) ~ We can use this formula to calculate the transition rate of the D1 line of 87 Rb, but some modifications need to be made. In Eq. (4.16), the delta function ensures energy conservation, so only the transitions whose energy difference match ~ωf 1 , are driven. This means that the transition in consideration has an infinitely narrow linewidth. Experimentally we observe that atomic transitions have a finite line width associated with them. In particular the D1 line has a linewidth of ΓD1 = 2π × 5.75 MHz, [26]. To incorporate the idea of a finite linewidth, we substitute the delta function for a Lorentzian in terms of the detuning ∆ ≡ ωf 1 − ωl , which is the difference between the transition and laser frequencies. Therefore: δ(∆) → Γ2 A + 4∆2 This function should be normalized over all ∆ such that: Z ∞ A d∆ = 1 2 2 −∞ Γ + 4∆ (4.17) (4.18) 4.2. SPLITTING THE MATTER WAVE 91 which constrains the value of A to 2Γ/π. Finally, we arrive at an expression which appropriately describes the transition rate for the atomic states of 87 Rb. µ ¶ 2Γ 1 R1→f = |hf |Ĥ 0 |1i|2 . (4.19) 2 2 ~ Γ + 4∆2 Using a detuning of ∆ = 2π × 6.890 THz (the detuning of the D1 line to the laser frequency used for the standing wave), an intensity I ∼ 5Isat , ΓD1 = 4.484 mW/cm2 [26] and substituting Hf21 /~2 = Ω2f 1 = Ω2D1 = Γ2D1 I/2Isat [35] into Eq. (4.19), the D1 line will have a transition probability RD1 = 63 × 10−6 s−1 which is small compared to the lenght of our typical pulses (see Sec. 4.2.5). In other words this transition is unlikely to occur. 4.2.2 The Two Level Solution We can proceed to calculate the solution to the two level Rabi problem. To do so, we will take a slightly different approach in writting the wavefunction as compared to that in the previous section. Going back to Eq. (4.4), we can expand it with a different version of ψ, X | ψ(t)i = cn (t) | ni (4.20) n where the time dependent phase has been absorbed into the cn coefficients. When plugged back into Eq. (4.3) this yields the following expression: i~ X ∂ 0 cj = Ej cj + Hjn cn ∂t n (4.21) In the equation above, the two energy levels considered will labeled such that 1 → g for ground and 2 → e for excited state. To obtain the full Hamiltonian of the system we use the interaction described by Eq. (4.8). The same dipole approximation is used, but instead of using the complex representation for the E field we use a real wave form such that E = k E0 cos (ky − ωt). 0 Hjn = −~ eE0 hj|z|ni cos (ωt) ~ (4.22) To simplify the notation, we can introduce the definition of the Rabi frequency, Ωjn ≡ eE~ 0 hj|z|ni and notice that because of odd parity, the spatial integral hj|z|ji 0 = 0. Because the energy scale vanishes, making the diagonal matrix elements of Hjn is defined up to a constant, for the stationary eigenenergies, we choose the value of Eg = 0 and Ee = ~ω0 . Combining all these ideas together we arrive at the following set of equations. ¸ ¸ · ¸· · ∂ cg 0 ~Ω cos (ωt) cg . (4.23) = i~ ce ~Ω cos (ωt) ~ω0 ∂t ce 92 CHAPTER 4. INTERFEROMETRY TECHNIQUES This translates to the following pair of coupled differential equations for the c0n s i ċg = Ω cos (ωt) ce i ċe = Ω cos (ωt) cg + ω0 ce (4.24) (4.25) A mathematical trick can be performed to facilitate solving these equations. One can map one of the coefficients, namely ce , by performing a unitary transformation causing the time dependence to be eliminated. We call the newly transformed coefficient d(t) and define it as follows: ce (t) ≡ d(t) e−iωt (4.26) Using the above definition, we can re-write the differential equations in terms of d to obtain ċg = −iΩ cos (ωt)d e−iωt d˙ = i(ω − ω0 )d − iΩ cos (ωt) cg eiωt (4.27) (4.28) We re-introduce the parameter ∆ ≡ ω −ω0 as the detuning of the laser frequency from the atomic transition (D2 ) in consideration. At this stage we make use of a technique known as the rotating wave approximation. This approximation consists of averaging out the terms whose oscillation frequency is considerably larger than the detuning. First, we expand the cosine terms in Eqns. (4.27) and (4.28) in terms of exponentials to obtain: ¤ iΩd £ 1 + e−i2ωt 2 ¤ iΩcg £ i2ωt d˙ = i∆d − e +1 2 ċg = − (4.29) (4.30) Assuming |∆| ¿ ω we can apply the rotating wave approximation and drop the two terms which oscillate at a rate 2ω. The above equations yield: Ω ċg = −i d 2 Ω d˙ = i∆d − i cg 2 which written in matrix form gives: ¸ · ¸ · ¸· ∂ cg 0 Ω2 cg i = Ω d −∆ ∂t d 2 (4.31) (4.32) (4.33) Here, we label the 2 × 2 matrix on the right hand side as Ĥef f . With Eq. (4.33) we recover the form of the Schrödinger equation which is analogous to Eq. (4.23) 4.2. SPLITTING THE MATTER WAVE 93 but with the advantage that this effective Hamiltonian has no time dependence. We can check the correspondence of this effective Hamiltonian to the original two level Hamiltonian by setting the coupling parameter Ω = 0. This means that the effective Hamiltonian becomes a simple diagonal matrix with two constant energy levels. The solution in this situation is the plane wave such that d(t) = ei∆t . Carrying out the transformation back to ce (t), we obtain ce (t) = e−iωt ei∆t . This results in ce (t) = e−iω0 t which is consistent with the expected result for the two-level Hamiltonian presented in Eq. (4.23) when Ω = 0. One approach to solving Eq. (4.33) is to apply one more time derivative to the equation for d(t), yielding a second order equation that has a term including ċg (t). This allows us to substitute Eq. (4.31) into Eq. (4.32) to obtain an uncoupled equation in terms of d(t) and its derivatives. Following the solution of d(t) we can obtain cg (t) by plugging in the appropriate derivatives of d(t) back into Eq. (4.28). Appendix F works through the mathematical details of how to obtain the solution to cg (t), d(t) and introduces the following substitutions which make the solution more elegant. √ X = ∆2 + Ω2 (4.34) c0 = cg (t = 0) (4.35) d0 = d(t = 0) (4.36) Using the above definitions, we can write solutions to the Schrödinger equation with the effective Hamiltonian in Eq. (4.33) as an operator Û . ¸ · ¸ · c0 cg (t) = Û (4.37) d0 d(t) where, Û = e · i∆t/2 ¸ cos(Xt/2) − i∆/X sin(Xt/2) −iΩ/X sin(Xt/2) −iΩ/X sin(Xt/2) cos(Xt/2) + i∆/X sin(Xt/2) (4.38) To check, we set Ω = 0 and obtain the following Û operator · −i∆t/2 ¸ e 0 i∆t/2 Û → e 0 ei∆t/2 (4.39) which yields a result consistent with an effective Hamiltonian that has no laser coupling. The result becomes cg (t) = c0 and d(t) = ei∆t d0 , as required by a constant potential Hamiltonian. Now we can modify the starting Hamiltonian, to one that incorporates a travelling wave with phase φ. · ¸ 0 ~Ω cos(ωt + φ) Ĥ = (4.40) ~Ω cos(ωt + φ) ~ω0 94 CHAPTER 4. INTERFEROMETRY TECHNIQUES This means that Eq. (4.31) and (4.32) get modified (as seen in appendix F) to include an extra phase factor giving a new set of equations Ω ċg = −i eiφ d 2 Ω d˙ = i∆d − i e−iφ cg 2 which means we obtain a new effective Hamiltonian of the form: · ¸ Ω iφ e 0 0 2 Ĥ ef f = ~ Ω −iφ e −∆ 2 (4.41) (4.42) (4.43) We note that the new effective Hamiltonian can be written in terms of the original effective Hamiltonian in Eq. (4.33) and a transformation matrix Ŝ such that Ĥ 0 ef f = Ŝ † Ĥef f Ŝ. · iφ/2 ¸· ¸ · −iφ/2 ¸ e 0 0 Ω2 e 0 0 Ĥ ef f = ~ (4.44) Ω −∆ 0 e−iφ/2 0 eiφ/2 2 This means that a new Schrödinger equation in terms of the new effective Hamiltonian can be written in terms of the original effective Hamiltonian as: i~ ∂ | ψi = Ĥ 0 ef f | ψi ∂t = Ŝ † Hˆef f Ŝ| ψi (4.45) If we act on this equation by the Ŝ operator on both sides from the right, we get an equation equivalent to Eq. (4.33) for the states | ψ 0 i = Ŝ| ψi. ∂ Ŝ| ψi = Ĥ Ŝ| ψi ∂t ∂ i~ | ψ 0 i = Ĥ| ψ 0 i ∂t i~ (4.46) As shown, the Ŝ and Ŝ 0 operators let us transform between the | ψi and | ψ 0 i basis. Similarly, by applying these operators, we can transform the time evolution of | ψi given by the operator Û . To obtain the solution to Eq. (4.46) we act on the operator Û from the left and right to obtain the new time evolution Ûφ of the state | ψ 0 (0)i Ûφ = Ŝ † Û Ŝ ¸ · cos(Xt/2) − i∆/2 sin(Xt/2) −ieiφ Ω2 sin(Xt/2) i∆t/2 = e cos(Xt/2) + i∆/2 sin(Xt/2) −ie−iφ Ω2 sin(Xt/2) (4.47) 4.2. SPLITTING THE MATTER WAVE 95 The result presented above is the solution to a quantum mechanical two-level system where the ground and excited state amplitudes cg (t) and ce (t) are coupled via an electromagnetic plane wave. It is important to note that recovering the amplitude for the excited state ce (t) can be done by multiplying d(t) by the phase e−iωt . At any rate, the populations for each state are obtained by taking the modulus squared of each amplitude so |ce |2 = |d|2 , making the overall phase irrelevant. Above all, this result will prove useful when we apply the two-level time evolution to the rest and moving states of the wave-packets in the waveguide with a standing wave potential. 4.2.3 The Light Shift Equation (4.33) shows the Hamiltonian for a two level system (like an atom), whose energy levels are coupled via the interaction with the E field. We can use this Hamiltonian to find out how the light intensity shifts the internal atomic states. Then we relate the shift to the E field of a standing wave discussed in Sec. 4.1 to obtain the potential generated by the counter propagating beams. The Hamiltonian in Eq. (4.33) can be diagonalized using the requirements on eigenvalue matrix equations. Specifically, we apply det(H − λ1) = 0, which gives: λg = ~ Ω2 4∆ λe = −~∆ − ~ (4.48) Ω2 4∆ (4.49) For a negative detuning ∆, the light shift reduces the energy of the ground state by λg . However, the light shift can depend on position. As it was described on chapter 2, the optical Bloch equations [35] yield the equations defining the saturation intensity. In turn, these reveal that Ω2 depends on the intensity I of the light seen by the atoms. In a 1-D standing wave, like the one we apply to split the atoms, the intensity of the light will vary as a function of space. For this purpose, we can use the standard result that the intensity of light I(y) depends on the electric field like I(y) = |E(y)|2 /2ξ0 , where ξ0 = 1/²0 c = 377 Ω is the impedance of free space [61]. We can then write Γ2 I(y) 2 (4.50) Ω (y) = 2Is where the Is is the saturation intensity for the atoms to scatter photons as discussed in Sec. 2.2. 4.2.4 The Bloch Picture In order to obtain an intuitive understanding of the time evolution of the state vector in the two-level problem, we can make use of the Bloch vector picture developed 96 CHAPTER 4. INTERFEROMETRY TECHNIQUES by Feynman et al. [62]. In the Bloch representation of a generic two level system in Eq. (4.33), one constructs a 3-dimensional vector in the {x̂, ŷ, ẑ} basis out of the time dependent coefficients cg , ce and their complex conjugates [35]. The Bloch vector R is then made up of three components which evolve in time and represents the state in which the two-level system can be found. The Bloch picture also includes the vector Ω, containing information about the Hamiltonian which couples the two energy levels. Specifically the vector Ω is defined as: Ω ≡ Re Ω x̂ + Im Ω ŷ + ∆ ẑ (4.51) Where Re Ω = Ω is the Rabi frequency and ∆ the detuning for a two level problem defined in Sec. 4.2.1. It can be demonstrated, using the equations for the coefficients in Eq. (4.7), that a vector R constructed from the components: £ ¤ rx = cg c∗e + c∗g cg x̂ (4.52) £ ∗ ¤ ∗ ry = i cg ce − cg cg ŷ (4.53) £ 2 ¤ rz = |ce | − |cg |2 ẑ (4.54) obeys the following vector equation known as the Bloch equation of motion dR = Ω × R. dt (4.55) The physics that arises from the Bloch equation of motion, describes the dynamics analogous to a classical top whose angular momentum vector Lc precesses around a constant gravitational field vector g. In the case of a two level quantum system, the Bloch vector R precesses around the vector Ω. Additionally, according to equation (4.55), R will evolve in time with constant length. Hence, its motion is confined to what is known as the Bloch sphere. When R points to the south or north poles of the sphere, the system is in the ground or excited state respectively. If the vector lies in the equator, the system is in an equal superposition of ground and excited states. Because we can experimentally control the direction of Ω, we can alter the precession angle and obtain different time evolutions for the system. 4.2.5 Splitting Operation In order to carry out the interferometer sequence we must split the condensate into two packets moving apart from each other. The atoms interact with a periodic potential set up by a standing wave from off-resonant beams created as described in Fig. 4.2 and 4.3. Because a periodic potential is set up, the off-resonant laser beams interact with the condensates via Bragg scattering [63, 64, 65]. A short time after the condensate atoms are loaded into the waveguide, we apply the pair of counterpropagating beams along the axis of the waveguide in order to split the condensate. 4.2. SPLITTING THE MATTER WAVE 97 In this section we aim to find a method that models the interaction of the standing wave created by the counter propagating beams with the condensate. The counter-propagating beams of a laser can be modeled by two travelling plane waves with opposite wave vector k. Because we use a mirror to retro-reflect the incoming beam, the amplitudes and frequencies of each plane wave are very similar. Adding the two plane waves gives the following field: Es (y) = k E0 ei(ky−ωt) + k E0 ei(−ky−ωt) (4.56) where y is the position of the atom. The magnitude squared of this field yields |Es (y)|2 = 2E02 + 2E02 cos(2ky) (4.57) Using the equation for the intensity in terms of the electric field, we can plug I(y) into Eq. (4.50) to obtain an expression for Ω which will expose its spatial dependence: Ω2 (y) = Γ2 2E 2 [cos(2ky) + 1] 4Is ξ0 0 (4.58) Next, we can plug the expression for Ω2 (y) into (4.48) to obtain an equation for the potential experienced by the atoms when a standing wave is applied along the axis of the waveguide. In the expression below the term corresponding to an over all constant energy shift has been disregarded. U (y) = ~Γ2 E02 cos(2ky) 8∆Is ξ0 (4.59) To obtain the final form for the potential of the standing wave, we introduce the variable β = Γ2 E02 /8∆ξ0 Is = Γ2 I/4∆Is where I = E02 /2ξ0 in order to make the above equation more manageable. Eventually, β will become time dependent allowing us to turn on or off the interaction. Additionally we introduce the standing wave phase φ such that cos(2ky) → cos(2ky + φ). Later, φ will be shown to control the zero of the standing wave. This gives U (y) = ~β cos(2ky + φ). (4.60) Having derived the above expression for the potential, we can write it as a an operator Û (y), and proceed to write the 1-D Hamiltonian for atoms that see a standing wave in the waveguide as Ĥs = p̂2 + ~β cos(2ky + φ) 2m (4.61) With p as the atomic momentum. One can write the potential energy term of this Hamiltonian as a sum of two complex exponentials. Consequently, the Hamiltonian is re-written in terms of two momentum translation operators e±i2~k . These 98 CHAPTER 4. INTERFEROMETRY TECHNIQUES two momentum transformations will convert stationary states into moving states of momenta ±2~k. To get an idea of the coupling mechanism, we can consider a situation where the interaction times are short thus simplifying the problem. However it should be noted that this kind of model is not applicable in our case because we will be applying the standing wave for long times. Similarly we consider a wave-packet confined to a one-dimensional box. This is also an approximation that will be relaxed later. For short enough interaction times, we can assume that the kinetic energy term is negligible since the wavefunction which describes the condensate atoms will not move while we apply the standing wave. ¤ ~β £ i(2ky+φ) Ĥs ' e + e−i(2ky+φ) (4.62) 2 We start with a stationary wave packet | ψ0 i described by a constant wave function that is normalized to a 1-D box of length L. Then the evolution of the wave-packet can be obtained by using the time evolution operator as follows: | ψ(t)i = e−iĤs t/~ | ψ0 i (4.63) To obtain an idea of how the time evolution occurs, we can start with an approximate treatment in which βt ¿ 1. In this way we can approximate the exponential to get βt βt (4.64) | ψ(t)i ' 1| ψ0 i − i ei(2ky+φ) | ψ0 i − i e−i(2ky+φ) | ψ0 i 2 2 Which shows the original wave packet | ψ0 i plus two other plane wave states moving along the y direction. The above example shows how a Hamiltonian of this form can operate on a stationary wave-packet and generate alternate wave packets travelling with momentum of 2~k. Other higher momentum states are generated, but their probability amplitude is small and therefore neglected. This is why we approximated the exponential to first order only. The result is analogous to an optical grating in which the zeroth order beam gets split into higher order diffraction beams that have higher momenta. It should be noted that this approximation has limitations when comparing it to a better model (as explained below) of the interaction. If we make the interaction time too short then we increase the probability to drive atoms into the higher momentum states ±4~k [64], making this approach invalid. We could use a long single pulse. However, using a longer pulse will also leave many atoms at rest. In practice, using a single pulse will at best put 1/3 of the atoms into the moving states ±2~k, which is not optimum for our interferometer. Our waveguide is one-dimensional. Implementing the successive operations to obtain a Michelson interferometer like the one in Fig. 4.4, means the condensate part | ψ0 i will obstruct the motion of the split condensates. Moreover, due to atomic interactions, the overlap adds phase shifts to the clouds which complicate the operation of the interferometer. 4.2. SPLITTING THE MATTER WAVE 99 In light of this difficulty, we seek to find an alternative to split the condensate evenly, without leaving any portion of atoms behind. Consequently we adopt a technique described by Wu et al. in [66]. In this technique a sequence of two laser pulses separated by the appropriate time are used to achieve even splitting. The pulses interact with the atoms through an off-resonant Bragg scattering process. Subsequently, we calculate the required pulse intensities and times to achieve a successful splitting technique. This implies that after splitting, 50% of the atoms move with p = +2~k, the other 50% move at p = −2~k and no atoms are left at rest. For this purpose, we make use of the Bloch sphere representation of a twolevel system. The Bloch sphere picture will help us visualize the dynamics of the quantum mechanical states. It will use a time evolving vector which we can track, helping us choose the right pulse lengths that will yield the correct quantum states. We start by restricting the Hamiltonian in Eq. (4.61) to a three dimensional Hilbert space. We no longer assume that βt ¿ 1. This gives us the required flexibility for the pulse lengths (given a fixed intensity of the laser) needed to split, reflect and recombine the condensate. Therefore in the following analysis, we choose to neglect the coupling to momenta states with p = ±4~k or higher [64]. For these reasons, we assume that the time evolution of the condensate’s translational states in the waveguide will be described by the following three states: | 0i atoms moving at p = 0~k | +2i atoms moving at p = +2~k | −2i atoms moving at p = −2~k (4.65) The coordinate representation of the moving states is given by plane waves of the form ψ0 (y) e±iky and the rest state is ψ0 (y). Here the function ψ0 (y) represents the condensate wavefunction and it should be normalized. Using this basis we can compute the matrix elements of Ĥs . Details of how to obtain each matrix element are given in appendix F, but the results are expressed by the following matrix using the states in the order of (4.65): 0 β iφ Ĥs = ~ e 2 β −iφ e 2 β −iφ e 2 4ωr 0 β iφ e 2 0 4ωr (4.66) where ωr = ~k 2 /2m = 2.36 × 104 s−1 is defined to be the recoil frequency of the atoms. At this point we make a change of basis that will decouple one of the states in the three-level system. For now we choose φ = 0 assuming no changes in the phase of the potential. Nevertheless, φ will become a parameter that has physical significance in our experiment. The meaning of φ and its relevance will be explained in Sec. 4.4. We aim to convert this Hamiltonian so that it contains a two-level system to which we can apply the results obtained in section 4.2.2. This can be achieved using a 100 CHAPTER 4. INTERFEROMETRY TECHNIQUES change of basis like: | 0i = | 0i | +i = √12 (| +2i + | −2i) | −i = √12 (| +2i − | −2i) (4.67) In order to calculate the matrix elements of Ĥs in our new basis, we can use the results found in Eq. (4.66). ³ ´ 1 √ h+|Ĥs |0i = h+2|Ĥs |0i + h−2|Ĥs |0i 2¡ ¢ ~β 1 (4.68) = √2 2 + ~β 2 1 = √2 ~β In a similar way h−|Ĥs |0i = √1 2 √1 2 = = 0 ³ ´ h+2|Ĥs |0i − h−2|Ĥs |0i ¡ ~β ~β ¢ − 2 2 (4.69) h i h+|Ĥs |−i = 12 h+2|Ĥs |+2i − h+2|Ĥs |−2i + h−2|Ĥs |+2i − h−2|Ĥs |−2i = 12 [4~ωr − 0 + 0 − 4~ωr ] = 0 (4.70) h i h+|Ĥs |+i = 21 h+2|Ĥs |+2i + h−2|Ĥs |−2i + h−2|Ĥs |+2i + h+2|Ĥs |−2i = 12 [4~ωr + 4~ωr + 0 + 0] = 4~ωr (4.71) h i h−|Ĥs |−i = 21 h+2|Ĥs |+2i + h−2|Ĥs |−2i − h−2|Ĥs |+2i − h+2|Ĥs |−2i = 21 [4~ωr + 4~ωr − 0 − 0] = 4~ωr (4.72) h0|Ĥs |0i = 0 (4.73) Because we know Ĥs is hermitian such that Ĥs† = Ĥs then † ³ (h+|Ĥs |0i) = h0|Ĥs |+i = ´† √1 ~β 2 √1 ~β 2 (4.74) 4.2. SPLITTING THE MATTER WAVE and 101 (h−|Ĥs |0i)† = 0 h0|Ĥs |−i = 0 (4.75) (h+|Ĥs |−i)† = (4~ωr )† h−|Ĥs |+i = 4~ωr (4.76) Combining all these results we can obtain Ĥs in its new representation using the | 0i, | +i, | −i basis vectors. The resulting Hamiltonian yields. 0 √β2 0 Ĥs = ~ √β2 4ωr 0 (4.77) 0 0 4ωr By inspecting Eq. (4.77), we can identify the {| 0i, | +i} sub-space as being analogous to the effective Hamiltonian found in Eq. (4.33) while the {| −i} state is decoupled. This means we can treat the {| 0i, | +i} sub-space exactly like the two level system√ and use the solution found in Eq. (4.38). Making the direct comparison we get Ω = 2β and ∆ = −4ωr , noting that the detuning is negative. Accordingly, in this case the ground state represents the rest state | 0i, and the excited state represents the symmetric superposition √12 (| +2i + | −2i) of the two travelling plane waves with momentum ±2~k. The latter is the desired output state after applying the standing wave. Having a two-level system allows us to take advantage of the Bloch vector model. We can construct the corresponding Ω and R vectors for our system and use the time evolution of Eq. (4.38) to get the time evolution for R. In the case of our standing wave potential, β is the direct analog of Ω in the generic two level-system. It is real, so we do not worry about the ŷ component. In particular this is due to Ω not having an imaginary phase. This means the Ω vector in our case lies in the x̂, ẑ plane. √ Ω = 2β x̂ − 4ωr ẑ (4.78) Experimentally, we can control the angle Ω makes with the x̂ axis. Because it is not within our control to easily change the recoil frequency of the atoms ωr , the value of ∆ remains constant. However, the power of the diode laser can be reduced by controlling the current control of the laser, permitting some intensity control of the standing wave at the position of the atoms. In this way, we can control the x̂ component of Ω, which in turn changes its angle with the x̂ axis. The Bloch picture allows us to visually follow the precession of the state vector, and give us insight as to what Ω should be in order to obtain the desired state. The atoms start in the ground state so that the Bloch vector points to the south pole of the Bloch sphere. Our aim is to manipulate Ω so that R precesses in such a way 102 CHAPTER 4. INTERFEROMETRY TECHNIQUES that its final position after the splitting sequence is done points to the north pole of the sphere. We make use of the optimized light pulse sequence technique proposed by Wang et al. in [12]. They demonstrate that for atoms whose state vector starts in the south pole of the Bloch sphere, a first pulse with the correct value of Ωx (Ω in the x̂ direction) causes R to precess around Ω so that at some later time, the Bloch vector will find itself in the equator of the Bloch sphere. A Ω in the +x̂−ẑ direction, transfers the state vector to the +x̂ axis at a time corresponding to half the period of precession At this point the standing wave is turned off but the recoil frequency −4ωr still exists. This implies Ω points directly downward and R precess perpendicular to it along the equator. By waiting a time corresponding to half the period of precession, the state vector is allowed to rotate 180◦ ending in the −x̂ direction. Finally, the standing wave is turned back on during a second pulse, causing the Bloch vector to precess once again about the axis defined by Ω as seen in Fig. 4.7. Keeping the standing wave on for the appropriate time causes the state vector to precess until it is pointing directly north. In terms of our experiment, we can choose the correct value of Ωx by controlling the intensity of the laser. We can also switch the standing wave interaction on or off by using an acousto optic modulator which we can switch on and off in ∼ 1 µs. Using our {| 0i, | +i} basis, for the first pulse we want the following time evolution at the peak of the precession. 1 | 0i → √ [| 0i + | +i] 2 (4.79) Inspecting the solution presented in Eqns. (4.38), (4.37) and starting with c0 = 1, d0 = 0 we get the following state vector as a function of time ¸ · ¸ · cos(Xt/2) − i∆/X sin(Xt/2) cg (t) i∆t/2 =e (4.80) d(t) −iΩ/X sin(Xt/2) From the Bloch picture, given that the vector Ω is in the +x̂ − ẑ direction and the starting Bloch vector points south, the Bloch vector will precess to the +x̂ position at a the time of half the oscillation cycle. To see this, we can calculate the components of R(t) with Eqns. (4.52), (4.53), (4.54) and use the initial conditions set forth by Eq. (4.80). 2Ω∆ 2 sin (Xt/2) X2 −2Ω = sin(Xt/2) cos(Xt/2) · X2 ¸ Ω ∆2 = − sin2 (Xt/2) − cos2 (Xt/2) X2 X2 rx = (4.81) ry (4.82) rz (4.83) 4.2. SPLITTING THE MATTER WAVE 103 When the Bloch vector reaches the equator, its rx component is at its maximum. Inspecting the above equations, specifically the rx component, we can conclude that this occurs when Xt = (2n + 1)π where n is an integer. Furthermore, by plugging in t = π/X into Eq. (4.80), we can obtain the following constraints |∆| 1 = √ X 2 Ω 1 = √ X 2 (4.84) (4.85) in order to have a state vector of the form shown in Eq. (4.79), which is the desired state after the first pulse. This is also consistent with rx = −1 at half the cycle time, meaning the unit length of R has been preserved. As a result we can obtain the time needed for Ω to reach the equator as: τ1 = (2n + 1)π √ 2|∆| (4.86) Immediately after the Bloch vector reaches the equator, we turn off the standing wave and let R evolve freely. This means Ω is pointing directly to the south pole. In this case the precession is perpendicular to √ Ω so R rotates in the equatorial plane of the Bloch √ sphere. Using√the state vector 1/ 2(| +i + | 0i) as a new initial condition, c0 = 1/ 2 and d0 = 1/ 2. Then in Eq. (4.38) we obtain the following state vector: · cg (t) d(t) ¸ ei∆t/2 = √ 2 · cos(Xt/2) − i∆/X sin(Xt/2) cos(Xt/2) + i∆/X sin(Xt/2) ¸ (4.87) Just as we did earlier, we can find the time evolution for the components of R, noting that when Ω = 0 means X = |∆|: rx = cos2 (Xt/2) − sin2 (Xt/2) ry = 2 sin(Xt/2) cos(Xt/2) rz = 0 (4.88) (4.89) (4.90) Starting with R(t = 0) = x̂, to achieve a 180◦ rotation, we want R(t) = −x̂. This implies that Xt = (m + 1)π/2 so that the required time for such a final state is: τ2 = (2m + 1)π . |∆| (4.91) This achieves the desired change in the state vector such that: 1 1 √ [| 0i + | +i] → √ [−| 0i + | +i] 2 2 (4.92) 104 CHAPTER 4. INTERFEROMETRY TECHNIQUES √ Finally we turn on the second pulse so that Ω = 2βx̂ − 4ωr ẑ, inducing √ the Bloch vector to precess once again. Using the initial conditions c 2, and = −1/ 0 √ d0 = 1/ 2 corresponding to R starting in the −x̂ direction, we obtain the following time evolution for the state vector. · ¸ · ¸ ei∆t/2 − cos(Xt/2) + i∆/X sin(Xt/2) − iΩ/X sin(Xt/2) cg (t) = √ (4.93) d(t) iΩ/X sin(Xt/2) + cos(Xt/2) + i∆/X sin(Xt/2) 2 This in turn yields the following time dependent components of R(t): · 2 ¸ Ω2 ∆ 2 rx = − cos (Xt/2) − sin(Xt/2) − X2 X2 ∆ ry = −2 cos(Xt/2) sin(Xt/2) X Ω∆ 2 rz = 2 2 sin (Xt/2) X (4.94) (4.95) (4.96) The Bloch vector must completely lie along the ẑ direction for the final state vector to be | +i. Moreover from the Bloch picture, the precession of R must be such that the maximum rz must occur at half the period of oscillation meaning Xt = (2n+1)π. Additionally we know that the length of R will not change. According to Eq. (4.80), we started the sequence with a vector of unit length. Consequently at the end of the pulse, R should equal ẑ meaning (Ω/X)(∆/X) = 1/2. In order to satisfy the final condition of t = π/X for Eq. (4.93), we see that Ω/X = |∆|/X, which yields the constraints |∆| 1 = √ X 2 Ω 1 = √ X 2 (4.97) (4.98) As a result we can see that the time required to reach the north pole of the Bloch sphere is given by (2n + 1)π τ3 = √ (4.99) 2|∆| The above result demonstrates the motion of R is equivalent to its precession during the first pulse, but located in the {−x̂, ŷ, ẑ} quadrant of the Bloch space. This is consistent with the symmetry of the Bloch sphere. Plugging in the constraints found in Eqns. (4.97), (4.98) and the required time set by (4.99) into Eq. (4.93), gives the final state of the two level system. The result shows that after the second pulse is over, the following transformation takes place: 1 √ [−| 0i + | +i] → | +i 2 (4.100) 4.2. SPLITTING THE MATTER WAVE 105 Figure 4.7: Illustration of the Bloch vector precession during the optimized double √ pulse sequence. (a) We start with Rx , during the first pulse Ω = 2βx̂ − 4ωr ẑ so that R precesses along the dotted circle going through the x̂ axis once every cycle. Waiting t = τ1 places R along the x̂ axis. (b) Turning off the laser means Ω = −4ωr ẑ, and R rotates along the equator. Waiting t = τ2 leaves R along the −x̂ axis. (c) A second light pulse is used and R precesses along the dotted line for t = τ3 corresponding to half the cycle time, giving the final position of R along the ẑ axis. The time dependence of Ωz is given by the bottom graph showing Ω vs t. Here τ1 = τ3 . In short, the dynamics of the Bloch vector for the optimized pulse sequence is best described and summarized by the three stages shown in Fig. 4.7. According to the optimized pulse sequence presented, we can summarise the theoretical values for the parameters of light intensity, pulse time and wait time required to split the rest condensate into two equal clouds moving at ±2~k. We use the simplest solutions for τ1√, τ2 and τ3 where n = 0 and m = 0. In our case we identify ∆ = −4ωr and Ω = 2β from the two level system presented in Eq. (4.77). √ β1 = 2 2ωr π τ1 = √ 4 2ωr π τ2 = 4ωr (4.101) (4.102) (4.103) 106 CHAPTER 4. INTERFEROMETRY TECHNIQUES Figure 4.8: Absorption imaging showing two wave packets after applying the double pulse sequence on the condensate at rest in the waveguide. Here two wave packets are seen travelling at ±2~k 10 ms after splitting. 4.2.6 Experimental Verification Experimentally, we have been able to corroborate the efficiency of the double pulse. Using the parameters calculated in the optimized double pulse sequence we obtained a ratio 1 : 1 for atoms in the | +2~ki and | −2~ki state respectively. Our absorption measurement with the camera was only accurate up to 95%. Hence, up to 5% of the atoms could be left behind by the splitting and we would have not been able to detect it. This occurs because the absorption coefficients are very small because there are so litte atoms to absorb the light. For this reason we say that the splitting using the double pulse technique was 95% efficient. Thus we could see a maximum of 95% of the atoms separated into two clouds travelling at ±2~k. The theoretically optimum values of τ1 = τ3 = 24 µs for the pulse durations and τ2 = 33 µs for the wait time between pulses provided the best results. To create the Bragg beam we used a laser detuned 7.8 GHz red of the D2 transition. The laser had a power of 0.7 mW and a Gaussian beam waist of approximately 1.5 mm which resulted in a peak intensity of 17.6 mW/cm2 which meant that β = 52 KHz. This power setting for both pulses corresponded to within 23% with the expected theoretical intensity given by the relationship in Eq. (4.101), which relates the recoil frequency ωr to the laser intensity. The results can be seen in Fig. 4.8. 4.3. REFLECTING THE MATTER WAVE 4.3 4.3.1 107 Reflecting the Matter Wave Three Level System Following the splitting of the atoms, we allow the two wave packets to propagate along the axis of the waveguide until they fully separate from each other. At some variable time after separation we apply another laser pulse similar to the splitting in order to reverse the momentum of each wave packet. The objective is to reverse the momentum of the wave packets twice at t = T /4 and t = 3T /4 as described by Fig. 4.6 in order for the groups of condensate atoms to travel through identical paths before becoming recombined. Making each wave packet traverse the same path means that both packets will experience the same energy phase shift if there are any asymmetrical imperfections and changes in the potential. We developed a technique to reflect the atoms via an off-resonant beam, [64]. To understand the reflection sequence we return to using the {| 0i, | +i, | −i} basis. Using the Hamiltonian containing a potential energy term describing a standing wave like in Eq. (4.61), we were able to write a representation for φ = 0 where the {| 0i, | +i} comprised a decoupled subspace from {| −i}. This meant we could use the two-level time evolution expressed in Eq. (4.38). If we add an additional decoupled sate with constant energy −4ωr to the two-level system, the time evolution for the three-level system would just acquire an additional diagonal term that contained the normal constant energy phase factor. Û = ei∆t/2 × cos(Xt/2) − i∆/X sin(Xt/2) −iΩ/X sin(Xt/2) 0 −iΩ/X sin(Xt/2) cos(Xt/2) + i∆/X sin(Xt/2) 0 0 0 ei∆t/2 (4.104) where once again ∆ = −4ωr . Our goal is to use this time evolution operator to transform the states obtained after the splitting sequence, e.g convert | ±2~ki as follows: | +2~ki ←→ | −2~ki 1 1 √ [| +i + | −i] ←→ √ [| +i − | −i] 2 2 (4.105) (4.106) This means that if our initial state is: 0 | ψ+2k i = 1 1 (4.107) then, by applying the time evolution operator Û in Eq. (4.104), the general final 108 CHAPTER 4. INTERFEROMETRY TECHNIQUES state has the form: −iΩ/X sin(Xt/2) 1 | ψf i = √ ei∆t/2 cos(Xt/2) + i∆/X sin(Xt/2) 2 ei∆t/2 To obtain the desired output we would like a final state of the form: 0 | ψf i ∝ 1 −1 (4.108) (4.109) which yields a set of constraints that can help us define what the intensity and the length of the pulse should be in order to achieve reflection. To eliminate sin(Xt/2) we require that Xt/2 = mπ where m is any integer which in turn means cos(Xt/2) = (−1)m giving us so far, 0 1 | ψf i = √ ei∆t/2 (−1)m (4.110) 2 ei∆t/2 m Observing the above equation, it is evident we want to have ei∆t/2 = −(−1) or √ m±1 2 equivalently (−1) . It is important to keep in mind that because X = ∆ + Ω2 then ∆ must be smaller than X by definition, thus specifically |∆| < X. The simplest solution satisfying these conditions is: ∆t = −π 2 Xt = 2π 2 (4.111) (4.112) This means the time required to reflect the atoms is τref = −2π/∆ = π/2ωr and X = −2∆. Using the definition of X we obtain: X 2 = Ω2 + ∆ 2 4∆2 = Ω2 + ∆2 Ω2 = 3∆2 (4.113) (4.114) (4.115) √ In a similar way to the splitting sequence, we identify Ω = 2β and ∆ = −4ωr and obtain the parameters for intensity and time of the standing wave pulse required to make the transition in Eq. (4.105). √ βr = 2 6ωr (4.116) π (4.117) τr = 2ωr 4.3. REFLECTING THE MATTER WAVE 4.3.2 109 Experimental Verification Using the above technique to reflect the atoms is not the only way to reflect the atoms. Previous experiments have used short pulses that couple the | +2~ki to the | −2~ki through second order Bragg scattering [64]. However this technique is very sensitive to velocity errors in the wave-packets. Given that, any fluctuation in the initial velocity of the wave-packets will degrade the performance of the reflection pulse. Ordinarily, because we are not interested in populating the | 0i state, a long weak pulse could be used in order to transfer the atoms from | −2~ki to | +2~ki. However, the long pulse poses a draw back. The transition less likely to happen if there are velocity errors present. A major difficulty arising when performing the interferometer operations is the residual motion acquired by the atoms after the waveguide is loaded. We have observed that the loading process is very sensitive to fluctuations in external magnetic fields. This causes the condensates to start with a non-zero velocity when starting the interferometer sequence. However the initial motion due to loading was resolved as described in Sec. 3.5.4. We have observed, using phase contrast imaging, initial condensate velocities of up to 0.5 mm/s. These offsets in velocity, denoted by δ, can decrease the efficiency of the reflection pulse. To understand how much these non-zero starting velocities affect the interferometer, we can analyze how sensitive the reflection pulse is to velocity variations. Using Fourier analysis [28], we know that for a light pulse of duration τ , the width of its frequency distribution is given by the relation: ∆ωτ ≥ 1 (4.118) If the velocity of a packet is v0 + δ before we apply the reflection pulse, then it will be −v0 + δ after the transition, giving an energy difference ∆E = 2M v0 δ. Using the energy-time uncertainty relation we can conclude that for a laser pulse of duration τr , the width of frequencies available to cause a transition is 1/τr . Hence the corresponding energy uncertainty width for the laser is ~/τr . As a result, the energy difference for the reflection transition ∆E, must be small compared to ~/τr , giving 1 ~ = (4.119) |δ| ≤ 2M v0 τr 4kτr in order for the transition to occur. Otherwise it is likely that it will not happen. For example, Wang et al. used a pulse length of τr = 150 µs. This means the velocity variation is limited to δ ≤ 0.2 mm/s which is more than 50% less than the variations we observe. For this reason we opted for the short pulse method described above and achieved better results. 110 CHAPTER 4. INTERFEROMETRY TECHNIQUES In the laboratory we tested the method of reflecting the atoms along the waveguide using the time and intensity parameters calculated in the optimized reflection single pulse sequence. We used an intensity value of 2 times the splitting intensity having a β within 11% of the theoretical calcalculation. Additionally, we used the corresponding pulse time of τr = 67 µs calculated above, and obtained reflection efficiencies which varied between 100% and 80% in the waveguide. The shorter pulse made the reflection technique less sensitive to initial velocity fluctuations. For a pulse duration of 67 µs, the velocity fluctuations in the waveguide are limited to δ ≤ 0.5 mm/s. Given our observations for δ, we minimally satisfy this requirement. 4.4 Recombination Using the optimized splitting and reflecting pulses we can achieve the desired motion of the atoms as described by Fig. 4.6. Up until now, we have assumed that no external agents change the phase of the condensate wave packets. Applying the optimized splitting double pulse when the atoms regroup at the center of the waveguide at the end of their oscillation means that all the atoms should come back to rest. The atoms come back to rest because in quantum mechanical two level systems, like the one describing {| 0i, | +i}, the operations like splitting are unitary and therefore reversible. The recombination operation of the condensates will be shown in this section. Because the standing wave potential described in Fig. 4.2 is generated by retroreflection from a mirror, we can choose to describe the intensity of the standing wave as (see Sec. 4.2.5): I(y) = I0 sin2 (ky − ky0 ) = 1/2I0 [1 − cos(2ky − 2ky0 )] (4.120) (4.121) where y0 is the location of the mirror. In this way, writing the expression for the potential generated by the standing wave will result in Eq. (4.60). In this case the additional phase incorporates the location of the retro-reflection mirror at y0 . In writing the potential for this form, we drop any constant term and obtain: U (y) = ~β cos(2ky + φ) (4.122) where φ = −2ky0 . The above expression is equal to Eq. (4.60). We now see a physical meaning to φ. A change in φ is caused by a shift in the mirror position, or more generally any shift in the nodes of the standing wave relative to the atoms. To observe the functioning of our interferometer, we vary the phase φ. Figure 4.2 shows that the Bragg beam standing wave is generated by using a mirror located outside the science cell. This mirror is positioned a distance of D = 22.5 cm away from the atoms along the y axis. At the location of the mirror the there is a node 4.4. RECOMBINATION 111 where the wave vanishes. If the laser frequency is shifted by an amount ∆ν, then the position of the nodes of the standing wave will change relative to the mirror. This will be reflected in a change of recombination phase φ. Specifically, the phase shift φ = 2y0 ∆k can be written in terms of the change in frequency, yielding φ = 4y0 π∆ν/c . This means that we expect N0 /N = 0 when: y0 π π 4 ∆ν = c 2 c ∆ν = (4.123) 8y0 Using the above equation, for y0 = 22.5 cm the expected change in frequency should be of 167 MHz. We achieved this change by applying a varying current to the diode laser. During the experiment, changing the frequency takes approximately 2 ms. With a nonzero φ, as in Eq. (4.66), the Hamiltonian we obtained using Û (y) in the {| 0i, | +2i, | −2i} basis is β −iφ β iφ 0 e e 2 2 β iφ Ĥs = ~ (4.124) e 4ωr 0 2 β −iφ e 0 4ω r 2 In a similar way to section 4.2.5, we look for a new basis to represent Ĥs such that one of the levels is decoupled leaving a coupled two level subspace. Likewise, if we set up a basis{| 0i, | +φ i, | −φ i} to obtain Ĥs | −φ i = 4ωr | −φ i we need 0 1 | −φ i = √ eiφ (4.125) 2 −e−iφ so an orthogonal vector to | −φ i is 0 1 | +φ i = √ eiφ 2 e−iφ (4.126) and the remaining state to complete our basis remains the same, so we keep | 0i. We proceed to calculate the new representation of Ĥs using the known matrix elements of Ĥs in the {| 0i, | +2i, | −2i} basis shown in Eq. (4.66). For example, ´ 1 ³ iφ e h0|Ĥs |+2i + e−iφ h0|Ĥs |−2i h0|Ĥs |+φ i = 2µ ¶ 1 β β β = + (4.127) = 2 2 2 2 Putting together the new representation of Ĥs we obtain: 0 β2 0 Ĥs = ~ β2 4ωr 0 0 0 4ωr (4.128) 112 CHAPTER 4. INTERFEROMETRY TECHNIQUES which is identical to the result obtained in Eq. (4.77). We note that our approach to modeling the recombination operation is equivalent to that presented in Sec. 4.2.5 but keeping track of the third state | −i. Now we can apply the solution to the two level problem to obtain a time evolution operator for the splitting sequence in the three level system. We start out by using the general time evolution operator obtained in Eq. (4.104), and plugging in the parameters for the first pulse in the optimized splitting sequence of section 4.2.5. This gets the time evolution operator for the first pulse. −1 1 0 1 1 0 √ −iπ/(2√2) 2e 0 0 −i Û1 = √ e 2 √ −iπ/2 2 (4.129) Next, we use the parameters of the free evolution in the optimized splitting sequence to get the time evolution operator during the time the laser is turned off. 1 1 0 Ûf ree = 1 −1 0 0 0 −1 (4.130) From section 4.2.5 we know that the dynamics of the Bloch vector for the second light pulse are symmetrical to those of the first pulse. For this reason, the parameters for the second pulse are identical to that of the first pulse, therefore the time evolution operator Û2 for the second pulse is just Û2 = Û1 . To get the total splitting operator for a three level system described by a Hamiltonian of the form in Eq. (4.128) and Eq. (4.77), we multiply the three operators in the order set by the double pulse sequence so Ûsplit = Û2 Ûf Û1 . 0 1 0 1 0 0√ −iπ/ 2 0 0 e √ −iπ/ 2 Ûsplit = e (4.131) Assuming no relative phase has been introduced between √ the arms of the interferometer, the state just before recombination is | +i = 1/ 2 (| +2i + | −2i). Here it has been written in the {| 0i, | +2i, | −2i} basis. It represents the two wave-packets travelling at ±2~k. The Ûsplit operator used during the recombination pulse is written and valid in the {| 0i, | +φ i, | −φ i} basis. Consequently, we must re-write | +i in this same basis in order to obtain the output state for the interferometer sequence. To get the representation of | +i in the desired basis, we project it onto the new 4.4. RECOMBINATION 113 basis. | +i = h+φ |+i | +φ i + h−φ |+i | −φ i ¢ ¢ 1 ¡ −iφ 1 ¡ −iφ = e + eiφ | +φ i + e − eiφ | −φ i 2 2 = cos(φ)| +φ i − i sin(φ)| −φ i (4.132) Finally we apply Ûsplit to | +i and obtain the output state of the interferometer as a function of φ. | ψf inal i = Ûsplit [cos(φ)| +φ i − i sin(φ)| −φ i] √ = cos(φ)| 0i − i sin(φ)e−iπ/ 2 | −φ i (4.133) Inspecting the result above, we can see that there are two states in the output. One state is the antisymmetric superposition of the plane wave states | ±2i with an additional phase included, while the the other is the rest state | 0i. In this way the probability to find the atoms in the rest state is given by: P (k = 0) = |h0|ψf inal i|2 = cos2 (φ) (4.134) In the laboratory we can measure the number of atoms in the rest state by taking a picture using the absorption imaging technique described in section [?]. Assuming no loss in the number of atoms loaded into the waveguide N after performing the interferometer sequence, the fraction of atoms brought back to the rest state N0 is given by the probability P (k = 0). Conversely, the fraction of atoms left in the moving state is given by P (k = ±2~k). For this reason, what we seek to measure during the interferometry experiment is the phase dependent fraction N0 /N given by: N0 /N = cos2 (φ) (4.135) We notice that if our interferometer is working correctly during the experiment, we should expect to get N0 = 0 when φ = π/2. Chapter 5 Experimental Results Up to now we have discussed the components that to be implemented in order to create our Bose-Einstein condensate interferometer. These components include the creation of a 87 Rb condensate, loading the condensate into a magnetic waveguide, and performing splitting and reflection operations on the condensate. The coordinate system used to describe the interferometer operations, Bragg beam and imaging system positioning and alignment is illustrated in Fig. 3.1. In this reference frame the origin is lined up with the center of the waveguide. To implement the interferometer we use the sequence of operations described in Chapter 4, and outlined in Figs. 4.4 and Fig. 4.6. Measurements of the number of atoms in the initial condensate and subsequent packets produced in the output state are carried out using absorption imaging. A black and white CCD camera in conjunction with its imaging lenses are mounted along the z axis directly above the center of the wave guide. The imaging system is described in Sec. 2.8. After the splitting and reflecting operations, it is important to ensure that we can eliminate all uncontrolled phases upon recombination of the wave packets. This condition guarantees that after having applied and controlled the relative phase between the packets, no external agents have contributed to the observed phase. Moreover, we must ensure that the packets remain coherent from shot to shot of the experiment causing the number fluctuation of the measurement N0 /N to remain small when taking measurements. This ensures that our number measurements as a function of the phase (see Sec. 4.4) has a smaller error, causing the contrast of our measurements to be increased. Before we took measurements of the output state described in the following section, we started by performing a simpler two-step scheme. The simple interferometer sequence involved a split, followed by a short propagation time (t1 < 8 ms), then a reflection followed by another propagation time equivalent to the first one t1 , and finally a recombination pulse. We label the interferometer sequences by the time between pulses like t1 − t1 . For example, the simple initial sequence to test the interferometers’ pulse operations is labeled as 5 - 5. This means 5 ms between the 114 5.1. EXPECTED OUTPUT STATE 115 initial split and the reflection, and 5 ms between the reflection and recombination pulse. We performed various t1 − t1 sequences (for t1 < 8 ms) and checked the output state after a applying no phase change and applying a π phase shift to the recombination pulse. Our results showed that most atoms came back to rest after no phase was applied in the recombination pulse. For example, in the 2-2 interferometer ∼ 73% of the atoms in the initial condensate returned to rest after applying a φ = 0 phase on the output. This demonstrated that our pulses were working correctly. The change in phase of the standing wave was achieved by controlling the current on the diode laser providing the Bragg beam which changed its frequency and in turn changed the position of nodes in the standing wave potential. The creation of the standing wave potential is explained in Chapter 4, and the dependence of the phase φ with the frequency change is given in Sec. 4.4. 5.1 Expected Output State We use the technique described in Sec. 2.8 to take absorption images of the condensates in the wave guide after they have completed the interferometry sequence described in Fig. 4.4. The experimental results observed after carrying out the interferometer sequence were consistent with the output state demonstrated by Eq. (4.133). Experimentally the results obtained included three basic types of output (see Fig. 5.1). If the phase of the splitting double pulse is kept fixed, then φ = 0 and all the atoms are brought back to rest. Applying a (2n + 1)π/2 phase shift (where n is an integer), meant all the atoms are transferred into the ±2~k states so that no atoms are observed at rest. Finally, any other phase would yield a linear combination of rest atoms and atoms moving at ±2~k, where the ratio of the moving atoms is 1 : 1. Depending on the phase applied upon recombination, the output could include up to 3 clouds of atoms to image and analyze. For this purpose, we wrote a specialized 2-D fitting program which analyzed the different cloud images. The fitting program is called AI 3 (Atom interferometer 3). It can simultaneously fit three wave packets. It also incorporates the ability for the fitter to zoom into the desired regions where the atoms are, reducing its exposure to background noise and decreasing the fitting time considerably. An outline of the program and its operation is given in appendix D. 5.2 Measurements Raw data is obtained in the form of absorption images which are then fit to a 2-D Gaussian function to obtain the number of atoms brought to rest N0 . The images observed match very well the expected output described in Sec. 5.1. We demonstrate 116 CHAPTER 5. EXPERIMENTAL RESULTS Figure 5.1: Illustration of the expected output upon recombination of the coherent wave-packets. (a) When φ = 0 the standing wave does not shift so in the output state all the atoms return to rest. (b) For φ = π/2 all the atoms are evenly distributed in the p = ±2~k states meaning no atoms will be observed at rest. (c) At an intermediate phase, a linear combination of p = ±2~k and rest wave packets are observed. 5.3. OUTPUT FIT FUNCTION 117 Figure 5.2: Absorption images of the output state for different phases of the recombination pulse. The condensate atoms and their position is shown by the dark clouds. As expected for φ = 0 all the atoms return to the stationary state | 0i. For φ = π/2 no atoms return to the rest state, implying the atoms must remain in the | ±2~ki. The phase φ = π/4 is half way between φ = 0 and φ = π/2. Applying it on recombination yields the expected linear combination of | 0i and | ±2~ki states. this agreement of the output states for three distinct phases φ of the recombination pulse in the images shown in Fig. 5.2. The interferometer sequences used include two reflection pulses between the split and recombine operations. This is to allow each wave packet to travel an equivalent path length. Each packet travels through both arms of the interferometer, requiring two reflection pulses, see Chapter 4. Accordingly, each interferometer sequence is labeled using the time experienced by the wave packets between splitting and reflection operations like t1 − 2t1 − t1 . For example, a sequence where the time between the initial splitting and the first reflection is 5 ms, the first reflection and the second reflection is 10 ms and the second reflection and the final recombination is 5 ms, is labeled as 5-10-5. The total interaction time of the interferometer operation is labeled T where T = t1 + 2t1 + t1 . We obtained data for several different operation times ranging from 3-6-3 ms to a maximum of 11-22-11 ms. We show the output signal for the 10-20-10 interferometer obtained from the average of two data sets in Fig. 5.3. 5.3 Output Fit Function Our interferometer characterization consists of measuring the number of N0 atoms brought to rest after recombination as compared to the total number of atoms N prior to splitting. In this respect, following the calculation in Sec. 4.4, we expect that 118 CHAPTER 5. EXPERIMENTAL RESULTS Figure 5.3: Output signal showing the fraction N0 /N as a function of φ. The data shown is the average of two runs for the 10-20-10 ms interferometer sequence. The data is fitted to the function A cos 2φ + y0 showing a visibility of V = 0.45 ± 0.10, demonstrating a coherence time of 40 ms. The data was obtained in 03/03/06 and 23/02/06. 5.3. OUTPUT FIT FUNCTION 119 Figure 5.4: Visibility of the output function for interferometer sequences of varying interaction time T . The error ∆V was calculated using the result in Eq. (5.10) and the visibility for T < 10 ms was obtained using Eq. (5.15). the fraction N0 /N will depend on the phase φ introduced during the recombination pulse. The dependence of the fraction N0 /N in φ is given by the expression in Eq. (4.135). Consequently, using a squared sinusoidal function with the appropriate phase will serve as an appropriate fit function. Hence we use the following form: N0 = A cos2 (φ) + y0 N 1 1 = A cos (2φ) + + y0 2 2 (5.1) (5.2) where A has been selected as a parameter for the amplitude of the probability of the output state, and y0 is a vertical offset. With this in mind, we can perform the substitutions 1/2A → A and 1/2 + y0 → y0 , in order to simplify the fit function. which gives: N0 Y ≡ = A cos (2φ) + y0 . (5.3) N Using absorption imaging, we expect the output signal of N0 (φ)/N after the recombination of the wave packets to have the above form. 120 5.4 CHAPTER 5. EXPERIMENTAL RESULTS Visibility A technique we can use to characterize the degree of coherence exhibited by the wave packets used in the interferometer sequence is to measure the visibility of the output signal over many runs. Before giving the exact equation from which to calculate the visibility, we must motivate its significance given the mathematical form of our output state and how it relates to the coherence of the wave packets. The various values for the fraction N0 (φ)/N will be fitted to the sinusoidal function described by Eq. (5.3). If we do not change the phase of the recombination pulse as compared to the splitting pulse, we expect all the atoms that were split into the ±2~k states to return to the rest state. This occurs because as explained in Sec. 4.4, quantum mechanical operations are reversible, and the recombination pulse is identical to the split pulse. However, if there are any external agents which cause the wave packets to acquire a relative phase shift, then on recombination, not all the atoms in the ±2~k states will come to rest. Moreover, if we desire to make multiple measurements of N0 /N for a fixed value of φ in the recombination pulse, any decohering effects will result in the value of N0 /N shifting from shot to shot. Hence, N0 /N will deviate from the expected value given by the model in Eq. (5.3), causing a decrease in the contrast of the sinusoidal signal. This effect has the tendency to “flatten out” the signal observed. In fact, the decrease in contrast of our signal is analogous to the decohering effects which cause a blurring in the interference pattern of light discussed in Sec. 1.4. For an output signal whose maximum and minimum values are given by Imax and Imin respectively, the visibility function is given by [3]: V = Imax − Imin Imax + Imin (5.4) An interpretation for the visibility function V is given by the ratio between the peak to peak value of the output function and twice its average value. Because the fraction N0 /N > 1, we multiply the average value by 2 in order to normalize the visibility such that 0 < V < 1. Applying such normalization means that the visibility value obtained will depend on the overall offset of the output signal. This makes sense because as the signal’s average value increases, the fluctuations (asuming the amplitude is fixed) become a smaller fraction of the total signal. This means the contrast is reduced. Using the fit function in Eq. (5.3), we obtain that Imax = y0 +A and Imin = y0 −A. Plugging in these values into Eq. (5.4) we obtain an expression for the visibility in terms of our fit parameters. V V (y0 + A) − (y0 − A) (y0 + A) + (y0 − A) A = y0 = (5.5) (5.6) 5.5. RESULTS 121 Given that, we can linearize the visibility function with respect to our fit parameters and obtain an expression for the error in the visibility. ·µ ¶ ¸2 ·µ ¶ ¸2 ∂V ∂V 2 (∆V ) = ∆A + ∆y0 (5.7) ∂A ∂y0 (5.8) Taking the partial derivatives found in the above expression we find: ∂V −A 1 ∂V = 2 = ∂A y0 ∂y0 y0 (5.9) Plugging the above derivatives into Eq. (5.7), we obtain the expression for ∆V yielding: sµ ¶2 µ ¶2 ∆AV ∆y0 V ∆V = + (5.10) A y0 sµ ¶2 µ ¶2 ∆A ∆y0 ∆V = V + (5.11) A y0 Finally, bringing together the above results, the expression for the visibility in conjunction with its error given our fit function parameter is: sµ ¶2 µ ¶2 ∆y0 ∆A A ±V + V = (5.12) y0 A y0 We measure V as a function of the sum of the time between pulses. In this way, the overall time of the interferometer sequence will reflect the total time the wave packets have evolved for. We seek to obtain an interferometer sequence in which the packets are propagating for the longest time, while still yielding a sinusoidal output signal like Eq. (5.3). In other words, we want to see how large T (the total time for the interferometer’s operation as explained next) can be while still having the packets coherent. Therefore, this will achieve the interferometer signal with longest coherence time. Applying the expression in Eq. (5.12) to each of the output signals of varying sequence times, we are able to obtain a quantitative analysis on the coherence of each sequence. The higher the visibility of each signal, the higher its contrast, therefore the higher its degree of coherence. Normally, we expect to have a drop in visibility as the time of the interferometer operation increases. 5.5 Results For the 10-20-10 interferometer the output signal was fit to the function in Eq. (5.3) yielding the following fit parameters, A = 0.24 ± 0.05, and y0 = 0.54 ± 0.04. Consequently, the visibility V = A/y0 for this signal yielded a value of V = 0.45 with 122 CHAPTER 5. EXPERIMENTAL RESULTS an error ∆V = ±0.10. We give the visibility of the output function for interferometer sequences of varying total time T in Fig. 5.4. The range of the total times for the interferometer sequences varies from 0 to 56 ms. As mentioned in Sec. 4.4, the rate at which we could change the laser frequency for recombination was limited. Therefore interferometer sequences with T < 10 ms used a set of points at φ = 0 to estimate the visibility. Assuming that y0 = 1/2 for φ = 0, we can obtain the minimum and maximum visibilities as: 1 Imax = A + (5.13) 2 1 Imin = −A + (5.14) 2 which means that the visibility V is equal to 2A. Using Eq. (5.3), the fit function at φ = 0 is Y (0) = A+1/2, and can be used to solve and substitute for A. Solving for A yields A = Y (0)−1/2. Plugging in this result into the visibility yields V = 2Y (0)−1. We know that Y (0) = N0 /N so we can finally write the average visibility using the form: V = 2hN0 /N i − 1. (5.15) The result of the output function of the 11-22-11 interferometer with T = 44 ms shows our longest attainable coherence time to date demonstrated by a visibility of V = 0.6 ± 0.17. For interferometer sequences with T > 44 ms, the visibility drops substantially, indicating a loss of coherence for the wave packets (see Sec. 5.6). Furthermore, the interferometer sequence having T = 44 ms exhibited the longest matter wave separation while still maintaining coherent wave packets. In other words, upon applying the recombination pulses using various values for the phase φ, the wave packets recombined according to the fit function in Eq. (5.3). The maximum matter wave separation obtained is pictured using absorption imaging in Fig. 5.5. We seek to obtain the largest possible arm separation. For this reason, it is to our advantage to maintain the best visibility for the longest time possible. In other words, maximizing the coherence time of the wave packets will permit us to maximize the time between pulses, hence maximizing the path length of the packets which can allow us to increase the arm separation. As Fig. 5.5 shows, we obtained two wave packets completely separated by a macroscopic distance of 0.26 mm from center to center of each packet. It should be noted that the picture shows atoms which are in a quantum superposition of being in the +2~k and −2~k translational states [67]. 5.6 Decohering Effects Unfortunately, we observe fluctuations in the measured value of N0 (φ)/N from run to run. This fluctuation has the effect of lowering the visibility of the interferometer’s 5.6. DECOHERING EFFECTS 123 Figure 5.5: Maximum matter wave separation yielding the largest arm separation of 260 µm for our Bose-Einstein condensate interferometer. This separation was obtained from the 11-22-11 interferometer, having imaged the packets 11 ms after the initial split. Wave packets are pictured using absorption imaging, 1 shows a 3-D representation of the absorption profile and 2 shows a 2-D image. Throughout this particular sequence, the wave packets remained coherent as demonstrated by the non-zero visibility of the T = 44 ms interferometer. Hence the atoms in this picture were in a quantum superposition of being in both peaks. Note, red color and height indicate the highest density of atoms. 124 CHAPTER 5. EXPERIMENTAL RESULTS output signal. One possible explanation is that fluctuations occur because of an instability in the frequency of the Bragg beam which creates the standing wave potential. We checked this supposition by setting up an optical interferometer derived from the Bragg beam and observed that there were no significant fluctuations in the beam. We did notice that the Bragg beam contained spatial noise that caused variations in the Bragg beam intensity of up to 20%. We believe that this fluctuation (from the expected Gaussian intensity cross-section) in the intensity cross-section of the beam is caused by imperfections in the glass cell. Additionally, multiple reflections inside the glass chamber cause random interference patterns see (Fig. 4.2). As a result the intensity of the Bragg beam varies randomly, causing imperfections in the standing wave potential. In turn this causes variations in the coupling strength of the different translational states | 0i, | ±2~ki to the Bragg beam, thus causing variations in splitting and reflection operations which cause fluctuations in the fraction N0 /N as a function of φ. The result is a decrease in the contrast of our output signal. Another decohering effect is the residual velocity experienced by the condensate after loading it into the magnetic wave guide. As mentioned earlier, this residual motion causes efficiencies of the reflection pulse between 80 - 100%. Clearly these ineficiencies will contribute to the lack of conservation in the total number of atoms in the experiment, consequently casusing the measurements of the fraction N0 /N to be inaccurate. Similarly, initial residual motion causes asymmetries in the splitting operation. This means that after the split, one packet will have a greater number of atoms than its counterpart. We observe that the difference in the number of atoms from packet to packet varied as much as 20%. The asymmetry in the number of atoms will cause one packet to have a larger self interaction energy. As a result, a relative phase shift between the packets is introduced, reducing the visibility of the output. This phase shift will fluctuate with velocity and increases with T , which is consistent with the observed data. Overall we see that V remains close to 0.5 for interferometer sequences whose T value ranges from 0 to 44 ms. For longer T ’s the visibility substantially drops to zero, suggesting a sharp drop of in the form of a step at T = 44 ms. However, the errors in the measurement are too large to be certain whether this sudden change is real, or just a reflection of the statistical noise. 5.7 Intrinsic Limits of the Output Next we discuss and explore the intrinsic limits for the output signal of our interferometer. These limits include fluctuations in the number of atoms as a result of the splitting ( and recombining) operation and the reduction of the interferometer’s 5.8. NUMBER FLUCTUATION 125 contrast due to the atomic interactions. We refer to the effect of the reduction in contrast due to interactions as phase diffusion. It will become clear that phase diffusion is an effect introduced as a direct consequence of the number fluctuation. 5.8 Number Fluctuation When the atoms are split using the Bragg beam, the number of atoms N+ and N− in their respective states | +2~ki and | −2~ki is not necessarily even. Due to the asymmetry in the splitting, the packets will have different self interaction energy causing a difference in phase between the two packets. Moreover, if the number of atoms after the split in the | ±2~ki states fluctuates randomly from run to run, so will the number of atoms N0 brought back to rest upon recombination. This means that there will be a fluctuation in the fraction N0 /N for a fixed φ from shot to shot. In the end the decrease in contrast of the output signal seen in Fig. 5.3 will be reflected in a decrease in visibility given by Eq. (5.12). To understand how the number fluctuations come into the variation of the total number of atoms in the separate clouds with N+ and N− , we make the following definitions wich represent the translational states after the split (see Sec. 4.2.5): | ψ+ i = | 2~ki | ψ− i = | −2~ki (5.16) (5.17) After the split of the condensate with N atoms, we assume the system can be written in terms of a product of state vectors in different Hilbert spaces, where each term of the product is a state representing a single atom which has some probability to be in the +2~k and −2~k state. Consequently there will be N such terms in the product such that: · ¸⊗N | ψ+ i + eiφ | ψ− i √ | ψi = (5.18) 2 where ⊗ is the Hilbert space product and φ is once again the relative phase shift acquired by one of the wave packets. This time the phase shift acquired by the packets travelling at −2~k is not due to a shift in the mirror position, but rather acquired through some external agent during its propagation. We can expand the above equation using the binomial coefficients given by the choose function: µ ¶ N (5.19) m This function gives the number of ways you can arrange m things out of N independent of the order. In our case m is an integer for the number of atoms in the −2~k 126 CHAPTER 5. EXPERIMENTAL RESULTS packet and N is the total number of particles. Writing out the binomial expansion we get, · µ ¶ 1 N N N −1 iφ | ψi = N/2 | ψ+ i + N | ψ+ i | ψ− ie + . . . + | ψ+ iN −m | ψ− im eimφ + m 2 i . . . + N | ψ+ i| ψ− iN −1 ei(N −1)φ + | ψ− iN eiN φ . (5.20) To find the expectation value and the variation for the number of atoms in each packet N+ and N− we define the following operators N̂+ and N̂− . N̂+ = N̂− = N X i=1 N X | ψ+ ii i h ψ+ | (5.21) | ψ− ii i h ψ− | (5.22) i=1 which then allows us to obtain the average number of particles in each of the ±2~k states. We can do this by applying hψ|N̂+ |ψi and hψ|N̂− |ψi giving hN+ i = hN− i = N/2. Similarly, we can obtain the variance for measuring the number of atoms in a packet corresponding to the +2~k or −2~k states. This is given by using the result for the variance of a measurement whose probability is given by the binomial distribution [17] as 1√ ∆N+ = ∆N− = N. (5.23) 2 In the end, this result tells us the intrinsic statistical variation in N± from shot to shot of the experiment and how we can expect the number of atoms in each packet to vary as a function of N . 5.9 Atomic Interactions We introduce the effects of atomic interactions by considering the Schrödinger equation using an approximation which models the interaction potential for atoms which scatter off each other. The function 4π~2 a U (rij ) = |ψ(rij )|2 M (5.24) gives the interaction between atoms [46, 45]. Above, a is the s−wave scattering length [15], M is the mass of 87 Rb and rij is the coordinate describing the distance between two colliding particles. Plugging this interaction into the Schrodinger equation with the relative coordinate rij gives the Gross-Pitaevskii equation [35, 46, 45]. · 2 2 ¸ ~∇ 4π~2 a ∂ 2 + Uext (r) + |ψ(r, t)| ψ(r, t) i~ ψ(r, t) = − (5.25) ∂t 2M M 5.9. ATOMIC INTERACTIONS 127 Above, Uext is the external potential sensed by the atoms. It should be noted that the interaction of Eq. (5.24) depends on density of the atoms which is just the probability |ψ|2 . Consequently, considering atom interactions in our interferometer would add a phase shift 4π~at N± φ± = (5.26) M V per atom in the 2~k or −2~k wave-packet. Here we have assumed that for large N± , N± − 1 ≈ N± . Setting κ = 4π~at/M V , the total phase shift for N+ and N− atoms will be given by: η+ = κN+ η− = κN− (5.27) (5.28) Because atomic interactions will add an additional phase shift to each wave packet, the observed phase shift in the output state will be the difference in the phase shifts for each packet η = κ(N+ − N− ). Accordingly, the output function derived in Eq. (5.3) will have an additional phase induced by interactions such that: N0 = A cos(2φ + η) + y0 N (5.29) As noted, the phase η depends on the difference between the number of atoms in each packet before recombination. Therefore any uncertainty in the number of atoms in each packet will be reflected in an uncertainty in the phase due to interactions ∆η. With this in mind we seek to find how to characterize ∆η. Assuming the total number of atoms is conserved then N = N+ + N− . This allows us to write N− = N − N+ . Additionally we can define the quantity q which is proportional to η such that, q = N+ − N− (5.30) Substituting N− = N − N+ into q yields the expression q = 2N+ − N , in which case the uncertainty in q is given by the following expression ∆q = 2∆N+ (5.31) In this way we have found an expression for the uncertainty in the quantity q which is directly proportional to the extra phase η acquired by the output signal of our interferometer. We know that η = κq therefore the uncertainty ∆η = κ∆q. From Eq. (5.23) we can get a result for the uncertainty ∆N+ which we can plug into Eq. (5.31) to get √ N (5.32) ∆(N+ − N− ) = √ (5.33) ∆η = κ N 128 CHAPTER 5. EXPERIMENTAL RESULTS This uncertainty in the phase η acquired due to atomic interactions will cause a reduction in the contrast and therefore the visibility of the output signal. The effect can be described as follows. We can assume that the probability P (η) to make a measurement with some value η is described by the Gaussian function which is normalized over all η: 2 1 − η √ e (∆η)2 P (η) = (5.34) ∆η π Given the above distribution for η, the output signal for a given value of N0 /N will vary for a fixed value of φ. Hence we take the average of N0 /N over the different vales of η. N0 (φ)/N ∼ hcos(2φ + η)iη Z ∞ 2 1 − η √ e (∆η)2 cos(2φ + η) dη ∼ −∞ ∆η π 2 /4 ∼ e(∆η) cos(φ) (5.35) (5.36) (5.37) The above equation shows that the signal obtained is equivalent to the original output given in Eq. (5.3) but with a coefficient which reduces its overall amplitude. As a result, due to the atomic interactions, we observe a signal with reduced visibility. This example illustrates in a very intuitive way how atomic interactions will cause a “blurring” effect to the output signal. Moreover, an increase in the interaction strength κ will increase ∆η hence decrease the visibility exponentially. Chapter 6 Conclusion The work presented in this thesis began in the summer of 2002. Specifically, I and several others had the opportunity to begin the task of setting up most of the apparatus used to carry out this experiment. Thankfully after four exciting years, the goal of implementing a functional Bose-Einstein condensate interferometer was achieved. 6.1 Achieved Interference Our interferometer has demonstrated that in general we can successfully split the condensate into two equal parts in the waveguide potential, then let the packets separate for some distance to later recombine them while maintaining their quantum coherence, Fig. 4.6. Moreover, upon recombination of the wave packets, the output state of the interferometer matched the predicted model in Eq. (5.3). Hence, we were able to achieve interference between matter waves. As described by Fig. 5.4, we have achieved an output interference signal like Fig. 5.3 which remains coherent for total interferometer times of T up to 44 ms. This is demonstrated by the non-zero visibility which remained on average around 0.5, of the output signal for 0 < T < 44 ms. This means that while the wave packets propagated along the wave guide, they remained in a coherent quantum superposition for a total time of 44 ms. Up to date most experiments dealing with coherent matter waves have had coherence times limited to 10 ms [12], however recent experiments ([54]) have reported coherence times up to 200 ms. In the latter case, G.-B. Jo et al. have loaded a 23 Na condensate into a single wire magnetic trap on a chip with radial frequencies such that ωr = 2.1 kHz and the vertical frequency ωz = 9 Hz. Using a radio frequency field ramp, they separated the original trap into a double well potential in which the minima of each well were separated by a distance of 8.7 µm. As a result of the split potential, the condensate was separated into two packets, located at the minimum of each well. The two 129 130 CHAPTER 6. CONCLUSION packets were held separated for varying times, then released from the trap causing them to fall and interfere when their expansion caused them to overlap during the time of flight. The phase shift between the packets was obtained by controlling the relative height of the minima in the double well potential. The relative phase of the packets was obtained by resolving the interference fringes of the overlapping condensates using absorption imaging. As their results demonstrate, they observe a dramatic decrease in the number fluctuations δN for each packet due to inter-atomic interactions. Due to repulsive interactions when the condensate is split, the atoms preferentially divide evenly among the wells as this is more energetically favourable. In other words they observe number squeezed states. In particular they observe squeezing by a factor of ≥ 10. Consequently for magnetic potentials with trapping frequencies as mentioned above, the coherence time of the wave-packets is increased by a factor of 100 as compared to the maximum coherence times limited by phase diffusion effects Sec. 5.6. However, number squeezing has the effect of increasing the quantum uncertainty in the phase. Given that, we believe that the leading cause for the long coherence times observed in our interferometer is the weakly confining waveguide potential used for the interferometer, see Sec. 5.7. Due to lower confinement forces, the density in the waveguide is reduced, lowering the interaction energies which introduce unwanted phase shits. These phase shifts cause the wavepackets to decohere, thus eliminating the contrast observed in the output state. Given the effects described in [2], for a condensate having a number of atoms NA ≤ 1.5 × 104 , we do not expect the phase diffusion effects in Sec. 5.7 to reduce the contrast of our interferometer for operation times of ≤ 1 s. Olshanii et al. have noted that the interaction between atoms during the initial splitting can cause a phase gradient in the different packets. As the atoms separate, one end of a cloud interacts for a time corresponding to a full length travel through the opposing cloud, while the end that separated first only interacts briefly, corresponding to a minimal travel time through the opposing cloud. If the condensate has a chemical potential µ, and the separation time is τs then the differential phase introduced is in the order of µτ /~. Due to this differential phase, when we apply the recombination pulse using a certain φ, not all the atoms will transfer to the expected translational state for that φ, therefore decreasing the visibility of the output signal. For example, applying the Thomas Fermi approximation [45] given the density in our waveguide, µ for our condensate is ≈ 2π~ × 10 Hz. This gives a differential phase of 0.2 rad using a separation time τs = 3 ms. We can compare this to the experiment by Wang et al. [12] which had a differential phase of 3.33 rad. This demonstrates how a weakly confining trap reduces the differential phase. To our advantage, the weakly confining trap used in this experiment also reduces the condensate’s sensitivity to mechanical vibrations of the trap structure. Additionally, it reduces the required precision of alignment of the Bragg beam standing wave to the guide axis. 6.2. LONG ARM SEPARATION 6.2 131 Long Arm Separation Another important achievement for this experiment was the long separation between the arms of the interferometer we had initially aimed for. Up to date, we believe to have obtained the first literal image of a matter wave that has been split and separated by a macroscopic distance of 0.26 mm, while still preserving quantum coherence. In other words, the atoms in Fig. 5.5 are in a quantum superposition of the translational states | ±2~ki. This is demonstrated by the a visibility of 0.6 Fig. 5.4 for an interferometer whose total interaction time is T = 44 ms. In this experiment, the coherence demonstrated by the condensates brings more experimental evidence of the wave-like nature of matter. 6.3 Future Adaptations The large arm separation shown in this interferometer promises several different future applications. For example, the long separation between packets may permit one arm of the interferometer to enter an optical cavity and acquire a phase shift due to to the electromagnetic field present. This type of experiment could be used to measure the number of photons in the cavity using non-destructive techniques similar to experiments by Nogues et al. [68]. In the case of such an interferometer, it would be more sensitive to smaller phase shifts, permitting the atoms-photon interaction to be off-resonant, thus making it a simpler technique. This type of experiment would have applications in quantum communication and QED [69]. Other examples include taking advantage of the arm separation to bounce one of the packets off a surface. The wave packet would bounce due to quantum reflection meaning the phase shift due to this effect could be measured. This could be used to measure effects like the Casimir-Polder force. Finally, our laboratory plans to set up an experiment where the electric polarizability of 87 Rb can be measured. The long packet separation can be used to position a set of electrically charged plates at the end of one arm of the interferometer. The plates will be aligned with the waveguide, permitting one packet to enter it momentarily during the interferometer operation. Then, the electric field of the plates will induce a phase shift in one of the packets that can be measured to obtain the polarizability of 87 Rb. We mentioned our limitations in Sec. 5.6. For this reason we are trying to improve the efficiency of the interferometer operations with the Bragg beam by improving the science cells’ windows, thus improving the uniformity of the beam. We also wish to reduce the residual motion of the condensate after loading the waveguide by varying the loading sequence. By controlling the magnetic fields we can avoid unwanted resonant oscillations in the waveguide. In conclusion, we have achieved and observed an atom interferometer with the greatest arm spacing to date. We believe our experiment has demonstrated a fun- 132 CHAPTER 6. CONCLUSION damental principle in quantum mechanics. It has done so by exposing the wave nature of matter, hence matter’s ability to interfere like a wave. My hope is that the work presented here will be of pedagogical value to anyone interested in science, contribute to the understanding of quantum mechanics, science in general and the human desire in understanding nature. Appendix A Temperature Interlock We use a spherical quadrupole field to generate the magnetic trap to transfer the atoms to the science cell and to create the TOP trap. In both situations we must apply 750 A of current (using a custom built high current switch [70]) to obtain the correct field gradient. This causes a large amount of heating in the coils (see Sec. 2.4.3). The coils are made of copper tubing through which we can pump chilled water to prevent overheating. However, the water cooling system requires constant flow of water at 2.5 L/min. Otherwise, when operating at full current, the water inside the coils can exceed 100◦ C and cause explosions of steam which cost hours worth of cleaning optics. For this reason we configured two interlock systems which were connected in series. A water flow interlock monitored that the flow remained at the correct level (see [21]), and a temperature interlock monitored the temperature of the copper coils themselves. In this way, if any of these two conditions failed, the current to the quadrupole coils would be turned off. So far the system has worked to great satisfaction. The circuit design of the temperature interlock is shown in Fig. A.1. It includes the usage of a chip specially designed to work in monitoring thermocouple signals, converting them to a convenient voltage output. 133 134 APPENDIX A. TEMPERATURE INTERLOCK Figure A.1: Circuit diagram for temperature interlock. Thermocouple leads which measure temperature are on the upper left corner, solid line represents constantan (alumel) and dashed represents iron (chromel). The leads are connected to an amplifier specially designed for thermocouple configurations. The output of the thermocouple chip is calibrated to 10 mV/◦ C and is fed to a comparator. The temperature signal is then compared to a set point which can be adjusted as needed. If the temperature signal exceeds the set point, the relay opens. All the chips on this circuit are labeled according to their data sheets. Each chip type can be identified by the part number. Appendix B Control Panel In order to control and synchronize the experimental apparatus used in making BEC and performing the interferometry experiment, we use the Adwin-Pro real time controller system. The current Adwin-Pro controller functions as a stand alone box communicating to a computer via an Ethernet connection. Adwin-Pro has 24 digital and 8 analog channels available, doubling the number of apparatus that we could originally control using the Adwin (computer card). The output bus, having twice as many channels as the original controller, connects to a new version of the switch panel also made in the lab see Fig. B.1. A description of the apparatus assigned to each digital/analog channel is given in Table B.1. There are two main functions for the switch panel. First, it allows users to switch the control of a particular device between computer or manual for all digital channels. In manual operation, the user can choose between a high (5V) or low (0V) output. Additionally, because the switch component inside the panel introduces unwanted fluctuations of the output signal, the panel includes a de-bouncing circuit which filters out any unwanted oscillations that could pass on to the controlled device. Details of the de-bounce circuit, its components and operation are shown in Fig. B.2 135 136 APPENDIX B. CONTROL PANEL Figure B.1: Set up of real time experimental control. Black dots are switches, clear dots are LED’s, red/black dots with circles are inputs/outputs. (a) Computer is connected to Adwin Pro via an ethernet connection. (b) Adwin Pro connected to (c) the output control panel. The left side of the panel contains twenty four threeway switches with LED’s that can be set to manual (on/off) or computer control. The respective outputs are on the right side in addition to synchronization inputs and RS 232 control input.(d) Output/monitor panel for the eight analog channels, user can select to monitor external inputs or internal analog channels. (e) BEC/ALT output selector panel, user can switch the outputs for different experiments e.g. BEC or alternative. Eight ethernet analog/digital alternate inputs 137 Figure B.2: De-bounce circuit for a single digital channel in the real-time control panel. There are twenty-four digital channels, each having a copy of this circuit in order to eliminate unwanted electrical noise when using the manual on/off setting. The labeling on each circuit component matches the description found in their data sheets. Each component is labeled with their respective part number. The Switch on the top left indicates the pin connections being used (depicted in the 5 V (ON) manual position). 7 8 1 2 3 4 5 6 Analog Channels Double pass frequency (−10 V → 10 V) Bragg beam Amplitude (0 V → 1 V) Big B field current (0 V → 10 V) Waveguide Quad Current (−5 V → 5 V) Wave Guide bias current (−5 V → 5 V) -EOM bias (0 V → 5 V) -Waveguide ext.coils amplitude(−5 V → 5 V) Double pass amplitude (0 V → −1 V) Bragg beam current control (0 V = φ = 0, 1.1 V φ = π) Table B.1: Description of the function associated with each digital and analog channel controlled by Adwin-Pro. 15 digital (out of the 24 digital channels) and all 8 analog channels were used. Digital channel “O” was used to trigger a switcher which selected between two outputs on analog channel 6 G Big B field on/off H Waveguide on/off I Pumping bias Field on/off J CCD trigger K Track move trigger L Waveguide Ext M Frame Grabber trigger N O Analog switcher doubler ch6. P Q R S MOT Shutter T Bragg beam Shutter (fast) U V W X RS232 out A B C D E F Digital Channels MOT + Re-pump AOM Pumping beam AOM Diode 2 AOM MBR Probe AOM 138 APPENDIX B. CONTROL PANEL Appendix C Sequences We include below the sequences used to make BEC and perform the interferometer operations using the digital and analog channel convention presented in Sec. B. Both the BEC sequence and the interferometer sequence have standard subsequences which are also given. It proved to be very useful and flexible to insert functioning sub-sequences into the larger more complex sequences. It also gave an object oriented approach to building sequences just like subroutines do in normal coding. loadcmot Time [ms] 88 15 0 1 0.2 Active acgks agks aks ciks bciks 1 2 0 0 0.5 0.6 0 0.05 3 0.25 0.25 0 3.2 3.2 Analog 4 0 channel 5 6 7 8 0 0 0 0 2 0 5 -0.3 5 0 5 0 Table C.1: Sequence showing steps used to load the CMOT. Blank space denotes previous value 139 140 APPENDIX C. SEQUENCES movetrap Time [ms] 4 1 50 200r 1850 Active gk cgk gk gk ga 1 2 3 -1.2 0 3.2 Analog channel 4 5 6 0 0 5 10 10 0 0 7 8 -1 0 0 0 Table C.2: Sequence showing steps used to move the translation stage holding the spherical quadrupole field. Blank space denotes previous value, r denotes a linear ramp from the previous value. probesplit Time [ms] 0.2 0.05 0.1 30 Active js djs js a 1 2 3 -0.07 0 0 Analog channel 4 5 6 0 0 5 5 5 7 8 0 0 0 -1 Table C.3: Sequence showing steps used to take absorption images of the condensate in the waveguide. Blank space denotes previous value splitpulse Time [ms] 0.024 0.033 0.024 Active ht 1 2 3 0.18 -0.016 0.18 Analog channel 4 5 6 7 8 Table C.4: Sequence showing steps used to split the condensate in the waveguide. Blank space denotes previous value reflectpulse Time [ms] 0.067 Active ht 1 2 3 0.27 Analog channel 4 5 6 7 8 Table C.5: Sequence showing steps used to reflect the condensate in the waveguide. Blank space denotes previous value 141 interferometer Time [ms] loadcmot movetrap 500 rs232 b ag 500 500 10000r rs232 d agh 100 1000r 1000r 800e 250r 10 splitpulse 10 reflectpulse 20 reflectpulse 10 splitpulse 40 probesplit 26000 500r 40 probesplit 1850 rs232 a k 100 Active 1 ag 0 ag agh agh 0 2 0 3 Analog 4 10 0 agh ht 2 1 0.007 -0.016 0 -0.016 het -0.016 ht -0.016 ht -0.016 hjs -0.07 -0.016 a agh ghjs 0 0 -0.07 k acgks 0 0 0 0 0 5 -1 -5 5 -3 3.3 -3 5 8 0 0 0.8 0 0 0 0 0 3.3 0 0 0 0.25 0 7 10 8 agh agh channel 5 6 0 5 0 0 5 0 -1 0 0 0 0 0 0 0 Table C.6: Sequence showing 10-20-10 interferometer operation. Blank space denotes previous value and r denotes a linear ramp from previous value. Using e denotes an exponential ramp. Pre-defined subsequences are used as subroutines. Rs232 command denotes which evaporation sequence to use with the first letter and remaining letters are channels that remain constant from the previous step. The RS 232 commands follow the format described in Table 2.3, different letters are used for different evaporation sequences, see [48] Appendix D Image Analysis Program Two image analysis programs were developed and thus used according to the experimental circumstances. The program Sponge was created to analyze images of single atom clouds. However, when operating the interferometer, the resulting images contained multiple smaller clouds which became cumbersome to analyse using Sponge. For this reason we developed a second image analysis program called by the acronym AI 3, meaning atom interferometer three. The program’s main feature is the capability to analyse up to three images in a single run. In summary, the program uses a two dimensional function described below to fit to each individual cloud. The fit outputs the absorption and width parameters of the clouds needed to calculate the number of atoms in each cloud. Upon start-up, the program consists of a graphical user interface containing a display for the image being analyzed (main image), 6 smaller displays for a zoom of the three clouds and their resulting fit, 6 displays for the “x, y” cross-sections of the fits and boxes for the parameters of the fits. D.1 Fit Function AI 3 uses an image S(x, y) which is derived from processing 3 images as described in Sec. 2.8. A script program is automatically run after taking the last image in the probing sequence which generates the final image to be analyzed by AI 3. The function used to fit the two dimensional absorption profile S(x, y) is given by: · 2 x−x0 F (x, y) = exp A − Be( wx ) 2 ¸ y−y − w 0 y · x − x0 × 10 ¸4 · y − y0 10 ¸4 (D.1) where x0 and y0 are the cloud’s center position, wx and wy are the widths of the cloud along their respective coordinate, A is an overall offset and B is the absorption coefficient. AI 3 uses the Matlab built in function “fminsearch” to search for the 142 D.2. OPERATION 143 parameters which minimize the value of a χ2 between the model presented above and the image values of the array S(x, y). The last two factors in brackets are there to significantly reduce the χ2 in the region outside the cloud. Therefore reducing the search performed by Matlab’s “fminsearch” function. D.2 Operation The program is stored in two locations, in the desktop of the computer casslab 6 (set up in case the network drive is not accessible) and the network drive location R:\\home\casslab\source\AI 3. The program is run by starting up Matlab and typing AI 3 at the prompt. The directory containing the desired copy of AI 3 to be run should be set in the path of Matlab. AI 3 has a startup file which sets the working directory to the previously used directory from where images were analyzed. Once the program is displayed, the user selects the image to be analyzed by using the browse button. This also sets the working directory which is stored in the startup file and displayed in the directory box. The next step is to provide AI 3 with the centers for each cloud. Depending on the output described in Sec. 5.1, the user should select the cloud with the highest “visible” absorption coefficient (we will refer to this as the main cloud). This is done by clicking the radio button (top, center or bottom) which corresponds to the relative position of the cloud with strongest absorption, and then clicking the main image on the center of the main cloud. AI 3 has a built in function which tries to calculate the center of the two remaining clouds. It does so by using the time in ms set in the “time after rec” box, which should be the time between the recombination pulse and the time the atoms image was taken. Additionally, this function requires setting the “x calibration” and “y calibration” boxes correctly. These boxes contain the number of pixels/mm along each dimension corresponding to the magnification of each image. Usually the calibration is done by taking an image of a ruler’s scale at the position of the atoms. AI 3 proceeds to draw three sub-images centered and zoomed around the calculated (and user provided) center for each cloud. If the sub-images are not properly centered on the the clouds, the user can click on the desired new center of each sub-image to recenter the sub-image. Every time the images are clicked, the corresponding centers are displayed in the “x o pos ” and “y o pos ” boxes (pos indicates whether it is top center or bottom). If previously not set (in the startup file), the user sets the “guess” value for each parameter of the fits by entering the value into their respective boxes. For each sub-image there are six different parameters. The parameters end with t, c, or b denoting the top, center and bottom image respectively. The parameters correspond 144 APPENDIX D. IMAGE ANALYSIS PROGRAM to those described in Eq. (D.1). The user can also choose to fix the fit parameter by clicking the check box to the left of each parameter box. In doing so, AI 3 will simply plug this value into Eq. (D.1) and not vary this parameter during the fminsearch. To perform the actual fits, the button “Analyze” is pressed. After some time, the resulting fit parameters overwrite the guess values in their boxes. Additionally, the fraction N0 /N is displayed in the box “N 0/N”. It calculates this number using the B coefficients of each cloud. AI 3 can also export the resulting fit parameters into a running Excel spread sheet. The user can select the export row by inserting the row number in the “Export Row” box and the export column by selecting a letter from the scroll menu next to the parameter to be exported. To export, the user should check the box to the right of the parameter to be exported. As a result of the fit, AI 3 will display the results as a two-dimensional absorption function for each cloud. The absorption for each cloud will be represented by a color map shown in Fig. D.1 as a function of position. Additionally, a cross section through the center position of each cloud along “x” and “y” is displayed comparing the fit function with the measured absorption. D.2. OPERATION 145 Figure D.1: Screen shot of AI 3. The main image is displayed on the top left. The upper right boxes include: the working directory, browse button, “x” and “y” calibration boxes and the “time after recombination” box. Below there are 6 boxes for each cloud (top, center and bottom). Each box corresponds to the fit parameters in Eq. (D.1). To the left of each parameter box is a check-box to choose whether the parameter remains fixed during the fit. To the right there is a check box to export and a scroll menu to choose the export column. Further below are the “Analyze” button, “Export Row” box and the “N 0/N” box. The top row of remaining axes display in adjacent pairs the measured cloud and the fit 2-D function. Similarly, the bottom row displays adjacent pairs of x y cross-sections comparing the fit function and the measured values through the centers of each cloud Appendix E Experiment Setup Probably one of the most important experimental tools in our interferometry experiment is the laser. We utilize three different lasers in total. To create a MOT we use a 10W, V-10 (Verdi) diode laser at 532 nm to pump a Ti:Sapphire crystal, monolithic ring cavity laser MBR-110 outputting 1.3W of light ranging from 700nm to 1000nm. The monolithic block design means the entire cavity is machined out of a single special aluminium alloy, ensuring passive stability. Both units are manufactured by Coherent. The second laser is a diode laser Toptica DL 100 outputting 15-18 mW of light in the 779 nm to 785.2 nm optical range (not mode hop free), we use this laser to create our standing wave Bragg beam that splits, reflects and recombines the condensates during the interferometer sequence. We label this laser Diode I. Finally, a custom laser system using a configuration including a diode in conjunction with an external cavity was built. It outputs 30 mW - 40 mW of power, lasing in the range of 780.2 nm to 780.5 nm. We use this system to provide additional re-pump light (780.232nm) to our MOT, increasing the number of atoms trapped by the MOT and eventually loaded into the magnetic wave-guide. Most importntly we used it during our optical pumping stage Sec. 2.4.2. To generate the re-pump laser frequency used in making a MOT we use an electro optical modulator at 6.8GHz. The output introduces additional frequency sidebands to the beam offset by ±6.8GHz from the input frequency of 780.246nm. As seen in Fig. E.1 the EOM does not introduce any spatial shift in the poynting vector of the laser. The output is used for the vertical beams of the MOT. The sidebands are created in a crystal inside the unit which interacts with the input light. In turn the phonons are made and modulated by an RF signal which is controlled and locked by a custom built driver circuit. Details on the specifics of the driver circuit can be found in J.M. Reeves’ thesis project [21]. 146 147 Figure E.1: A Top view of the layout of the main beam path, not to scale. Beam starts at the bottom right corner after exiting the Mbr-110 (Ti:Sapphire) leakage light enclosure. The letters denote beams that are matched up to to the same lettered beam on Fig. E.2. Dashed lines denote a beam going in or out of the page, labeled up or down. Although not shown, the glass chamber would be located above the figure itself. Diode I and Diode II not shown. 148 APPENDIX E. EXPERIMENT SETUP Figure E.2: Top view of the two glass chambers with MOT and imaging beams configuration. This diagram continues the layout of the beams labeled by letters on Fig. E.1. Dashed lines denote a beam going in or out of the page, labeled up or down. Diode I and Diode II not shown. 149 Figure E.3: A top view of the entire optical table illustrating the beam configuration for Diode I and Diode II. A flip mirror soon after the beam exits the MBR-110 leakage light enclosure, redirects the normal beam path of the beam to-wards a fiber coupler which sends the light to a separate table. When the flip mirror is down the beam path goes to the first λ/2 retarder of the beam path shown in Fig. E.1. Appendix F Mathematical Calculations F.1 Two Level Solution In order to obtain the time evolution of the state vectors in the two level problem described in chapter 4, we must find the solution to the Schrödinger equation containing the effective Hamiltonian Ĥef f in Eq. (4.33). Writing out the time dependent equations we obtain: ċg = −i Ω d 2 Ω d˙ = i∆d − i cg 2 (F.1) (F.2) Taking one more time derivative of Eq. (F.2) yields: Ω d¨ = i∆d˙ − i ċg 2 (F.3) were we can plug in the corresponding expression for ċg found in Eq. (F.1). This gives a second order equation for d such that: µ ¶ Ω Ω d¨ = i∆d˙ − i −i d (F.4) 2 2 Ω2 d (F.5) d¨ = i∆d˙ − 4 which can be re-written as a second order homogeneous equation. Ω2 d¨ − i∆d˙ + d=0 4 (F.6) Inspecting Eq. (F.6), we can extract a characteristic quadratic equation corresponding to the orders of the time derivatives of d in terms of the parameter m (which 150 F.1. TWO LEVEL SOLUTION 151 asumes a solution of the form eimt ): m2 − i∆m + Ω2 m=0 4 (F.7) In the equation above, m is no longer used as an integer (as in previous chapters). Solving the equation for m we obtain two solutions: m± = i ´ √ 1³ ∆ ± ∆ 2 + Ω2 2 (F.8) √ where m± denotes the two distinct solutions. We can define X ≡ ∆2 + Ω2 in order to make our solution to m more elegant such that m± = i1/2(∆ ± X). Given the solution to the characteristic equation, we can then write the solution to d(t) as a sum of exponentials with the powers of m± t. d(t) = Aeim+ t + Beim− t ¡ ¢ d(t) = ei∆t/2 AeiXt/2 + Be−iXt/2 (F.9) (F.10) where A and B are constants. By adding the right constants and exponentials, we can re-write the above equation such that we can make the replacements AeiXt/2 → A0 cos (Xt/2) and Be−iXt/2 → B 0 sin (Xt/2). d(t) = ei∆t/2 (A0 cos (iXt/2) + B 0 sin (iXt/2)) (F.11) We can find A0 by using the initial condition d(0) = d0 , therefore allowing us to write: dt = ei∆t/2 (d0 cos (iXt/2) + B 0 sin (iXt/2)) (F.12) Additionally we can obtain the time derivative of d using the chain rule giving: µ ¶ −X X ∆ i∆t/2 0 ˙ = i d(t) + e d0 cos (iXt/2) + B sin (iXt/2) (F.13) d(t) 2 2 2 where we can introduce the value for d(t) in Eq. (F.2) giving µ ¶ ∆ −X X 0 Ω i∆t/2 d0 sin (iXt/2) + B cos (iXt/2) . (F.14) i∆d − i cg = i d(t) + e 2 2 2 2 If we apply the initial condition cg (0) = c0 for t = 0 we can obtain a result for B 0 such that: i∆d0 − i Ω ∆ X c0 = i d0 + B 0 2 2 2 ∆d − Ω c0 0 B0 = i X (F.15) (F.16) 152 APPENDIX F. MATHEMATICAL CALCULATIONS Introducing the value of B 0 into Eq. (F.12) we obtain the final expression for d(t): · ¸ Ω i∆t/2 d(t) = e d0 cos (iXt/2) + id0 sin (iXt/2) − i c0 sin (iXt/2) . (F.17) X In order to find the solution for cg (t) we can plug the above result into Eq. (F.2) and solve for cg (t). First we write: cg = i i 2 h˙ d − i∆d Ω (F.18) then the right hand side of the above equation becomes: · ∆ −X i∆/2 d˙ − i∆d = −i d + e − d0 sin (Xt/2) 2 2 ¸ ∆ Ω +i d0 cos (Xt/2) + i c0 cos (Xt/2) 2 2 h 1 i∆t/2 ∆2 ∆Ω = e − i∆d0 cos (Xt/2) + d0 sin (Xt/2) − c0 sin (Xt/2) 2 X X i −Xd0 sin (Xt/2) + i∆d0 cos (Xt/2) − iΩc0 cos (Xt/2) h = ∆ Ω i∆t/2 e − ic0 cos (Xt/2) − c0 sin (Xt/2) 2 X µ 2 ¶ i ∆ X + − d0 sin (Xt/2) XΩ Ω (F.19) We can simplify the above expression by inspecting the last term and noting that: µ ¶ ∆2 X 1 ∆2 X 2 − = − (F.20) XΩ Ω X Ω Ω µ ¶ 1 ∆2 − (Ω2 + ∆2 ) = (F.21) X Ω Ω (F.22) = − X so that: ¸ · Ω Ω ∆ i∆t/2 d˙ − i∆d = e −ic0 cos (Xt/2) − c0 sin (Xt/2) − d0 sin (Xt/2) (F.23) 2 X X therefore, writing the final form of cg (t) we obtain: ¸ · Ω ∆ i∆t/2 cg = e c0 cos (Xt/2) − i c0 sin (Xt/2) − i d0 sin (Xt/2) X X (F.24) F.2. MATRIX ELEMENTS OF ĤS 153 In the end, the solution for the state vector [cg (t), d(t)] can be written in matrix form giving: · · ¸ ¸ cg (t) c0 i∆t/2 M̂ =e (F.25) d(t) d0 where: · M̂ = Ω ∆ sin (Xt/2) −i X sin (Xt/2) cos (Xt/2) − i X Ω ∆ −i X sin (Xt/2) cos (Xt/2) + i X sin (Xt/2) ¸ (F.26) Next, we show how to obtain Eqns. 4.41 and 4.42 which use the Hamiltonian in Eq. (4.33) including an extra phase φ. If we have a Hamiltonian like that in Eq. (4.40), when we include it in the Schrödinger equation we obtain: d˙ = i∆d − iΩ cos (ωt + φ) cg Ω = i∆d − i (ei2ωt+iφ + e−iφ )cg 2 (F.27) Similarly for cg we obtain: ċg = −iΩ cos (ωt + φ)e−iωt d ¢ Ω ¡ iφ = −i e + e−i(2ωt+φ) d 2 (F.28) We apply the rotating wave approximation, which means that the terms oscillating at a rate ω average out to 0. In this way we get: Ω ċg = −i eiφ d 2 Ω d˙ = i∆d − i e−iφ cg 2 F.2 (F.29) (F.30) Matrix Elements of Ĥs Finally, the following calculation explains how to obtain the matrix elements of Ĥs presented in Eq. (4.66). We use the coordinate representation of the three states | ±2~ki and | 0i such that: ψ0 (y) = hy|0i ψ0 (y)ei2ky = hy|2~ki ψ0 (y)e−i2ky = hy|−2~ki (F.31) (F.32) (F.33) where ±2~k is the recoil momentum given by the standing wave potential in Eq. (4.61). Here the function ψ0 (y) is normalized over all y space. In this case ψ0 (y) represents the initial wave-packet loaded into the wave-guide, hence it can be thought as the 154 APPENDIX F. MATHEMATICAL CALCULATIONS condensate wave-function described by the Thomas Fermi model [45]. First we note the completeness relation [15] which we will make use of: Z | yi ih yi | dyi = 1 (F.34) where i is an integer representing the different positions in y−space. Additionally we use the ortho-normality relation of our chosen basis (j is an integer equivalent to i): hyi |yj i = δij . (F.35) In calculating the matrix elements of Ĥs we note that the kinetic energy term can be handled as follows: p̂2 | 0i = 0 2M p̂2 4~2 k 2 | +2i = | +2i = 4~ωr | +2i 2M 2M p̂2 4~2 k 2 | −2i = | −2i = 4~ωr | −2i 2M 2M (F.36) (F.37) (F.38) where p̂2 /2M is the kinetic energy operator having p̂ as the momentum and M as the packet’s mass. In this way we define the recoil frequency ωr = ~k 2 /2M just as in Eq. (4.66). We use the convention where the rows of Ĥs are indexed according to the momentum states in the order {0, +2, −2}, representing the order of the row entry from top to bottom. Similarly the entries for the columns are indexed in the same way from left to right. Using the orthogonality relation Eq. (F.35), we can find out that the off-diagonal kinetic energy terms of Ĥs vanish and the only non-zero terms are those corresponding to Ĥ2,2 and Ĥ−2,−2 . The corresponding kinetic energies for these two terms are equivalent and equal to 4~ωr . Similarly we seek to find the matrix representation for the potential shown in Eq. (4.60) using the above basis. We proceed to obtain the matrix element h2|Ĥs |0i by calculating the potential energy term using the operator V̂ = ~β cos (2ky + φ). Therefore by inserting the completeness relation into h+2|V̂ |0i we get: Z Z h+2|V̂ |0i = h+2|yi ihyi |V̂ |yj ihyj |0idyi dyj (F.39) yi yj Z Z = dyi h+2|yi i dyj V (yj )hyi |yj ihyj |0i (F.40) yi yj Z Z −i2kyi ∗ dyj hyi |yj i V (yj )ψ0 (yj ) = dyi ψ0 (yi )e (F.41) | {z } yj yi δij Z = yi dyi ψ0∗ (yi )e−i2kyi V (yi )ψ0 (yi ) (F.42) F.2. MATRIX ELEMENTS OF ĤS 155 Z dyi |ψ0 (yi )|2 e−i2kyi V (yi ) = (F.43) yi We drop the subscript i because it becomes superfluous, and introduce the nate representation of the potential V (y) = ~β cos (2ky + φ) Z h+2|V̂ |0i = dy|ψ0 (y)|2 e−i2ky ~β cos (2ky + φ) Zy ¡ ¢ β = dy ~ |ψ0 (y)|2 e−i2ky ei(2ky+φ) + e−i(2ky+φ) 2 Zy ¡ ¢ β = dy ~ |ψ0 (y)|2 eiφ + e−i(4ky+φ) 2 y Z Z iφ β 2 −iφ β = ~e dy|ψ0 (y)| + ~e dy|ψ0 (y)|2 e−i4ky 2 y 2 y coordi- (F.44) (F.45) (F.46) (F.47) As shown above the matrix element yields two terms. Because the wavefunction ψ0 is normalized, the first term gives ~βeiφ /2. However, the real part of the exponential in the second term oscillates rapidly in the region where |ψ0 |2 is non-zero, therefore causing it to vanish when performing the integral. β h+2|V̂ |0i = ~ eiφ 2 (F.48) We use the same procedure as illustrated above to obtain the matrix element for h−2|V̂ |0i. An inspection of Eq. (F.39) reveals that changing the state h +2| to h −2| yields: Z h−2|V̂ |0i = dy|ψ0 (y)|2 e+i2ky V (y) (F.49) y Z ¡ ¢ β = dy ~ |ψ0 (y)|2 ei(4ky+φ) + e−iφ (F.50) 2 y In this case the first term is oscillating thus causing it to vanish. This gives the result: β (F.51) h−2|V̂ |0i = ~ e−iφ 2 For the term h−2|V̂ |+2i we can inspect Eq. (F.39) and introduce the states h −2| and | +2i to obtain: Z h−2|V̂ |+2i = dyi |ψ0 (yi )|2 ei4kyi V (yi ) (F.52) yi Z ¢ ¡ β (F.53) = dy ~ |ψ0 (y)|2 ei(6ky+φ) + ei(2ky−φ) 2 y 156 APPENDIX F. MATHEMATICAL CALCULATIONS which means both terms oscillate where ψ0 is non-zero, meaning they average out to zero when integrated over y yielding: h−2|V̂ |+2i = 0 (F.54) Additionally, each diagonal term of V̂ will only contain integrals having oscillating terms (similar to Eq. (F.47)) that will average out to zero. Hence these diagonal matrix elements vanish. We can make use of the hermitian properties of Ĥs in order to calculate the remaining terms of the potential V . 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