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ENGINEERING OF COMPLEX OPTICAL FIELDS AND ITS APPLICATIONS Dissertation Submitted to The School of Engineering of the UNIVERSITY OF DAYTON In Partial Fulfillment of the Requirements for The Degree Doctor of Philosophy in Electro-Optics By Wei Han UNIVERSITY OF DAYTON Dayton, Ohio August, 2013 ENGINEERING OF COMPLEX OPTICAL FIELDS AND ITS APPLICATIONS Name: Han, Wei APPROVED BY Qiwen Zhan, Ph.D. Advisory Committee Chairman Professor Electro-Optics Program Joseph W. Haus, Ph.D. Committee Member Professor Electro-Optics Program Partha Banerjee, Ph.D. Committee Member Director and Professor Electro-Optics Program Guru Subramanyam, Ph.D. Committee member Chair and Professor Electrical and Computer Engineering John G. Weber, Ph.D. Associate Dean School of Engineering Tony E. Saliba, Ph.D. Dean, School of Engineering & Wilke Distinguished Professor ii © Copyright by Wei Han All rights reserved 2013 iii ABSTRACT ENGINEERING OF COMPLEX OPTICAL FIELDS AND ITS APPLICATIONS Name: Han, Wei University of Dayton Advisor: Dr. Qiwen Zhan Generation of optical fields with complex spatial distribution in the cross section is of great interest in application areas where exotic optical fields are desired, including particle manipulation, optical nanofabrication, beam shaping and optical imaging. The dissertation is organized in two parts. In the first part, different aspects of the optical field are controlled with different approaches used in four projects. First, a diffractive optics element (DOE) Simulator consisting of 4-f imaging systems and reflective spatial light modulator (SLM) is introduced, where the phase is modulated. In the second project, a complex optical filter design using optical antennas is presented for optical needle field generation, using the amplitude and binary phase modulation. In the third example, a “Bull’s Eye” structure on fiber end is analyzed and demonstrated as a polarization sensitive device for cylindrical vector beam generation, where the SOP can be controlled. As the last demonstration, the vectorial beam is constructed by superimposing x-polarized Gaussian and y-polarized Laguerre Gaussian is introduced as iv one type of second order full Poincaré beams, which can be realized using liquid crystal (LC) based device. The demands to arbitrarily tailor the properties of optical fields lead to our Vector Optical Field Generator (VOF-Gen). In the second part, a vectorial optical field generator capable of creating arbitrarily complex beam cross section is designed, built and tested. Based on two reflective phase-only liquid crystal spatial light modulators, this generator is capable of controlling all the parameters of the spatial distributions of an optical field, including the phase, amplitude and polarization (ellipticity and orientation) on a pixel-bypixel basis. Various optical fields containing phase, amplitude and/or polarization modulations are successfully generated and tested using Stokes parameter measurement to demonstrate the its capability and versatility. v Dedicated to my wife and my parents vi ACKNOWLEDGEMENTS I am greatly indebted to the people who have helped me over the last six years. Above all, I would like to acknowledge my advisor, Dr. Qiwen Zhan, for his tremendous amount of help and support through my Ph.D. period. I couldn’t thank him enough. I would like to thank him for the great amount of time, effort and thoughts he put in my research and for the inspiring discussions and interactions with him, which leads to the successful conclusion of my dissertation. He is a knowledgeable and diligent professor and a leading scientist in the fields of space variant polarization engineering and I am especially grateful for his experienced guidance and vision in my research of complex optical fields engineering. I would also like to thank my committee members, Dr. Joseph Haus, Dr. Partha Banerjee and Dr. Guru Subramanyam for their continuous support during my Ph.D. research. I am very grateful for their valuable revision advice on my dissertation manuscript. Dr. Haus is a very knowledgeable and passionate professor and always ready to start discussion on any subject in optics. I am very grateful for his mentor as the advisor for my master’s study. Dr. Banerjee is the Director of the Electro-Optics Program and is a very nice and vii knowledgeable professor with strong disciplines. Dr. Guru Subramanyam is the Chair of the Electrical and Computer Engineering Department and is a very humble and knowledgeable professor. I also want to take this opportunity to express my sincere appreciation to all the professors from whom I have had the honor to take the courses. My sincere thanks go to Dr. Loomis, Dr. Duncan, Dr. Powers, Dr. Sarangan, Dr. Vorontsov, Dr. Watson and Dr. McManamon as well as my committee members. My wishes go to Dr. Powers for a full recovery. I have learned a lot of knowledge and experience from all the professors and am deeply impressed with their love and passion for optics. I would like to thank the former members of Dr. Zhan’s group, including Dr. Weibin Chen, Dr. Zhi Wu, Dr. Jian Gao, Dr. Wenzao Li, Dr. Alain Tschimwangan, Xue Liu, Shuangyang Yang and Mengshu Pan. I have received a lot of help from them since I came to the USA to pursue the graduate study in 2007. I also want to thank the current members of Dr. Zhan’s group, including Shiyi Wang, Zhijun Yang, Hongwei Chen, Zhenyu Yang, Renjie Zhou and Chenchen Wan for their help and support. My special thanks also go to my close friends and former ECE graduate, Dr. Hai Jiang and his wife Xiaoyan Ruan. They are very nice people and always ready to help. They have offered me countless help and valuable advice both inside and outside the academics with their experience. Last but not least, I would like to thank my family. My parents are always there for me. My most special thanks goes to my wife, Wen Cheng. We met here in the Electro-Optics viii Program. None of this could have happened without her accompany and support. She is always there for me whenever I am down. ix TABLE OF CONTENTS ABSTRACT ...................................................................................................................... iv ACKNOWLEDGEMENTS ........................................................................................... vii LIST OF FIGURES ....................................................................................................... xiv LIST OF TABLES .......................................................................................................... xx LIST OF ABBREVIATIONS AND NOTATIONS ..................................................... xxi CHAPTER 1 INTRODUCTION ..................................................................................... 1 CHAPTER 2 OVERVIEW OF RESEARCH BACKGROUND .................................. 4 1. STATE OF POLARIZATION, STOKES PARAMETERS AND POINCARÉ SPHERE ........... 4 2. INTRODUCTION TO CYLINDRICAL VECTOR BEAMS................................................. 7 3. LIQUID CRYSTAL SPATIAL LIGHT MODULATOR AND ITS LIGHT MODULATION CAPABILITY ..................................................................................................................... 9 4. LIGHT MODULATION USING SUBWAVELENGTH METALLIC STRUCTURES ............ 13 4.1. Wiregrid polarizer for polarization modulation ........................................... 13 4.2. Periodic grating structure for amplitude and phase modulation................. 14 4.3. Antenna structure for amplitude, phase and polarization modulation ....... 14 CHAPTER 3 DOE SIMULATOR USING PHASE MODULATION CREATED BY A REFLECTIVE SLM ................................................................................................... 16 x 1. INTRODUCTION ...................................................................................................... 16 1.1. 4-f imaging system ......................................................................................... 16 1.2. Beam propagation and its paraxial approximation ...................................... 20 2. EXPERIMENTAL SETUP OF DOE SIMULATOR ....................................................... 22 3. COMPLEX SCALAR FIELD REALIZATION USING DOE SIMULATOR: BIFOCAL LENS AND TORIC LENS ............................................................................................................ 24 4. 3.1. DOE bifocal lens ............................................................................................ 24 3.2. Toric lens ........................................................................................................ 28 SUMMARY .............................................................................................................. 31 CHAPTER 4 SECOND-ORDER FULL POINCARÉ BEAMS ................................. 32 1. INTRODUCTION ...................................................................................................... 32 2. FULL POINCARÉ BEAM AND ITS STATE OF POLARIZATION................................... 33 3. SUMMARY .............................................................................................................. 39 CHAPTER 5 GENERATING CYLINDRICAL VECTOR BEAM WITH SUBWAVELENGTH CONCENTRIC METALLIC GRATING FABRICATED ON OPTICAL FIBER ........................................................................................................... 40 CHAPTER 6 COMPLEX OPTICAL FILTER FOR HIGH PURITY OPTICAL NEEDLE FIELD GENERATION ................................................................................ 47 1. INTRODUCTION ...................................................................................................... 47 2. ELECTRIC FIELD CALCULATION AT PUPIL PLANE ................................................ 48 3. DISCRETIZATION OF THE PUPIL FILTER................................................................ 54 xi 4. SUB-WAVELENGTH METALLIC GRATING IMPLEMENTATION FOR OPTICAL NEEDLE GENERATION ................................................................................................................. 56 4.1. Introduction ................................................................................................... 56 4.2. Pupil filter design and proposed experiment setup ...................................... 57 5. PRELIMINARY RESULTS ......................................................................................... 59 6. DESIGN BASED ON SUBWAVELENGTH METALLIC LINEAR ANTENNA .................... 60 7. 6.1. Introduction ................................................................................................... 60 6.2. Initial analysis................................................................................................ 60 6.3. Complex optical filter design ......................................................................... 65 6.4. Realization of complex optical filter with slot antennas .............................. 72 SUMMARY .............................................................................................................. 73 CHAPTER 7 VECTOR OPTICAL FIELD GENERATOR....................................... 74 1. INTRODUCTION ...................................................................................................... 74 2. PRINCIPLES ............................................................................................................ 77 2.1. Spatial light modulator .................................................................................. 78 2.2. Spatially variant polarization rotator ............................................................ 79 2.3. System flow chart ........................................................................................... 82 2.4. Modulation of Light....................................................................................... 83 2.4.1. Phase modulation (SLM Section 1) ......................................................... 83 2.4.2. Amplitude modulation (SLM Section 2) ................................................. 83 2.4.3. Polarization ratio modulation (SLM Section 3) ..................................... 84 2.4.4. Phase retardation modulation (SLM Section 4) ..................................... 85 3. EXPERIMENTAL SETUP .......................................................................................... 87 xii 4. 3.1. Experimental setup of the generator ............................................................. 87 3.2. Gamma Curve Calibration Using Polarization Rotator ............................... 91 3.3. 4-f imaging system and its alignment procedure .......................................... 93 EXPERIMENTAL RESULTS ...................................................................................... 97 4.1. Spatially variant phase modulation: vortex generation ............................... 97 4.2. Spatially variant amplitude modulation ........................................................ 99 4.3. Spatially variant polarization rotation: radially polarized beam ............... 102 4.4. Spatially variant phase retardation ............................................................. 108 4.5. Stokes parameters measurement and complex vectorial optical field generation with multiple parameters ..................................................................... 111 4.5.1. Stokes parameters and its measurement .............................................. 111 4.5.2. Experimental results for complex vector field generation with multiple parameters .......................................................................................................... 114 4.6. 5. Realization of full Poincaré beam and the singularities ............................ 122 SUMMARY ............................................................................................................ 126 CHAPTER 8 CONCLUSIONS AND FUTURE WORK .......................................... 127 BIBLIOGRAPHY ......................................................................................................... 129 VITA............................................................................................................................... 137 xiii LIST OF FIGURES Fig. 2-1: Polarization ellipse. .............................................................................................. 5 Fig. 2-2: Poincaré sphere. ................................................................................................... 6 Fig. 2-3: Cylindrical vector beams. (a) Radial polarization; (b) azimuthal polarization; (c) generalized CVB. ................................................................................................................ 7 Fig. 2-4. Twisted nematic LC molecules with external voltage applied. Here LC directors are shown in cylinders. The front surface is rubbed in vertical direction while the back is in horizontal direction. ...................................................................................................... 10 Fig. 2-5: Illustration of the extraordinary refractive index for uniaxial LC molecules .... 10 Fig. 3-1. Schematic diagram of 4-f imaging system. ........................................................ 17 Fig. 3-2. Schematic diagram of DOE Simulator. .............................................................. 23 Fig. 3-3. Experimental setup of the DOE Simulator. ........................................................ 24 Fig. 3-4: Phase pattern of the bifocal phase with the 20 D base power. ........................... 25 Fig. 3-5. Through focus PSF of ReSTOR with 20 D base power for 4 mm pupil size. ... 26 Fig. 3-6. Experimental results of 2D through focus PSF for 4mm pupil size................... 27 Fig. 3-7. Simulation results of 2D through focus PSF. ..................................................... 27 Fig. 3-8. 3 D toricity phase pattern. .................................................................................. 28 Fig. 3-9. Evolution of 3 D toricity near focus. The upper column is simulation results and the lower is the experimental measurement. The defocus from left to right is 0 mm, -4 mm and -6.5 mm, respectively. ......................................................................................... 29 xiv Fig. 3-10. Evolution of 0.5 D toricity near focus. The upper column is simulation results and the lower is the experimental measurement. The defocus from left to right is 0 mm, 0.6 mm and -1.2 mm, respectively. ................................................................................... 30 Fig. 3-11. Evolution of 0.1 D toricity near focus. The upper column is simulation results and the lower is the experimental measurement. The defocus from left to right is 0 mm, 0.12 mm and -0.24 mm, respectively. ............................................................................... 31 Fig. 4-1. Intensity and phase pattern for LG02 mode. ....................................................... 34 Fig. 4-2. SOPs evolution for second order FP beam at 1). z = -10zR, 2). z = -zR, 3). z = 0, 4). z = zR and 5). z = 10zR. ................................................................................................ 37 Fig. 4-3. One slice (shown in red) of the Poincaré sphere at fixed ϕ and r/w(z) with δ spanning from 0 to 2π. ...................................................................................................... 38 Fig. 5-1. Experimental setup for generalized CV beam generation. [46] ......................... 41 Fig. 5-2. SEM pictures of the Bull's Eye structure. [46] Sample is prepared by Don Abeysinghe using FIB....................................................................................................... 42 Fig. 5-3. Simulated energy density and local SOP. [46] ................................................... 44 Fig. 5-4. Experimental results for generalized CV beam generation. [46] ....................... 45 Fig. 6-1. High NA focusing of pupil plane field in the focal volume (shown in red). ..... 49 Fig. 6-2. Schematic configuration of reversing radiation of an electric dipole array. ...... 49 Fig. 6-3. Far field intensity along focus (upper) and its line scan (lower) [48]. The longitudinal coordinate is normalized to the wavelength. ................................................ 52 Fig. 6-4. Intensity distribution in the pupil plane (upper) and its line scan (lower) [48]. The transverse coordinate is normalized to the pupil radius of the high NA objective. ... 53 Fig. 6-5. Discrete filter design. ρ is normalized to the pupil radius for the high NA objective. ........................................................................................................................... 54 Fig. 6-6. Electric field along focus (a) and its line scan (b) for discrete pupil filter. The horizontal axis is normalized by the wavelength. ............................................................. 55 Fig. 6-7. Grating structure (upper) and proposed experimental setup (lower). The radii are normalized to the radius of the pupil. ............................................................................... 58 xv Fig. 6-8. SEM of sample (by Don C Abeysinghe). ........................................................... 59 Fig. 6-9: Linear antenna oriented at angle θ from the incident polarization. .................... 61 Fig. 6-10. Normalized amplitude (upper) and phase (lower) of the longitudinally polarized scattered field. ................................................................................................... 62 Fig. 6-11. The absolute value of the Ez component of the scattered field off the rod antenna. ............................................................................................................................. 63 Fig. 6-12. The absolute value of the Eρ component of the scattered field off the rod antenna. ............................................................................................................................. 63 Fig. 6-13. 2D amplitude plot of linear antenna versus length L and θ.............................. 65 Fig. 6-14. 2D phase plot of linear antenna versus length L and θ. ................................... 65 Fig. 6-15. Normalized amplitude (upper) and phase (lower) of the longitudinally polarized scattered field for 25 nm radius rod antenna. .................................................... 67 Fig. 6-16. Normalized amplitude (upper) and phase (lower) of cross-polarized scattered field as a function of L and θ for 25-nm radius rod antenna. ............................................ 68 Fig. 6-17. Rectangle linear antenna and its complementary design. ................................ 72 Fig. 6-18. SEM pictures of antenna structure as complex optical filter fabricated by Don C Abeysinghe using FIB. .................................................................................................. 73 Fig. 7-1. Taiji pattern coded in circular polarization. The total field (left), the upper half Taiji pattern (upper right) in RCP and the lower half Taiji pattern (lower right) in LCP. 78 Fig. 7-2. Illustration of the Polarization Rotator setup. (a) The Polarization Rotator comprised of QWP and reflective SLM; (b) Illustration of the effective rotation of the QWP fast axis for the incident (upper) and the reflected (lower) beams due to the mirror imaging of the laboratory coordinates in dashed lines...................................................... 80 Fig. 7-3. Flow chart of the system. The VOF-Gen System consists of light source, 4 subsystems for control of all the aspects of light, 4-f imaging subsystems and detection subsystem. PR: Polarization Rotator................................................................................. 82 Fig. 7-4. Schematic diagram of the VOF-Gen. ................................................................. 88 Fig. 7-5. Experiment Setup of the VOF-Gen. ................................................................... 89 xvi Fig. 7-6. Driver circuits for the color channels of the VOF-Gen system. The upper one is the red channel responsible for the control of SLM1 and the lower one is the green channel for SLM 2. ........................................................................................................... 90 Fig. 7-7. Calibration setup consists of a PR and a polarizer. ............................................ 92 Fig. 7-8: Pattern with fine features for 4-f imaging system alignment. Each line is 100 μm wide. .................................................................................................................................. 94 Fig. 7-9: 4-f imaging system alignment procedure ........................................................... 95 Fig. 7-10: Test results for (a) amplitude modulation: the intensity is directly captured by the CCD camera; (b) polarization rotation: the intensity is captured after a linear polarizer; (c) Retardation: the intensity is captured after a circular analyzer. .................................. 95 Fig. 7-11: Comparison of the same patterns generated by VOF-Gen system without and with well aligned 4-f imaging systems. ............................................................................ 96 Fig. 7-12. Pure phase modulation with spiral phase of topological charge 1 (upper), 10 (middle) and 15 (lower). The images are captured in the focal plane of 75-mm planoconvex lens........................................................................................................................ 99 Fig. 7-13. x-polarized "EO" logo coded in amplitude (upper) and its phase pattern (lower). ......................................................................................................................................... 101 Fig. 7-14. Phase patterns for radially polarized beams without (upper) and with (with) pre-compensation. For the latter phase pattern, the variation in green color indicates the pre-compensation phase. ................................................................................................. 104 Fig. 7-15. Focused field by a 75-mm plano-convex lens. (a) Radially polarized beam without proper phase cancellation; (b) radially polarized beam with phase cancellation. ......................................................................................................................................... 105 Fig. 7-16. Radially polarized beam generated by the VOF-Gen. Upper graphs show the fields after a polarizer with polarization axis orientation indicated by black arrows at 0°, 45°, 90° and 135°, respectively; Lower graph shows a polarization map of radially polarized beam overlapped with the intensity distribution and the local polarization directions are indicated by the bars. ................................................................................ 107 Fig. 7-17. Phase pattern for "EO" logo generation VOF-Gen. ....................................... 108 Fig. 7-18. "EO" logo coded in circular polarization. The total field (left), the EO logo (upper right) in RCP and the complimentary “EO” logo (lower right) in LCP. ............. 109 xvii Fig. 7-19. Phase pattern for Taiji pattern generation. ..................................................... 110 Fig. 7-20. Taiji pattern coded in circular polarization. The total field (left), the upper half (upper right) in RCP and the lower half (lower right) in LCP. ....................................... 110 Fig. 7-21. Full Stokes parameters measurement setup. .................................................. 113 Fig. 7-22. The ideal vector field where the SOP varying from azimuthal to radial as radius increases. .............................................................................................................. 114 Fig. 7-23. The phase pattern for VOF-Gen. .................................................................... 115 Fig. 7-24. Ring structure with SOP continuously varying from azimuthal to radial direction as radius increases. The upper set of graphs show the field components along 0°, 45°, 90° and 135° respectively and the lower graph shows the measured field overlapped with polarization map. .................................................................................................... 116 Fig. 7-25. The ideal field for double ring pattern where inner ring has azimuthal polarization and outer ring has radial polarization. ........................................................ 117 Fig. 7-26. The phase pattern for VOF-Gen. .................................................................... 118 Fig. 7-27. Double ring structure with amplitude and polarization rotation modulation: (upper) the linear polarization components with polarizer at 0°, 45° and 90°; (lower) the polarization map.............................................................................................................. 119 Fig. 7-28. Ideal field distribution with polarization map. ............................................... 120 Fig. 7-29. Phase pattern for VOF-Gen. ........................................................................... 121 Fig. 7-30. Experimental results (left) for optical field with constant ellipticity and elevation angle along radial direction as well as the histogram (right) of the ellipticity in the unit of π. .................................................................................................................... 121 Fig. 7-31. Simulation of FP beam with polarization map superimposed........................ 122 Fig. 7-32. Experimental result for FP beam with polarization map superimposed. Two singularities are highlighted by green circles.................................................................. 123 Fig. 7-33. Phase pattern for retardation modulation for the FP beam............................. 124 Fig. 7-34. The phase pattern for the generation of the FP beam. .................................... 125 Fig. 7-35. Diffraction pattern after propagation distance of 1 mm. ................................ 125 xviii Fig. 8-1. Experiment setup for linear antenna design. .................................................... 128 xix LIST OF TABLES Table 1: Parameters of dipole array for N = 2 .................................................................. 51 Table 2: Grating parameters for each concentric ring ...................................................... 57 Table 3: Design parameters .............................................................................................. 66 Table 4: Antenna design parameters for optical needle field generation .......................... 70 Table 5. Tolerance study of the antenna structure ............................................................ 71 xx LIST OF ABBREVIATIONS AND NOTATIONS CCD CV DOE F FIB FP HWP (λ/2) LCP LG LP NA PR QWP (λ/4) RCP RCWA SF SLM SOP VOF-Gen PSF DOF NSOM CP OAM SAM EM TE TM Charge coupled device Cylindrical vector Diffractive Optics Element Focal length Focused ion beam Full Poincaré Half wave plate Left-hand circular polarization Laguerre Gaussian Linear polarizer Numerical aperture Polarization Rotator Quarter wave plate Right-hand circular polarization Rigorous coupled wave analysis Spatial filter Spatial light modulator State of polarization Vector optical field generator Point spread function Depth of focus Near-field scanning optical microscope Circular polarizer Orbital angular momentum Spin angular momentum Electro-magnetic Transverse electric Transverse magnetic HDTV NPBS LC SEM xxi High-definition television Non-polarizing beam splitter Liquid crystal Scanning electron microscope CHAPTER 1 INTRODUCTION As a form of electromagnetic field, optical fields governed by the Maxwell’s Equations also exhibit vectorial nature in addition to phase and amplitude of the scalar field. Engineering of complex optical fields has drawn tremendous amount of research in various fields of applications. Optical trapping, or particle manipulation is made possible by the laser beam shaping or focus shaping. Shaped optical fields have enabled researchers to better understand the biophysics and colloidal dynamics through the trapping, guiding or patterning of molecules or nano/micro particles. Spatial engineering of focal field intensity has been studied to reach resolution far beyond diffraction limit in microscope system. Vortex beam, also known as “twisted light”, has also drawn a lot of interest owing to its spiral phase wavefront carrying orbital angular momentums. Better integrity of vortex beam through propagation in turbulent atmosphere has been shown and a lot of research has been done using the orbital angular momentum as information carrier for free space communication due to its orthogonality and multiplexing capability. Besides the manipulation of intensity and phase, as the vector nature of electromagnetic 1 wave, the state of polarization (SOP) also plays an important part in beam shaping for flattop generation, focus shaping, optical tweezing and surface plasmon sensing using cylindrical vectorial beams, ellipsometry. All the above applications require local control over all variables of the optical fields. The need to generate arbitrarily complex optical fields led to the development our vectorial optical field generator (VOF-Gen), which is capable of tailoring all aspects of the light field. Various techniques of manipulating degrees of freedom for complex optical fields are investigated from Chapter 3 to Chapter 6, which demonstrated partial control of complex optical field using SLM and subwavelength structure and in the meanwhile served as motivations for our VOF-Gen. In Chapter 3, we show that a DOE Simulator using the phase modulation capability of liquid crystal spatial light modulator (LC-SLM). In Chapter 4, the modulation of polarization is added for the generation of a more complex optical field. We show that, by adjusting the weighting of the x- and y-polarized components and loading corresponding phase, the complex SOP can be realized using SLM, which is then found to be one type of the full Poincaré beams. In Chapter 5, a vectorial optical field whose polarization possesses a rotational symmetry is achieved with a metallic grating structure. A concentric ring structure (Bull’s Eye) on fiber end is shown to have polarization sensitivity. More specifically, a generalized cylindrical vector (mostly radially polarized) beam is generated after the propagation of a circularly polarized input beam through the fiber. A more complex engineering of optical field is shown in Chapter 6, where modulations of phase, amplitude and polarization are simultaneously realized using a complex filter design. An optical antenna structure is proposed as a complex optical filter with amplitude, phase and polarization modulation to 2 achieve optical needle field in the focal volume of a high numerical aperture (NA) objective. An optical needle field features a mostly longitudinal polarization and a flattop intensity profile along axial direction with an extended depth of focus. All these projects lead to the need for a universal system that’s capable of manipulating all degrees of freedom for vectorial optical field, as the complexity of the conventional system increases and fabrication of the individual filter design gets more and more challenging. In Chapter 7, VOF-Gen that is capable of generating vectorial optical field with arbitrary phase, amplitude and polarization on a pixel by pixel basis is proposed and experimentally demonstrated. Various exotic vectorial optical fields are generated with desired spatial distribution of amplitude, phase and polarization. 3 CHAPTER 2 OVERVIEW OF RESEARCH BACKGROUND 1. State of polarization, Stokes parameters and Poincaré sphere Polarization in nature is the oscillation of electromagnetic wave and the SOP describes the oscillation trajectory. The vectorial form of electric field after normalization can be represented using Jones vector as: E0 x E j E0 y e cos j , sin e (2-1) where the tangent of χ represents the absolute value of the ratio between y- and xcomponents (E0y/E0x) and δ is the phase retardation. Polarization can also be viewed in terms of a polarization ellipse, as shown in Fig. 2-1. An elliptically polarized electric field is shown as an example, where E0x and E0y are given in the figure. A more intuitive way to represent the SOP is through elevation angle α and ellipticity ε. The laboratory coordinate (x, y) is rotated to (x’, y’) by the amount of α so that the horizontal axis ox’ is aligned with the major axis of the polarization ellipse, as depicted in Fig. 2-1. Mathematically, it is given as: 4 cos E . jsin (2-2) ε is the ellipticity of the polarization ellipse, whose tangent is defined as b/a, as shown in Fig. 2-1. Fig. 2-1: Polarization ellipse. Stokes parameters are all measurable quantities (intensities), which is an alternative of the SOP representation discussed above. Stokes parameters are given as 2 2 S 0 I x I y E0 x E0 y S I I E 2 E 2 x y 0x 0y 1 S 2 I I 2 E0 x E0 y cos . 4 4 S I I 2 E E sin R L 0x 0y 3 5 (2-3) After normalization, the Stokes parameters can be written as: S0 1 S cos 2 cos 2 cos 2 1 . S cos 2 sin 2 sin 2 cos 2 S3 sin 2 sin 2 sin (2-4) Note that S12+S22+S32 = 1 after normalization. Thus any combination of S1, S2 and S3 can be found on a sphere with constant radius (r = S12+S22+S32 = 1) using the coordinate (S1, S2, S3). In other words, the sphere defined by Stokes parameters contains all possible SOP on its surface. This is the so called Poincaré sphere, which is shown in Fig. 2-2. From Eq. (2-4), it can be shown that in Fig. 2-2 the azimuth angle with respect to S1 axis is equal to 2α and the elevation angle is equal to 2ε measured from the S1-S2 plane. Fig. 2-2: Poincaré sphere. 6 2. Introduction to cylindrical vector beams In order to engineer complex optical field, it is of fundamental importance to introduce spatially inhomogeneous polarization where the distribution of SOPs adds another degree of freedom for the manipulation of such beams. As the most well-known and investigated inhomogeneously polarized optical field, cylindrical vector beams (CVBs) are solutions to Maxwell’s Equations, whose SOPs possess rotational symmetry [1]. Radial and azimuthal polarization are the most common CVBs (Fig. 2-3 (a) and (b)) where the SOP follows radial and azimuthal direction at any point on the beam, respectively. Due to the orthogonality, radial and azimuthal polarizations form the basis for CVBs. And for any generalized CVB as shown in Fig. 2-3 (c), it can always be represented as a linear combination of radial and azimuthal modes. Fig. 2-3: Cylindrical vector beams. (a) Radial polarization; (b) azimuthal polarization; (c) generalized CVB. The unique properties of CVBs have attracted much research interest recently. Plasmonic focusing [2] [3] can be realized using radial polarization due to the TM polarization direction with respect to the nanostructure. The focal spot of radially polarized beam can 7 be much smaller than the diffraction limited spot size of spatially homogeneously polarized beams under using high NA objective [4] [5] [6]. High resolution imaging [7] can thus be realized using CVBs. When tightly focused, the radially polarized beam also exhibits a strong axial component with a smaller spot size centered on optic axis. The strong axial component provides a large gradient force while due to the non-propagating property, the axial scattering and absorption forces will be reduced [8] [9], which leads to the successful trapping of gold nanoparticles with a higher transverse trapping stiffness [10] and micrometer-sized dielectric particles with a higher axial and transverse trapping efficiency for radially and azimuthally polarized beams, respectively [11]. Evanescent Bessel beam generation has also been confirmed via surface plasmon resonance using tightly focused radially polarized beam [12]. In 4Pi microscopy, both dark and bright spherical focal spot can be created using radial polarization with spatially engineered amplitude and phase distribution [13] [14]. By carefully designing pupil apodization function, optical fields with unique amplitude, phase and polarization distribution can be obtained in the 3D focal volume of a high NA objective. It is possible to achieve a flattop focal shape by balancing the radial and azimuthal components and using a high-pass filter in the pupil apodization function [15]. By designing a DOE pupil mask with binary phase, optical needle field can be generated with significant longitudinal polarization component and an extended depth of focus [16]. Optical chain along longitudinal direction for stably trapping and delivering particles has been proposed by using a DOE with spatially engineered amplitude and phase modulation for different concentric ring regions [17]. Three-dimensional optical cage for 8 optical trapping can also be obtained by using spatially patterned generalized CVBs as the illumination for a high NA objective [18]. 3. Liquid crystal spatial light modulator and its light modulation capability 3.1. Liquid Crystal and Spatial light modulators In order to engineer complex optical fields, phase-only liquid crystal spatial light modulator (LC-SLM) is introduced for the realization of phase modulation. Liquid crystal (LC) is a phase of matter where the properties of the molecular order are between liquid and crystal. The molecules of LC differ from liquid as they demonstrate anisotropy as seen in crystalline structures. However, at the same time, unlike crystals, LC molecules show a flow behavior of liquid with randomly positioned and oriented molecules. The nematic LC phase can be characterized by rod-like molecules with no positional order but tend to self-align to have long range directional order. For LC display (LCD), the LC cells are spatially separated in cell (pixel) structures with carefully chosen dimensions. The transvers direction of LC molecules can be surface-aligned, which is done be rubbing the surface to introduce micro-grooves. Such direction is called rubbing direction. The longitudinal orientation of LC molecules (director) can be manipulated by externally applied electric field. The dipole-like director is excited by the external electric field and tends to align parallel to the electric field. Due to the long-range order of the nematic LC molecules, the LC cells will exhibit a voltage-dependent birefringence. In general, for twisted nematic-LC cells (TN-LC), the LCD structure with directors indicated by cylinders is shown in Fig. 2-4. 9 V- V+ Fig. 2-4. Twisted nematic LC molecules with external voltage applied. Here LC directors are shown in cylinders. The front surface is rubbed in vertical direction while the back is in horizontal direction. For uniaxial LC molecule, if the wave vector k of the incident beam has an angle θ with respect to the director as depicted in Fig. 2-5, the extraordinary refractive index ne can be found by Eq. (2-5). Fig. 2-5: Illustration of the extraordinary refractive index for uniaxial LC molecules 10 cos 2 sin 2 ne 2 no 2 n e 1/2 , (2-5) where angle θ is dependent on voltage V, ne and no are the properties of the LC material. Therefore, assuming the extraordinary direction is aligned along the x-axis, a single LC molecule can be regarded as a thin wave plate, whose Jones matrix is given by, W e jno 2 d j ne no 2 d e 0 0 , 1 (2-6) where d is the thickness of the LC molecule. A twisted nematic LC cell (in a LC layer) can thus be modeled as a succession of thin wave plates whose optic axes follow the molecular axes of the LC molecules as shown in Fig. 2-4. The overall Jones Matrix can be written as [19], WTN LC cos j sin j R e 0 sin sin , cos j sin (2-7) where R is the rotation matrix, α is the overall twist angle, β is the overall birefringence of the LC molecule defined as πdΔn/λ, Φ0 is the common phase and γ2 = α2 + β2. For the phase-only LC-SLM, the twist angle α is set to 0 so the Jones matrix can be simplified as WPhaseonly SLM e j 0 11 e j 0 0 . e j (2-8) It can be shown for LC cells with parallel rubbing directions, the LC cells become a variable retarder whose birefringence is a function of voltage applied. For a reflective-type phase-only LC-SLM, the phase pattern is imposed onto the reflected beam for incident beam with polarization parallel to the fast axis of the LC-SLM (or the rubbing direction of LC molecules). Thus phase modulation can be readily realized using a LC-SLM. However, for arbitrarily polarized input beam, the parallel component will carry the prescribed phase pattern while the orthogonal component remains unaffected after reflection. In other words, simple polarization control can also be realized where the phase retardation between the orthogonal polarization components is modulated using a single reflective-type LC-SLM for arbitrarily polarized incident beam. 3.2. Light modulation using LC-SLM based systems Tremendous amount of research has been conducted by scientists in the community developing versatile systems to generate optical field with exotic properties. Arbitrary vector fields with inhomogeneous distribution of linear polarization were realized using a LC-SLM and an interferometric arrangement [20]. A recent study showed that in order to fully control the SOP, two spatially addressable retarders need to be used [21]. Researchers constructed such system consisting of two LC-SLMs with the fast axes 45° from each other and were able to generate optical fields that cover the entire Poincare Sphere. Another non-interferometric method for vector field generation was proposed [22]. However, the complete control of both polarization elevation angle and ellipticity can only be realized by modifying the experimental setup. Complete amplitude, phase and polarization control was reported [23] with the help of a double modulation system 12 which requires two transmissive LC-SLMs whose modulation depth can be controlled to achieve amplitude modulation for certain diffraction order. However, this approach comes with the limitation that each area must contain a large number of periods to achieve the ideal diffraction efficiency, which leads to optical field with limited spatial resolution for practical applications. Very recently, a technique for generating arbitrary intensity and polarization was reported with interesting results using transmissive LCSLMs and Mach-Zehnder interferometry setup [24]. Due to the nature of the technique, the absolute phase of each electric field component does not cover an entire 2π range. As a result, a complete phase control cannot be fully realized. The limitations of this technique also include limited transmittance and relatively low spatial resolution. All the present techniques mentioned above have limitations when it comes to generating a spatially-invariant arbitrary vectorial field with high spatial resolution on a pixel basis. 4. Light modulation using subwavelength metallic structures The interactions between optical fields and specially engineered structures have long been investigated and demonstrated for the generation of beams with spatially inhomogeneous polarization such as CVBs or with prescribed amplitude or phase modulation. For instance, subwavelength metallic structures with exotic subwavelength geometries have been extensively studied for polarization control as well as amplitude and phase modulation. 4.1. Wiregrid polarizer for polarization modulation It has been demonstrated that a wiregrid grating with a period smaller than the wavelength of incident light strongly reflects TE polarized light and allows TM polarized 13 light to transmit through [25]. Subwavelength concentric metallic slits have been used for creating two-lobe shaped radially polarized or azimuthally polarized beam with linearly polarized illumination [26]. When an azimuthally polarized light is focused onto the axially symmetric metallic grating, the entire beam is TE polarized with respect to the interface and therefore experiences high reflection. In contrary, a radially polarized beam is entirely TM polarized with respect to the metallic grating and can pass through the device with higher transmittance than the azimuthal polarization. Therefore such structure can behave as a TM polarizer. 4.2. Periodic grating structure for amplitude and phase modulation Periodic metallic grating structure can also be used for the modulation of amplitude and phase of the diffracted orders. Rigorous coupled wave analysis (RCWA) is used to evaluate the reflected and diffracted waves [27] [28] [29] [30]. Based on Fourier series expansion and using Floquet’s theorem, the optical field in each layer of the grating is calculated by matching boundary conditions for each layer and each order. RCWA can in principle provide analytical solution if the infinite number of orders are kept. In practical application, finite number of orders are kept based on the accuracy and speed requirements. 4.3. Antenna structure for amplitude, phase and polarization modulation The scattered field off V-shaped nano antenna has recently been theoretically studied for its ability to control the amplitude and phase of the cross-polarized component [31] [32]. Thanks to the greater-than-2π phase coverage, the design of plasmonic nano V-shaped antenna array to introduce a phase gradient from 0 to 2π at the interface of two media in 14 order to steer the beam has been proposed and experimentally demonstrated. The amplitude and phase of the scattered field can be engineered by appropriately choosing the design parameters, the length of the rod antenna and the angle between the two arms. 5. High NA focusing of vectorial optical field The focusing of electromagnetic field over a three dimensional volume has always been an interesting and important area for both theoretical and applied optics. The focusing properties of linearly polarized (scalar) field have been well established by Richards and Wolf [33]. However, for spatially inhomogeneously polarized beams, the focusing properties hadn’t been thoroughly investigated until recent years. The vectorial optical field distribution in the focal volume of a high NA objective for radially and azimuthally polarized illumination can be found by the following equations respectively [4]. Ex 2 E C sin cos L , e jk Z r y 0 0 Ez S cos S sin cos S Ex 2 E C sin cos L , e jk Z y 0 0 Ez cos cos cos sin d d (2-9) sin S cos S sin cos S sin cos d d (2-10) 0 Coordinates (zS, ρS, ϕS) describe the locations in the image space measured from the focal point. Lr and Lϕ are the field distribution in the pupil plane of the high NA objective for radial and azimuthal illumination, respectively, where ϕ and θ are the azimuth angle in the pupil plane and polar angle. 15 CHAPTER 3 DOE SIMULATOR USING PHASE MODULATION CREATED BY A REFLECTIVE SLM 1. Introduction In this chapter, phase modulation using a LC-SLM based DOE Simulator is demonstrated as the start point for modulations of complex optical field. Two types of LC-SLMs have been investigated and used for DOE Simulator. The BNS XY series is a reflective LCSLM with a resolution of 512 x 512 and 15 μm pitch size. The SLM is set up to work with a He-Ne laser at 632.8 nm. The HOLOEYE HEO 1080P is another reflective phaseonly LC-SLM with a resolution of 1920x1080 and 8 μm pitch size and is set up to work with a He-Ne laser at either 543 nm or 633 nm. 1.1. 4-f imaging system 4-f imaging system is widely used for holography reconstruction [34]. The optical field at the image plane can be a reconstruction of that at the object plane without diffraction effect or quadratic wavefront. In our DOE simulator, 4-f imaging system is also 16 introduced to relay the optical fields between the object and image planes. The schematic diagram of 4-f imaging system is depicted below in Fig. 3-1. Fig. 3-1. Schematic diagram of 4-f imaging system. Assuming L1 and L2 have the same focal length denoted as f, the incident transparency t(x’, y’) is located at one f before L1. Based on Fresnel diffraction, the field T 1 right in front of Lens L1 (in Plane (ξ, η)) can be found by Eq. (3-1): T1 , t x ', y ' h , ; f t x ', y ' e e jk 2 2 2f jk x '2 y '2 2f t x ', y ' e jk dx ' dy ' x '2 y '2 2f e jk (3-1) x ' y ' f dx ' dy ' The field T2 immediately after Lens L1 can be calculated by multiplying the transformation function of the lens, giving rise to the following expression (Eq. (3-2)): 17 T2 , T1 , e jk 2 2 2f (3-2) The field T3 at one f distance from L1 (the focal plane Plane (x, y)) is then given by Eq. (3-3): T3 x, y T2 , e e e jk x2 y 2 2f x2 y 2 jk 2f jk x 2 y 2 T , e 1 T , 1 d d 2f jk x y f d d k kx f k ky f (3-3) Remember in spatial frequency domain, T , t x ', y '; z f t x ', y ' e 1 j k 2 2 x ' k y ' 2k f (3-4) By equating the spatial frequencies kx’ and kξ, ky’ and kη, respectively, Eq. (3-3) can be simplified as: 18 T3 x, y e x2 y 2 jk 2f t x ', y ' e t x ', y ' kx 2 ky 2 f f f j 2k kx' kx f ky' ky f kx kx' f ky' (3-5) ky f The field T3(x, y) at Plane (x, y) is proportional to the Fourier transform of the transparency t(x’, y’), without quadratic phase term. Thus, the output field Tout at Plane (x1, y1) can be determined similarly, which turns out to be proportional to the Fourier transform of the field at T3(x, y). As a result, Tout at Plane (x1, y1) can be written as T x, y Tout x1 , y1 3 kx kx1 f ky ky1 f kx1 kx k x f f t x ', y ' ky ky ky' ky 1 f f kx' f kx1 f ky1 , t k f k f t x1 , y1 f k 19 (3-6) Through rigorous derivation, one can find that for a 4-f imaging system, the output field Tout is directly proportional to the inverse of the original transparency t as shown in Eq. (3-6) without any approximation or quadratic phase term. In other words, the object (transparency) can be reimaged at the image plane in terms of both amplitude and phase. 1.2. Beam propagation and its paraxial approximation From Helmholtz Equation, we have 2 k 2 E r, z 0 (3-7) For scalar case, E field can be Fourier transformed into plane wave decomposition in angular frequency space. E r, z 1 2 2 U kr , z e jkr r dkr 2 (3-8) Plug into the Helmholtz Equation, yielding, d2 U kr , z kr 2U kr , z k 2U k r , z 0 2 dz (3-9) Assuming U (kr, z) has a exp (-j kz z) dependence, we then can rewrite the equation as k z 2 k r 2 k 2 U k r , z 0 (3-10) Therefore, k z k 2 kr 2 U kr , z U 0 kr e j 20 (3-11) k 2 kr 2 z (3-12) In paraxial case, kr/k is much smaller than 1, thus, U kr , z U 0 kr e jkz e kr 2 z 2k j (3-13) In space domain, the input E field can be viewed as a collection of point sources located at different 2D coordinates. The diffraction of point source will introduce a spherical wavefront to the field at the point source. Therefore, we have the following expression Eq. (3-14) for the diffraction in the space domain. E r , z E0 r 1 jkR e R E0 x0 , y0 e jk 1 x x0 x x0 y y0 2 2 z2 2 y y0 z 2 2 (3-14) dx0 dy0 In paraxial case, r/z is much smaller than 1, yielding, E r , z E0 x0 , y0 e x x0 2 y y0 2 jkz 1 2 z2 x x0 y y0 2 E0 x0 , y0 e jkz e E0 x, y e jkz e jk jk 2z dx0 dy0 2 dx0 dy0 (3-15) x2 y 2 2z The propagation of optical field be viewed as a linear, time-invariant system problem where the output (response) is equal to the convolution of the input with the impulse response (point spread function) in space domain or the multiplication of the input with the system function (amplitude transfer function, ATF) in angular frequency domain. Mathematically, it follows, 21 U kr , z z U kr , z ATF z where ATF z e 2 2 j k kr z e jkz e j kr 2 z 2k . E r , z z E r , z PSF z where PSF z e jkR e jkz e jk (3-16) (3-17) x2 y 2 2 z 2. Experimental setup of DOE Simulator Based on the 4-f imaging system previously discussed and the phase-only LC-SLM, we designed the following DOE Simulator consisting of a 4-f imaging system and the SLM with schematic diagram shown in Fig. 3-2. Here the field right after the reflection from the SLM, which is the input transparency multiplied by the phase loaded onto the SLM, can be reimaged at the output plane, so that precise measurements can be performed without introducing any phase aberration. The experimental setup is also shown in Fig. 3-3. 22 Output (x2, y2) Input (x1, y1) f SLM (x’, y’) f L1 (ξ, η) f (x, y) f L2 Fig. 3-2. Schematic diagram of DOE Simulator. 23 Fig. 3-3. Experimental setup of the DOE Simulator. 3. Complex scalar field realization using DOE Simulator: bifocal lens and toric lens As an illustration of the capability of our DOE Simulator, two types of lens functions have been realized and tested. 3.1. DOE bifocal lens A bifocal DOE design is investigated to test the performance of our DOE Simulator system. A bifocal power of 3 diopters (D) is added to a base power of 20 D. The phase pattern is shown in Fig. 3-4. 24 Fig. 3-4: Phase pattern of the bifocal phase with the 20 D base power. Optical powers of 20 D and 23 D are expected and the spacing d between two foci can be calculated as: d 1 1 1 1 6.52mm p1 p2 20 23 The experiment was done with 4 mm pupil size. The one dimensional (1D) through-focus point spread function (PSF) simulation and experimental data for 4 mm pupil size is shown in Fig. 3-5. Fresnel propagation simulation is used for PSF evaluation in the MATLAB environment. The locations of the peaks appear as predicted with the spacing of about 6.49 mm. The difference between experimental data and simulation could be due to scattering from the 87% filled SLM pixels, vibrations and other perturbations. 25 1 Through focus PSF of ReSTOR with 20D for 4 mm pupil size Simulation Experimental results 0.9 Normalized Intensity 0.8 0.7 0.6 0.5 0.4 0.3 0.2 0.1 0 -8 -7 -6 -5 -4 -3 -2 Defocus (mm) -1 0 1 2 Fig. 3-5. Through focus PSF of ReSTOR with 20 D base power for 4 mm pupil size. The two dimensional (2D) through-focus PSF are shown in Fig. 3-6 for 4 mm pupil size. Fig. 3-7 shows the simulation result. Good agreement has been obtained. Note that the captured image is not affected by other diffraction orders since the separation in the far field is large. 26 40 30 20 x (m) 10 0 -10 -20 -30 -40 -7 -6 -5 -4 -3 -2 Defocus z (mm) -1 0 1 Fig. 3-6. Experimental results of 2D through focus PSF for 4mm pupil size. 40 30 20 x (m) 10 0 -10 -20 -30 -40 -7 -6 -5 -4 -3 -2 Defocus z (mm) -1 0 Fig. 3-7. Simulation results of 2D through focus PSF. 27 1 3.2. Toric lens In order to verify the astigmatism effect from toric lens and the spacing between its sagittal and tangential foci, we tested toric lenses consisting of a 20 D base power with different toricities of 3 D, 0.5 D and 0.1 D on x-axis, respectively. As one example, toric phase pattern of 3 D toricity is shown in Fig. 3-8. This combined with base power of 20 D is then loaded onto the SLM and tested on our DOE Simulator with 4-f system. Fig. 3-8. 3 D toricity phase pattern. The spacing between the tangential and sagittal foci is found to be 6.52 mm, 1.2 mm and 0.24 mm, respectively and the evolution is in Fig. 3-9, Fig. 3-10 and Fig. 3-11. In each figure, the tangential focus, mid-point between two foci and sagittal focus are shown with the simulation results for each toricity. Even for 0.1 D toricity, low space-bandwidth 28 product is present due to the small beam size and limited pixel size of the detector. However, even at 0.1 D, we were able to observe the transition of the energy concentration from along horizontal direction to along vertical direction as the CCD is translated from the tangential focus to the sagittal focus. Fig. 3-9. Evolution of 3 D toricity near focus. The upper column is simulation results and the lower is the experimental measurement. The defocus from left to right is 0 mm, -4 mm and -6.5 mm, respectively. 29 Fig. 3-10. Evolution of 0.5 D toricity near focus. The upper column is simulation results and the lower is the experimental measurement. The defocus from left to right is 0 mm, 0.6 mm and -1.2 mm, respectively. 30 Fig. 3-11. Evolution of 0.1 D toricity near focus. The upper column is simulation results and the lower is the experimental measurement. The defocus from left to right is 0 mm, 0.12 mm and -0.24 mm, respectively. 4. Summary The DOE Simulator is proposed and experimentally verified. The DOE phase has been imaged on the output plane of the DOE Simulator and the through-focus PSF for both bifocal and toric lens designs show very good agreement with the simulation results based on beam propagation method. The DOE Simulator has well demonstrated the phase modulation capability using the SLM. 31 CHAPTER 4 SECOND-ORDER FULL POINCARÉ BEAMS 1. Introduction Phase modulation capability has been previously demonstrated using LC-SLM based DOE Simulator. As discussed before, for incident beams with arbitrary polarization direction, phase retardation can be introduced between the polarization components along the fast and slow axes of the LC-SLM. Thus, more complex modulation can be achieved by spatially engineering the retardation within each LC-SLM pixel as prescribed by the phase pattern. It is well known that electromagnetic waves carry both energy and momentum and the interactions between light and matter involves both energy and momentum exchange. As a fundamental nature of light, the momentum can be further divided into two categories, spin angular momentum (SAM) and orbital angular momentum (OAM). SAM is associated with polarization while OAM describes the angular distribution of the phase or wave front. If the EM wave has an azimuthal dependence of exp(ilφ), where φ is the azimuthal angle, then it’s said to have an OAM of lħ or a topological charge of l. The 32 origin has an abrupt change in phase, which is defined as a singularity point. OAM has attracted a lot of research interest recently due to its potential applications in optical communications [35], optical trapping [36], optical tweezers, Full Poincaré (FP) Beams generation [37] [38] and laser beam shaping [39]. 2. Full Poincaré beam and its state of polarization Full Poincaré (FP) beam is a new class of beams that have been proposed and studied recently [38] [37]. Beams whose SOPs within the cross-section span the entire Poincaré sphere are defined as FP beams. FP beams can be generated through superimposing orthogonally polarized beams with spatially different intensity distributions [1]. Generation of the first order FP beams has been previously studied using fundamental Gaussian (LG00) and first order Laguerre Gaussian (LG01) beams of right hand circular polarization (RCP) and left hand circular polarization (LCP), respectively [38]. 2D flattop beam shaping has been reported in one previous paper using the linear combination of xpolarized fundamental Gaussian and y-polarized LG01 mode [40], which in fact generated the first order FP beam. Smooth flattop profile has been obtained for chosen parameters. However, the edge roll-off is not steep due to the gentle roll-off of the transverse profile for the focused LG01 component. This can be improved through the using of LG modes with higher topological charges. The interest in flattop generation leads to our investigation on the second order FP beam. Here we report the second order FP beams generated through linear combination of horizontally polarized (x-polarized) fundamental Gaussian (LG00) and vertically polarized (y-polarized) second order Laguerre Gaussian (LG02) beams. 33 Vortex beams with spiral wavefront carry OAM, or phase singularity in the center. In the far-field, the vortex beam takes the form of Laguerre Gaussian mode where the phase singularity evolves into a doughnut distribution. The far-field intensity and phase pattern of vortex beam with topological charge of 2 are shown in Fig. 4-1. In this example, LG02 is expected. LG beams are a set of solutions to Maxwell’s Equations that carry OAM with rotational symmetry expressed in cylindrical coordinates. P denotes radial nodes while l represents the topological charge associated with the beam. Generally speaking, as l increases, the dark center of the donut-shaped beam also increases. Fig. 4-1. Intensity and phase pattern for LG02 mode. Generation of scalar vortex beam (LG02) is reported in this section. A novel beam with spatially variant polarization has been demonstrated theoretically and experimentally by superimposing orthogonally polarized fundamental Gaussian (LG00) and second order Laguerre Gaussian (LG02) beams [39]. This beam in fact belongs to the family of the second order FP beams. The evolution of the SOPs along propagation will be discussed in details. 34 The fundamental Gaussian beam can be represented as: LG00 r , z A0 A0 w0 e w z w0 e w z j kz z jkr 2 2 q z 1 jk , j kz z r 2 z 2 z02 w0 2 1 2 z z z0 (4-1) where A0 is the amplitude, w0 is the beam waist, q(z) is the Gaussian beam propagation parameter as a function of axial distance z, w(z) is the beam size, φ(z) is the Gouy phase for fundamental Gauss and z0 is the Rayleigh range. A more detailed discussion on general Laguerre Gaussian modes LGpl can be found on Chapter 7, Section 4.1. Similarly, second-order Laguerre Gaussian (LG02) beams can be written as: LG02 r , , z A0 2 r2 w z 2 w0 j kz 3 z j 2 e w z 2 , jk 1 exp r 2 2 z 2 z 2 z 0 w 1 0 z z 0 (4-2) where ϕ is introduced as the azimuthal angle due to the spiral wave front. Note that the Gouy phase for LG0,2 is 3 times larger than the one for the fundamental Gauss. 35 A superposition of orthogonally polarized LG00 and LG02 can be expressed as follows: EFP r , z cos LG00 xˆ sin LG02 yˆ 1 C j 0e , (4-3) Here we denote the second term in Jones vector as ρ0ejδ, where ρ0 is the ratio between y and x components and δ is the phase difference. Angle γ is the angle between the polarization direction and the horizontal axis, which is used to adjust the weighting between the x and y components of the FP beam. Then we would have the following expressions: 0 2 tan r2 w z 2 , 2 z 2 , (4-4) Simple algebra shows that close to axis, the polarization is mainly along x-axis while away from axis the polarization evolves to y-polarization. The phase delay is twice the difference of azimuthal angle and Gouy phase shift. Therefore at any cross section of the superimposed beam along propagation, the phase delay between two components will range from 0 to 4π. Thus, the SOP of in the superimposed beam cross section second will span the entire surface of Poincaré sphere twice. Hence, we call this the second order FP beam. Along propagation, the Gouy phase shift will further introduce an additional phase delay of 0 to -π, which will cause the SOP to rotate by 2π as it propagates. Numerical simulation agrees well with the prediction, as illustrated in Fig. 4-2. 36 Fig. 4-2. SOPs evolution for second order FP beam at 1). z = -10zR, 2). z = -zR, 3). z = 0, 4). z = zR and 5). z = 10zR. In the above figure, the local SOP is denoted as lines, ellipses or circles. The ± 10zR represent z at ± infinity. Between adjacent plots, a change of π/2 in the phase difference δ has been introduced for the local polarization as the beam propagates. For instance, the polarization of the red circled area evolves from 45° linear to RCP, 135° linear, LCP and finally back to 45° linear as the beam propagates from minus infinity to plus infinity. In other word, as the beam propagates from negative infinity to positive infinity, the local polarization at each relative position (azimuth φ and normalized radius r/w(z)) experiences a continuous rotation in phase difference δ from 0 to 2π. 37 Recall that normalized Stokes Vector can be written as S1 cos 2 cos 2 cos 2 S 2 cos 2 sin 2 sin 2 cos S3 sin 2 sin 2 sin (4-5) where tan(χ) = ρ0 = 2tan(γ)(r/w(z))2, describing the ratio of the amplitudes of y and x components. The evolution of SOP at fixed azimuthal angle φ and relative radius r/w(z) along propagation covers one slice (shown in red) of the Poincaré sphere perpendicular to the S1 axis as shown in Fig. 4-3 where δ spans from 0 to 2π due to Gouy phase at a constant S1 (cos(2χ)). However, the intensity, as a function of γ and r/w(z), remains unchanged during propagation. Fig. 4-3. One slice (shown in red) of the Poincaré sphere at fixed ϕ and r/w(z) with δ spanning from 0 to 2π. 38 3. Summary Second-order full Poincaré beams are introduced. As one type of 2nd order FP beams, the vectorial beam as a superposition of x-polarized Gaussian and y-polarized LG02 is investigated in details. The SOPs in the cross section are shown to cover the entire Poincaré sphere twice, hence the 2nd order FP beams. The evolution of the SOP during propagation is also investigated. Potential applications of such beam include laser beam shaping, where the beam has been experimentally generated both using the SLM [39] [41]and compact beam shaper [42]. The flattop beam profile has been demonstrated in both cases. 39 CHAPTER 5 GENERATING CYLINDRICAL VECTOR BEAM WITH SUBWAVELENGTH CONCENTRIC METALLIC GRATING FABRICATED ON OPTICAL FIBER Subwavelength grating structures have long been used to modify optical fields [43] [44]. In this chapter, a metallic grating structure is used to realize polarization selection by generating generalized cylindrical vector beams, as an example of more complex control of complex vectorial optical field. As one example of polarization control using subwavelength metallic structures, we report the generation of cylindrical vector (CV) beam with a subwavelength concentric metallic grating fabricated on an optical fiber, eliminating the widely used conical devices or birefringent crystals. It has been demonstrated that a wiregrid grating with a period smaller than the wavelength of incident light strongly reflects TE polarized light and allows TM polarized light to transmit through [25]. Subwavelength concentric metallic slits have been used for creating two-lobe shaped radially polarized or azimuthally polarized beam with linearly polarized illumination [26]. When an 40 azimuthally polarized light is focused onto the axially symmetric metallic grating, the entire beam is TE polarized with respect to the interface and therefore experiences high reflection. In contrary, a radially polarized beam is entirely TM polarized with respect to the metallic grating and can pass through the device with higher transmittance than the azimuthal polarization. It has been shown that circular polarization can be decomposed into the combination of radial polarization and azimuthal polarization components with a spiral phase wavefront [45]. Therefore, if a circularly polarized beam is coupled into a fiber with a subwavelength concentric metallic grating integrated on the core region, the radial polarization component has much higher transmittance than the azimuthal polarization component. Consequently, a doughnut-shaped CV beam can be created. LP QW Lens Metallic rings LP Laser CCD Fiber Fig. 5-1. Experimental setup for generalized CV beam generation. [46] The diagram of the experimental setup is illustrated in Fig. 5-1. A subwavelength concentric metallic grating fabricated on the core of an optical fiber was used as a polarization selector for generating CV beams. First, a 200 nm gold film was deposited onto a cleaved fiber (Thorlabs 630HP) facet with e-beam evaporation. This thickness was chosen to prevent high direct transmission of the laser through the gold layer. Then twenty periods of concentric annular slits were fabricated into the gold film with focused 41 ion beam milling (FIB, FEI dual beam SEM-FIB NOVA 200 Nanolab system) with the center of the concentric rings coincides with the center of the fiber. The number of rings is chosen to ensure that the concentric grating is larger than the core region of the fiber. Fig. 5-2 shows the scanning electron microscope (SEM) images of the fiber based concentric grating (Bull’s Eye structure) fabricated by Don Abeysinghe with focused ion beam (FIB) and a zoom-in of the metallic annular structure. The grating has a period of 200 nm, which is smaller than the laser wavelength (Nd:YAG second harmonic 532 nm green laser). The duty cycle was chosen to be 50%. A circularly polarized Gaussian beam was focused onto the fiber end with the concentric grating structure. The output beam at the other end of the fiber was imaged onto a CCD camera. A linear analyzer was placed in front of the camera to investigate the SOP of the light. Fig. 5-2. SEM pictures of the Bull's Eye structure. [46] Sample is prepared by Don Abeysinghe using FIB. 42 A left-hand or right-hand circularly polarized beam (LCP or RCP) is a linear superposition of uniformly distributed radially polarized and azimuthally polarized vortex beams with a topological charge of 1 [45]. j E LHC P ( r ) e ( er je ) 2 , E RHC P ( r )e j ( er je ) 2 , (5-1) where P(r) is the amplitude distribution of the beam in cylindrical coordinate, er and eφ are amplitude of unit vectors in radial and azimuthal directions, respectively. Due to much higher transmittance of radial polarization component, a mostly radially polarized beam can be obtained at the output end. A finite element method model (COMSOL Multiphysics) was developed to numerically investigate the polarization selection properties of the subwavelength concentric metallic grating fabricated on optical fiber under circularly polarized illumination. 3D model was used and the thickness is chosen at 200 nm to balance the polarization conversion efficiency and the milling time using FIB. The simulated energy density and local electric vector field distributions are illustrated in Fig. 5-3. The extinction ratio between radial polarization and azimuthal polarization was found to be 50.7, therefore the electric vector field orientation of the output CV beam has a small angle (~8 degrees) deviating from the radial direction. 43 Fig. 5-3. Simulated energy density and local SOP. [46] 44 Fig. 5-4. Experimental results for generalized CV beam generation. [46] 45 Fig. 5-4 (upper) shows the total intensity distribution of the output laser beam captured by the CCD camera. A doughnut spot with a dark center was obtained at the output end. Fig. 5-4 (lower) shows the pictures of the output laser beam after it passes through a linear analyzer oriented at different angles indicated by the arrows. The two-lobe spot follows the rotation of the linear analyzer, indicating the generation of a CV beam. The beam can be conveniently converted into an azimuthally polarized beam or radially polarized beam with two cascaded half-wave plates [47]. The transmission efficiency of the CV beam was measured to be 1.96%. This efficiency can be improved by adjusting the thickness of the metal film and annular ring parameters. The integrated subwavelength structure on the fiber end provides a compact and convenient way for CV beam generation in fiber laser cavity design. If the concentric metallic grating is used as one end mirror coupler, the axially symmetry of the metallic rings ensures that the oscillation mode has axially polarization symmetry and radial polarization output will be resulted due to its polarization selectivity. Summary In this project, the polarization-sensitive Bull’s Eye structure is designed and experimentally verified. The generation of generalized cylindrical vector beam with mostly radial polarization is confirmed with the all-fiber device. This approach eliminates the needs of conventional conical devices or birefringent crystals in fiber laser cavity design and enables a compact all-fiber laser design. It also avoids the requirement of precise alignment, which could improve the stability of the CV beam generation. 46 CHAPTER 6 COMPLEX OPTICAL FILTER FOR HIGH PURITY OPTICAL NEEDLE FIELD GENERATION 1. Introduction In this chapter, a more complex engineering of the optical field is proposed, where modulations of phase, amplitude and polarization are simultaneously realized using complex filter designs with subwavelength grating and optical antennas. The engineered optical field will then be focused by a high NA objective and high-purity optical needle field is expected with flattop distribution along longitudinal direction and an extended depth of focus. The investigation of focused electromagnetic field over a three dimensional volume has always been an interesting and important area of theoretical and applied optics. The focusing properties of linearly polarized (scalar) field have been well established by Richards and Wolf [33]. However, beams that possess polarization axial symmetry, i.e. radial and azimuthal polarization, hadn’t been thoroughly investigated until recent years. These beams characterized by a spatially inhomogeneous SOP, are also called cylindrical 47 vector beams (CVBs). Of particular interest, it is found that under tight focusing, an azimuthally polarized beam maintains its polarization property while a radially polarized beam acquires a significant longitudinal polarization component [4] [6]. By using a carefully designed pupil apodization function, it is possible to achieve a tighter focusing spot and increase the resolution of the system by a factor of two [47] [15]. By using a DOE pupil mask with binary phase coding, it is also possible to achieve a flattop profile at focal plane with extended depth of focus [16]. The generation of an optical needle field proposed in [48] provides a new approach to obtain an electrical field with uniform axial intensity profile, extended depth of focus and high-purity longitudinal polarization. The unique electric field distribution opens the door to applications in polarization sensitive imaging [49], light-matter interaction on the nanometer scale and particle trapping and acceleration [50]. For instance, the uniform axial intensity profile along with extended depth of focus ensures a uniform and elongated trapping force in longitudinal direction for increased trapping efficiency. 2. Electric field calculation at pupil plane Reversing radiation of an electric dipole array located around the focus of a high NA lens is used to calculate the incident field at the pupil plane [48]. A high NA focusing of engineered optical field at the pupil plane is depicted in Fig. 6-1, where the vector field in the focal volume near focal plane shown in red is of interest. An array of equally spaced electric dipoles is placed in the vicinity of the focal plane, which is shown in Fig. 6-2 [48]. 48 Fig. 6-1. High NA focusing of pupil plane field in the focal volume (shown in red). Fig. 6-2. Schematic configuration of reversing radiation of an electric dipole array. 49 where N pairs of dipoles (N = 2) shown in red in Fig. 6-2 are located symmetrically with respect to the focal point along the optical axis. Due to the symmetry, we only need to adjust the amplitude An, the spacing between two dipoles in each pair dn and additional phases ±βn associated with both dipoles in each pair. The superposition is written as, N AFn An e n 1 where kdn cos n j kd n cos n /2 e j kd n cos n /2 , (6-1) is the phase difference between both dipoles in each pair and it has been divided by 2 to achieve equal distribution on both dipoles. For an objective lens that follows sine condition, the incident field can be represented as [4] [33], Ei i , C sin / cos AFn cos xi sin yi , (6-2) where φ is the azimuthal angle in the pupil plane. For a radially polarized beam, the radial and longitudinal electric field near focus may be expressed using the vectorial Debye theory [4] as Er r , z C max AF sin n 2 cos J1 kr sin eikz cos d , (6-3) 0 Ez r , z C max AF sin n 3 0 50 J 0 kr sin eikz cos d , (6-4) respectively, where C is a constant. Generally, the higher the number of dipole pairs N is, the longer the DOF of the resulting field will be. However, the complexity of the corresponding pupil plane distribution will also increase. A trial and error methodology is employed and a DOF of 5λ with a uniform intensity in the longitudinal direction around the focus has been achieved using the transparency reconstructed from an array of 2 pairs of dipoles. The parameters of the dipole array are shown in Table 1 [48]. Table 1: Parameters of dipole array for N = 2 An dn βn 1 1.39 λ π 0.87 4.10 λ 3π The far field intensity along focus is shown in Fig. 6-3 (upper) and the line scan of the normalized intensity in Fig. 6-3 (lower) [48]. This demonstrates very high longitudinal field purity and a nearly flat top axial distribution in focal volume. Therefore, the optical needle field is expected near the focal volume. Beam purity of 86%, which is defined as the intensity of the longitudinally polarized component confined within the optical needle over the total intensity, has been achieved. 51 Fig. 6-3. Far field intensity along focus (upper) and its line scan (lower) [48]. The longitudinal coordinate is normalized to the wavelength. The depth of focus is found to be 7.9 λ. In order to generate such optical needle field, the required intensity distribution of the optical field in the pupil plane and its line scan are calculated via Eq. (6-2) and Table 1 and shown in Fig. 6-4 [48]. We noticed that the highest transmittance occurs at the outermost ring. 52 Fig. 6-4. Intensity distribution in the pupil plane (upper) and its line scan (lower) [48]. The transverse coordinate is normalized to the pupil radius of the high NA objective. 53 3. Discretization of the pupil filter The desired field at pupil plane can be considered as the transmitted field of a radially polarized electric field from a filter located at the pupil plane. The filter has a complex transmittance for both amplitude and phase. To realize the optical needle field in practice, we introduce a simplified discrete filter design with non-continuous transmittance and binary phase. The amplitude and phase of the filter are plotted along radial direction as shown in Fig. 6-5 [48]. Fig. 6-5. Discrete filter design. ρ is normalized to the pupil radius for the high NA objective. 54 The resulting field is further calculated and the performance is shown in Fig. 6-6 [48]. Fig. 6-6. Electric field along focus (a) and its line scan (b) for discrete pupil filter. The horizontal axis is normalized by the wavelength. The results show a good agreement with the continuous complex filter. Implementation is made possible with the discretized design discussed here and liquid crystal devices, such as SLMs and subwavelength metallic structures are good candidates to realize such pupil filter. 55 Nikon CFI Plan Apo VC is used as the high NA objective. The lens has a magnification of 100X and NA of 1.4 in oil. The focal length is found to be 2 mm and NA in air is 0.924. The radius of pupil is found to be 1.85 mm and the diameter is 3.7 mm. 4. Sub-wavelength metallic grating implementation for optical needle generation 4.1. Introduction Sub-wavelength metallic gratings have been thoroughly investigated for its reflection and transmittance properties by researchers in this field [34]. The degrees of freedom in the grating design include the choice of metal, depth of grating, periodicity and duty cycle of the grating. By carefully choosing the parameters, the amplitude and phase of the zeroth order of the transmitted electric field can be adjusted to the desired combination in each annular ring. For each annular ring, the structure can be approximated as a rectangular grating with infinite number of periods. Rigorous Coupled Wave Analysis (RCWA) [27] [28] [29] is used to evaluate the diffraction of electric field by a periodic grating structure. A thorough search is performed to generate the desired amplitude and phase of the transmitted electric field for the three inner rings with lower transmittance. The zero transmittance is simply obtained by coating a layer of Al film and high transmittance is approximated by the transparent glass substrate. 56 4.2. Pupil filter design and proposed experiment setup In our proposed design, aluminum (Al) is chosen as the metal and the highest amplitude at the outmost ring is provided by using a glass substrate. Al gratings on the glass substrate are engineered such that the three inner rings share the same period of 1 um and 50% duty cycle. By varying the depth of the grating, different amplitude and phase can be achieved. Fig. 6-7 has a schematic plot of the pupil filter. The black region is covered by the Al film and is opaque, the white region is the transparent glass substrate, the green region has a 180 nm thick Al grating structure and the blue region has a 675 nm thick Al grating structure. The parameters for different regions of the pupil mask are shown in Table 2, where Ring 1 refers to the innermost ring and Ring 7 is the outermost area of the pupil. FIB is to be used for the fabrication of the subwavelength metallic structure. The technique limits the radius of the pupil filter to 250 μm and in order to cover the entrance pupil of the Nikon objective, a telescope relay is required. The radius in Table 2 is given in microns and scaled with respect to the radius of the pupil filter. Table 2: Grating parameters for each concentric ring Ring 1 2 3 4 5 6 7 Radius (μm) 37.5 87.5 132.5 162.5 180 215 232.5 The proposed experimental setup is also included in Fig. 6-7. A linearly polarized laser beam is converted to radial polarization by a circular polarizer, a phase plate and a radial analyzer before passing through the pupil filter. With a telescope relay setup discussed 57 above, the beam can be expanded to match the NA of the 1.4-NA oil immersion objective lens. The resulting longitudinal field along the focus then can be detected using near-field scanning optical microscope (NSOM) setup. Filter λ=1.064μm Pinhole with 0.5 mm in dia. Radial Analyzer Telescope 1.4 NA oil immersion objective Fig. 6-7. Grating structure (upper) and proposed experimental setup (lower). The radii are normalized to the radius of the pupil. 58 5. Preliminary results Initial FIB sample is shown in Fig. 6-8. The depth of the trench is 100 nm. However, for grating thickness as much as 675 nm, even with the largest available current, it would take days of milling time to fabricate a deep trench. Therefore, a different fabrication technique needs to be adopted for the optical needle field generation using subwavelength metallic grating structure. Fig. 6-8. SEM of sample (by Don C Abeysinghe). 59 6. Design based on subwavelength metallic linear antenna 6.1. Introduction As an alternative approach, we also investigate the properties of subwavelength linear antenna design for its much smaller cross section, which as a result reduces the amount of metal removing. The scattered field off V-shaped nano antenna has recently been theoretically studied for its ability to control the amplitude and phase of the crosspolarized component [31] [32]. Thanks to the greater-than-2π phase coverage, the design of a plasmonic nano V-shaped antenna array to introduce a phase gradient from 0 to 2π at the interface of two media in order to steer the beam has been proposed and experimentally demonstrated. The amplitude and phase of the scattered field can be engineered by appropriately choosing the design parameters, the length of the rod antenna and the angle between the two arms. One cell of the nano V-shaped array consists of 8 V-shaped antennas providing a phase shift from 0 to 2π in one direction while exhibiting constant amplitude of the cross-polarized component. This is also referred to as generalized laws of reflection and refraction, or light bending using plasmonic nano-antenna. 6.2. Initial analysis Since our design of the discrete pupil filter only requires two phase values, 0 and π, we decided to investigate a linear rod antenna for its simplicity in numerical simulation and fabrication. 60 Fig. 6-9: Linear antenna oriented at angle θ from the incident polarization. A linear antenna with a certain length and angle θ from the incident polarization (as illustrated in Fig. 6-9) has the potential to spatially modify the amplitude and phase of cross-polarized scattering field. The Hallen and Pocklington Integral Equations [51] are given as 4 l /2 I z ' G z z ' dz ' j 2z k 2 Ein z , 1 (6-5) l /2 4 l /2 I z ' 2 z k 2 G z z ' dz ' j Ein z , (6-6) l /2 where G z z ' 1 2 2 0 e jkR d ' and R R z z ' 2 2a 2 2a 2 cos ' . Based on these equations, the normalized amplitude and phase of the scattered field polarized in the axial direction (z direction) off the linear rod antenna can be calculated numerically and plotted as a function of the length L as shown in Fig. 6-10. 61 1 0.9 Normalized amplitude 0.8 0.7 0.6 0.5 0.4 0.3 0.2 0.1 0 0.2 0.3 0.4 0.5 L/0 0.6 0.7 0.8 0.3 0.4 0.5 L/0 0.6 0.7 0.8 0 -20 Phase (degree) -40 -60 -80 -100 -120 -140 -160 0.2 Fig. 6-10. Normalized amplitude (upper) and phase (lower) of the longitudinally polarized scattered field. The z (along antenna) and ρ components of the scattered field of the rod antenna placed along z direction with L = 0.5 λ are shown in Fig. 6-11 and Fig. 6-12, respectively. COMSOL Mulitphysics is a finite element method (FEM) based simulation tool. 62 Compared with COMSOL results, good agreement is observed between the two simulation tools. Fig. 6-11. The absolute value of the Ez component of the scattered field off the rod antenna. Fig. 6-12. The absolute value of the Eρ component of the scattered field off the rod antenna. 63 Here we assume the antenna is parallel to the polarization of the incident light, λ0 denotes the wavelength and the radius of the rod antenna is λ0/100. By putting the antenna at an angle from the incident polarization, the projection of the incident light to the antenna direction follows a cosine rule. Consider the cross-polarized component of the scattered field, another projection of the longitudinally excited electric field to the orthogonal direction of the incident polarization needs to be performed in order to calculate the resulting field. Assuming the angle between the antenna and the incident polarization is θ, the cross-polarized component of the scattered field and the original scattered field follows such relationship: scattered scattered Ecross cos sin polarized E , (6-7) A phase jump of 180 degrees can be achieved if the product of cosine and sine functions becomes negative. The amplitude and phase of the cross-polarized scattered field off linear rod antennas then can be calculated as a function of both antenna length (L) and orientation (θ) from the incident polarization in Fig. 6-13 and Fig. 6-14, respectively. In both figures, the dashed line refers to a constant 0.5 amplitude contour plot. As can be seen from Fig. 6-14, the phase coverage is greater than π but less than 2π 64 Fig. 6-13. 2D amplitude plot of linear antenna versus length L and θ. Fig. 6-14. 2D phase plot of linear antenna versus length L and θ. 6.3. Complex optical filter design The maximum amplitude occurs at L = 0.4744 λ. Since we only need a phase change of 0 and π, a horizontal line at L = 0.4744 λ is the area of interest. In our proposed pupil filter 65 design, both the amplitude and phase can be regarded as relative quantities for different annular rings. Amplitude modulation can be obtained by rotating the linear antenna with respect to the local polarization, in other words, to change the angle θ. The parameters are shown in the following table (Table 3) for different annular rings on the pupil mask. Table 3: Design parameters Amplitude 0.07 0.077 0.132 0.48 1 Phase 0 (π) π (0) 0 (π) π(0) π(0) Orientation (θ) 2.0 2.2 3.8 14.3 45 The orientation angle θ listed above all have phase of 0. To change the phase from 0 to π, one can use a simple transformation as follows. new 2 or , (6-8) Since the required electric field before tight focusing needs to be radially polarized, a radial analyzer is required in front of the high NA objective. The incident field onto the antenna pupil mask needs to be azimuthally polarized to ensure correct field distribution in the cross-polarized component, which is a radial polarization in this case. The illumination wavelength is 1.064 μm so the length of the rod antenna is set to be 0.505 μm. To ensure the fabrication is feasible, we set the radius of the cross section of the rod antenna to be 25 nm. The 1D plots (Fig. 6-15) of normalized amplitude and phase of 66 longitudinally polarized scattered field and 2D plots (Fig. 6-16) of the cross-polarized scattered field as a function of length L and orientation θ have been regenerated for 25 nm radius rod antenna. 1 0.9 Normalized amplitude 0.8 0.7 0.6 0.5 0.4 0.3 0.2 0.1 0 0.1 0.2 0.3 0.4 0.5 L/0 0.6 0.7 0.8 0.9 0.2 0.3 0.4 0.5 L/0 0.6 0.7 0.8 0.9 0 -20 Phase (degree) -40 -60 -80 -100 -120 -140 -160 0.1 Fig. 6-15. Normalized amplitude (upper) and phase (lower) of the longitudinally polarized scattered field for 25 nm radius rod antenna. 67 Fig. 6-16. Normalized amplitude (upper) and phase (lower) of cross-polarized scattered field as a function of L and θ for 25-nm radius rod antenna. Note that the maximum amplitude occurs at L = 0.4739 λ, only with a negligible shift. Since the amplitude modulation is achieved by adjusting angle θ, the design is identical as the previous model. The complete design is shown in Table 4, where the antenna 68 direction is measured from the local polarization direction (azimuthal direction). A tolerance study of all of the design parameters for +/- 10% fluctuation in the orientations of the linear antennas is performed in 69 Table 5. Table 4: Antenna design parameters for optical needle field generation Annular ring # 1 2 3 4 5 2° 92.2° 3.8° 104.3° 135° Amplitude 0.007 0.0077 0.0133 0.0481 0.1005 Phase (radians) -2.096 1.048 -2.094 1.048 1.050 0.070 0.077 0.132 0.479 1 Antenna direction Normalized Amplitude 70 Table 5. Tolerance study of the antenna structure Upper limit Lower limit Phase (-93.4 ◦) +0.2π (-57.4◦) -0.2π Length (0.4744) 0.4256 0.5663 Amplitude1 (0.07) +10% (0.077) -10% (0.063) Orientation (2.0) 2.2 1.8 Amplitude2 (0.077) +10% (0.0847) -10% (0.0693) Orientation (2.2) 2.4 2.0 Amplitude3 (0.132) +10% (0.145) -10% (0.119) Orientation (3.8) 4.2 3.4 Amplitude4 (0.48) +10% (0.528) -10% (0.432) Orientation (14.3) 15.9 12.8 Amplitude5 (1) +10% (1.1) -10% (0.9) Orientation (45.0) n.a. 32.0 71 6.4. Realization of complex optical filter with slot antennas The linear antenna design may offer the ultimate method to achieve optical needle field after tight focusing. Rectangle cross section needs to numerically simulated and compared with circular one. We expect a cross section of 100 nm x 50 nm rectangle to behave similarly as the rod antenna with 50 nm radius. COMSOL simulations are performed for both original design and the complimentary design (slot in metal) based on Babinet’s Principle as depicted in Fig. 6-17. Fig. 6-17. Rectangle linear antenna and its complementary design. Due to the vector Babinet’s principle [52] [53], the transmitted polarization will be orthogonal to the long axis of the slot antenna. The orthogonal component of the transmitted field will follow the same relationship as the original design of the linear antenna. In other word, for azimuthally polarized input field, the radial component of the transmitted field will have the designed amplitude/phase distribution. The new slot antenna design requires much less metal to be removed compared to the grating, which 72 thus made the FIB a suitable and reliable fabrication technique. The antenna sample is fabricated by Don Abeysinghe using FIB shown in Fig. 6-18 Very good uniformity of the antenna in terms of direction and shape has been achieved. Fig. 6-18. SEM pictures of antenna structure as complex optical filter fabricated by Don C Abeysinghe using FIB. 7. Summary The complex optical filter design with optical antennas is presented for optical needle field generation. The tolerance study is performed and it shows a reasonable tolerance to the fabrication error. The slot antenna design is proposed and investigated based on Babinet’s principle and the fabrication is made possible using FIB. It has been theoretically shown that with the complex optical filter, we are able to obtain the desired amplitude and binary phase distribution at the pupil plane of a high NA objective for optical needle field generation. 73 CHAPTER 7 VECTOR OPTICAL FIELD GENERATOR 1. Introduction All these projects discussed in previous chapters lead to the need for a universal system that’s capable of manipulating all degrees of freedom for vectorial optical field, as the complexity of the conventional system increases and fabrication of the individual filter design gets more and more challenging. In this chapter, VOF-Gen that is capable of generating vectorial optical field with arbitrary phase, amplitude and polarization on a pixel by pixel basis is proposed and experimentally demonstrated. Optical trapping, or particle manipulation in colloidal and biomedical sciences, is made possible by the shaping of light [54]. Shaped optical fields have enabled researchers to better understand the biophysics and colloidal dynamics through the trapping, guiding or patterning of molecules or nano/micro particles. Spatial engineering of focal field intensity has been studied to reach resolution far beyond diffraction limit in microscope system [55]. Vortex beam, also known as “twisted light”, has also drawn a lot of interest owing to its spiral phase wavefront carrying orbital angular momentums [45]. Better 74 integrity of vortex beam through propagation in turbulent atmosphere has been shown [56] and a lot of research has been done using the orbital angular momentum as information carrier for free space communication due to its orthogonality and multiplexing capability [57]. Besides the manipulation of intensity and phase, as the vector nature of electromagnetic wave, the SOP also plays an important part in beam shaping for flattop generation [39], focus shaping [15], optical tweezing and surface plasmon sensing using cylindrical vectorial beams [58], ellipsometry [59]. All the above applications require modulations of certain aspect of optical fields. Tremendous amount of research has been conducted by scientists in the community developing versatile systems for the generation of the optical fields with exotic properties. Arbitrary vector fields with inhomogeneous distribution of linear polarization were realized using a spatial light modulator (SLM) and an interferometric arrangement [20]. A recent study showed that in order to fully control the SOP, two spatially addressable retarders need to used [21]. Researchers constructed such system consisting of two SLMs with the fast axes 45° from each other and were able to generate optical fields that cover the entire Poincare Sphere. Another non-interferometric method for vector field generation was proposed by Tripathi and Toussaint [22]. However, the complete control of both polarization elevation angle and ellipticity can only be realized by modifying the experimental setup. Complete amplitude, phase and polarization control was reported by Moreno et al. [23] with the help of a double modulation system which requires two transmissive SLMs whose modulation depth can be controlled to achieve amplitude modulation for certain diffraction order. However, this approach comes with the limitation that each area must contain a large number of periods to achieve the ideal 75 diffraction efficiency, which leads to optical field with limited spatial resolution for practical applications. Very recently, a technique for generating arbitrary intensity and polarization was reported with interesting results using transmissive SLMs and MachZehnder interferometry setup [24]. However, due to the nature of the technique, the absolute phase of each electric field component does not cover an entire 2π range. As a result, complete phase control cannot be fully realized. The limitations of this technique also include relatively low transmittance and poor spatial resolution. All the existing techniques have limitations and cannot be used to generate a spatially-invariant arbitrary vectorial field with high spatial resolution on a pixel basis. In this work, we propose and demonstrate a Vectorial Optical Field Generator (VOF-Gen) that is capable of creating an arbitrary beam with independent controls of phase, amplitude and polarization on the pixel level utilizing high resolution reflective phase-only LC-SLM. The scalar optical wave is typically written in the following complex form: E x, y E0 x, y e j k r t , (7-1) where Eo(x, y) denotes the amplitude and the exponential part carries phase information. However, in most cases, desired optical field takes vector form, which can be represented as a superposition of two orthogonal polarization components. Using Jones vector representation, the desired field is usually written as: E d x, y Ad x, y e jd x , y 76 E xd x, y E x, y e j d x , y yd , (7-2) where Ad(x, y) represents the amplitude distribution, ϕd(x, y) is the common phase for both x and y components and the Jones vector contains the polarization information where Exd and Eyd are both real and normalized (Exd2 + Eyd2 = 1). δd(x, y) is the desired phase retardation between the y and x components. As we know the polarization state can be represented either in terms of linear polarization rotation χ and retardation δ or in terms of polarization elevation angle α and ellipticity ε as shown in Eq. (7-3). cos sin e j cos sin at , or (7-3) These two representations are equivalent and can both describe any SOP on the Poincare’s Sphere. They can be converted using Eq. (7-4). tan e j tan j tan 1 j tan tan , (7-4) Clearly four degrees of freedom, namely the phase, amplitude, polarization ratio and retardation between the x and y components are necessary in order to fully characterize a vectorial optical field. Thus a true vectorial optical field generator needs to be able to control all of these four parameters on a pixel-by-pixel basis for the generation of arbitrarily complex vectorial optical field. The principles of our proposed VOF-Gen will be discussed in details in the following. 2. Principles As one example, a Taiji pattern is generated using VOF-Gen with one half polarized in right-hand circular polarization (RCP) and the other in left-hand circular polarization 77 (LCP) as depicted in Fig. 7-1. The principles of the VOF-Gen will be discussed in details in this section. Fig. 7-1. Taiji pattern coded in circular polarization. The total field (left), the upper half Taiji pattern (upper right) in RCP and the lower half Taiji pattern (lower right) in LCP. 2.1. Spatial light modulator As a key component for the VOF-Gen, the SLM, Holoeye HEO 1080P, is used as a variable and addressable retarder. The SLM is a phase-only, reflective liquid crystal (LC) device featuring a HDTV resolution of 1920 x 1080 with pixel pitch of 8 μm and fill factor of 87%. The retardation for each pixel on the SLM can be described as a function of the voltage (V) applied: (V ) 2 / ne V no d , where d is the thickness of the LC layer, ne and no are the extraordinary and ordinary refractive indices of the LC retarder, respectively. Due to the birefringent nature, the SLM in our system only responds to the horizontal polarization parallel to the LC directors, meaning that the horizontal 78 component of the reflected beam will carry the wavefront specified by the SLM while the vertical one will be reflected unaffected. Since four degrees of freedom in Eq. (7-2) need to be independently controlled in the system, four reflections are required where each SLM section is loaded with one of the phase patterns for the modulations of phase, amplitude, polarization rotation and retardation. First we show in detail how the modulations of the four degrees of freedom in the VOFGen can be achieved step by step with the introduction of the key components and the calculation of the required phase patterns. Then we discuss the system integration, experiment setup and extra care we took in building the system to ensure excellent results. 2.2. Spatially variant polarization rotator Our proposed system relies on one key component called Polarization Rotator (PR) based on the concept of a pure polarization rotator in order to realize the amplitude modulation and linear polarization rotation. Pure polarization rotator that consists of a quarter-wave plate (QWP), variable optical retarder with fast axis at 45° and anther QWP with its fast axis perpendicular to that of the first QWP has been proposed to achieve fast, nonmechanical polarization rotation [60]. 79 Fig. 7-2. Illustration of the Polarization Rotator setup. (a) The Polarization Rotator comprised of QWP and reflective SLM; (b) Illustration of the effective rotation of the QWP fast axis for the incident (upper) and the reflected (lower) beams due to the mirror imaging of the laboratory coordinates in dashed lines. In our design, the variable retarder is replaced with the LC-SLM to realize spatially variant polarization rotation function on a pixel-by-pixel basis as shown in Fig. 7-2(a). The fast axis of the QWP is 45° with respect to the horizontal axis. The incident light passes the QWP with fast axis oriented at 45° (upper part in Fig. 7-2(b)) in the laboratory coordinate (x, y) for the incident beam, then gets reflected off the SLM surface. The reflected light goes through the same QWP for the second time (lower part in Fig. 7-2(b)). However, due to the opposite propagation direction, the new laboratory coordinate (x’, y’) is a mirror image of coordinate (x, y) about the y axis. Therefore, the fast axis of the QWP has been effectively rotated to 135° in the coordinate (x’, y’). Thus, the Jones matrix representation of the PR can be calculated as: 80 3 3 M PR R J QWP R 4 4 1 0 M SLM R J QWP R 0 1 4 4 i x , y 1 1 i 1 i 1 0 e 4 1 i 1 i 0 1 0 0 1 i 1 i 1 1 i 1 i x, y x, y sin cos x, y 2 2 i e 2 x, y x, y cos sin 2 2 e x, y i 2 , (7-5) 3 x, y R 2 2 Equation (7-5) describes the Jones matrix of PR in terms of a rotation matrix R with an extra phase term. The rotation matrix R indicates an effective polarization rotation of 3 / 2 x, y / 2 at each pixel. In other words, the counter-clockwise polarization rotation at each pixel is found to be x, y / 2 / 2 , which depends on the phase loaded onto the SLM. The PR setup is also used to calibrate the look up table (gamma curves) for both SLM panels. By precisely measuring the amount of rotation based on the nulling effect with a linear analyzer for each gray level, we are able to calibrate the gamma curves so that the gray level and the actual phase imposed by the SLM are more concisely correlated. 81 2.3. System flow chart Fig. 7-3. Flow chart of the system. The VOF-Gen System consists of light source, 4 subsystems for control of all the aspects of light, 4-f imaging subsystems and detection subsystem. PR: Polarization Rotator. The VOF-Gen consists of the light source, four SLM sections as subsystems to realize the modulation of all degrees of freedom for arbitrary optical field generation, 4-f imaging subsystems [34] to relay the optical field from one SLM section to the next or to the image plane and a CCD camera for detection. The 4-f imaging system is introduced to minimize the diffraction effect after careful alignment. The SLM sections (subsystems) are integrated to achieve the full control functionality as described in Fig. 7-3. For the desired complex optical field that we want to generate, the phase patterns for the SLMs are calculated based on a collimated Gaussian input beam. Then the phase patterns are loaded onto the generator and the modulations of phase, amplitude, polarization ratio and retardation are realized through SLM Sections 1 to 4 as shown in the flow chart, respectively. At the output plane, the beam is expected to have the desired complex optical field distribution and can be analyzed thereafter. The 4-f imaging systems are 82 introduced to relay between SLM sections to minimize the diffraction effects. Details of the modulations and phase pattern calculations are given in the following. 2.4. Modulation of Light 2.4.1. Phase modulation (SLM Section 1) Phase modulation can be readily realized as the phase information loaded on the SLM will be directly imposed on the horizontal component of the reflected beam. This is done in SLM Section 1 with a horizontally polarized, well collimated Gaussian input beam. The resulting field can be represented in terms of Jones Vector as: J1 x, y e i1 x , y 1 E0 x, y , 0 (7-6) where Eo(x, y) is the amplitude of the input field and ϕ1(x, y) is the phase pattern loaded onto SLM Section 1 of the VOF-Gen. As will be discussed later, the phase ϕ1(x, y) will contain not only the desired phase ϕd(x, y) according to Eq. (7-2), but also a precompensation phase that are due to the geometric phase effect for the polarization rotator described in Section 2.2 above. 2.4.2. Amplitude modulation (SLM Section 2) Amplitude modulation is achieved by putting a linear polarizer with transmission axis oriented along horizontal direction after a PR setup utilizing the second SLM section. For horizontally polarized input field defined in Eq. (7-6), the resulting output field can be represented in Jones Vector form as: 83 J 2 x, y e x, y i 1 x , y + 2 + 2 x, y 1 sin 2 E x , y , 0 2 0 (7-7) where ϕ2(x, y) is the phase pattern for SLM Section 2. Equation (7-7) shows that amplitude modulation can be achieved with the sine function while the output is still horizontally polarized. For ϕ2(x, y) = 0 radian, 0 amplitude can be obtained and unit amplitude is expected for ϕ2(x, y) = π. Recall the general expression for desired field as shown in Eq. (7-2). Compared to the definition for the desired field, ϕ2(x, y) can be given via the following expression: 2 x, y 2 sin 1 Ad x, y , 2.4.3. (7-8) Polarization ratio modulation (SLM Section 3) As described in Eq. (7-7), the output field of SLM Section 2 is horizontally polarized. Using another PR setup consisting of the third SLM section, the SOP at each location can be linearly rotated to any direction prescribed by the local phase pattern to realize the desired polarization ratio distribution between the x- and y- polarization components. Assuming the phase pattern for SLM Section 3 is ϕ3(x, y), we have the output field of SLM Section 3 given by: 84 J 3 x , y E0 x , y e x , y 3 x , y i 1 x , y 2 2 2 3 x, y cos 2 2 x, y , sin 2 2 x, y sin 3 2 2 (7-9) Similarly, ϕ3(x, y) can be found from the desired field distribution given by Eq. (7-2): E yd x, y 3 x, y 2 tan E xd x, y 1 2.4.4. , (7-10) Phase retardation modulation (SLM Section 4) Phase retardation can be introduced by directly shining the linearly polarized output field of Section 3 as shown in Eq. (7-9) to the last SLM section due to the birefringence nature of the LC molecules. Assuming the phase pattern is ϕ4(x, y) for SLM Section 4, the final output field of the VOF-Gen can be written as: J 4 x , y E0 x , y e x , y 3 x , y i 1 x , y 2 2 2 3 x, y i4 x , y cos e 2 2 2 x , y , sin 2 3 x, y sin 2 2 85 (7-11) where 4 x, y d x, y , (7-12) as given by the desired field distribution Eq. (7-2). As we previously discussed, the first SLM section is responsible for the phase modulation. As we can see in Eq. (7-11), the phase of the final output will have the following expression: output x, y 1 x, y 2 x, y 3 x, y 2 2 , (7-13) Additional phase information is acquired throughout the steps of amplitude and polarization ratio modulations due to the geometrical phase effects arising from the two PRs used in the setup. Therefore, in order to correctly generate the desired phase in the final output, ϕ1(x, y) must contain both the desired phase information ϕd(x, y) and a precompensation phase that compensates the accumulated geometrical phases. By equating ϕoutput(x, y) to ϕd(x, y), we have: 1 x, y d x, y c x, y , (7-14) where the pre-compensation phase c x, y 2 x, y / 2 3 x, y / 2 . The verification of the need for this phase pre-compensation will be shown in Section 4.3. Note that the phase patterns ϕ1(x, y), ϕ2(x, y), ϕ3(x, y) and ϕ4(x, y) can all be spatially inhomogeneously distributed. For any desired output field with arbitrary spatial 86 distributions of phase, amplitude and polarization, Eqs. (7-8), (7-10), (7-12) and (7-14) can be used to calculate the required phase patterns. By loading the phase patterns onto each of the SLM sections of the VOF-Gen, arbitrarily complex desired output field can thus be generated. 3. Experimental setup 3.1. Experimental setup of the generator From the discussions above, in general four SLMs would be needed in order to fully control all of the degree of freedoms to create an arbitrarily complex optical field. However, taking the advantage of the HDTV format of the Holoeye HEO 1080P SLM, in our VOF-Gen setup two SLM panels are used with each of the SLM panel divided into two halves. Each half of the SLM panels is used to realize the control of one degree of freedom. This architecture utilizes the high resolution of the SLM panel while keeps the complexity of the experimental setup is kept manageable. 87 Fig. 7-4. Schematic diagram of the VOF-Gen. 88 Fig. 7-5. Experiment Setup of the VOF-Gen. The schematic diagram and actual experiment setup of the VOF-Gen are shown in Fig. 7-4 and Fig. 7-5, respectively. He-Ne laser of 632.8 nm wavelength is used as the input. Polarizer P1 and half wave plate λ/2 are used in combination to adjust input Gaussian beam intensity. Non-polarizing beam splitters (NPBSs) are used to properly direct the beam, thanks to its insensitivity of the polarization direction of the input beam. The SLM panels are divided into 4 sections, as shown in Fig. 7-4. The input beam first incidents on SLM Section 1 where phase modulation can be directly obtained. Lens L1 and Mirror M1 are used as a 4-f system. The optical field at the SLM surface in SLM Section 1 can be relayed to SLM Section 2 by carefully controlling the distances from the SLM to L1 and from L1 to M1 to be both equal to the focal length of L1, which is 300 mm. The QWP λ/4 combined with SLM Section 2 works as a PR discussed in Section 2.2. Amplitude modulation is achieved in this SLM section by using the PR setup and a polarizer P2 89 while the output beam is still polarized horizontally. The second 4-f system comprised of lenses L2 and L3 is used to image the optical field from SLM Section 2 to SLM Section 3, where polarization rotation is obtained with a second PR setup. Lens L4 and Mirror M2 work as another 4-f system to relay the field at SLM Section 3 to SLM Section 4. Retardation is added to the optical field after being reflected from SLM Section 4. Finally, lenses L5 and L6 are used to relay the field from SLM Section 4 to the Detector (LBAFW-SCOR by Spiricon) as the last 4-f imaging system in the entire VOF-Gen. Fig. 7-6. Driver circuits for the color channels of the VOF-Gen system. The upper one is the red channel responsible for the control of SLM1 and the lower one is the green channel for SLM 2. As previously mentioned, the VOF-Gen consists of two SLM panels as shown in Fig. 7-6. Therefore a simultaneous and independent control of both panels is required. This is realized through a color channel coding scheme such that the phase pattern for SLM 1 is coded into the green color (green channel) while the pattern for SLM 2 is coded in the red color (red channel). Then the two colors are combined to generate a color image as the 90 overall phase pattern as shown in Fig. 7-4. Note that we have divided each SLM panel into two halves. Therefore the control signal (overall phase pattern) is also multiplexed spatially into right and left halves to control the left and right sections of both SLMs, respectively. Thus the entire VOF-Gen can be operated with one computer that is capable of outputting 1920 x 1080 resolution color graphics. In order to generate arbitrary beams, diffraction effects have to be taken into consideration. The diffraction needs to be minimized so that sharp edges or high frequency information in phase, amplitude and polarization can survive. This is achieved by the four 4-f imaging systems used in our setup. Spatial filters SF1 and SF2 located in the Fourier planes of the 4-f systems are used to suppress the interference caused by bulk cube beam splitters. Opaque cardboards (shown as black bars between NPBSs in Fig. 7-4) are placed to block the direct illumination. Before proceeding to the complex optical field generation, gamma curves of both SLM panels need to be calibrated for accurate phase generation. 4-f systems also need to be well aligned to minimize the diffraction effects. 3.2. Gamma Curve Calibration Using Polarization Rotator In order to calibrate the gamma curve of the SLM, a calibration setup is proposed to perform the fine measurement of the actual phase-grey level relationship. The calibration setup consists of a PR, a beam splitter (BS), a polarizer with transmission axis at angle θ with respect to horizontal direction and a detector as depicted in Fig. 7-7. 91 Fig. 7-7. Calibration setup consists of a PR and a polarizer. The input beam is horizontally polarized (x-polarized) and it goes through the PR setup. The beam goes through a polarizer after passing through the BS and is collected by the detector. The polarizer is rotated by angle θ so that the transmission is minimized, which is the so-called nulling effect. For grey level X, based on the property of the PR the actual phase value imposed by the SLM pixel δ(X) can be found by X 2 X 2 X , 2 2 (7-15) where θ(X) is the amount of rotation of the polarizer as a function of grey level X. The same calibration procedure is performed for many grey levels and a precise calibration of the gamma curve can then be realized by generating the one to one mapping of actual phase-grey level relationship. For any phase value to be generated by 92 the SLM, a grey level is found by interpolating the phase value in the nonlinear relationship as opposed to using the linear relation: Grey _ level mod , 2 255 . 2 3.3. 4-f imaging system and its alignment procedure In order to generate arbitrary beams, diffraction effects have to be taken into consideration. The diffraction needs to be minimized so that sharp edges or high frequency information in phase, amplitude and polarization can survive. In our setup, four 4-f imaging systems [34] are used as discussed previously. In order to test the resolution of our system, the alignment of the 4-f imaging system is crucial in our experiment as shown in Fig. 3-1. In a well aligned 4-f imaging system, the image is an inverted replica of the object without any diffraction or any additional phase introduced. Thanks to the 4-f systems, the optical field at the SLM surface in SLM Section 1 with the phase modulation is imaged to SLM Section 2, adding the amplitude modulation, then to SLM Section 3 with polarization rotation, to SLM Section 4 with retardation information, and finally to the camera without the introduction of diffraction. Since the input beam is well collimated in our system, a shearing interferometer can be used as a collimation checker to align the 2f distance between the two lenses. Once the output beam is well collimated based on the collimation checker, the 2f distance can be precisely determined. In order to align the entire 4-f imaging system, mostly the f distance before the first lens and f distance after the second, we designed a pattern with fine features and used the 93 CCD camera to resolve the pattern as a figure of merit for the alignment. In our experiment, 3 horizontal lines crossed with 3 vertical lines are generated where each of the lines is only 100 μm wide shown in Fig. 7-8. Fig. 7-8: Pattern with fine features for 4-f imaging system alignment. Each line is 100 μm wide. The alignment is performed in a sequential order, as shown by the arrows in Fig. 7-9. The first 4-f system needs to be aligned is the one between CCD and SLM Section 4, where the retardation modulation is achieved. A beam is designed so that the pattern with fine features as shown in Fig. 7-8 is polarized in RCP while the rest of the beam polarized in LCP. The longitudinal distances in the 4-f system are adjusted until the sharpest pattern is detected by the CCD camera in front of which a circular analyzer is used to resolve the RCP component. At this point the first 4-f imaging system is well aligned. Then the alignment needs to be performed for each following 4-f imaging system in a similar way where different sets of patterns with fine features and the complementary are generated. The patterns are designed so that the degree of freedom to be realized in the specific SLM 94 section can be revealed. Then the 4-f imaging system’s alignment is determined by adjusting the distances to obtain the maximum sharpness where diffraction is eliminated. Fig. 7-9: 4-f imaging system alignment procedure The results for the alignment are shown in Fig. 7-10 below. Fig. 7-10: Test results for (a) amplitude modulation: the intensity is directly captured by the CCD camera; (b) polarization rotation: the intensity is captured after a linear polarizer; (c) Retardation: the intensity is captured after a circular analyzer. In all cases, the rectangular dark areas of 100 μm x 100 μm are visible with fairly sharp edges. This shows that the 4-f systems are well calibrated and the VOF-Gen is free of diffraction. 95 To test the 4-f imaging subsystems, ring and “EO” logo patterns are generated by the VOFGEN system without and with the 4-f imaging systems as shown in the left and right parts of Fig. 7-11, respectively. As we can see without the 4-f imaging system, the field captured by the CCD camera is blurred or smoothed out, where the high frequencies are not present. This is an indication of the diffraction effect. By introducing and aligning the 4-f imaging subsystems, the diffraction effects have been eliminated and sharp edges are observed with the help of the reconstruction from the 4-f imaging systems. Fig. 7-11: Comparison of the same patterns generated by VOF-Gen system without and with well aligned 4-f imaging systems. 96 4. Experimental results 4.1. Spatially variant phase modulation: vortex generation We first demonstrate the phase modulation capability with the generation of optical vortex beams. Optical vortices with spiral wavefront carry orbital angular momentum (OAM). If the phase of the beam has an azimuthal dependence of exp(ilφ), where φ is the azimuthal angle, then it’s said to have an OAM of lħ or a topological charge of l. Vortex beam with topological charge l in the far-field will have Laguerre Gaussian distribution of LG0,l. The mathematical representation of a general Laguerre Gaussian beam LGp,l can be shown as: l 2 w0 r l r2 E p ,l r , , z 2 L p 2 2 w z w2 z w z 2 kr 2 r 2 , (7-16) exp j kz pl z l 2 R z w2 z where 2 z z w02 z2 pl z 2 p l 1 tan , z0 , w z w0 1 and R z z 0 . z z0 z0 1 Lpl is the associated Laguerre polynomials and satisfies the following equation: x d 2 Llp x dx 2 (l 1 x ) dLlp x 97 dx pLlp x 0 . (7-17) Here p gives the number of nodes in radial direction and l gives the topological charge of the phase pattern. For the case where p = 0, the associated Laguerre polynomials reduces to 1. Further assuming z = 0 (no propagation), Eq. (7-16) can then be simplified as: l 2 r r2 E0,l r , ,0 2 2 exp j kz l 2 , w0 w0 2 (7-18) Since phase cannot be directly measured using a camera without resort to interferometric method, we first generated optical beams with pure spiral phase in order to demonstrate the phase modulation capability. Here only the first SLM section is controlled with a spiral phase and the phase patterns for the rest of VOF-Gen remain flat. The generated field is focused by a lens and the intensity is recorded at the focal plane by the CCD camera. Vortex beams with topological charges 1, 10 and 15 are generated here and the far-field intensities are as shown in Fig. 7-12. As we can see, LG0,1, LG0,10 and LG0,15 are observed in the focal plane of the lens. As the topological charge increases, the size of the dark center also increases according to the property of Laguerre Gaussian beams as described in Eq. (7-18) for LG0,l modes. This phenomenon can be understood as the larger phase singularity (higher topological charge) will inevitably lead to a larger dark center. This example shows the phase modulation capability of our VOF-Gen and we are able to generate vortex beams with topological charge up to 15 with good beam quality and integrity. 98 Fig. 7-12. Pure phase modulation with spiral phase of topological charge 1 (upper), 10 (middle) and 15 (lower). The images are captured in the focal plane of 75-mm planoconvex lens. A weak central spot is also observed and it may be caused by the direct reflection due to the filling factor, finite pixel size and level of quantization. The relative amplitude of the central spot is more pronounced for higher topological charges due to the enlarged ring area. 4.2. Spatially variant amplitude modulation In order to demonstrate the functionality of amplitude modulation, we designed an “EO” logo binary amplitude pattern. SLM Section 2 is loaded with “EO” shaped pattern for 100% 99 transmission and zero for the rest of the window. SLM Section 1 is loaded with a precompensation phase and SLM Section 3 and 4 both have flat phase. The output is directly captured by the CCD camera shown in Fig. 7-13 along with the phase pattern loaded onto VOF-Gen. It shows that fine features such as sharp edges in amplitude modulation are well preserved in the output beam. Note that the entire window would have been illuminated by the input Gaussian beam without the amplitude modulation. The result shows that fine features such as sharp edges in amplitude modulation are well preserved in the output beam. 100 Fig. 7-13. x-polarized "EO" logo coded in amplitude (upper) and its phase pattern (lower). 101 However, as one can see, the interference pattern has not been entirely removed. This is due to the fact that reducing the pinhole size in the Fourier plane of the 4-f system will remove both the interference pattern and high frequency components. In order to maintain a high resolution, we balanced the pinhole size so that high frequency terms are well preserved while only allowing a minimum amount of interference pattern. 4.3. Spatially variant polarization rotation: radially polarized beam Cylindrical Vector (CV) beams are a group of beams whose spatially variant SOP possesses cylindrical symmetry [1]. Due to the unique properties when focused by a high NA objective [15], there has been a great increase in the research of the CV beams recently, which has led to applications in high-resolution imaging [7], plasmonic focusing [2] and particle manipulation [61]. Numerous approaches have been proposed to generate such beams, including both active [62], [63] and passive methods [64], [59]. We illustrate the capability of using our generator to create these CV beams through the generation of a radially polarized beam, one important subset of CV beams. Essentially the CV beams such as the radial polarization can be generated with the polarization rotation function of the SLM Section 3. A horizontally polarized input beam can be locally rotated pixel-by-pixel to the desired polarization direction. However, as we pointed out in Eq. (7-5), the spatially variant polarization rotation introduces an additional geometric phase. It is important to pre-compensate this additional phase by the phase pattern for SLM Section 1, as shown in Eq. (7-14). When radially polarized beam is focused by low NA lens, a doughnut distribution will be resulted in the focal plane owing to the polarization singularity at the center. In order to 102 generate radially polarized beam, the phase pattern for SLM Section 3 ϕ3(x, y) will have an azimuthal dependence of 2φ according to Eq. (7-10), where φ is the azimuth angle. Based on Eq. (7-11), we know that the extra phase to be introduced by the following modulations will carry a phase with azimuthal dependence of φ, in other words, a spiral phase with topological charge l = 1. In order to generate the radial polarization with flat phase, a spiral phase with topological charge l = -1 needs to be incorporated in the precompensation phase. Therefore, to verify the phase pre-compensation, we generate radially polarized beams without and with pre-compensation phase. The required phase patterns for radial polarization without and with phase pre-compensation are shown in the upper and lower parts of Fig. 7-14, respectively. Then the far field intensities are captured at the focal plane of a lens, as shown in Fig. 7-15. 103 Fig. 7-14. Phase patterns for radially polarized beams without (upper) and with (with) pre-compensation. For the latter phase pattern, the variation in green color indicates the pre-compensation phase. 104 Fig. 7-15. Focused field by a 75-mm plano-convex lens. (a) Radially polarized beam without proper phase cancellation; (b) radially polarized beam with phase cancellation. In the phase pattern for the radially polarized beam with pre-compensation phase, the introduction of and variation in green color indicate the existence of the precompensation phase and its spiral nature as shown in Fig. 7-14. From Fig. 7-15(a), we can see that without proper phase pre-compensation, a bright spot is obtained when such beam is focused. This can be understood as the additional spiral phase cancelled the polarization singularity at the center of the focused radially polarized beam. Once precompensation phase is introduced a doughnut distribution is achieved as expected (shown in Fig. 7-15(b)). This confirms that the geometrical phase generated due to the operation of SLM Section 3 is successfully compensated. In general, the phase pre-compensation scheme can be used to compensate any additional phases that are introduced in the following modulation steps from SLM Sections 2, 3 and 4, as shown in Eq. (7-14). Moreover, this confirmation of the phase pre-compensation also serves as another evidence of the phase modulation capability discussed in Section 4.1. 105 The generation of radially polarized beam is then shown in Fig. 7-16. The arrows in the upper set of graphs indicate the directions of the linear analyzer in front of the camera and the intensity of each linear polarization component (0°, 45°, 90° or 135°) is shown respectively. The polarization map is given in the lower graph that is calculated based on partial Stokes parameter measurement of S0, S1 and S2. The orientation of the lines indicates the local polarization direction while the length of lines indicates the local intensity. As shown in the figure, radial polarization in the output field is generated. Thus the polarization rotation capability is demonstrated. 106 Fig. 7-16. Radially polarized beam generated by the VOF-Gen. Upper graphs show the fields after a polarizer with polarization axis orientation indicated by black arrows at 0°, 45°, 90° and 135°, respectively; Lower graph shows a polarization map of radially polarized beam overlapped with the intensity distribution and the local polarization directions are indicated by the bars. 107 4.4. Spatially variant phase retardation Right-hand circular polarization (RCP) and left-hand circular polarization (LCP) have phase retardation of +π/2 and -π/2, respectively. To demonstrate the capability of optical field with spatially variant phase retardation, we designed patterns with zero phase, unit amplitude modulation and spatially patterned retardation distribution. In the first example, we designed the beam where the “EO” logo is polarized in RCP while the rest of the window polarized in LCP. The required phase pattern for VOF-Gen and the total field as well as the RCP and LCP components are shown in and Fig. 7-17 and Fig. 7-18, respectively. Fig. 7-17. Phase pattern for "EO" logo generation VOF-Gen. 108 Fig. 7-18. "EO" logo coded in circular polarization. The total field (left), the EO logo (upper right) in RCP and the complimentary “EO” logo (lower right) in LCP. In the second demonstration, we designed the Taiji pattern with one half coded in RCP and the other in LCP. The required phase pattern and the output beam are shown in Fig. 7-19 and Fig. 7-20, respectively. 109 Fig. 7-19. Phase pattern for Taiji pattern generation. Fig. 7-20. Taiji pattern coded in circular polarization. The total field (left), the upper half (upper right) in RCP and the lower half (lower right) in LCP. 110 From the results shown in Fig. 7-18 and Fig. 7-20, it shows that the polarization retardation modulation can also be achieved using our VOF-Gen. At this point, the modulation of each individual degree of freedom in describing an optical field has been successfully demonstrated. In the next two examples, we would like to generate optical fields that require controls in different aspects of light. 4.5. Stokes parameters measurement and complex vectorial optical field generation with multiple parameters 4.5.1. Stokes parameters and its measurement Arbitrary optical field can be represented in Jones vector form as shown in Eq. (7-2), where the polarization can also be expressed using elevation angle and ellipticity, cos SOP at , sin (7-19) where α is the elevation angle and ε is the ellipticity. The conversion between the elevation angle and ellipticity form and the polarization rotation and retardation form can be found in Eq. (7-4). As previously discussed, Stokes parameters are all measurable quantities (intensities), which is an alternative of the SOP representation. Stokes parameters are given as 2 2 S 0 I x I y E0 x E0 y S I I E 2 E 2 x y 0x 0y 1 S 2 I I 2 E0 x E0 y cos 4 4 S I I 2 E E sin R L 0x 0y 3 111 , (7-20) For normalized Stokes parameters, we have S0 1 S cos 2 cos 2 cos 2 1 S 2 cos 2 sin 2 sin 2 cos S3 sin 2 sin 2 sin (7-21) , Both polarized and partially polarized light can be characterized by the Stokes parameters in terms of degree of polarization p, given as: p S12 S 22 S32 S0 (7-22) , For partially polarized light, the Stokes parameters can be shown as: S0 pS 0 1 p S0 S S 0 1 1 S S S P UP S2 S2 0 S S 0 3 3 , (7-23) In order to compensate the absorption from the quarter-wave plate, the quarter-wave plate and polarizer are used in combination to perform the full Stokes Parameters measurement as shown in Fig. 7-21. Here θ is the angle between the polarizer’s transmission axis and the horizontal direction and φ is the angle of the quarter-wave plate’s fast axis and the horizontal direction. 112 Fig. 7-21. Full Stokes parameters measurement setup. The Stokes parameters can be measured in terms of I(θ, φ) as: S 0 I 0,0 I 90,90 S1 I 0,0 I 90,90 S 2 2 I 45, 45 S 0 S3 2 I 45,0 S 0 , (7-24) Then Eq. (7-21) can be used to calculate the local SOP via either α and ε or χ and ϕ at the cross section of the beam provided that the intensities are well aligned as the polarizer and QWP are rotated. 113 4.5.2. Experimental results for complex vector field generation with multiple parameters At this point, the modulation of each individual degree of freedom in describing an optical field has been successfully demonstrated. In the next two examples, we would like to generate optical fields that require controls in different aspects of light. First we propose a ring structure with the local SOP continuously varying from azimuthal to radial direction as the radius increases. The desired ideal field and the required phase pattern are shown in Fig. 7-22 and Fig. 7-23, respectively. The experimental result is shown in Fig. 7-24. The filed distribution after polarizer at 0°, 45°, 90° and 135° and the total field overlapped with SOP map are shown in the upper and lower portions of Fig. 7-24, respectively. It clearly shows the gradual change from azimuthal to radial for local SOP. The weak pattern in the center part of the output beam is due to the interference. Fig. 7-22. The ideal vector field where the SOP varying from azimuthal to radial as radius increases. 114 Fig. 7-23. The phase pattern for VOF-Gen. 115 Fig. 7-24. Ring structure with SOP continuously varying from azimuthal to radial direction as radius increases. The upper set of graphs show the field components along 0°, 45°, 90° and 135° respectively and the lower graph shows the measured field overlapped with polarization map. 116 In the next example, we generate a double ring pattern where the inner ring is azimuthally polarized with 0.5 amplitude while the outer ring is radially polarized with unit amplitude. The ideal field and the required phase pattern for VOF-Gen are shown in Fig. 7-25 and Fig. 7-26. The linear polarization components along 0°, 45° and 90° are shown in the upper set of graphs in Fig. 7-27 and the polarization map is given in the lower part of Fig. 7-27. As we can see in the figure, the outer ring has a higher intensity than the inner one as opposed to Gaussian illumination and the polarization distribution follows the design. Fig. 7-25. The ideal field for double ring pattern where inner ring has azimuthal polarization and outer ring has radial polarization. 117 Fig. 7-26. The phase pattern for VOF-Gen. 118 Fig. 7-27. Double ring structure with amplitude and polarization rotation modulation: (upper) the linear polarization components with polarizer at 0°, 45° and 90°; (lower) the polarization map. As another demonstration, complex vector optical field with local polarization elevation angle along radial direction and constant ellipticity π/10 is designed. In other words, the SOP at each location is elliptical with constant ellipticity and the major axis of the ellipse is always along the radial direction. The ideal field distribution with polarization map, the required phase pattern for VOF-Gen and the experimental result with the histogram of the 119 ellipticity (in unit of π radian) generated experimentally are shown in Fig. 7-28, Fig. 7-29 and Fig. 7-30, respectively. In this case, the full Stokes parameter measurement of S0, S1, S2 and S3 is performed to reveal the spatial distribution of the SOP of the generated beam. It can be shown that the experiment results generally agree with the design. The histogram of the ellipticity peaks around 0.1π, which shows the generation of the designed ellipticity. At some points the local SOP is slightly different from the expected and we think it is due to the fact that the interference patterns with vertical polarization coming from the SLM surface will change the local SOP and the vibration also affects the accuracy of the full Stokes parameters measurement. Fig. 7-28. Ideal field distribution with polarization map. 120 Fig. 7-29. Phase pattern for VOF-Gen. Fig. 7-30. Experimental results (left) for optical field with constant ellipticity and elevation angle along radial direction as well as the histogram (right) of the ellipticity in the unit of π. 121 4.6. Realization of full Poincaré beam and the singularities As a continued research from Chapter 4, an example of the full Poincaré beam is shown in Fig. 7-31. In the cross section of the beam profile, the elevation angle follows the radial direction while the ellipticity varies from π/4 to –π/4 so that the SOP changes from RCP to LCP from the center to the edge of the beam. In the polarization map of Fig. 7-31, the blue color indicates positive ellipticity while the black indicates negative ellipticity. Fig. 7-31. Simulation of FP beam with polarization map superimposed. In the radial direction, from the center to the edge, the polarization evolves from RCP to LCP, which covers from the north pole to the south pole on the Poincaré sphere. The elevation angle α ranges from 0 to 2π, which translates to a coverage of 4π for the 122 azimuth angle 2α in the Poincaré sphere as shown in Fig. 4-3. Therefore, the SOP on the cross section of the beam covers the entire Poincaré sphere two times. Using the VOF-Gen, we are able to generate such FP beam experimentally. The intensity profile as well as the polarization map is shown in Fig. 7-32. Two singularity points were discovered and highlighted by green circles in the figure. Fig. 7-32. Experimental result for FP beam with polarization map superimposed. Two singularities are highlighted by green circles. The singularities can be understood by investigating the phase pattern used for the generation of such beam. It can be shown that the phase retardation shown in Fig. 7-33 has four vortex-like singularity points at the mid-points on both the horizontal and the 123 vertical direction, where the SOPs are horizontal and vertical polarizations. However, due to the fact that the SLM only responds to the horizontal polarization, the retardation singularities on the vertical direction are not reflected in the generated beam. Therefore, only the retardation singularities on the horizontal direction affect the beam as shown experimentally. The phase pattern used for the VOF-Gen generation is shown in Fig. 7-34. Numerical simulation of such beam also confirms the beam singularities. The diffraction pattern is shown in Fig. 7-35 after a propagation distance of 1 mm. It has been found that the two is the least number of singularities for different approaches of generating such FP beam using VOF-Gen, which coincides with how many times the SOP on the cross section of the beam covers the entire Poincaré sphere. Fig. 7-33. Phase pattern for retardation modulation for the FP beam. 124 Fig. 7-34. The phase pattern for the generation of the FP beam. Fig. 7-35. Diffraction pattern after propagation distance of 1 mm. 125 5. Summary We reported a novel and versatile vectorial optical field generator (VOF-Gen) that is capable of generating arbitrary optical fields by spatially modulating all aspects of optical field (including phase, amplitude and polarization) on a pixel-by-pixel basis. Various complex vector fields are generated and tested to demonstrate the functionality and flexibility of the proposed VOF-Gen. To the best of our knowledge, it is the first successful experimental demonstration of a beam generation system with high spatial resolution that is capable of tailoring all the aspects of optical fields. This arbitrary complex optical field generator may find extensive applications in areas where exotic input fields are required, such as particle manipulation and beam shaping. 126 CHAPTER 8 CONCLUSIONS AND FUTURE WORK VOF-Gen is discussed in details and successfully demonstrated as a promising arbitrary vectorial complex optical field generator. Exciting results have been obtained and discussed which show the capability of arbitrary phase, amplitude and polarization modulation on a pixel by pixel basis. If a single piece device can be made to replace the optical components of the VOF-Gen, the alignment can be greatly simplified, which may lead to potential commercialization. In addition Labview or other automation technique can be introduced to realize the automation of the vectorial optical field generation. The motivations for such a full control beam generation system are also introduced with examples focused on the modulations of different aspects of light. As the future work, the experimental verification of optical needle field needs to be achieved with the antenna based complex optical filter design. The experimental setup to generate optical needle field is proposed here shown in Fig. 8-1. In order to generate desired radially polarized field as the desired pupil plane field for needle field generation, azimuthal input polarization is required for the complex filter (shown in green) due to the 127 fact that the amplitude and phase of the cross-polarized component are modulated. Recall that the circular polarization can be decomposed into uniform distribution of radial and azimuthal polarization with a spiral phase. Therefore, in order to generate azimuthal polarization, a circular polarizer (CP), a spiral phase plate and an azimuthal analyzer are used in the setup. After the complex filter, a radial analyzer is used, only allowing the cross-polarized component to go through. Then the beam is expanded to match the NA of the objective and focused by the high NA objective. A near-field scanning optical microscope is proposed to perform the detection of the generated optical needle field. Fig. 8-1. Experiment setup for linear antenna design. An alternative to generate azimuthally polarized beam is to use fiber to perform automatic mode selection. Careful alignment is required to ensure the generation of azimuthal (radial) polarization. 128 BIBLIOGRAPHY 1. Q. Zhan, "Cylindrical vector beams: from mathematical concepts to applications," Advances in Optics and Photonics, vol. 1, no. 1, pp. 1-57, 2009. 2. Yanai and U. Levy, "Plasmonic focusing with a coaxial structure illuminated by radially polarized light," Optics Express, vol. 17, no. 2, pp. 924-932, 2009. 3. J. Bar-David, G. M. Lerman, L. Stern, N. Mazurski and U. Levy, "Generation of a periodic array of radially polarized Plasmonic focal spots," Opt. Express, vol. 21, no. 3, pp. 3746-3755, 2013. 4. K. Youngworth and T. Brown, "Focusing of high numerical aperture cylindricalvector beams," Optics Express, vol. 7, no. 2, pp. 77-87, 2000. 5. R. Dorn, S. Quabis and G. Leuchs, "Sharper Focus for a Radially Polarized Light Beam," Phys. Rev. Lett., vol. 91, no. 23, p. 233901, 2003. 6. D. Biss and T. Brown, "Cylindrical vector beam focusing through a dielectric interface," Optics Express,, vol. 9, no. 10, pp. 490-497, 2001. 7. D. P. Biss, K. S. Youngworth and T. G. Brown, "Dark-field imaging with cylindrical-vector beams," Applied Optics, vol. 45, no. 3, pp. 470-479, 2006. 8. Q. Zhan, "Trapping metallic Rayleigh particles with radial polarization," Opt. Express, vol. 12, no. 15, pp. 3377-3382, 2004. 129 9. H. Kawauchi, K. Yonezawa, Y. Kozawa and S. Sato, "Calculation of optical trapping forces on a dielectric sphere in the ray optics regime produced by a radially polarized laser beam," Opt. Lett., vol. 32, no. 13, pp. 1839-1841, 2007. 10. L. Huang, H. Guo, J. Li, L. Ling, B. Feng and Z.-Y. Li, "Optical trapping of gold nanoparticles by cylindrical vector beam," Opt. Lett., vol. 37, no. 10, pp. 16941696, 2012. 11. Y. Kozawa and S. Sato, "Optical trapping of micrometer-sized dielectric particles by cylindrical vector beams," Opt. Express, vol. 18, no. 10, pp. 10828-10833, 2010. 12. W. Chen and Q. Zhan, "Realization of an evanescent Bessel beam via surface plasmon interference excited by a radially polarized beam," Opt. Lett., vol. 34, no. 6, pp. 722-724, 2009. 13. N. Bokor and N. Davidson, "Generation of a hollow dark spherical spot by 4pi focusing of a radially polarized Laguerre-Gaussian beam," Opt. Lett., vol. 31, no. 2, pp. 149-151, 2006. 14. W. Chen and Q. Zhan, "Creating a spherical focal spot with spatially modulated radial polarization in 4Pi microscopy," Opt. Lett., vol. 34, no. 16, pp. 2444-2446, 2009. 15. Q. Zhan and J. Leger, "Focus shaping using cylindrical vector beams," Opt. Express, vol. 10, no. 7, p. 324, 2002. 130 16. W. Chen and Q. Zhan, "Three-dimensional focus shaping with cylindrical vector beams," Optics Communications, vol. 265, no. 2, pp. 411-417, 2006. 17. Y. Zhao, Q. Zhan, Y. Zhang and Y.-P. Li, "Creation of a three-dimensional optical chain for controllable particle delivery," Opt. Lett., vol. 30, no. 8, pp. 848850, 2005. 18. X.-L. Wang, J. Ding, J.-Q. Qin, J. Chen, Y.-X. Fan and H.-T. Wang, "Configurable three-dimensional optical cage generated from cylindrical vector beams," Opt. Comm., vol. 282, no. 17, p. 3421–3425, 2009. 19. J. A. Davis, I. Moreno and P. Tsai, "Polarization Eigenstates for Twisted-Nematic Liquid-Crystal Displays," Applied Optics, vol. 37, no. 5, pp. 937-945, 1998. 20. G. R. Bird and J. Maxfield Parrish, "The wire grid as a near-infrared polarizer," J. Opt. Soc. Am., vol. 50, no. 9, p. 886, 1960. 21. F. Wang, M. Xiao, K. Sun and Q.-H. Wei, "Generation of radially and azimuthally polarized light by optical transmission through concentric circular nanoslits in Ag films," Opt. Express, vol. 18, no. 1, p. 63, 2010. 22. M. G. Moharam and T. K. Gaylord, "Rigorous coupled-wave analysis of metallic surface-relief gratings," JOSA A, vol. 3, no. 11, pp. 1780-1787, 1986. 23. M. G. Moharam, E. B. Grann, D. A. Pommet and T. K. Gaylord, "Formulation for stable and efficient implementation of the rigorous coupled-wave analysis of binary gratings," JOSA A, vol. 12, no. 5, pp. 1068-1076, 1995. 24. M. G. Moharam, D. A. Pommet, E. B. Grann and T. K. Gaylord, "Stable implementation of the rigorous coupled-wave analysis for surface-relief gratings: 131 enhanced transmittance matrix approach," JOSA A, vol. 12, no. 5, pp. 1077-1086, 1995. 25. P. Lalanne and G. M. Morris, "Highly improved convergence of the coupledwave method for TM polarization," JOSA A, vol. 13, no. 4, pp. 779-784, 1996. 26. X. Ni, N. K. Emani, A. V. Kildishev, A. Boltasseva and V. M. Shalaev, "Broadband Light Bending with Plasmonic Nanoantennas," Science, vol. 335, no. 6067, p. 427, 2011. 27. N. Yu, P. Genevet, M. A. Kats, F. Aieta, J.-P. Tetienne, F. Capasso and Z. Gaburro, "Light Propagation with Phase Discontinuities: Generalized Laws of Reflection and Refraction," Science, vol. 334, no. 6054, p. 333, 2011. 28. X.-L. Wang, J. Ding, W.-J. Ni, C.-S. Guo and H.-T. Wang, "Generation of arbitrary vector beams with a spatial light modulator and a common path interferometric arrangement," Optics Letters, vol. 32, no. 24, pp. 3549-3551, 2007. 29. F. Kenny, D. Lara, O. G. Rodríguez-Herrera and C. Dainty, "Complete polarization and phase control for focus-shaping in high-NA microscopy," Optics Express, vol. 20, no. 13, pp. 14015-14029, 2012. 30. S. Tripathi and K. C. Toussaint, "Versatile generation of optical vector fields and vector beams using a non-interferometric approach," Optics Express, vol. 20, no. 10, pp. 10788-10795, 2012. 31. Moreno, J. A. Davis, T. M. Hernandez, D. M. Cottrell and D. Sand, "Complete polarization control of light from a liquid crystal spatial light modulator," Optics Express, vol. 20, no. 1, pp. 364-376, 2012. 132 32. D. Maluenda, I. Juvells, R. Martínez-Herrero and A. Carnicer, "Reconfigurable beams with arbitrary polarization and shape distributions at a given plane," Optics Express, vol. 21, no. 5, pp. 5432-5439, 2013. 33. B. Richards and E. Wolf, "Electromagnetic Diffraction in Optical Systems. II. Structure of the Image Field in an Aplanatic System," Proc. R. Soc. Lond. A, vol. 253, no. 1274, p. 358, 1959. 34. J. Wang, W. Chen and Q. Zhan, "Engineering of high purity ultra-long optical needle field through reversing the electric dipole array radiation," Optics Express, vol. 18, no. 21, pp. 21965-21972, 2010. 35. L. Novotny, M. R. Beversluis, K. S. Youngworth and T. G. Brown, "Longitudinal Field Modes Probed by Single Molecules," Phys. Rev. Lett., vol. 86, no. 23, pp. 5251-5254, 2001. 36. M. E. Friese, T. A. Nieminen, N. R. Heckenberg and H. Rubinsztein-Dunlop, "Optical alignment and spinning of laser-trapped microscopic particles," Nature, vol. 394, no. 6691, pp. 348-350, 1998. 37. S. Zhang, W. Fan, N. C. Panoiu, K. J. Malloy, R. M. Osgood and S. R. J. Brueck, "Experimental Demonstration of Near-Infrared Negative-Index Metamaterials," Phys. Rev. Lett., vol. 95, no. 13, pp. 137404-137408, 2005. 38. J. Wang, J.-Y. Yang, I. Fazal, N. Ahmed, Y. Yan, B. Shamee, A. Willner, K. Birnbaum, J. Choi, B. Erkmen, S. Dolinar and M. Tur, "Demonstration of 12.8bit/s/Hz spectral efficiency using 16-QAM signals over multiple orbital-angularmomentum modes," in Optical Communication (ECOC), 2011 37th European Conference and Exhibition on , 2011. 133 39. J. Ng, Z. Lin and C. T. Chan, "Theory of Optical Trapping by an Optical Vortex Beam," Phys. Rev. Lett, vol. 104, no. 10, p. 103601, 2010. 40. M. Beckley, T. G. Brown and M. A. Alonso, "Full Poincaré beams II: partial polarization," Opt. Express, vol. 20, no. 9, p. 9357, 2012. 41. M. Beckley, T. G. Brown and M. A. Alonso, "Full Poincare beams," Opt. Express, vol. 18, no. 10, p. 10777, 2010. 42. W. Han, W. Cheng and Q. Zhan, "Flattop focusing with full Poincaré beams under low numerical aperture illumination," Optics Letters, vol. 36, no. 9, pp. 1605-1607, 2011. 43. J. Dai and Q. Zhan, "Beam shaping with vectorial vortex beams under low numerical aperture illumination condition," in Proceedings of the SPIE, 2008. 44. W. Cheng, W. Han and Q. Zhan, "Generation of flattop focusing with second order full Poincaré beams," in SPIE Proceedings Vol. 8130, 2011. 45. W. Cheng, W. Han and Q. Zhan, "Compact Flattop Laser Beam Shaper Using Vectorial Vortex," Applied Optics, 2013. 46. Q. Zhan, "Properties of circularly polarized vortex beams," Opt. Lett., vol. 31, no. 7, p. 867, 2006. 47. Q. Zhan, "Cylindrical vector beams: from mathematical concepts to applications," Advances in Optics and Photonics, vol. 1, no. 1, p. 1, 2009. 48. R. W. P. King, The theory of linear antennas, Harvard University Press, 1956. 49. Z. Zhao, J. Wang, S. Li and A. E. Willner, "Metamaterials-based broadband generation of orbital angular momentum carrying vector beams," Optics Letters, vol. 38, no. 6, p. 932, 2013. 134 50. Z. Ruan and M. Qiu, "Enhanced Transmission through Periodic Arrays of Subwavelength Holes: The Role of Localized Waveguide Resonances," Phys. Rev. Lett., vol. 96, no. 23, pp. 3901, 2006. 51. K. Dholakia and T. Čižmár, "Shaping the future of manipulation," Nature Photonics, vol. 5, p. 335–342, 2011. 52. S. W. Hell, "Far-field optical nanoscopy," Science, vol. 316, no. 5828, pp. 1153, 2007. 53. W. Cheng, J. W. Haus and Q. Zhan, "Propagation of vector vortex beams through a turbulent atmosphere," Optics Express, vol. 17, no. 20, pp. 17829-17836, 2009. 54. G. Gibson, J. Courtial, M. Padgett, M. Vasnetsov, V. Pas'ko, S. Barnett and S. Franke-Arnold, "Free-space information transfer using light beams carrying orbital angular momentum," Optics Express, vol. 12, no. 22, pp. 5448-5456, 2004. 55. K. J. Moh, X.-C. Yuan, J. Bu, S. W. Zhu and B. Z. Gao, "Surface plasmon resonance imaging of cell-substrate contacts with radially polarized beams," Opt. Express, vol. 16, no. 25, p. 20734, 2008. 56. Q. Zhan and J. R. Leger, "Microellipsometer with Radial Symmetry," Appl. Opt., vol. 41, no. 22, pp. 4430, 2002. 57. C. Ye, "Construction of an optical rotator using quarter-wave plates and an optical retarder," Optical Engineering, vol. 34, no. 10, pp. 3031, 1995. 58. B. E. Saleh and M. C. Teich, Fundamentals of Photonics, Wiley-Interscience, 2007. 135 59. Y. Kozawa and S. Sato, "Optical trapping of micrometer-sized dielectric particles by cylindrical vector beams," Optics Express, vol. 18, no. 10, pp. 10828-10833, 2010. 60. J. F. Bisson, J. Li, K. Ueda and Y. Senatsky, "Radially polarized ring and arc beams of a neodymium laser with an intra-cavity axicon," Optics Express, vol. 14, no. 8, pp. 3304-3311, 2006. 61. M. A. Ahmed, A. Voss, M. M. Vogel and T. Graf, "Multilayer polarizing grating mirror used for the generation of radial polarization in Yb:YAG thin-disk lasers," Optics Letters, vol. 32, no. 22, pp. 3272-3274, 2007. 62. V. G. Niziev, R. S. Chang and A. V. Nesterov, "Generation of inhomogeneously polarized laser beams by use of a Sagnac interferometer," Applied Optics, vol. 45, no. 33, pp. 8393-8399, 2006. 136 VITA Wei Han was born on April 3rd, 1984 in Hefei, Anhui Province, People’s Republic of China, the son of Jie Han and Zhongping Wang. After completing his high school at Hefei No. 1 High School, he entered Nanjing University for undergraduate study majored in Electrical Engineering in 2002. He graduated in 2007 with a bachelor’s degree and came to the Electro-Optics program at the University of Dayton for graduate study. He received his master’s degree in 2009 under the supervision of Dr. Joseph W. Haus. He received his Ph.D. degree in August 2013 under the supervision of Dr. Qiwen Zhan. His research is focused on the engineering of complex optical fields and its applications. 137