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Atomic quantum phase studies with a longitudinal Stern-Gerlach interferometer J. Robert, Ch. Miniatura, O. Gorceix, S. Le Boiteux, V. Lorent, J. Reinhardt, J. Baudon To cite this version: J. Robert, Ch. Miniatura, O. Gorceix, S. Le Boiteux, V. Lorent, et al.. Atomic quantum phase studies with a longitudinal Stern-Gerlach interferometer. Journal de Physique II, EDP Sciences, 1992, 2 (4), pp.601-614. <10.1051/jp2:1992155>. <jpa-00247659> HAL Id: jpa-00247659 https://hal.archives-ouvertes.fr/jpa-00247659 Submitted on 1 Jan 1992 HAL is a multi-disciplinary open access archive for the deposit and dissemination of scientific research documents, whether they are published or not. The documents may come from teaching and research institutions in France or abroad, or from public or private research centers. L’archive ouverte pluridisciplinaire HAL, est destinée au dépôt et à la diffusion de documents scientifiques de niveau recherche, publiés ou non, émanant des établissements d’enseignement et de recherche français ou étrangers, des laboratoires publics ou privés. J. Phys. II France (1992) 2 601-614 1992, APRIL 601 PAGE Classification Physics Abstracts 03.65W 07.60L 32.60V phase quantum Atomic with studies longitudinal a Stern-Gerlach interferometer Robert, J. and Laboratoire J-B- Av. de Physique des Lasers(*), Institut C16ment, 93430 Villetaneuse, France (Received 31 R4sumd January1992, On donne diffusion. de rateur sentd O. Gorceix, S. Le Miniatura, Ch. Boiteux, V. Lorent, J. par 5 montre l'action que polar1s6 d'onde se ramkne atomiques longitudinal sur interf4romktres des interf6rom+tre d'un £ A Abstract given. The polarized general description ofatomic interferometers of a longitudinal interferometer on action wavepacket is shown atome un On examine champ pr4cessant m6tastables d'hydrog+ne est pr6c6dentes sont discut6s. On des champs de quelques 10 G, et celui d'un scattering by an leading to a of the terms described atom operator incident "beaded" transformation, magnetic field and that of a spatially examined. precessing field are metastable hydrogen atoms is presented and the results obtained in both situations mentioned above are discussed. Properties of beaded produced by relatively strong fields (od 10 G) are investigated by means of the intensity atoms diagram of their electrically induced radiative decay. The atom. special of case to pure a be equivalent in an d'opdreprd- termes en r4fdrentiel. de transformation une cas is Paris-Nord, Universitd February 1992) description g6n6rale une On paquet un accepted Gali16e, particulier d'un champ magn4tique I gradient longitudinal spatialement. Une r4alisation exp4dmentale utilisant des atomes prdsent6e et les r6sultats ensuite obtenus dans les deux situations chalelet" dtudie enfin les firopr16t6s des "en produits par atomes £ partir du induit champ 61ectrique. rayonnement par un le Reinhardt Baudon J. to a frame longitudinal gradient An experiment «sing of Introduction. 1 In the states representation, arises generally definite (*) the system assoc16 based problem of problem of bra the au of kets CNRS, is the upon the phase and used URA 282. as superposition principle, of associated conjugation. representation to ket a of quantum any given state (cf. a This question is of states insofar as it Dirac system by [ii) and importance leads a more when priori to a a JOURNAL 602 phase-dependent representation of cancels perform measurements choice of phases is adopted. observables. the N°4 II by chance, the usual However difficulties, these all to PHYSIQUE DE least at if a way and permanent we use coherent necessity of a renewal of phase studies (for a that, with systems containing several degrees of answer see relative phases. The idea freedom, it is possible in a real or "gedanken" experiment to exhibit (by filter) whereas the degrees of freedom of is to lock with respect to each other some some of interferometric the evolution observes, by of the other degrees measurement, means an one that has been made on the of freedom, in an elTective sub-space depending on the preparation locked degrees of freedom. It may be noticed that this type of methods is commonly used in scattering experiments on atoms or molecules, as well as in light-matter interaction studies. atomic interferometry experiments is not the evidence for What is really new in the recent the de Broglie wavelength but rather the variety of methods to "freeze" or "lock" degrees some made feasible by the use of atomic control techniques. AH these experiments of freedom beam that each particle (atom) interferes with itself. So far of the one-particle type in the sense are coherent elTect has been observed or even, to our knowledge, proposed. collective no Atomic systems are particularly very well fitted for fine studies of quantum phases »ince external degrees of freedom can be manipulated rather easily by means of external inner and of a rich internal in atoms is an advantage, compared to photons fields. The structure occurence be exploited which the external degrees of freedom via the internal to act on neutrons, can or provides and This flexibility the methods control vice in specify to great a versa. ones, or interferometer. phaseshifts and consequently to build an interferometers is presented and In part 2 of this article, a general description of atomic discussed. the problem of dynamical and topological phases h In part 3, the principle of the Stern-Gerlach interferometer longitudinal is given and the theoretical methods used to study presented. is devoted Part 4 the description of the its operation experiJnent and to to are either with a the results obtained magnetic field with a longitudinal gradient (pure transverse dynamical phases) or with a conical field configuration (dynamical and topological phases). In part 5, experiments using a strong field are presented. They are devoted to the study of special optical properties exhibited by the atoms emerging from the interferometer l'~beaded" atoms). this In context, 2. may one about wonder the [2]). One possible general review Description ofatomic is interferometers. Any atonfic interferometer consists of an arrangement slits, grating, etc...) which perturbs the atomic within a finite domain of space. evolution From this view point, it is quite s1nlilar (except device. Just like a collision, the operation of the interferometer for the size) to a scattering is contained in a "scattering operator" § which transforms asymptotic (free) incident state any (~l~~) into an asymptotic outgoing state (~1°~~) GENERAL 2.I of external CONSIDERATIONS. fields (among which includes one § j~inj l~outj Let us variable define £ now '~principal path the (discrete or continuous), being / = A Stieltjes in discrete integral and with continuous a measure cases. ofthe states" as interferometer, [p(£)), labelled by eigenstates of this operator: has been quantities used s(£) are in a vectorial (2) dP(f)lw(f))e'~~~~(~2(t)1 p(£) The the (~) order real to phases get a insofar similar as all expression scattering QUANTUM ATOMIC N°4 channels is case the atomic actually is ultra-cold of of the that tion This open. are (the beams is in describe to further then ossible m the of = set Is with #~, flint [k, by states iven basis and dk / SELECTED ~ genvalues = e(x), dE such E,x)lk, P(x)a"(k, tt°(r,t, d restrict We further bution of which is choice our peaked at value some With a°(k, E,x) jr, kP = + u, [u[ « -kfl = m asymptotic the jr, = = kP, i,y j~t outgoing) states analysed) wave-packet, or (4) ° these ~l E a°(k,x)b exp[I(k ~ distri- momentum corresponds that such by projection obtained is wavepackets, the the (y[ selection asumptions and reminding that and to a asymptotic these (x)j ~ Et/h)] r ~~~~ EP~ = = (particle) velocity, group + 2m and wavepacket now labelled with kfl and slowly variable envelop: a (x~) ~ h2 (kfl)2 Ef x~ = can be ~ m written In such in the conditions, form of a the carrier multiplying 1~" the (kfl, x~; r, t) ; kfl = exp r envelop is given by: £" The spectively. (kfl h vfl = k, E) t E where e(x) or quasi-monochromatic to given eigenstate of flint, say (x~[ wavepackets are free, one gets: wave + ~~ (3) described, for each atom in the beam, by a selected implies a choice of a phase reference insofar as the wavepacket of [~l") onto the bra jr, t, y[, where y labels the internal state: are Let ~ asymptotic (incomin g If WAVE-PACKETS. ASYMPTOTIC # Ei this k are #, E, ~~, (prepared with which '~mixers" the after m lt~°) 2 choije the interferometer, I.e. to of the principal path states [~g(£)). In combinations linear include not and before = il, of eigenstates 2 a the does It the atomic interferometer state, one can expand on in, out) on a basis set realizing a complete description of the interferometer being of the short-range The interaction, in the asymptotic states [~1°) (a #~. Hamiltonian asymptotic tonian, atomic experiments using thermal carefully). descripthis Actually more separatrices and the arms), in which of the elTect the the internal ariable (say beam atomic 603 of the most adiabatic. cases charge to prepare or analyse the specify (~li~, °~~) which are definite STUDIES examined be interferometer most in order in case should of the "core" evolution the atoms PHASE special (r case vflt; x~) of a plane = exp wave [-ie (x~) t/h] is readily / obtained (~ t)j du a° £° (u, x~) by setting (r exp in a° vflt; x~) (I u (5) (r (u,x~) vflt)) = a° (x~) b(u). (6) JOURNAL 604 SPATIAL 2. 3 AND TEMPORAL SHIFTS PHYSIQUE DE II DEGENERATE IN A N°4 LONGITUDINAL INTERFEROMETER. degenerate longitudinal interferometer h a device such that (I) the asymptotic channels internal variables, an degenerated with the I.e. there exists single value respect to e of are a e(x) (we shall take e 0 in the following) (it) any incoming beam of atoms at a given direction results propagating in the same direction, regardless to the external into an outgoing beam A = (all trajectories motion such In concept is relevant) within the of the § operator reduces if this matrix the case, a form (k, E',x'(S(k, E, # and principal path the states stands y for internal the E') simply: are z) 1~2(t)ilk, E, where k') b (E (k, E, x'(S[k, E, x) b (k = interferometer. of the arms to phaseshifts corresponding The state. (7) by equation (2) defined are: S(t) An incoming The prepared (polarized) along (x') state (l#°~~) dk # outgoing dp (X') dp(y) (X' (r,t,x°) / dk = (r,t,x° = of powers u s(k, y) (Vk s)~, outgoing one: where s' one = ~1°~~ / makes fl explicitely appear k, x') a~" (k, x') e'~~ ((°) refers and to X' (8) ~'~~ ~~~ ~ + u (9) s'(k", £ incident the wavepacket within the expression (r,t, x°) = dv(y) (x° y) (y x") tt~" [r + Ar (k', fl t + At (k', fl , spatial -j 2m , = The J~2 ~2 fit°~~) s° (k", ci state: k' in the vicinity of k" k = outgoing the to then: is dp(y) (x° y) e'~(~,Y) (y By expanding s(k, y) in leads y) e'~~~'~~ (y X') a~'~ (k, X') packet polarized along (x°) wave lV°~~ of the S(k,z) = temporal shifts fl Ar (k~, At (k",fl the s° are s° h ~ (k') ~ ~~ = (k') ~ dependent part (lo) given by: ~ =2 x"] , (s° of Ar s' 2 k" and ~' (k') ~ s') At) (k' s') At° = = + At' Ar° + Ar' (11) QUANTUM ATOMIC N°4 noting packet. worth It is envelop of the In the that (spatial) one Ar°/At° as dimension case, V", the phase velocity, which packet. conclude To this phaseshift the part, well as carrier as In wave. averaging the a Ar that these on of k'. one The interference then does result not h source (cf used similar is the carrier = of the wave and adiabatic dealing with atoms adiabatic topological phaseshifts The the Az'/At' has: one the alTect not dynamical parts of The topological case. aiect the envelop but only the of dilTerent velocities, I.e. with the is pattern. light monochromatic k" and involve not in topological the about k~6z, = absent are At° do and hi and k" shifts wavepacket, in the 605 Ar° shifts Az = remark a elTects experiment real of the extended an does distribution incoherent an Ar°, as make us their v', = where indicates let part, regards hk'/m = STUDIES PHASE to Young's will that holes involved be not optics experiment used observed in in when as a spatial correlator), longitudinal The 3. PRINCIPLE 3. I AND profile B(z) opposite directions restricted field on the section t6 a which means The 2.3. finite in the in and zero, the to energy The izer, is atom in device This DESCRIPTION. described type of the eter polarization Stern-Gerlach core The range. interferometer. is longitudinal-degenerated a of this interferometer gradient of its modulus integral out-sides that the that net transfer in such a way there is finally no is of interferom- magnetic longitudinal, with consists of of the a force exerted neither momentum of atom. core of the which selects interferometer a specific preceeded by is Zeeman preparation by a (x"), state followed section a mixer consisting of builds which a polar- a linear superposition of such states. Experimental details will be given further. The principle of this (with the direction of field rapidly mixer is basically to turn respect to the Larmor a magnetic frequency). Similarly the core is followed by a second mixer and an analyzer selecting (x°). Actually, (x'>°) are eigenstates of the component of the atomic spin J along a fixed axis u". fl~ reduces to the kinetic energy operator. The principal Hamiltonian Here the asymptotic determined following the lines path states [~g(y)), belonging to the [k E J) manifold, can be developed by Majorana [3]. Within both mixers and core domains, the Hamiltonian also can be written in the form: fi ~ fl(r) where B(r) 3.2 is g = the Land6 B(r)fiB(r), THE with SCHWINGER'S factor and pB LimjrjcoB = TREATMENT. gvBJ = the 0, so Bohr that In B(r) The magneton. fl his reduces paper to fl~ field in the "Non-adiabatic has limit general [r[oo. the processes in form: non- homogeneous fields" [4], Schwinger has developed all the theoretical background needed in time-dependent description of the spin evolution in the spin-state subspace. However to a properly the interferometer describe simply transpose this time-dependent theory cannot we the external motion is given by the classical expression z One has in assuming that vi. solve the complete atomic motion, by adding the kinetic the internal operator to to energy The field configuration will be assumed Hamiltonian. In a first part the field to be as follows: has a longitudinal gradient but a fixed direction, its magnitude rhing from zero up to some value B. In a second part of length L it keeps direction in magnitude but its constant preBfiB(z), with a (spatial) angular velocity Q 2~/L and uniformly around z : B(z) cesses making a constant angle with z-axis. In a third part, the field goes down to zero keeping = = = JOURNAL 606 direction. constant a referred the to concentrate be and attention our z-dependent a fl is fltM with: £ (6) As the be restritted £ fit of the coupled FM(z)fltM (6(z)). = M We shall adiabatic. Let fi(z) fl + sin a(z)iiy sin eigenstates fltM The + phi cos u(z) of J parametrized are (hi Mi ~0)FM = FM (z) describing the Functions by 6, external definite of energy will problem The the IVM over motion (6) solutions are equations: dilTerential FM(z) E Qz. states difficulty. is time-independent it is allowed to look for a state being independent of z, y, these variables are separated. only z coordinate. The complete state be expanded can the to basis: a(z)6~ = any not spin the among occurs Hamiltonian total interaction The transition no form: l8~, ~,(0, -fl, -a(z))lV = Mi E. of the cos a(z) and constant a fl sin N°4 without parts can be treated central part in which the evolution is vector = parts II these the unitary third and then to 6 where first the In ads B PHYSIQUE DE £ (-gpB) + ~2 (M (0z( M') (M(J B(M') m 0zFM/- m -~ (M (0)( M') MJj ~, (12) m where matrix all algebra [5] allows (M Using JWKB the 0z FM is of the value totic energy. terms K M') (0z in -iQ = (M 2~/A the because hand (M (0)( if') are order the the compare local of dilTerent very As L » to those in of Jz momentum J) and : (M (J) M') -Q~ = are I/L. negligible with respect those of terms equation (12): close to the asymp- small compared to the kinetic A, wavenumber energies Zeeman Q is of to K is the angular standard The 0) by and (M (0)( M') M') where basis. of 0z elements is able one K(z)FM, of (3~ (6) the fltM in matrix approximation order = taken are replace to one another On the elements (M very Q~ one has QK, then (0z M'). Obviously these « interaction compared to E but not compared to the "static" terms (M [-gpBJ B[ M') and they must be kept in the form of the ampliThe eikonal treatment. and SM a rapidly tudes is FM = AM(z)exp [iSM(z)], where AM is a slowly varying function S + aM with aM < S. The approximate JWKB form of varying real phase such that SM the coupled equations is now: latter terms are small = E AM (z) = £ (M gpBJ. B )S'~AM ~~' ~, The due parts oIT-diagonal coupling to the cancel z terms contain dependence of the basis eachother by a convenient ~~ B + gfiBm hQ6z = a set. static In choice Be6(z) the of = Q6zj + gPBm M') part (in J B) and a dynamical part (in present case it is possible to make these 6(z) : if 6 is such that: Be(elTective magnetic field) QS') two QUANTUM ATOMIC N°4 the then equations decouple ~2 solution takes 607 in: the (M (gpBJ Be M') -S'~ E Finally the STUDIES PHASE = form: +CO FM Reafisation of 4. I GENERAL DESCRIPTION already sented here. continuous, (TOF). The OF dz EXPERIMENT details elsewhere but a it TOF thermal molecular beam. In results. (see Fig. I). [6] and only its general principle developed in parts Hydrogen atom H* (2si/2) beam. metastable of wM(z) experimental THE in ~co The of a bombardment case the described been ikz + interferometer, 4. has Amexp = most 2.3 and 3.I beam This of the The main is experiments H~m~ '~ ~~ ~j)fj~j~i~~j~flj)~ ~ @~~~ C P C'B~ [--,--) setup be pre- been bombardment this easily pulsed in view of an analysis or selection can dhtribution is well fitted by the following function: Bp will applied to the produced by electronic has be KA experimental features of the time of h flight la) D j --_z P (b) (a) Scheme of the apparatus. K, A: electron gun, Bp,A Poladzing and analysing fields, quasi-zero field chambers, p: magnetic shieldings, iC (b) axisparallel intensities, D detector. Principle of the experiment. P,A: polarizer, analyzer; M, M' : mixers; R: region where the longitudinal (a J magnetic field gradient induces phaseshifts among Zeeman 1 value being assumed). states Fig. 1. CC' = f(z) where vo =10 z t/to,to being km/s. = The preparation lowing steps: of the the most beam at = C~~z~~exp probable the entrance time (-z~) of of the flight, corresponding interferometer consists to the of the velocity two fol- JOURNAL 608 PHYSIQUE DE N°4 II Lamb-Retherford method [7], (I) a partial polarization of the beam h achieved by use of the by passage through a transverse field Bp parallel to z-axis, of about 600 G in magnitude: only the two hyperfine Zeeman states F I, MF +1, 0 remain within the beam, with equal between them. populations and no coherence (ii) Starting from one or the other of these filtered levels, a linear superposition of hyperfine sublevels F I, MF +1, 0, -1, referred to the y-axis is built in a "mixer" (AI in Fig. I). reduce the fringe field of the polarizer (parallel to z-axis) to Its principle is simply to first distance y-direction, of 5 mm. The the field to the few tens of mG and then turn over a I-e- = = # = evolution non-adiabatic spin makes of the the desired result without appreciable any elTect on According to a general treatment given by Schwinger [4] applied to a spin show J I (which is fully justified owing to the low magnitude of the magnetic field), one can that the operation of the mixer is representable by a Wigner matrix Dl') in which the Euler characteristics of the field in the mixer. angles depend on the The mixer is followed by a region 7l where a magnetic field B(Z), with a longitudinal gradient dilTerent interferometer of B, induces phaseshifts on the dilTerent eigenstates ("arms") of the external motion of the atom. and acts at the time on the Two dilTerent field configurations same field parallel to y-axis, (it) a conical magnetic field. These have been used: (I) a transverse the external motion. = two ending consists of discussed be will cases The side (M') parallel or anti-parallel emerging metastable either further. detail more (analysis) apparatus mixer second a in of the followed by a symmetric to entrance polarisation analyzer, the is (preparation). side field BA of which It is Bp. to finally counted in a detector specific of H*(2s) atoms. atoms are other species (detectable by a standard requirement since electron many an multiplier) are produced by the electronic bombardment of H2 (metastable molecules, ions). detector a static electric field of 40 V/cm induces the 2s-2p transition. The Lyman a In this photons resulting from the decay of the 2p level are detected by a channel electron multiplier through a MgF~, window. The This important is 4.2 TRANSVERSE described conical in to to states part 2.3, this is of wave the are shown and t. In the AZM recalled a definite here GRADIENT. in order to This experiment, already emfihasize the contrast with the following paragraph. Two wires The interference figure 2a. case 3s[ /K pattern It is well of the of VB eTect a magnetic field Bc(z) -4l on the -1 interferometer. of the create in region lZ is y-axis. In this particular mono-kinetic, each of If the beam was resp.). According to the theory given in +1, 0, = given phaseshift (+4l, 0, evolution the referred to motion: external an incident atomic diTerentially shifted outgoing plane waves. momentum almost monokinetic incident wavepacket is used, the 3 outgoing an incident providing convenient changes in thi origins of z to the one gives K present " "arms" a MF states manifestation before, when wavepackets are identical As LONGITUDINAL A Zeeman accumulate would plane for adiabatic these case them WITH [6], is briefly configuration which will be considered in the (+ ic) z-axis and transporting opposite intensities the y-axis- As the direction of field is not varied, field parallel parallel strictly FIELD reference (M and to 3 +1, 0, -1) = AtM obtained interpreted by 1= rise /~ o # 4ms[ / (hk~) by scanning ic, use of the dz f(z)~ s[ where without any = ~°~~~~~ 8 ~ ~ ~'~~~~ j~~~~~~ velocity selection, is shown formula: ~ ~~ M ~~~ in QUANTUM ATOMIC N°4 PHASE STUDIES 609 a b N -300 300 o mA mA DA ,04 ic,A Fig. 2. -Interference experimental data TOF (8t/t selection where with = The data. with magnetic transverse a fives the field region in (a) prediction. theoretical R. give Points selection; TOF no (b) 0.3) parameter the the obtained pattern the brokenline while characteristic broadness mixers of the has adjusted been (bt/t distribution TOF order interferences of the I) ci to causes a get the best fit damping fast of visibility of the fringes when the increases. By chopping the beam and selecting a slice in the TOF spectrum (St It ci 0.3), a significant improvement of the visibility is achieved, as expected (Fig. 2b). Whilst a wavepacket description would be able to reproduce the loss of visibility due to the distribution width, it is not possible in the present TOF experiment to discriminate in between wavepackets (which should be the roles of the "true" source) determined by the operation of the beam and that of the statistical distribution of the these packets. An other experiment including a velocity selector with a group velocity among the well-defined transmission CONICAL 4.3 experiment Of the factor FIELD has CONFIGURATION. to by Its creates spatial frequency The order to get field BH a is Q = information some typical time compare a the magnetic field. It of 0.I TOPOLOGICAL G, spin one gets T evolution ci and of flight turns 7L, the 2~/L. On almost diTerent another constant B is (BH/Bj) T of an that Therefore correlative the a constant Dubbers around the and on period (L one hand over Artan and turn one where about out making (see Fig. 3). This type of conditions regarding the value PHASES somewhat spin dud the adiabaticity of the evolution) by Bitters parallel wires are now replaced by field B II which can be considered as B then takes the form: B = 86(z), of axis z and apex angle f = a cone In [8]. necessary already performed (in been [9]. In region 7l, the two helix (intensity iH) which [0, L]. be would the solenoid a interval 6 a z = cm) of over the axis creates vector a double interval longitudinal a resulting field [0, L]. The unit beam neutron a 6 which describes validity of the adiabatic approximation one has Larmor period 7L imposed atom through [0, L] to the at a velocity of10 km/s and a typical magnetic field adiabatic approximation is not valid here in general. the eTect on the external motion have been examined in JOURNAL 610 PHYSIQUE DE II N°4 a ', Z ' ' ' ' iH b ~ i e ~e E i i e ~ ~ ~ ~ l Z ---+ e II Fig. Conical 3. field configuration: field Be = configuration (a) experimental setup: H double helix; S B + Afiz where A is proportional to spatial frequency part 3.3. As explained spin the Be lated B + = hQ/g~Bi1z. along path the of the axis For L is: lbM principal paths the before along component each of states, these interferometer magnetic field: labelled by M, the the 3 are phase total eigenstates shift of accumu- Mlb, with: = 16 Actually Be of the effective (b) magnetic solenoid Q. l) (~(~~~~ h QK 2~ = ill and K. Because of the K depenaveraging the TOF distribution. an over The topological part fl of the phase is proportional to the solid angle of the cone described by with its geometric Be. Therefore it depends explicitely on K, which to be contradictory seems non-adiabatic character. In fact however this is not paradoxial since, in the case, the geometric dence the character followed does not refer but rather to to encloses +0A A +6 mA (+ (+ worthnoting of the experiment same cone. Bj,16 has = that a to sign 16 is single out rotation an ilz). even minimum ibm;n iH is way: z), for fixed ill, Bj is iH For BH = one " 2~ has the same sign as Bj. This means only when Bjj < 0. Consequently the " the present values about scanned of ((gpBBjjm/(hKQ) the zero-order dose 15 value 16 = + I( 0 is bright fringe in the range curve when the the cyclic -0A A up ip ranging from -6 mA times larger than BH. It of iH> not of I II. As a function minimum 0. The value: that the case, states around function at (in [10]: fl remains the same provided that Be (which defines of the following in the iH> also parameters space another into the Bj of the Hilbert carried of here include space the to changed is refers the to given values of for will is hamiltonian states) defined are pattern by B) Zeeman The then 16 and interference of BH for a fixed up is value I] obtainable still exists at at some value of (BH( of negative values QUANTUM ATOMIC N°4 STUDIES PHASE 611 it disappears at positive values of Bjj. peak present in all patterns is only due seen complete calculation qualitative: This solely mechanism is mixing not [6]). agreement to the a 4b in figure which in good agreement the shown interference fives of the patterns are curves with the experiment, except at large values of BH because of a failure of the model adopted to Bjj (but it is shifted behaviour This describe the is at value some clearly in (BH( # 0), figure whereas (the 4a central mixers. b,mA ;,,,~A a N o 2 2 4 OA -O.4 iH,A Fig. 4.- (a) intensity iH in predictions. 5. Interference the Experiment 5. I helix is in a patterns scanned strong As EXPERIMENT. longitudinal gradient of i~,A using for field. mentioned magnetic field conical the fixed values properties Optical before can be configuration depicted in figure 3. The intensity ill in the solenoid. (b) Theoretical field of the the spatial increased of shifts beaded the induced 1 on atoms. an by use up to few 10~ out of the complete by a wave "strong~ fields atomic of of Gauss. In such conditions interferometer will atom going an following properties: (I) its internal state is we[I defined (by the analyzer), for instance I); (it) its external motion consists of 3 wavepackets the envelops and the I, M (2sij2, F largely shifted in space and time as explained in 2:3 (beaded atom). carrier of which waves are Because of the large values of the corresponding phaseshifts (few 10~ rad) the visibility of the distribution. interference fringes is completely cancelled by the averaging over the TOF atomic preserved multiple wavepackets generated Nevertheless coherence is &om a given among the a if it through interference of the shortness incident one, even be seen the atomic because cannot associated wavelength. of the coherence by The present experiment has been carried out in view of investigating this electrostatic field, the transition 2s-2p is beaded another atom is passed through an way. If the induced without external motion. It is followed by the emission any appreciable change in the conformation of the of a Lyman a photon. The question which arises is: does the special now external motion affect in some emission of the atom ? way the optical of few have tens the = = JOURNAL 612 PHYSIQUE DE II N°4 diagram of such atoms, the range of the electrostatic field along z-axis and the photons Lyman detected at a mm are angle this axis, (Az, At) given with through finite solid angle As shifts respect to a a a w. K-dependent, a TOF technique can be used to scan these quantities experimentally. The are experiment has been carried out as follows: In a first step for given a and w, a TOF distribution field in shift). is obtained without magnetic regibn without 7l (I.e. This distribution any any I) (maximum normalized equal is practically independent of and In second to once a a w. step a longitudinal magnetic field Bp produced by a solenoid (2000 tums~ 10 cm in length) is applied in 7l. The difference A between the intensities measured without and with this field is then plotted as a function of th~e time of flight, in the scale as that used for the normalized same order In has study to (standard) of B II, ues A is been Table (£ in 6il of the Characteristics figures 5a,b modulation both been in carried The with out figures 5a,b,c,d. long acquisition rather bars. error have shown are and is main in various The val- difference (few 10~ s) times features the cases these distribution, which results have are the magnetic field; the to d. a /BjjdZ(G.cm) AZ(I) 1200 45 1000 1200 45 0.2 c 2000 2400 45 0.5 d 1000 1200 90 0.2 at with a are 45° = with 2 better contrast normalized with a that means are elongating strong a figures 5, in 1000 A(t) curves with shown a A on (d) to b obtained seen experiments the of experiments (a) of the In results flux) total get sufficiently small to Expt. I) I. The table ones: I. results w small necessary following given experiments Four DISCUSSION. AND a I distribution. and generally emission about to TOF RESULTS 5.2 the restricted been decrease the values of in figure in seen (0.5 and 5b. It resp.) srd 0.2 should be the (b) is not the noted corresponding to respect of A w 0.5 same that standard due to the smaller in TOF value of w. ii) seen is In figure that the iii) Data now 90°. shown order In and to the the Tab. A in Bp I). get In that quenching case case and could electric = be field is 90° in the (again but faster Bjj has than in conditions same normalized with multiplied by been 2. It is (a). as in respect (b) the angle a corresponding but the to wavelength the that would characteristic be obtained modulation of the (with the values same one has of a, emitting coherently Lyman a photons and located at of the multiple wavepackets. Then the difference 6(t) between with Bp is calculated (see broken in Figs. sa~b,c~d and curves unlikely smallness of obviously 6 is that the 0. It gets one ci attributed not (a) twice small. about light centers without (d) (a obtained in as about patterns I(t) with the as I(t) of same of A is very insight some interference points same figure 5d are magnitude distribution) the are oscillates of A the before) as values in Clearly the calculated w modulation TOF standard conditions the 5c well sources to a light polarization defined all over the effect atomic insofar beam as the section, direction and also of the because N°4 ATOMIC -QUANTUM PHASE STUDIES 613 a b o o ~ o o o o o j o ~ £ o q ~ , , £ ~ o ~ Z ~ Z ' o t o , , i , a t t ' ' , , , o t ', ' ' ', o ' t , ' a t ° , , , ' , i ' ' , 1 , , ,, _. Vt~ 2 t/tm 2 ~o d o C o o o oo ° o o o a o a o o o ~ ~ o o o o o o o Z o q o o £ , ~ Z o o o ~, ~ o o o I a i o ° i o I i a i o i I a ' ' , o ~ ~ ~ ~ °°o ° ', ° , ', %m Fig. Time 5. TOF spectra difference A refer a to small small in the of with flight Bjj between = signal these is not without conditions observed conditions. of spectra in presence normalized such and with defined when Bjj strong the that 0 spectra experimental tj~ Bjj. maximum Broken curve: value is I. fields Full Young's holes difllerence A Bjj. Open circles and calculation. circles: full line: (a,b~c,d) table 1. in = longitudinal magnetic 0 : it is only the which is particularly JOURNAL 614 conclusion In it this Lyman a experiment is also because does one priori a N°4 phenomenon characterized by optical emission. The theoretical difficult, not only because of the emission in occur rather wavelength close interpretation of a the of the combined field II interference an complexity of the profile of electric that seems the to PHYSIQUE DE induced present 2p the with emission process (2s process 2p itself transition but in a transition). ls Conclusion. 6. opportunities to study more deeply the wave easily controlable tools one is allowed systems. are (the the incident projectile) insofar as the properties interferometer to concentrate atom on configuration (the target) is well defined at a macroscopic scale. The ability of producing beaded with splittings much larger than the atomic wavelength lead to new atoms information about the correlation of atomic wavepackets which can be now considered experimentally as an testable quantity rather than as a mere theoretical concept. Atomic interferometers properties of atomic provide with us new interferometers As these Acknowledgements. The Rubin, City College, New-York, for many wavepackets in an interferometer, interesting suggestions for future experiments. authors cussions very wish about to the thank Pr behaviour enlightening K. of atomic as well as for dhhis References iii DIRAC P-A-M-, The Principles of Mechanics~ Quantum 4th Edition (Oxford University Press, 1958). [2] Geometrical Phases in Physics, (World Scientific, 1989) and Adv. Ser. in References Math. Phys., 5, F. Wilczek and A. Shapere Eds. therein. Cime~lto 9 (1932) 43. [3] MAJORANA E., Nuovo [4] SCHWINGER J., Phys. Rev. 51 (1937) 648. [5) LANDAU L. et LIFSCHITZ E., M4canique Quanti.jue, 3rd Edition (Editions Mir, Moscou, 1974). [6) MINIATURA Ch., PERALES F., VASSILEV G., IiEINHARDT J., ROBERT J. and BAUDON J., I. Phys. II 1 (1991) 425; ROBERT J., AiINIATURA Ch., LE BOITEUX S., REINHARDT J., BOCVARSKI V, and BAUDON J., Europhys. Lett. 16 (1991) 29; AiINIATURA Ch., ROBERT J., LE BOITEUX S-i REINHARDT J. and BAUDON J-i submitted to AppJ. Phys. B, Special Issue: Optics and interferometry with Atoms [7) LAMB Jr W-E- and RETHERFORD R-C-, Phys. Rev. 86 (1952) 1014. communication. [8] RUBIN K., private Lett. 59 (1987) 251. [9] BITTERS T. and DUBBERS D., Phys. Rev. [10] AHARONOV Y. and ANANDAN J., Phys. Rev. Lett. 58 (1987) 1593. (1992).