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Selective Oxidation Reactions of Natural Compounds with
Selective Oxidation Reactions of Natural Compounds with

... Methyltrioxorhenium (CH3ReO3, MTO) in the presence of H2O2 has proven itself as an efficient and versatile oxidation catalyst with interesting selectivity towards natural compounds, which can be oxidized under quite mild conditions [3–21]. In previous work [22] we have observed good regio- and stere ...
Large coordination complexes: synthesis, characterisation and
Large coordination complexes: synthesis, characterisation and

... presence of two methyl groups remote from the coordination centre. Their coordination properties would be expected to be identical, the only difference being their molecular weight, 28 units greater for 2 than for 1. We will call these two ligands pseudoisotopic molecules, defined as two species whi ...
Chapter 24 Transition Metals and Coordination Compounds part 2
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... electrons in the d orbitals, this will cause ________________ This will cause those orbitals to be ________________ This will result in them having ______________ A. For an octahedral complex, there are 6 ligand attachment points (along the x, y, & z axes)  Three of the orbitals are farther away fr ...
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PREPARATORY PROBLEMS (Theoretical)
PREPARATORY PROBLEMS (Theoretical)

LECTURE 7 REDUCTIVE ELIMINATIONSa
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... activation, enamine activation, and palladium-catalyzed enyne cycloisomerization [46]. Córdova’s methodology allows the preparation of functionalized optically active cyclopentenes with all-carbon quaternary stereocenters in good diastereo- and high enantioselectivities from simple starting material ...
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Lecture note Part II (Coordination Chemistry)

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... Lukehart prepared a fascinating monorhenium compound displaying both acyl and hydroxycarbene ligands32 – the synthesis is shown in Scheme 1.9. The intermediate was referred to as a metalloacetylacetonato complex because it is the organometallic analogue of acac and may itself be a ligand to other me ...
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... Organometallic compounds are those which contain a metal-carbon bond. The variety of the organic moiety in such compounds is practically infinite, ranging from alkyl substituents to alkenes, alkynes, carbonyls, aromatic and heterocyclic compounds. Although some organometallic compounds have been kno ...
chapter 6-hydroxyl compounds
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... - Reason: a more highly substituted alkyl group inhibits solvation of the alkoxide ion and drives the dissociation equilibrium to the left. - For example: methanol is more acidic than t-butyl alcohol. • The present of electron-withdrawing atoms enhances the acidity of alcohols. - Reason: the electro ...
Future perspectives in catalysis - NRSC
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... It was also launched a quest to research and understand the underlying process. In 2007, the German scientist Gerhard Ertl was awarded the Nobel Prize for Chemistry for unraveling the mechanisms of the Haber-Bosch process. In the 1960s, he began using the equipment used in the burgeoning semiconduct ...
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... Mechanism occurs in two stages. The first is addition of the nucleophile to the carbonyl carbon to form a tetrahedral intermediate. The second stage in collapse of the tetrahedral intermediate to reform a carbonyl with expulsion of a leaving group (Y). There is overall substitution of the leaving gr ...
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...  separation was achieved by adjusting pH and organic complexant  Separation of Cm from Am was performed with 0.01 % ethylenediamine-tetramethylphosphonic acid at pH 3.4 in 0.1 M NaNO3 with a separation factor of 1.4 Separation of gram scale quantities of Am and Cm has been achieved by cation and a ...
Rules and Clues for Determining Oxidation Number
Rules and Clues for Determining Oxidation Number

... F: Always –1, except F2 O: Almost always –2 (exceptions: cmpds. w/ O-O or O-F bonds) Alkali metals: Always +1 (except pure metal (0)) Alkaline earths: Always +2 (except pure metal (0)) H: +1 when bonded to main group (C, O, N, halide groups) -1 when bonded to metals 5. Ranges of oxidation states for ...
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Hydroformylation



Hydroformylation, also known as oxo synthesis or oxo process, is an important homogeneously catalyzed industrial process for the production of aldehydes from alkenes. This chemical reaction entails the addition of a formyl group (CHO) and a hydrogen atom to a carbon-carbon double bond. This process has undergone continuous growth since its invention in 1938: Production capacity reached 6.6×106 tons in 1995. It is important because the resulting aldehydes are easily converted into many secondary products. For example, the resulting aldehydes are hydrogenated to alcohols that are converted to plasticizers or detergents. Hydroformylation is also used in specialty chemicals, relevant to the organic synthesis of fragrances and natural products. The development of hydroformylation, which originated within the German coal-based industry, is considered one of the premier achievements of 20th-century industrial chemistry.The process typically entails treatment of an alkene with high pressures (between 10 to 100 atmospheres) of carbon monoxide and hydrogen at temperatures between 40 and 200 °C. Transition metal catalysts are required.
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