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GEOPHYSICALRESEARCHLETTERS, VOL. 20, NO. 9, PAGES851-854,MAY 5, 1993 EVOLUTION OF SEAFLOORSPREADING RATE BASED ON 4øAtDEGASSING HISTORY EiichiTajika1 and TakafumiMatsui Departmentof EarthandPlanetaryPhysics, Universityof Tokyo Abstract A new degassing modelof 4øAt coupledwith thermal evolution of the mantle is constructedto constrain the temporalvariationof seafloorspreading rate. In thismodel,we take into accountthe effectsof elementalpartition and solubil- ity duringmeltgeneration andbubbleformation,andchanges in both seafloorspreading rate andmelt generation depthin the mantle. It is suggested that the seafloorspreading rate wouldhavebeen almostthe sameas that of today over the historyof the Earth in orderto explainthe presentamountof 4øAtin theatmosphere. Thisresultmayalsoimplythemild mantle potassiumconcentratesinto melt being associatedwith melt generationin the mantle belowthe mid-oceanridge, and eventually solidifiesas the oceanic crusts. Thus, potassium concentrates into the oceanic crust from the mantle concur- rentlywith4øAtdegassing. Potassium in theoceanic crustalso decayto 4øAtwhichwoulddegasto the atmosphere probably by diffusionthrough the oceaniccrust or by arc volcanismsat the subductionzone. Potassiumremainingin the oceaniccrust would finally return to the mantle. The continental crust is consideredto have formed by remelting of the oceanic crust with water at the subduction zone[e.g.,Campbelland Taylor, 1983]. If this werethe case, degassinghistory of volatilesfrom the mantle. the parts of potassiumin the subductingoceaniccrustsmight be transported to the continental crust at the time of its for- Introduction mation. 4øAtproducedby potassium in the continentalcrust Temporalvariationof seafloorspreadingrate overthe his- KAr hasdegassed to theatmosphere withdecayconstant D,cc-- tory of the Earth hasprofoundinfluences on the globalgeo3.71 x 10-•ø yr-1 whichis estimatedfroma relationbetween chemical cyclethroughvolatiledegassing fromandregassing K-At mineral ages and Rb-Sr whole rock agesfor the same into the mantle. In other words, it affectsthe evolutionsof crustalrock [Hamanoand Ozima,1978]. the atmosphereand oceans,and thus the terrestrialenviron- ment[e.g.,McGovern andSchubert, 1989;TajikaandMatsui, 1992,1993].It is, however,difficultto reconstructsucha tem- poralvariationof seafloor spreading rate fromany geological evidence. This is because the ancient seafloor itself has sub- We can calculate transportation of K and Ar between various reservoirs using a simple box model composedof three potassium reservoirs (mantle,oceaniccrust,continental crust) and of four argonreservoirs(mantle,oceaniccrust,continental crust,atmosphere).The massbalanceequations for argonand ductedinto the mantle. Because the seafloor spreading rate playsa dominant rolein transfer ofinternalheat[e.g.,Turcotte potassium are as follows: and Schubert,1982],we may obtain the evolutionof seafloor D •(4øK)ma, , = -• Tk'40 K,}mant-- KK(4øK)ma,t+(1-AK)tr-X(4øK) spreading rate by studyingthe globalgeochemical cyclecou- d pled with the thermal evolution of the mantle. In this paper, we try to infer the temporalvariationof seafloorspreading rate, usinga newdegassing modelof 4øAt coupled withthermalhistoryof themantlein whichtemporal variationof degassing rate is assumed to dependon changes in seafloorspreading rate and melt generation depthin the •t(4øK)oc =--AT(4øK)oc +KDK(4øK)m•,t --tr-X(4øK)oc (2) + dt d 40 •( Ar)m•,t = A•(4øK)m•,tK•"(4øAr)m•,t(4) mantle. Models dt We use4øAtasa tracerfor the mantledegassing. 4øAxis -dtd consideredto be the best tracer for the degassing history of the mantle amongvariousvolatile components.This is because d -4o - (1) 4øAtis a decayproductof potassium, andsoverylittle amount of 4øAt existed at the time of formation of the Earth. This meansthat 4øAtmay not haveexperienced impactdegassingwhichis considered to haveoccurredduringaccretion of the Earth [e.g.,Matsuiand Abe, 1986].(2) The existence of 4øAtin the presentatmosphere suggests the occurrence of subsequent continuousdegassing overthe historyof the Earth [e.g.,Turekian, 1964;Hamano andOzima,1978].And(3)4øAt probablyhas not experiencedany regassinginto the mantle, which meansthat we can only considerthe degassingprocess for the caseof 4øAt. In theserespects,4øAtis considered to be an adequateindicatorto constrainthe degassing historyof the Earth after its accretion. 4øAtis produced by potassium decayas 4øK+e- -,4øAt, wherethe decayconstantis ;•e=5.85x10 -n yr-•. 4øAtproducedin the mantle degasses to the atmospheremainly through the mid-oceanridge volcanismaccompanied by the formation of oceaniccrusts. Sincepotassiumis an incompatibleelement, = - = - = (5) D,cck wheretr is the residence time of seafloor(=area of seafloor/ seafloor spreading rate), K}) ia thecoefficient ofdegassing rate, and),T is thetotal4øKdecayconstant (= 5.305x 10-•øyr-•). ß Subscriptsrepresent as follows: mant = mantle, oc = oceanic crust, cc = continental crust, and arm = atmosphere,respectively. A•½is the accretionratio of potassium,which is a free parameter in this model. The fraction A•½ of potassium in the subducting oceaniccrust is assumedto be transported to the continentswith continental growth. A•½is iteratively determined so that the amount of potassiumin the continental crust at present may be equal to the observedamount. We consideredvariousmodelsof continentalgrowth. However,the continentalgrowth model did not affect the numericalresults seriously(Table2), andthenwe usethe modelwith a constant growth rate as a standard. The degassing processof Ar is modeledas follows:4øAt Copyright 1993by theAmericanGeophysical Union. in a certain volume Vo of the mantle degasto the atmosphere when oceanicplates are formed at the mid-oceanridge. This volume Vo probably dependson the seafloorspreadingrate Sr and the melt generationdepth d,• in the mantle. Assuminga Paper number93GL00731 first orderrate process (i.e., assuming a homogeneous mantle), 0094-8534/93/93GL-00731503.00 the degassing rate Fo of 4øAtfromthemantleis expressed by •Nowat Geological Institute,Universityof Tokyo 851 852 Tajika and Matsui: Evolutionof SeafloorSpreadingRate rv - 'ß (8) whereK• r is thecoefficient ofdegassing rateofargon. In the previousstudiesof degassing history[e.g., Turekian,1964;Hamduoand Ozima, 1978],the coefficient of degassingrate was given as an adjustableparameter for the degassinghistory and called "degassingconstant". However, in this study, we define the coefficientof degassingrate as follows[e.g.,TajikaandMatsui,1992]: Forsythand Uyeda(1975)suggested that platemotionmay be driven by the forcesacting on the downgoingslab and that drag force on the bottom of oceanic plates may be less important. If this were the case, the oceanichthospherewould couple weakly with the' underlying flow becauseof lower vis- cosityof asthenosphere [Forsythand Uyeda, 1975]. This is consistentwith the numerical result of thermal history of the mantlewith variableviscosity[Christensen, 1985]. According to Christensen (1985),the Rayleigh-Nusselt exponent/•should be nearlyzerounderthe conditionof the mantleconvection, K•V(t) -=far' VD(t)IVM-- far' St(t). dm(t)/VM (9) and in sucha caseseafloorspreadingrate becomesto be constuntin spiteof drasticchangein convective vigor. Therefore whereVM is the volumeof the mantle,VD(t) is the volumeof mantle material from which degassing occursin an unit time, weconsider anothermodelin which/• is setto be zero("the modelB"). In this model,the seafloorspreading rate is con- St(t) is theseafloor spreading rate,anddin(t)is themeltgen- stant at the presentvalueoverthe historyof the Earth. We needto knowthe total amountof potassiumto calculate erationdepth in the mantle. Here we assumethe degassing of4øAtproduced bythepotassium decay. Because volumeVt>= Sr x din, whichis time-dependent in this case. theamount it is difficultto estimatepotassium contentin the presentmanJAr is the degassing fractionof argonwhichrepresents the massratio of argonpartitioninginto the gasand melt phases tle, we useits upperestimateof 400 ppm and lowerestimate to the total amountoriginallyincludedin the degassing volume of 100 ppm derived from the discussionof surfaceheat flow [TajikaandMatsui,1992].Theeffectofprocesses suchasmelt generation, partitionofvolatileelements to themelt,andbub- [HamduoandOzima,1978].Recentgeochemical estimates on ble formationunder the mid-oceanridge are includedin this theabundance ofmantlepotassium [e.g.,Jochum et al., 1983], however, agreewellwith the average of the two(= 250ppm). factor. far can be estimatedfrom observation and physical We thereforeregard250ppmasthe mostprobablevaluein this quantitiessuchas partition coefficient,solubility in the sihcate study.Theinitialaverage mantletemperature Tø•issimplyas- melt and so on. [Tajikaand Matsui, 1992].For concentration sumedto be in the range of 2000-3000K. of potassium into melt,we usef•c and (4øK)mam insteadof far and (4øAt)main. The valuesof JArandf•c areestimated Numerical Results to be 0.93and0.99,respectively [Tajika,1992].It isnotedthat Figure 1 shows the temporal variations of the seafloor the coefficientof degassingrate in this model has a physical spreading rate, the melt generation depthin the mantle,and meaning(not an adjustableparameter)and varieswith time (not constant)sincethe seafloorspreadingrate and the melt generationdepth changewith the mantle cooling. 100 • The melt generation depth is defined by the depth where the ascendingmantle material intersectsthe mantle solidus, thus extensivemelting and melt segregationoccurat this depth. We assume that mantle volatile componentsare released effectively with the melt segregationat this depth. Temporal variation of the melt generationdepth can be calculatedfrom that of the averagemantle temperature and the mantle sohdus I ' I ' I , ! , (a) MODEL A if.:::.' .......... profile[TajikaandMatsui,1992].On the otherhand,temporal variation of the seafloorspreadingrate is related to the mantle heat flow. Both the mantle heat flow and the averagemantle temperature are obtained by solvingthe thermal evolution of the mantle [Tajikaand Matsui, 1992]. We use the parameterized convectionmodel to calculate 0.1 m I I I I I m I • 100 , • , • , • , , , the wholemantleconvection [e.g.,Schubertet al., 1980;Chris- (b) MODEL B tensen, 1985; McGovern and Schubert, 1989; Tajika and Mat- sui, 1992]. In this model,we trace the temporalvariationsof averagemantle temperature Tm and heat flow q from the mantle which is parameterizedin terms of the Rayleighnumber Ra. The equation of conservationof energyis given by atto- -3R•q+ (RS• •Q pC•( RS• - R•S)-•--•_ Rc) .. VD, dm (10) wherep is the density,Cp is the specific heat at constantpressure,and R, and Rc are the outerand innerradii of mantle, respectively.Q is the energyproductionrate by decay of radiogenicheat sourcesin the mantle. Mantle heat flow q is parameterized in termsof the RayleighnumberRa as, 0.1 I 0 i 2 I I 3 I I 4 I 5 q ock(Tm- Ts)/(Rm- Rc)Ra Is,wherek isthethermal con- TIME (Ga) ductivityand Ts is the surfacetemperature.The factor/• is a Rayleigh-Nusselt exponent, usuallytakenas0.3 [e.g.,Schubert Fig. 1. Temporalvariationof the seafloorspreadingrate St, the melt generationdepth in the mantle din, and the mantle degassing volumeVD (fromwhichthe degassing is assumed to et al., 1980].Because q ccv/• [e.g.,Turcotte andSchubert, 1982], wecanestimate Sr fromqbyusing arelation ofSr ccqa occur)for (a) the modelsA and (b) the modelB. Eachvalue [e.g.,Christensen, 1985;McGovern andSchubert, 1989;Tajika is normalized by the presentvalue(St* = 2.84x 10iama/Ma, andMatsui,1992].In thisway,wecanobtainthe average mantle temperatureandthe seafloorspreading rate by solvingthe aboveequations(wecall this "modelA"). temperature is assumed to be 2000-3000 K for the model A d• = 40x 10am,andV/• = 11.4x 1016mS/Ma). Initialmantle and2000-2500K forthe modelB (expressed ashatchedarea). Tajika and Matsui: Evolutionof SeafloorSpreadingRate the mantledegassing volumefrom whichthe degassing is assumedto occur. Thesevariationsare closelylinkedwith thermal evolutionof the mantle. In the modelA, averagemantle temperature, mantle viscosity,and mantle heat flow are shownto be greatly changedthroughoutthe historyof the Earth. Thesefeaturesare qualitativelysimilarto the results of previousstudies[e.g.,Schubert,etal., 1980;McGovernand Schubert,1989;Tajika andMatsui,1992].As a consequence, the seafloorspreadingrate in Arcbeanis estimatedto be 4-16 timeslargerthan that of todayand the melt generation depth at that time to be about 70-100 km (i.e., 2-3 timeslarger than that of today),resultingin a largemantledegassing volume about8-45 timesgreaterthan that of todayin the model 853 Table1. 4øAtdegassing history forthemodels A andB (forthe mantlepotassium content 250ppm).TOm is theinitialaverage mantletemperature. The superscript ß represents the present valueand the overlinerepresents the time averageoverthe history of the Earth. X is the ratio of the amount of 4øAr degassed to the atmosphere to the totalamountof 4øArproducedby potassiumdecay. model Tøm(K)St/St* dm/d• V•v/v• 4øArt X 3000 2500 2000 2500 2000 2500 A (Figurela). Thisstrongly suggests thevigorous degassing duringthe Hadeanand Arcbeanperiods,and thus the total amount of 4øAtdegassed to theatmosphere wouldbelarger. In the modelB, however,degassing from the mantlewouldbe 8.69 5.48 3.72 1.0 0.5 2000 lesseffectivecompared to the modelA (Figurelb) because the mantledegassing volumevariesonlywith melt generation depthin thiscase.The numerical resultson 4øAtdegassing 2500 2000 2.0 1.93 1.73 1.52 2.33 1.50 2.04 30.75 11.12 6.44 2.33 1.50 1.02 13.30 13.30 12.90 8.42 6.61 4.96 0.70 0.70 0.67 0.44 0.35 0.26 1.25 0.62 3.53 0.18 2.93 1.89 5.87 3.78 13.30 11.60 0.70 0.61 history are summarized in Table 1. Figure2 showsthe total amountof 4øAtdegassed to the atmosphere as a consequence of eachcorresponding degassing history (the error bars representuncertaintiesof the mantle potassiumcontent,100-400ppm).In the modelA, compared to the observed value,4øAthasdegassed too muchto the atmosphere for any initial average mantletemperature (Figure 2a). As shownin Table 1, the degassing fractionX, which represents the ratio of the amountof 4øAtdegassed to the atmosphere to the totalamountof 4øAtproduced by the potassium decay, is about 0.7. These results reflect more effective degassinghistory of the model A. On the other hand, in the modelB, theamountof4øAtdegassed to theatmosphere shows a goodagreement with the presentobserved value(Figure2b). The degassing fractionX is about0.35forthismodel(Table1). This meansa mild degassinghistory of the model B. Figure 2c $ axnountof 4øAtdegassed to the atmosphere in 1016kg at t=4.6 Ga (cf. theobserved valueis 6.6x 1016kg). and 2d show the results for the cases with different constant seafloorspreadingrate (larger and smallerthan the present one)for comparison.In the casehigherthan the presentvalue, the amountof 4øAtdegassed to the atmosphere is muchlarger (Figure2c), whereasin the caselowerthan the presentvalue, the amountis muchsmaller(Figure2d). This resultstrongly suggests that the seafloorspreadingrate may not havechanged greatly from the present value over the Earth's history. It is alsosuggestedthat volatile degassingrate from the mantle may have been as same as that of today, with possiblevariations of at most 2-3 times larger than that of today. Discussion 25 a A •o •' MODEL A b MODEL B ( Sr,= 1.0x Sr* )- 20 15- 5 - 2O . amountof 4øAtin the atmosphere. In thisrespect,the parameterized convectionmodel with fl = 0 is more reasonablethan the usual model with fl = 0.3. This would be, in turn, consistent with the idea that the oceaniclithospherewould couple weakly with the underlying asthenospherebecause of lower viscosity of the latter. The plausibility of constant seafloor spreaaqng rate werediscussed by Christensen(1985) basedon c ( Sr=2.0xSr* ) d ( Sr.=0.SxSr* ) A The seafloorspreadingrate is suggestedto have been almost constantduring the Earth's history to explain the present . theoretical considerationsand geologicalevidence. The numerical results, however,include somesort of ambiguities becauseof simple assumptionsfor the model and also uncertaintiesin physicalparameters.Therefore,we performed sensitivityanalysiswith respectto the standardmodel(model . B: TOm =2000 K, (K)•ant =250ppm)whichgivesa proper amountof 4øAtdegassing to the atmosphere. The resultsare summarized in Table 2. As shown in Table 2, the ambiguities causedby uncertainties of the model parameters and assumptionsmay not drastically changethe results. Even if we take into account the effectsof hot spot volcanismand mantle plumeson the 4øAtdegassing, we do not needto changeour Fig. 2. Totalamountof 4øAtdegassed to the atmosphere for the modelsA and B as the consequence of eachdegassing his- tory (figuresb, c, d correspond to the modelswith constant seafloorspreadingrate once,twice, and half of the present value,respectively). The presentpotassium abundance in the mantleis assumedto be 100-400ppm (rangeof changein the resultsdue to potassiumabundances is representedby error bars),and the initial mantletemperature is assumed to be 2000K (circles), 2500K (diamonds), and3000K (stars),respectively. The brokenlinerepresents the observed amountof 4øAtin thepresentatmosphere (6.6x1016 kg). conclusions. This is simply becausemuch larger amount of 4øAtmusthavedegassed in this case. The assumptionsof homogeneousmantle, constant partition coefficient under the variable conditions from the melt generationdepth to the surface,and the definitionof the mantle degassingvolumewould provideanothersourcesfor uncertainties. Becausethe extent of mantle heterogeneityand the change in partition coefficientshave not been known, there remain ambiguities due to these assumptions. Although the mantle degassingvolume is defined as Sr x dm in this study, the studiesof flow patterns of ascendingmantle materials and 854 Tajika and Matsui: Evolutionof SeafloorSpreadingRate Table 2. Summaryof sensitivityanalysis parameters/asumptions accretion ratio AK continental degassing rate K D,cc ar mantle solidusprofile continentalgrowth model degassinghistory " uncertainties errorst 0•1.0 +50% +50% -5.0% • 6.2% +3.c% +30% (nocontinental growth) (growthafter2.5GaBP) (nodegassing for the first1.0Ga) -5.0% -3.3% -6.0%t Difference between theresult ofdegassed 4øAtforthestandard case (model B' Tø•:2000K, =250ppm) andthatforsensitivity analysis (values areshown relative tothestandard result in %). Relative to the result of the model A. melts below the spreadingcenter might suggestmore complex geometryof mantle degassing volume[e.g., Spiegelmanand McKenzie, 1987].Here we modifythe definitionof the mantle degassingvolume by introducing the geometricalfactor • as VD ----St. drn/•. In order to explainthe observedamountof 4øAtby the modelA, • •20 is required.This seems to be too large for consideringmodification due to the flow pattern. Although someof the problemsstill remain unknown, the model B seems much more reasonable than the model A. Sleep(1979) has alsoattemptedto constrainthe seafloor spreadingrate and the amount of mantle potassiumby usinga simpleanalyticformulation of the 4øAtdegassing andthermal evolutionmodels. Accordingto his result, the averageseafloor spreadingrate during the last 3 bilhon years is no more than twice the present value. The differencebetween his and our results would be partly becausehe did not take into account the effect of temporal variation of melt generationdepth on the degassingrate. As shown in Table 1, the faster constant seafloorspreadingrate model(twicethe presentvalue)restfits in deeperaveragemelt generationdepth(about 2-3 timesthe presentone), whichmeansthe averagemantledegassing volume is about 4-6 times the present one. In such a case, as described earher(Fig. 2c), muchmore4øAtdegasses to the atmosphere. This suggeststhat more reahstic treatment of temporal variation of melt generation depth is required to constrain the seafloorspreadingrate. It is noted that the temporal variation of melt generationdepth is an inevitable result as far as the mantle has been coohngover the history of the Earth. Acknowledgments. This researchwas partially supported by the grants-in-aidfor ScientificResearch(No. 02804023)of the Ministry of Education of Japan. References Campbell I. H. and S. R. 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Left., 96, 27-37, 1989. Schubert G., D. Stevenson, andP. Cassen, Wholeplanetcooling and the radiogenicheat sourcecontentsof the Earth and Moon,J. Geophys. Res.,85, 2531-2538,1980. SleepN.H., Thermalhistoryanddegassing oftheEarth: Some simplecalculations, J. Geology, 87, 671-686,1979. Spiegelman M., andD. McKenzie,Simple2-D modelsfor melt extractionar mid-ocean ridgesandislandarcs,EarthPlanet. Sci. Left., 83, 137-152,1987. Tajika, E., Evolutionof the atmosphere andoceanof the Earth: globalgeochemical cyclesof C, H, O, N, and S, and degassing historycoupled withthermalhistory,pp. 416,Doctoral Thesis,Universityof Tokyo,Tokyo,March1992. Tajika,E., andT. Matsui,Evolutionof terrestrialproto-CO2atmosphere coupledwith thermalhistoryof the Earth, Earth Planet. Sci. Let.; 113, 251-266,1992. Tajika,E., andT. Matsui,Degassing historyandcarboncycle of the Earth:Froman impact-induced steamatmosphere to thepresent atmosphere, Lithos(submitted), 1993. TurcotteD. R., andG. Schubert, Geodynamics, 450pp,Wiley, New York. Turekian, K. K., Degassingof argon and helium from the Earth, in The Originand Evolutionof Atmosphere and Oceans, editedbyP. J. Brancazio andA. G. W. Cameron, pp.74-82, Wiley, 1964. T. Matsui,Department of Earth andPlanetaryPhysics, Facultyof Science, University of Tokyo,Tokyo113,Japan. E. Tajika,Geological Institute,Facultyof Science, University of Tokyo,Tokyo113, Japan. (ReceivedDecember15, 1992; revised March 8, 1993; acceptedMarch 17, 1993.)