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Design and Analysis of Chain and Network Structures from Organic
Design and Analysis of Chain and Network Structures from Organic

... in this study: a difunctional cluster, [W6O25H(AsR)2]5(R ) C6H4-4-NH2), and a tetrafunctional cluster, [Mo12O46(AsR)4]4- (R ) C6H4-4-NH3+). The former is isostructural with the previously reported phenyl derivative17 and similar to the molybdenum derivatives, [Mo6O24(AsC6H4NH2)2]4-.18 The cluster co ...
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... These results indicated that thermodynamics alone would not prevent the synthesis of nitroacetate from carbon dioxide, nitromethane and magnesium meth-oxide, although the yield achievable under these conditions could not be high. To investigate this possibility, a solution of magne-sium methoxide in ...
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Hydroformylation



Hydroformylation, also known as oxo synthesis or oxo process, is an important homogeneously catalyzed industrial process for the production of aldehydes from alkenes. This chemical reaction entails the addition of a formyl group (CHO) and a hydrogen atom to a carbon-carbon double bond. This process has undergone continuous growth since its invention in 1938: Production capacity reached 6.6×106 tons in 1995. It is important because the resulting aldehydes are easily converted into many secondary products. For example, the resulting aldehydes are hydrogenated to alcohols that are converted to plasticizers or detergents. Hydroformylation is also used in specialty chemicals, relevant to the organic synthesis of fragrances and natural products. The development of hydroformylation, which originated within the German coal-based industry, is considered one of the premier achievements of 20th-century industrial chemistry.The process typically entails treatment of an alkene with high pressures (between 10 to 100 atmospheres) of carbon monoxide and hydrogen at temperatures between 40 and 200 °C. Transition metal catalysts are required.
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