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Transcript
NEGATIVE CORONA DISCHARGE IN THE MIXTURE N2 + SF6 AT THE PRESSURE 26.6 kPa J. Kúdelčík, [email protected], M. Kúdelčíková, [email protected], FPV ŽU Hurbanova 15 Žilina INTRODUCTION Electronegative gases, as SF6 and mixture N2+SF6, are widely used in many industrial devices such as circuit breaker or gases insulating systems. The transmission from negative corona discharge to breakdown in these systems is unwelcome and elimination of this process depends on the understanding of the mechanism of the initial stage of discharge. Initial stage of negative corona discharge is in regime of Trichel pulses. Trichel mechanism presents wide and evident formation of cathode region at high pressure by streamer mechanism. The basic aspect of the corona discharge in a pointto-plane configuration at atmospherical pressures may be explained on the basis of the streamer theory. At a certain stage of the development of a single avalanche the space charge generated can partially shield itself from the applied field, creating a streamer initiating plasma. The condition of its generation is defined by Meek conditions [1] in the form: N e exp x dx 108 [cm -3 ] waveforms at the lowest gap voltage values (i.e., at the corona onset voltage values) were measured with UV illumination. At higher gap voltages the discharge started spontaneously. It can be seen for the lowest gap voltage values the current pulse had the form of a simple hump and its rise was rather slow with no sign of stepwise pulse on the leading edge. At higher gap voltages it was observed that the formation of a step on the pulse leading edge. At even higher gap voltage this step was found to develop into a new peak, i.e., the waveform took the form of a double peak. (1) If few electrons are just in front of the plasma, avalanching in the locally enhanced field can cause primary cathode- and anode-directed streamers to propagate. Thus, the feedback-to-cathode Towsend ionization mechanism is supplanted by faster feedforward-to-gas streamer mechanism. The streamers can be viewed as ionizing-potential waves characterized by the fact that the background gas is initially not ionized. After the initial acceleration lasting for about 1 ns, velocity of the cathode-directed streamer increases exponentially reaching the order of 108 cm/s. The streamer front propagation is really a phase movement, and can easily be much faster than the charged particles it contains. Choosing of used mixture was motivated by the fact, that when the concentration of SF6 is changed, at the same conditions it is possible to find characteristic aspects of streamer mechanism and we can also verify the physical model of streamer generation [2]. Presented results refer to the previous measurements for N2+SF6 [3] and O2 +SF6 [4]. EXPERIMENTAL PROCEDURE AND RESULTS General scheme of the experimental set-up and procedure used at the study of negative corona discharge in the mixture of nitrogen with SF6 are identical with these described in the related papers [3, 5]. The results in the Fig. 1 illustrate development of the first negative corona current pulse with increasing gap voltage at the pressure of 26.6 kPa for 5% admixture of SF6 in the buffer nitrogen gas. The Fig. 1. Current pulse waveforms taken for various gap voltages in mixture N2+5 %SF6 at pressure 26.6 kPa (distance point-to-plane 12 mm a radius of the point 0.1 mm) COMPUTATIONS The goal of computations was to find out, if the condition for streamer (eq. (1)) is fulfilled for measured values. So we dealt with the calculating of distance of the space charge center from the cathode surface, and its number. On the basis of these results it will be possible to explain forms of measured current pulses shown in the Fig. 1., i.e., if the current maximum responds to the contact of streamer with the cathode, and step on the leading edge to the i emission. If it is assumed that before the onset of the cathode directed streamer the discharge develops according to Townsend ionization mechanism, it is reasonable to suppose [6] that the maximum number of positive ions (a center of the positive ion space charge) is generated at a distance xc from the cathode, where the expression: xc ( E x c ). exp ( E z )dz 0 (2) reaches the maximum value ( is effective Townsend ionization coefficient). The value for the mixture N2 + 5% SF6 used in this relation was calculated using the program SIGLO based on the analysis of Boltzman equation [7]. To compute values in dependence from the distance from the cathode, the axial component of Laplacian’s field was calculated using hyperboloid approximation [8]. All computations and also finding the maximum of (2) were realized using the program MATHEMATICA. Our results were calculated for experimental data set shown in the Fig.1 and written in the Tab. 1. The value of xc and corresponding reduce field intensity E(Xc)/N, where expression (2) is the cathode [9]. All this process is quite long what influences the form of current pulse. xc a maximum, VZ1 : exp[ y dy ] is corresponding 0 number of electrons generated in the distance of xc, xcrit and corresponding reduce field intensity E(Xcrit)/N, where 0 . Results of computation of the characteristic distances and fields for measured experimental conditions TAB. 1. Voltage [V] 3300 3700 3900 Xc [μm] 199 237 257 (E(Xc)/N) [Td] 373 323 318 Xe[μm] 334 380 6 8.51710 403 7 4.621108 VZ1 3.17310 Xcrit [μm] 334 380 403 (E/N)crit [Td] 215 214 214 In the Fig. 2 there are shown results of computations for N2 + 5% SF6 at the pressure 26.6 kPa and gap voltage 3900 V. There is displayed behavior of , the dependence of number of positive ions and electrons from the axial distance from the cathode in arbitrary units. In the figure it is very well seen the separation of positive ions from electrons before streamer initiating plasma, which corresponds to the ionizating trajectory 1 (146 μm). Maximum number of generated electrons is reached when 0 . RESULTS AND DISCUSSION On the basis of measured results and computations it can be proclaimed, that at the gap voltage of more than 3600 V, for given experimental conditions, the form of current pulse is determined by streamer ionization mechanism. In the Tab.1 it can be seen, that the number of electrons developed of a single avalanche at the gap voltage of more than 3600 V, is sufficient to fulfill the criterion (1) for streamer initiating. This proclamation is also supported by ultra fast increase of the current to maximum of order ns, what would not be able in the case of Towsend ionization mechanism, because time of arrival of positive ions in mixture N2+5%SF6 exceeds hundreds of ns [2]. Also the total charge of observed current pulses of the negative corona discharge, i.e., cathode-oriented streamer, is typically of order ≈10-11 C, what corresponds to about 108 ions. In the case of gap voltage 3300 V, for the generation of streamer there are needed several generations of avalanches which are connected through the photoemission of secondary electrons from Fig. 2. Development for the mixture N2 + 5% SF6, expressions VZ1 and (2) in the dependence from axial distance from the cathode (p = 26.6 kPa, U = 3900 V, S = 12 mm, r0 = 0.1 mm). SUMMARY According to the streamer-based theory [2] the stepped pulse leading edge, the current pulses in mixture N2 + 5% SF6 (Fig. 1), forms as follows: The initial current rises to the step (denoted by A), it is due to a Towsend ionization mechanism fed by cathode secondary process (γp – emission). After decay of the current rises due to the rapidly shrinking cathode fall region, the current begins to rise again because of the development of cathode-direct streamer-like ionization wave. The pulse maximum is attained just as the streamer reaches the cathode. Next quick current fall in mixture N2+SF6 is due to negative space charge. This information about changing the mechanism of discharge is very important when isolating and switching apparatus are designed. By choosing the suitable equipment and electrode geometry required conditions for practice can be achieved. ACKNOWLEDGMENT: This work was supported by the institutional Grant no. 15/705/04 of FPV ŽU. REFERENCES 1. D. Meek, in Električeskij proboj v gazach (1960) 2. M. Černák, J. Phys. D 26, 607 (1993). 3. A. Zahoranová, J. Phys. D: Appl. Phys. 35, 762 (2002). 4. J. Kúdelčík, Contrib. Plasma Phys. 42, 546 (2002). 5. J. Kúdlečík, PhD. work (2003) 6. T. Ushita, Elec. Eng. in Japan 88, 45 (1968) 7. www.siglo-kinema.com 8. P. Espel, J. Phys. D: Appl. Phys. 35, 318 (2002) 9. R. Hodges et all, Phys. Rev. A 31, 2610 (1985)