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Republic of Iraq Ministry of Higher Education And Scientific Research University of Baghdad College of Science Dust Grain Charge Process in Negative Ion Plasma A Thesis Submitted to the Department of physics College of Science-University of Baghdad In partial Fulfillment of the Requirements for The Degree of Master of Science in Physics By Zainab Abdulla Mankhi (B. Sc. 2006) Supervised by Dr. Thamir H. khalaf January, 2012 Rab’i Al-awal, 1433 جوهىريت العراق وزارة التعلين العالي والبحث العلوي جاهعت بغداد /كليت العلىم عوليه شحي الحبيبت الغباريت في بالزها ذاث االيىى السالب رسالة هقدهة إلى قسن الفيزياء كلية العلوم – جاهعة بغداد وهي جزء هي هتطلبات ًيل درجة الواجستير في الفيزياء هي قبل زينب عبداهلل منخي (بكالىريىس ) 0226 بأشراف د .ثامر حميد خلف ربيع االول 0311, كاًوى الثاًي 2102 بِسْمِ اللّهِ الرَّحْمَنِ الرَّحِيمِ ك الَ ِع ْل َم لَ َنا َقالُو ْا ُسب َْحا َن َ ك أَ َ نت إِالَّ َما َعلَّمْ َت َنا إِ َّن َ ْال َعلِي ُم ْال َح ِكي ُم {البقرة}32/ Supervisor’s Certification We certify that this thesis was prepared by Zainab Abdullah Mankhi under our supervisionat the Physics Department, College of Science- University of Baghdad as partial requirement for the degree Master of Science in physics. Signature: Name: Dr. Thamir. H. khalaf Title: Assist Professor Address: Collage of Science University of Baghdad Date: / / 2012 In view of the available recommendation, I forward this thesis for debate by the examination committee. Signature: Name: Dr. RaadM.S.Al-haddad Title: Professor Address: Chairman of Physics Department College of Science University of Baghdad Date: / /2012 Examining Committee Certification We certify that we have read this thesis and examined “Dust Grain Charge Process in Negative Ion Plasma" and as an examining committee the student Zainab Abdullah Mankhi in its contents and in what is related with it, and in opining, it has adequate standard of the thesis of the degree of Master of Science in Physics. Signature: Signature: Name:Dr. Mahdi HadiJasim Name: Dr. KadhimAbdulwahidAadim Title: Assistant Professor Title: Assistant Professor Data: Data: / /2012 (Chairman) / /2012 (Member) Signature: Signature: Name: Dr. Khalid Abbas Yahya Name:Dr. ThamirHamidkhalaf Title: Assistant Professor Title: Assistant Professor Data: / /2012 Data: (Member) / /2012 (Supervisor) Approved by the Department of Physics / College of Science / University of Baghdad. Signature: Name: Dr. Saleh Mahdi Ali Title: Professor Dean of the College of Science. Data: / /2012 To my father’s soul, To my mother, who embraced me with her love and kindness. To my brothers and sisters, who encourage me. To my best friends, who helped me to see my success. Zainab Acknowledgements First of all, thanks to Allah are due for helping me to complete this thesis. Then, I would like to express my sincere appreciation and deep gratitude to my supervisor Dr. Thamir Hamid Khalaf for suggesting the topic of this thesis, guidance, suggestions and continuous encouragement throughout the research. My special thanks are exposed to the staff of the department of Physics in Baghdad University for their assistant and support during the years of my study and research. Finally, my thanks are also given everyone who helped me in one way or another, and who contributed in making this thesis possible particularly. I Abstract This work presents a computer studying to simulate charging process of dust grain immersed in plasma (electrons-K+ potassium ions) with negative ions ( sulfur hexafluoride ions) by basing on discrete model. In this work, the discrete model is developed to take into account effect negative ions on charging process of dust grain. The model was translated to a numerical calculation by using computer programs. The program of model has been written in FORTRAN programming language to calculate the charging process for a dust particle in a plasma with negative ion, the time distribution of a dust charge, number charge equilibrium and charging time for parameter (ratio of number density of electron to number density of positive ion) =10-1, 10-2, 10-3, 10-4, 10-5, and different grains size. The phase speed for negative ion dustacoustic wave has been calculated at different value of (ratio of number density of negative ion to number density of positive ion). The results of the work reveal that the charging of dust grains in negative ion plasma can be controlled by varying the relative fraction of negative ions in the plasma. As the negative ion density is increased in plasma, more electrons become attached by negative ion and there is a corresponding reduction in the negative current of electrons and allow the more mobile positive ions to charge the dust. Therefore, the negativity of charge number on dust grain decreases gradually to positive charge number. II The results also revealed that the effect of negative ions concentration and negative ions temperature on phase speed negative ion dust-acoustic wave. III List of Symbols a The grain radius µm D d The grain diameter Intergrain distance The electric field the electric field in the strata The electron charge the acceleration due to gravity The ion current The electron current The negative ion current The positive ion current The Boltzmann constant The dust grain mass The ion mass The electron mass The negative ion mass The number density of electron The number density of positive ion The number density of negative ion The number density of dust grain The electrostatic pressure on the surface charges The probability per unit time for electron The probability per unit time for ion The probability per unit time for negative ion The probability per unit time for positive ion The electron temperature The ion temperature The dust thermal energy The negative ion temperature The positive ion temperature µm µm Volt Volt C m/sec2 A A A A J/Ko kg kg kg kg m-3 m-3 m-3 m-3 C2/m4 e mi me Te Td IV Sec-1 Sec-1 Sec-1 Sec-1 eV eV eV eV eV Wi Wf mfp the phase speed of the dust-negative ion acoustic wave The negative ion thermal energy The ionization potential energy The work function of the dust grain material The number of charges on the surface of dust grain The number of charges of negative ion The collisional mean-free-path the dust plasma frequency the ion plasma frequency m/sec The Coulomb coupling parameter The thermal speed of the species of plasma particle z The permittivity constant for space The ratio of number density of dust grain to number density of positive ion The ratio of number density of electron to number density of positive ion The ratio of number density of negative ion to number density of positive ion Debye shielding distance The Debye lengths associated to electrons The Debye lengths associated to ions The surface charge density The scattering cross section The dust-neutral collision frequency The electron-neutral collision frequency The ion-neutral collision frequency The plasma frequency the electron plasma frequency m/sec The dust grain floating (surface) potential The secondary electron yield The charging time Volt sec V J J J µm Hz Hz farad/m µm µm µm C/m-2 m2 Hz Hz Hz Hz Hz Contents Subject Chapter One Page Introduction 1.1 Introduction 1 1.2 Dusty plasma in space 4 1.3 Basic dusty plasma characteristics 7 1.3.1 Macroscopic neutrality 7 1.3.2 Intergrain spacing 8 1.3.3 Debye length 9 1.3.4 Coulomb coupling parameter 10 1.3.5 Characteristic frequencies 10 1.4 Dust charging mechanisms 12 1.4.1 Collection of plasma particles 12 1.4.2 Secondary electron emission 13 1.4.3 Photo-detachment 15 1.4.4 Thermionic emission 1.4.5 Field emission 16 16 1.5 Production of Dusty Plasmas 17 1.5.1 Modified Q-machine 17 1.5.2 DC Discharges 19 1.5.3 RF Discharges 20 1.6 Literature review 22 1.7 Aim of the work 28 Chapter Two Theoretical Background 2.1 Introduction 29 2.2 Orbital-motion limited theory 30 2.3. Particle charging 32 2.3.1 Continuous Charging Model 33 2.3.2 Discrete Charging Model 35 2.4 The Dust-Negative Ion Acoustic Wave Chapter Three 36 Simulation and Results 3.1 Introduction 38 3.2 The Phenomenon modeling 39 3.3The Simulation 40 3.4 The program of model 42 3.5 3.3.1The Program Input Data 44 3.3.2 The Program Calculations 45 The Results 47 3.5.1 The charge dust grain fluctuations 47 3.5.2 The Time Distribution of a Dust Charge 52 3.5.3 The Equilibrium Charge Number 56 3.5.4 The dust surface potential 60 3.5.5 The Charging Time 62 3.5.6 RMS Level of Charge Fluctuation 65 3.5.7 The Dust-Negative Ion Acoustic Wave 67 3.6 Conclusions 70 3.7 Future works 71 Reference 72 CHAPTER ONE INTRODUCTION 1.1 Introduction About 80 years ago Tonks and Langmuir (1929) first coined the term „plasma‟ to describe the inner region (remote from the boundaries) of a glowing ionized gas produced by means of an electric discharge in a tube. The term plasma represents a microscopically neutral gas containing many interacting charged particles (electrons and ions) and neutrals. It is likely that 99% of the matter in our universe (in which the dust is one of the omnipresent ingredients) is in the form of a plasma. Thus, in most cases a plasma coexists with the dust particulates. These particulates may be as large as a micron. They are not neutral, but are charged either negatively or positively depending on their surrounding plasma environments. An admixture of such charged dust or macro-particles, electrons, ions and neutrals forms a“dusty plasma” [1]. Dusty plasmas are low-temperature multispecies ionized gases including electrons, ions, and negatively (or positively) charged dust grains [2]. Dust grains are massive (billions times heavier than the protons) and their sizes range from nanometers to millimeters. Dust grains may be metallic, conducting, or made of ice particulates [1]. The size and shape of dust grains will be different, unless they are man-made. Dust particles that are dispersed into plasmas for experimental studies, tend to be glass or plastic particles (melamine formaldehyde is a commonly used particle) and are spherical with a very narrow distribution of diameters. For example, a typically used particle may have a diameter of 3.50 ± 0.05 μm and a mass ~ 3×10−11 kg. Such narrowly sized particles are termed monodisperse. Some experiments used fine powders, such as aluminum silicate (kaolin) with a broad size distribution ranging from the sub-micron to tens of microns, and contain particles having laminar shapes with jagged edges [3]. However, they 1 CHAPTER ONE INTRODUCTION can be considered as point charges [1] figure (1.1.a). In such circumstances, The dust particles can be charged due to the collection of electron and ion currents from the background plasma, the grain charges negatively owing to the larger electron mobility [4, 5], photoelectric emission in the presence of a flux of sufficiently energetic ultraviolet (UV) photons, thermionic emission when the grain is heated, or secondary electron emission in the presence of higher energy ( 50 eV) electrons, dust grains acquire a positive charge. [6] In this work investigated the charging of dust in a plasma consisting of positive ions, electrons and negative ions (this is referred to a negative ion plasma). The charged dust grains can effectively collect electrons and ions from the background plasma. There has been a considerable interest in new wave modes, electrostatic potential and energy loss of charged projectiles in dusty plasmas recently and this is currently a rapidly growing area in dusty plasma physics. Numerous unique types of electrostatic and electromagnetic waves exist in dusty plasmas because of the dust charging process. For typical space and laboratory plasmas, the condition a ≪ , d is fulfilled, where a, , and d are respectively the grain radius, Debye shielding distance and the average intergrain distance. In the case where < d, the dusty plasma can be considered as a collection of isolated screened grains (which may be referred to as dust-in-plasma) whereas in the case where d < , the charged dust also participates in the screening process and therefore in the collective behavior of the ensemble (a true dusty plasma) [7]. Dusty plasmas are ubiquitous in the universe; examples are protoplanetary and solar nebulae, molecular clouds, supernova explosions, interplanetary medium (figure (1.1.b)), circumsolar rings, and asteroids. 2 CHAPTER ONE INTRODUCTION Within the solar system there are the planetary rings, cometary tails and comate [3, 8], and dust clouds on the moon. Closer to earth, are the noctilucent clouds composed of small ice particles that form in the summer polar mesosphere at an altitude of about 85 km where the temperature can dip as low as 100 K0. Dust also turns out to be common in laboratory plasmas, such as tokamaks, plasmas used in the processing of semiconductors, and even in electron storage rings. In plasmas used to manufacture semiconductor chips, dust particles are actually formed in the discharge from the reactive gases used to form the plasmas. These particles can then grow by agglomeration and accretion and eventually fall onto the semiconductor chips contaminating them, resulting in an overall significant reduction in yield [8]. Impuritycontaining plasmas are also relevant to many laboratory and technological plasmas, such as low temperature rf and dc glow discharges, rf-plasma etching and the wall region in fusion plasmas [5]. Because the positively charged dust occurs in the presence of strong ultraviolet (UV) radiation or fast electrons, plasmas with positive charged particles occur widely in space and also in the earth‟s mesosphere [9]. a b Figure (1.1) a: An SEM image of the 3±1 μm polydisperse dust used in this experiment [10]. b: The appearance of interplanetary dust particles [1]. 3 CHAPTER ONE INTRODUCTION The largest in the increase of the interest in dusty plasmas came from a completely different field - the semiconductor industry. Dust appeared to be a critical issue in the development of microelectronics. As the semiconductor industry aims at miniaturization, the contamination of the processing plasma with even very small particles became crucial. Initially, it was considered that contamination originates from external sources, but soon it was discovered that the plasma itself can create dust particles. Many efforts have been dedicated to investigate and understand the particle growth, charging and transport in plasmas [1]. In the meantime, positive aspects of the dusty plasma have been discovered. For example, the specific feature of dusty plasma to decrease the density of free electrons and, respectively, to increase their energy can be used for dust-plasma-enhanced chemical vapor deposition. Another area showing high interest in dusty plasmas is the solar cell industry. Initially, this industry (just like the microelectronics) was interested in removal of the dust, which grows in glow discharges in silane. Later, it has been shown that the incorporation of nanometer-sized dust particles in the amorphous silicon film can substantially increase the stability of the solar cell [11]. 1.2 Dusty plasma in space The attention is focused on dusty plasmas in space where they occur in a wide variety of environments. Dust is present in such diverse objects as interstellar clouds, solar system, cometary tails, planetary rings and noctilucent clouds etc. See figure (1. 2). Since charged dust grains are common in low earth orbit and in the interplanetary medium, the presence of this charged material can cause both physical damage and electrical problems for spacecraft. The charged dust particles in space plasmas may help to 4 CHAPTER ONE INTRODUCTION explain the formation of the planets, planetary rings, comet tails and nebulae. Given the variety of arenas in which a dusty plasma may play a role, it is important to understand the physical properties of this plasma system in space. The space between the stars is filled with cosmic dust and elements like hydrogen and helium which make up the “interstellar medium”[12]. Figure (1.2): Examples of dusty plasmas: (a) the Orion Nebula, (b) Halle Bop comet, (c) Saturn‟s rings, (d)fire and the soot particulate matter suspended in it. (Figures courtesy of NASA)[9] The interstellar medium is mainly made of hydrogen atoms. The density of hydrogen in interstellar space is on average about 1 atom per cubic centimeter. In the extremes, as low as 0.1 atom per cubic centimeter has been found in the space between the spiral arms and as high as 1000 atoms per cubic centimeter are known to exist near the galactic core[7]. The interstellar medium also contains cosmic dust. These particles are much bigger than hydrogen atoms. However, there are far fewer particles of cosmic dust than there are hydrogen atoms in the same volume of space. It is 5 CHAPTER ONE INTRODUCTION estimated that cosmic dust is 1000 times less common than hydrogen atoms in the interstellar medium. The dust grains in the interstellar or circumstellar clouds are dielectric (ices, silicates, etc.) and metallic (graphite, magnetite, amorphous carbons etc.) [7, 12]. Typical parameters of dust-laden plasmas in interstellar clouds are ne = 10−3–10−4 cm−3 cm−3, a 0.2 μm, nn 104 cm−3 , Te 12 , nd 10−7 ,and a/λD ≤ 0.3. The most important part of our Earth‟s environment, where the presence of charged dust particles are observed, is the polar summer mesopause located between 80 and 90 km in altitude. The most significant phenomenon observed in the polar summer mesopause is the formation of a special type of cloud known as „noctilucent clouds‟ (NLCs). Figure (1. 3). The NLCs were reported for the first time in 1885 and were, from the beginning, recognized as being different from other clouds [1]. Figure (1.3): Noctilucent clouds [Photographed by P. A. Dalin, Space Research Inst., Russia, 1999][2]. 6 CHAPTER ONE INTRODUCTION 1.3 Basic dusty plasma characteristics To understand the basic dusty plasma principles properly, it seems useful to re-examine some basic characteristics such as macroscopic neutrality, intergrain spacing, Debye length, Coulomb coupling parameter and characteristic frequencies, etc. In the following few sections:1.3.1 Macroscopic neutrality When no external disturbance is present, like electron–ion plasma a dusty plasma is also macroscopically neutral. This means that in an equilibrium with no external forces present, the net resulting electric charge in a dusty plasma is zero. Therefore, the equilibrium charge neutrality condition in a dusty plasma reads [1] where is the concentration of plasma electrons, singly charged positive ions (with charge e) and dust particles respectively, e is the magnitude of electron charge and is the amount of charge present on the dust grain surface when the grains are positively (negatively) charged with being the number of charges residing on the surface of dust grain. Note that the charge of the dust particle can vary significantly depending on plasma parameters. In studying the basic physics of dusty plasmas, the third term on the left in equation (1.1) carries very interesting implications. The presence of the dust particles in the plasma allows the formation of electric fields within the plasma, alters the local plasma potential profile, modifies the transport of particles in the plasma, modifies certain types of ion plasma waves, and introduces new dust plasma wave modes [12]. 7 CHAPTER ONE INTRODUCTION 1.3.2 Intergrain spacing A multi-component dusty plasma are composed of electrons, positively charged ions, and extremely massive charged dust grains, in a neutral background. The dust grain radius a is usually much smaller than the dusty plasma Debye length than . When the intergrain spacing d is much smaller , the charged dust particulates can be treated as massive point particles similar to multiply charged negative (or positive) ions in a multispecies plasma. Note that for dusty plasmas and the dust particles can be considered as massive point particles where the effect of neighboring particles can be significant. For dust-in-plasma , and in this situation the dust particles are completely isolated from their neighbors [7] . d a d d a a b Figure (1.4): a: The Debye length is greater than the average distance between ions. b: The Debye length is less than the average distance between the ions. 8 CHAPTER ONE INTRODUCTION 1.3.3 Debye length The Debye length is an important physical parameter in a plasma: it provides the distance over which the influence of the electric field of an individual charged particle is felt by other charged particles (such as ions) inside the plasma. The charged particles actually rearrange themselves in order to shield all electrostatic fields within a Debye distance. In dusty plasmas, the Debye length can be defined as follows [12]: √ Where √ √ and are the Debye lengths associated to electrons and ions respectively, and , , and are the electron and ion mean temperatures and densities. Dust grains of radius a, separated by a given distance d, can only be considered as individual isolated grains if the criterion is met, i.e. if the physical dimensions of the plasma are large enough for the shielding to take place. If so, considering that the electron‟s mobility is higher than that of the ions, shielding is primarily performed by electrons and equation (1.2) becomes [7]: √ 9 CHAPTER ONE INTRODUCTION 1.3.4 Coulomb coupling parameter One other important special characteristic of a dusty plasma is its Coulomb coupling parameter which is defined as the ratio of the dust potential energy to the dust thermal energy [1]. Charged dust grains can be either weakly or strong correlated depending on the strength of the Coulomb coupling parameter [2] ⁄ Where is the intergrain spacing, nd0 is the initial dust density, is the dust charge, Td is the dust thermal energy. When , the dust is strongly coupled and this condition is met in several laboratory dusty plasmas, such as dust “plasma crystals”. A dusty plasma is considered as a weakly coupled as long as [2]. 1.3.5 Characteristic frequencies A dusty plasma is macroscopically neutral, Like the usual electron-ion plasma. The disturbance of such a plasma from its equilibrium position can result in collective particle motions and hence can lead to the built up of an internal space charge field. This internal space charge field in turn will then try to restore the original space charge neutrality but due to inertia, there will be a collective oscillation of plasma particles around their equilibrium positions. These collective oscillations are characterized by the frequency of oscillation known as the plasma frequency. In order to derive an expression for the plasma frequency, the continuity equation, momentum equation and poison‟s equation for the electrons, ions and dust particles shall be taken into account. Linearization and simplification these equations results 10 CHAPTER ONE INTRODUCTION in the following expression for the plasma frequency associated with species z[1]: ∑ ∑ Where z = e for electrons, for ions and d for the dust .This can be understood in the following fashion. For the purpose of understanding, over attention is focused to the electron motion only. In this case, the internal space charge field (which is build up when the plasma particles are displaced from their equilibrium position) will try to attract electrons back to their equilibrium positions but due to inertia, the electrons will overshoot and move to the other extreme and will again be pulled back by the space charge field of opposite polarity. In this way, the electrons will continuously oscillate around their original positions with a frequency called the electron plasma frequency. A similar analogy can be true for ions and dust particles and they will oscillate around their equilibrium positions with ion plasma frequency and dust plasma frequency respectively. Since the frequency of such oscillations depends on mass, charge and number density of plasma particles, it is different for the electrons, ions and dust grains [7]. The electrons oscillate around ions with the electron plasma frequency ⁄ ⁄ , ions oscillate around the charged dust grains with the ion ⁄ plasma frequency ⁄ and dust particles oscillate around their equilibrium positions with the dust plasma frequency ⁄ ⁄ . In partially or low ionized plasma when there is a significant number of neutral particles present inside the plasma, the collisions is encountered 11 CHAPTER ONE INTRODUCTION frequent between plasma particles (electrons, ions and dust grains) and neutrals. These collisions can be characterized by collision frequencies. There are three types of collision frequencies known as electron-neutral collision frequency collision frequency frequency , ion-neutral collision frequency and dust-neutral respectively. The general expression for collision for scattering of plasma species z by the neutrals can be written as [12] Where cross section and the number density of neutral particles, √ is the scattering is the thermal speed of the species z. 1.4 Dust charging mechanisms The dust charge is an important property of dust grains since it affects the particle dynamics. The main point in dealing with the study of dusty plasmas is the understanding of the charging of dust grains once they are immersed/ introduced into the ordinary electron-ion plasmas. There are many elementary processes like the collection of plasma particles, photoemission and thermionic emission…etc. which can lead to the charging of grains. These processes could be quite complex and mainly depend on the environment around the dust grain itself. Assuming that the particles that are formed in the plasma from monomers or externally added are initially neutral, and then there exist different mechanisms for charging. They are: 1.4.1 Collection of plasma particles When a particle of solid matter is immersed in a plasma, it acquires an electric charge. The plasma particles (electrons and ions) start impinging on 12 CHAPTER ONE INTRODUCTION the surface of these newly introduced dust particles and some of them get collected on the dust grain surface. As the electrons possess much higher thermal velocities as compared to ions and therefore, the electrons will reach the dust grain surface much earlier than the ions this will make the dust grain charge and its surface potential negative [13]. On the other hand, the collections of positively charged ions tend to make the dust grain charge and its surface potential positive. These electron and ion currents are also affected by the grain surface potential. When the grain surface potential is negative, it starts repelling the electrons and attracting the ions. In other words, the current carried by the electrons is reduced while the current carried by the ions is increased and vice versa [12]. The charge on a grain of solid matter immersed in a plasma is an unknown parameter, which depends on the size of the particle and the plasma conditions. The charge is not a constant, but can fluctuate randomly, or in response to fluctuations in plasma parameters such as the electron density [14]. 1.4.2 Secondary electron emission The electrons and ions bombarding the dust particle can have an additional effect if they are very energetic. They can lead to the secondary electron emission by ionizing the dust particle material and ejecting electrons from it, the dust grain acquires positive charge. The probability for secondary electron emission depends on the energy of the bombarding particles as well as on the secondary electron yield (the average number of electrons emitted per incident ion), which in turn depends on the work function W [11].the electron and ion impact can be explained in detail as following 13 CHAPTER ONE INTRODUCTION Electron impact In case of electrons, secondary electron emission is a phenomenon that occurs when electrons impact on a dust grain surface with sufficient energy to „knock‟ additional electrons from the surface of that grain. This electron outflow can be considered as positive current onto the particle. Generally, one electron gives rise to several secondary electrons. When the electron strikes the dust grain surface, several things can happen: An electron may be scattered or reflected by the dust grain surface without penetration. It may be stopped and stick at the grain surface. If the electron penetrates the dust grain surface, it may excite other electrons which may then be emitted at the surface. Some electrons may pass through the grain and leave with a little loss of energy [7]. For plastic materials similar to the grains used in most of the experiments, high electron and ion energies are necessary for producing secondaries, and thus the contribution of the secondary electron emission to the particle charging is small (negligible) [12]. Ion impact The electron secondary emission can also be produced by ion bombardment. When the low energy ions are incident on a dust grain surface, these ions may become neutralized by the electrons tunneling from within the grain across the potential barrier [7, 12]. The energy released in this process may excite additional electrons which can then be emitted from the dust grain surface. The number of excited electrons depends on the available potential energy (after neutralization) which is determined by the ionization potential energy Wi and the work function Wf of the dust grain material. When a conduction electron is captured by the incident ion, it makes available a maximum energy of 14 CHAPTER ONE INTRODUCTION Wi − Wf. At least Wf of this must be used to free another electron from the material so that the condition for the secondary emission is Wi > 2Wf [1]. 1.4.3 Photo-detachment When photons with energies above the work function interact with the dust, electrons can be removed through the effect of photo-detachment. Many plasmas in space are exposed to intense ultraviolet radiation, for instance plasmas around young stars, and also the dusty plasma in the ionosphere. In fusion reactors there can also be significant UV fluxes. Plasma itself can also emit UV radiation, even though the intensity is relatively weak, however, commercially available UV sources are abundant, which could provide an interesting tool to control dust charge in laboratory dusty plasmas [13]. Absorption of UV radiation releases photoelectrons; hence it causes a positive charging current. Just like secondary electron emission, it can make the particle positively charged. The electron emission depends on the material properties of the particle (its photoemission efficiency). It also depends on the particle‟s surface potential, because a positively charged particle can recapture a fraction of its photoelectrons [14]. a b c Figure (1.5): Charging of dust particles in a dusty plasma takes place mainly by (a) collection of plasma particles,(b) photoemission and (c) secondary electron emission[12]. 15 CHAPTER ONE INTRODUCTION 1.4.4 Thermionic emission One of the important charging processes which charge up the dust grains positively is thermionic emission [1]. When a dust grain is heated to a high temperature, for instance by recombination of the collected charged plasma particles, the electrons and ions collected on the surface gain thermal energy. When this energy becomes larger than the binding energy, the collected particles can be emitted into the plasma. For the negatively charged particles this is most likely for the electrons, due to the repelling potential [13]. Electrons or ions may be thermionically emitted from the dust grain surface. The thermionic emission may be induced by laser heating or by thermal infrared (IR) heating or by hot filaments surrounding the dust grain [1]. In this work, the electrons and ions is low thermal energy, which collected on the surface gain. Therefore, thermionic emission is not included here. 1.4.5 Field emission Charged particles can be emitted from a surface when the local electric field is high enough. Assume a spherical particle with radius a and a surface charge density then given by charges is given by is had. The electric field at the surface is , and the electrostatic pressure on the surface , which acts outwards, against the forces binding the charges onto the surface. For metal tip field emitters, such as used in field emission microscopes, it can be as large as 1-10 V nm-1. Such strong fields then require sharp points or edges, which locally enhance the macroscopic field [13]. However, in this thesis results of particles are only presented which are assumed to be perfectly spherical, so that field emission plays no role. In 16 CHAPTER ONE INTRODUCTION many experiments, specially fabricated dust particles are used, which are spherical, or have other pre-defined shapes, but are typically very smooth. Insitu grown particles can have a different shape, for instance fractal-like. In that case, field emission might play an important role also, for the smaller particles. It results in a reduction of the number of electrons carried by the dust. 1.5 Production of Dusty Plasmas To produce/confine dusty plasmas in laboratories, a number of techniques have been developed in the last few years. Explanation of some techniques/methods was done below: 1.5.1 Modified Q-machine A simple device for producing dusty plasmas is a dusty plasma device (DPD), which is a single-ended Q-machine modified to allow the dispersal of dust grains over a portion of the cylindrical plasma column in which a potassium plasma column of ~ 6 cm diameter and ~ 1 m long is produced by surface ionization of potassium atoms from an atomic beam oven. The atoms are ionized on a tantalum surface which is heated by electron bombardment to a temperature of 2300 K0. For this The surface will be hot enough to emit large amounts of thermionic electrons which, together with the K+ ions . The plasma is radially confined by a longitudinal magnetic field of 0.3 T. The electrons and ions have roughly the same temperature of 0.2 eV at a density of 1010 cm−3 [15, 16]. The main diagnostic is a planar (2 mm diameter disk) Langmuir probe with its surface normal parallel to the magnetic field. Dust grains can be dispersed into a portion of the plasma column using a rotating cylinder described in detail by Xu et al [15] the rotating cylinder surrounds a 17 CHAPTER ONE INTRODUCTION 30 cm portion of the plasma column and is lined with aluminum wool into which dust particles are embedded. As the cylinder rotates around the plasma, dust grains fall through the plasma where they are charged by collection of electrons and ions, A schematic illustration of a DPD is shown in figure (1.6). Figure (1.6): Schematic of the negative ion dusty plasma device [17]. The dust grains were hollow glass microspheres with a relatively broad size distribution, with the majority if particles having a diameter of approximately 35 µm. A plasma containing negative ions was produced by leaking into the vacuum chamber the highly electronegative gas sulfur hexafluoride SF6 at partial pressures in the range of 10−6−10−3 Torr. The sulfur hexafluoride gas is admitted into the vacuum chamber through a variable leak valve. The attachment efficiency depends on the electron energy and is most pronounced 18 CHAPTER ONE INTRODUCTION for electrons with energies in the range of a few tenths of an eV, which coincides quite well with the electrons in the Q machine plasma. At higher electron energies, dissociation of the SF6 molecule becomes increasingly likely, leading to the formation of additional negative ion species such as and F−. For this reason the Q machine is an ideal device in which to form negative ion plasmas. In fact, it is possible to produce a negative ion plasma in which the electron concentration relative to the positive ions, ne/n+, is so small that the positive ion/negative ion plasma is had essentially [17]. 1.5.2 DC Discharges Dusty plasmas are produced by suspending micron-sized dust particles in a stratum of a dc neon glow discharge(Fortov et al 1997) .The discharge is formed in a cylindrical glass tube with cold electrodes. A 3 cm inner diameter and 60 cm long glass tube is positioned vertically. The electrodes are separated by 40 cm. The discharge current is varied from 0.4 to 2.5 mA, the pressure of neon is varied from 0.2 to 1 Torr. These conditions allow the formation of the natural standing strata in between two electrodes as shown in figure (1.7). A few grams of micron-sized particles are placed in a dust dropper in the upper side of the glass tube. The falling grains are trapped and suspended in the strata where the gravitational force acceleration due to gravity and (g is the is the electric field in the strata) [1, 18]. 19 CHAPTER ONE INTRODUCTION Figure (1.7): Schematic illustration of how dusty plasmas are produced in strata of a dc neon glow discharge (after Fortov et al 1997)[1]. 1.5.3 RF Discharges Radio-frequency (RF) discharges between parallel electrodes are the main tool of dusty plasma research because RF discharges easily tolerate impurities and they are also used in plasma processing where dustcontamination occurs. RF discharges for dusty plasma research are typically operated at 13.56 MHz at relatively low RF powers (usually <10 W) and gas pressures in the range between 1 and 100 Pa. The general setup for dust experiments in RF parallel plate discharges is shown in Fig. (1.8a). A discharge is operated between the parallel electrodes, usually the lower is RF powered and the upper is grounded. Often, the upper electrode 20 CHAPTER ONE INTRODUCTION has openings or is transparent to have optical access from top. The dust grains are then dropped into the discharge using dust containers with tiny holes. Typical dust for basic research consists of spherical plastic grains of well-defined diameter in the micrometer range (see Figure 1.8b). For micrometer particles, the dominant forces are the electric field force and gravity. A force balance is achieved in the plasma sheath above the lower electrode where the electric field is strong enough to levitate the grains against their weight. Since the electric field is increasing towards the electrode the force balance is fulfilled at a unique vertical position and the grains are confined in an effective vertical potential well (Figure 1.8c) [14]. Figure (1.8): a) Scheme of the experimental setup in a typical experiment on complex plasmas. The particles are illuminated by vertical and horizontal laser sheets. The particle motion is recorded from top and from the side with video cameras. b) Electron micrograph of the melamine-formaldehyde (MF) particles typically used in the experiments. c) Trapping of the particles in the sheath of an rf discharge [14]. 21 CHAPTER ONE INTRODUCTION 1.6 Literature review The increased interest in dusty plasmas was due to two major discoveries in very different areas: (1) the discovery by the Voyager 2 spacecraft in 1980 of the radial spokes in Saturn‟s B ring, and (2) the discovery in the early 80‟s of the dust contamination problem in semiconductor plasma processing devices. 1. Wenjun Xu et al [15] described a rotating-drum dust-dispersal device, which thy have used, in conjunction with an existing Q machine, to produce extended, steady state, magnetized plasma columns. The dusty plasma device (DPD) is to be used for the investigation of waves in dusty plasmas and of other plasma/dust aspects in 1992. 2. Chunshi Cui et al [19] studied theoretically fluctuation of charge on a dust grain in a plasma in 1994. 3. A .Braken et al [20] investigated experimentally charging of micronsized dust grains in a plasma. Dust grains were dispersed into a fully ionized, steady-state, magnetized plasma column consisting of electrons and K+ ions, both at a temperature of≈0.2 eV in 1994. 4. S. J. Choi, and m. j. Kushner [21] reported on Pseudoparticle-in-Cell (PIC)Simulation of Dust Charging and Shielding in low pressure Glow Discharges in1994. 5. Y. N. Nejoh [5] investigated the effects of the dust charge fluctuation and ion temperature on large amplitude ion-acoustic waves in a plasma with a finite population of negatively charged dust particles by numerical calculation in 1997. 6. E. Thomas and M. Watson [22] used The Fisk Plasma Source (FPS) is a plasma device operating at Fisk University Dusty plasmas in the FPS device are produced by suspending 40 µm diameter silica (SiO2) particles in an argon dc glow discharge plasma. They measured the 22 CHAPTER ONE INTRODUCTION charging of silica particles and showed that the dust particles become negatively charged with up 105 electrons in 2000. 7. Samarian et al [9] observed experimentally the trapping of dust particles in a dc abnormal glow discharge dominated by electron attachment. A dust cloud of several tens of positively charged particles was found to form in the anode sheath region. An analysis of the experimental conditions revealed that these particles were positively charged due to emission process, in contrast to most other experiments on the levitation of dust particles in gas-discharge plasmas where negatively charged particles are found. They take into account the processes of photoelectron and secondary electron emission from the particle surface in 2001. 8. S. I. Popel et al [23] considered the nonstationary problem of the evolution of perturbation and its transformation into nonlinear wave structure in dusty plasmas .They based on a set of fluid equations, Poisson‟s equation, and developed a charging equation for dust For this purpose two one-dimensional models in 2001. 9. Konstantin Ostrikov et al [24] studied accounting for the background density variation associated with electron capture and release by the dust grains. They showed that if the dust charge and density are sufficiently high, the effect of the background electron density variation on dust-charge relaxation is important. The equilibrium dust charge and its rate of variation are obtained for dusty plasmas subject to strong UV irradiation. The latter releases photoelectrons from the dust surface and can significantly affect the equilibrium dust charge, its variation rate, as well as the overall charge neutrality in the plasma in 2001. 23 CHAPTER ONE INTRODUCTION 10.In 2003, Mamun and Shukla[25] examined the role of negative ions on the charging of dust grains in plasma. They considered two models for negative ion distributions, the first is streaming negative ions, and the second is Boltzmannian negative ions. 11.M. K. Islama and Y. Nakashima[26] improved estimation in dust grain charging current in the retarding field is presented in the case of streaming dusty plasmas, where the particles streaming velocity is much larger than their thermal velocity in 2003. 12.Barbara Atamaniuk and Krzysztof Zuchowski[27] considered the influence of dust charge fluctuations on damping of the dust-ionacoustic waves. They considered Fluid approximation of longitudinal electrostatic waves in unmagnetized plasmas, and they showed that for a weak acoustic wave the attenuation depends on a phenomenological charging coefficient in 2003. 13.In 2005, A.G. Zagorodny[28] developed the kinetic theory of electromagnetic fluctuations in dusty plasmas on the basis of the microscopic description of the grain charging dynamics. The main difference of such a theory from that formulated with the use of a phenomenological assumption is that the effective charging crosssections are replaced by the k-dependent quantities describing the electron and ion absorption by grains with regard for the influence of a plasma inhomogeneity on the fluxes of absorbing particles. 14.Muhammad Shafiq[7] reported analytical results for the electrostatic response to a test charge moving through dusty plasma in his licentiate thesis. Two particular cases for a slowly moving test charge, namely, grain size distribution and grain charging dynamics are considered. Analytical results for the delayed shielding of a test charge due to 24 CHAPTER ONE INTRODUCTION dynamical grain charging in dusty plasma are also reported. In the first case, he considered a dusty plasma in thermal equilibrium and with a distribution of grain sizes. In the second case, he presents an analytical model for the shielding of a slowly moving test charge in a dusty plasma with dynamical grain charging for the both cases with and without the collision effects in2005. 15.Muhammad Shafiq reported analytical and numerical results for the electrostatic response to a test charge moving through dusty plasma in his doctoral thesis in 2006[12]. 16.Su-Hyun Kim and Robert L. Merlino[16] investigated experimentally charging of dust grains in a plasma with negative ions. When the relatively mobile electrons are attached to heavy negative ions, their tendency to charge the grains negatively is reduced. The grain charge can be reduced in magnitude nearly to zero (“decharging” or charge neutralization) in 2006. 17.Su-Hyun Kim and Robert L. Merlino[17] investigated experimentally the effect of negative ions on the charging of dust particles in a plasma. A plasma containing a very low percentage of electrons is formed in a single-ended Q machine when SF6 is admitted into the vacuum system. The relatively cold Q machine electrons (Te≈0.2 eV) readily attach to SF6 molecules to form negative ions. Calculations of the dust charge indicate that for electrons, negative ions, and positive ions of comparable temperatures, the charge of the dust can be positive if the positive ion mass is smaller than the negative ion mass and if the ratio of the electron to positive ion density, is sufficiently small in 2006. 25 CHAPTER ONE INTRODUCTION 18. Robert L. Merlino[18] studied a dusty plasma is an ionized gas containing dust particles, with sizes ranging from tens of nanometers to hundreds of microns. The interaction of the dust particles with the plasma and ambient environment results in a charging of the dust grains ,and reported applications of dusty plasmas in space, industry and the laboratory in 2006. 19.S.A. Maiorov et al [29] numerically investigated various kinetic characteristics of micron-sized dust grains in plasmas of gas discharge. They considered two-temperature stationary and moving plasma. For the simulation, they employed particle-in cell (PIC) method when a heavy macroparticle is placed in the center of the simulation Box and Newton equations are solved for the system involving also plasma particles. They simulated the process of charging of grain absorbing all electrons and ions colliding with its surface characteristics of the transitional and stationary regimes in 2007. 20.In 2007, K. Matyash et al [30] newly developed 3-dimensional Particle-Particle Particle-Mesh (P3M) code is applied to study the charging process of micrometer size dust grains confined in a capacitive RF discharge. In their plasma model, plasma particles (electrons and ions) are treated kinetically (Particle-in-Cell with Monte Carlo Collisions (PIC-MCC)), which allows to self-consistently resolve the electrostatic sheath in front of a wall. 21.I. Goertz et al [31] studied experimentally ion acoustic waves in plasmas containing dust or negative ions in 2007. 22.V.R.Ikkurthi et al [32] computed dust charge and potential on static spherical dust grains located in argon rf discharge using a threedimensional particle-particle-particle mesh code in 2008. 26 CHAPTER ONE INTRODUCTION 23.Erica K. Snipes[10] investigated experimentally thermal effects in the dispersion relations for a vertically propagating dust acoustic wave in a dc glow discharge dusty plasma. It was found that, the dust has a temperature that is well above the room temperature in 2009. 24.F. X. Bronold et al [33] proposed a surface model for the charge of a dust particle in a quiescent plasma which combines the microscopic physics at the grain boundary (sticking into and desorption from external surface states) with the macrophysics of the discharge (plasma collection fluxes). Within this model the charge and partial screening of the particle can be calculated without relying on the condition that the total electron collection flux balances on the grain surface the total ion collection flux in 2009. 25.S. Ali [34] investigated theoretically and numerically the modification in the Debye–Huckel and wake potentials due to the effects of dust relaxation rate, dust absorption frequency, dust grain radius, and negative ion temperature, and employed fluid equations to obtain the dielectric constant of the dust-negative-ion acoustic wave involving the negative ions and dust charge fluctuation effects in 2009. 26.S. S. Duha [35] investigated theoretically dust negative ion acoustic shock waves in a dusty multi-ion plasma with positive dust charging current by employing the reductive perturbation method in 2009. 27.S. Ratynskaia et al [36]carried out laboratory experiment where submicron dust was produced in a gas phase and diagnosed by surface analysis of samples and by measurements of its influence on the plasma density fluctuation spectra. Quantitative comparison of the latter with the theory yields information on dust density, size, and 27 CHAPTER ONE INTRODUCTION distribution in agreement with the results of the surface analysis in 2010. 28.S. S. Duha et al [37] investigated theoretically nonlinear dust-ionacoustic waves in a multi-ion plasma with trapped electrons in 2011. 1. 7 Aim of the work This work aims to study charging process of dust grain immersed in negative ions plasma by computing simulation and reveals the effect of negative ions concentration on the magnitude of the dust charge is reduced and a transition to positively charged dust and phase speed dust-negative ion acoustic wave in dust plasma with negative ion . It also reveals the fluctuation of the charge on the surface of grain and other related calculations. 28 CHAPTER TWO THEORETICAL BACKGROUND 2.1 Introduction When dust grains are immersed in a gaseous plasma, the plasma particles (electrons and ions) are collected by the dust grains which act as probes. The dust grains are therefore, charged by the collection of the plasma particles falling onto their surfaces. Since ions are much heavier than electrons, initially the ion current (Ii) is much smaller than the electron current (Ie), and the dust grain becomes negatively charged. This increases | | and decreases | | until| | | | . When energetic plasma particles (electrons or ions) are incident onto a dust grain surface, they are either backscattered/reflected by the dust grain or they pass through the dust grain material. During their passage, they may lose their energy partially or fully. A portion of the lost energy can go into exciting other electrons that in turn may escape from the material. The emitted electrons are known as secondary electrons. The release of these secondary electrons from the dust grain tends to make the grain surface positive. The interaction of photons incident onto the dust grain surface causes photoemission of electrons from the dust grain surface. The dust grains, which emit photoelectrons, may become positively charged. The emitted electrons collide with other dust grains and are captured by some of these grains which may become negatively charged [1, 25]. The charging of dust grains in a plasma consisting of positive ions, negative ions and electrons. In typical laboratory plasmas containing electrons and positive ions, dust grains acquire a negative charge. In negative ion plasmas, charging due to the negative ions, in addition to positive ions and electrons, must be taken into account. 29 CHAPTER TWO THEORETICAL BACKGROUND A number of theoretical and experimental investigations have carried out for understanding the charging of dust grains in a plasma under different conditions [25]. 2.2 Orbital-motion limited theory Most theories for predicting the charge of a dust grain in a plasma were originally developed to model electrostatic probes in plasmas. A dust grain is just a solid object immersed in plasma. One can view the dust particle as essentially a small probe, except that the dust grain has no wires connected to it. The starting point of these theories is a prediction of the electron and ion currents to the probe. The currents are termed “orbitlimited” when the condition a ≪ D ≪ mfp applies, where a is the particle radius, D is Debye length, and ¸mfp is a collisional mean-free-path between neutral gas atoms and either electrons or ions. In that case, the currents are calculated by assuming that the electrons and ions are collected if their collisionless orbits intersect the probe’s surface [14, 38]. In this work the charging of dust is investigated in plasma consisting of positive ions, electrons and negative ions (this plasma is called a negative ion plasma). a. The dust grain charge:Consider an isolated spherical dust grain of radius a introduced into a plasma consisting of electrons of density ne, singly charged positive ions of density n+, and singly charged negative ions of density n−. Define 30 CHAPTER TWO THEORETICAL BACKGROUND …………………….. (2.1) As the fraction of negative ions relative to positive ions. Using the charge neutrality condition [16] ………………… (2.2) We have that ………………………… (2.3) Analytic models including the OML model typically assume that the particle is spherical, and its surface is an equipotential. In this case, even if the particle is not made of a conductive material, it can be modeled as a capacitor [14]. The charge is then related to the particle’s surface potential as, with respect to a plasma potential of zero, by ……………………………… (2.4) Where a is the radius of the dust particle, and s is the dust grain surface potential relative to the plasma potential. [17]. b. Currents to the dust grain:For the collection of Maxwellian electrons and ions, characterized by temperatures Te and Ti, the orbit-limited the electron and positive ion currents to the isolated spherical dust grain of radius (a) are given by [16]: { …….. (2.5) 31 CHAPTER TWO THEORETICAL BACKGROUND { ……. (2.6) The negative ion current participates in the charging of a dust grain in a plasma is [25]: { ……. (2.7) The intial currents Ie0 , I-o and I+0 represent the current that is collected for s = 0, and are given by[16] ( ) The temperatures of the positive ions, electrons and negative ions are T+, Te and T-, respectively. nj is the number density of plasma species j(the positive ions, electrons and negative ions) [16]. The grain surface potential is then obtained by requiring this condition [17]:- 2.3 Particle charging A grain of solid matter acquires an electric charge, if it is immersed in plasma. This charge is in many cases, the reason that the particle is interesting. It is therefore of great interest to know how large the charge is. Ordinary plasmas consisting of only electrons and ions are complicated enough, but at least a physicist can trust that the charge of the constituents is known. For a dusty plasma, one cannot trust even that. In 32 CHAPTER TWO THEORETICAL BACKGROUND general, the charge on a particle of solid matter immersed in a plasma is an unknown parameter, which depends on the size of the particle and the plasma conditions. The charge is not a constant, but can fluctuate randomly, or in response to fluctuations in plasma parameters such as the electron density. To estimate the charge of a grain, there are several theoretical models and some experimental methods as well. In general, none of them yields a result with perfect precision. Here the theoretical models of charging will be considered, which in general are useful for estimating the charge with an accuracy of about a factor of two. These models will also be useful for gaining a conceptual understanding of how the charge varies with plasma parameters, and how it can vary in time [14]. There are some models, often implemented numerically to calculate the charge and potential of grain in a plasma, as described below. 2.3.1 Continuous Charging Model A dust grain with zero charge that is immersed in plasma will gradually charge up, by collecting electron and ions currents, according to[19] ∑ The currents are continuous quantities, and the dust particle’s charge Qd is allowed to vary smoothly, rather than in integer multiples of the electronic charge. To find the equilibrium, one can set in Eq. (2.10). This yields the steady-state potential fl and steady-state charge 〈 〈 〈 〉 〉⁄ 33 〉. CHAPTER TWO THEORETICAL BACKGROUND Where the coefficients and are functions of Ti/Te and mi/me, and the ion flow velocity, and they must be determined numerically. Useful values for these coefficients are listed in table 2.1 for cases with no ion flow. The charging time indicates how rapidly a particle’s charge can vary, when plasma conditions vary. One way of defining a charging time is the ratio of the equilibrium charge and one of the currents, electron or ion, collected during equilibrium conditions. Another definition assumes that hypothetically the particle has no charge and is suddenly immersed in a plasma with conditions that remain steady, so that the grain’s charge gradually varies from zero toward its equilibrium value; in this case the charging time has been defined as the time required for a grain’s charge to reach a fraction ( ) of its equilibrium value. The charging time varies inversely with plasma density and grain size, according to [14] √ Where for a non-drifting plasma K is a function of Ti/Te and mi/me. The fact that is inversely proportional to both a and ni means that the fastest charging occurs for large particles and high plasma densities [14]. Values of the constant K are summarized in table 2.1. Table (2 .1): Coefficients for fl , Q and appearing in Equations (2.11), (2.12) and (2.13). These values were found by a numerical solution of the continuous charging model, assuming non-drifting Maxwellians and no electron emission [19]. Ti/Te 0.05 1 0.05 1 34 CHAPTER TWO THEORETICAL BACKGROUND 2.1.2 Discrete Charging Model Continuous charging model neglects the fact that the electron and ion currents collected by the grain actually consist of individual electrons and ions. Therefore a charging model developed that includes the effect of discrete charges. The charge on the grain is an integer multiple of the electron charge, Qd = Ne, where N changes by -1 when an electron is collected and by zi when an ion is absorbed. Electrons and ions arrive at the particle’s surface at random times, like shot noise. The charge on a particle will fluctuate in discrete steps (and at random times) about the steady-state value〈 〉 [14, 21]. There are two key aspects of the collection of discrete of plasma particles (the term “plasma particle” is to refer to either electron or ions). First is that the time interval between the absorption of plasma particles varies randomly. Second is that the sequence in which electrons and ions arrive at the grain surface is random. But neither of these is purely random; they obey probabilities that depend on the grain potential s. Let us define pe(s) and pi(s) as the probability per unit time for absorbing an electron or ion, respectively. As the grain potential becomes more positive, more ions will be repelled and more electrons will be attracted to the grain, so pi should decrease with s and pe should increase. pj(s) (j refers to the ions, electrons) is calculated from the OML currents Ij(s), 35 CHAPTER TWO THEORETICAL BACKGROUND This equation is the key to developing the discrete charging model. Basically, it converts the OML currents into probabilities per unit time of collecting particles. This relates the discrete charging model with its probabilities to the continuous charging model with its currents. The total probability per unit time of collecting plasma particle is [19] ∑ The currents Ij depend on the grain surface potentials, so ptot also depends on s and hence on charge Qd. This assumption retains an important part, but not all, of the physics arising from the discreteness of the charge carriers. The discrete nature of an electron or ion is recognized when it is absorbed from the plasma by the grain, but not when it remains in the Debye sheath surrounding the grain. This is equivalent to treating the plasma with a continuum model that is characterized by the currents, Ij [19]. 2.4 The Dust-Negative Ion Acoustic Wave A dusty multi-ion plasma system consisting of electrons, light positive ions, negative ions, and extremely massive (few micron size) charge fluctuating stationary dust have been considered. The electrostatic waves associated with negative ion dynamics and dust grain charge fluctuation. The equilibrium state of the dusty multi-ion plasma system under consideration is defined as [35]: ⁄ Where is the dust grain charge at equilibrium. When electron and ion currents at equilibrium, it is noted here that in order to have a nonzero 36 CHAPTER TWO THEORETICAL BACKGROUND , | |⁄ negative ion current, i.e., ⁄ it must be had which reduces to ,where[37] √ In which | | √ , ⁄ , ⁄ , and . The linear dispersion relation for the ion acoustic waves associated with negative ions, which are significantly modified by the presence of the charge fluctuating stationary dust is [37] Where mn is the , negative , | | , T- is the negative ion thermal energy, ion mass, , , , , [35]. If no dust (ηd=0) and cold negative , and ion (T-=0) limits, the phase speed of this wave is equal to[37] √ ⁄ This means that the DNIA (Dust-Negative Ion Acoustic) waves are associated with dynamics of negative ions, where the inertia comes from the mass of the negative ions and restoring force is provided by the thermal pressures of electrons and light ions [37]. 37 CHAPTER THREE 3.1 SIMULATION AND RESULTS Introduction In recent years computer simulations are playing an important role in theoretical investigations in various branches of human activities. Similarly is the situation in the research of dusty plasma that is interesting not only for astronomers (interstellar clouds, comet tails etc.) but also in for finding the place the complicated technological processes like powder modification, plasma etching of semiconductor devices and plasma diagnostic. The understanding of processes like charging and dynamics of dusty particles is necessary for the effective development of technological devices. In this work, the discrete charging module have been employed in order to simulate the dust charge on spherical dust grains in plasma consisting of positive ions (K+ potassium ions), electrons and negative ions ( sulfur hexafluoride ions), for this plasma is called a negative ion plasma. The computation of dust charges dates back to earliest probe theories, Probe theories calculate the current to an electrostatic probe as a function of probe potential and probe shape. The floating potential is derived as the point where ion and electron currents balance. First probe theories based on orbit motion limited (OML). Later, Probe theory has been applied to dust charging. 38 CHAPTER THREE SIMULATION AND RESULTS 3.2 The Phenomenon modeling This model of charging is considered to be the development for discrete model that includes the effect of negative ion on the charging process of dust grain in a plasma negative ion instead of plasma electron-ion. The model will be useful for gaining a conceptual understanding of how the charge varies with plasma negative ion parameters, and how it can vary in time, which in general is useful for estimating the charge of dust grain. The model has described the charging process of an isolated dust grain immersed in a negative ion plasma and assumed a spherical grain with radius a which initially uncharged under the condition the particle radius, is Debye length, and ¸ , where a is is a collisional mean-free- path between neutral gas atoms and either electrons or ions In this case. The charging process is characterized by: 1. It is based on the assumption that the plasma particles arrive to grain surface at random time intervals , which is not fixed 2. The probabilities of arriving electrons or ions (negative or positive) in equations (2.14) depend on the surface potential of the dust grain. 3. The total probability per unit time of collecting plasma particle is calculated from equation (2.15) 4. The time interval depends on the potential of the grain and the random number R1 that we generated. 5. The model assumes that plasma particles (electron, positive ion, or negative ion) arrive in a random sequence in consistent with the probabilities. 39 CHAPTER THREE SIMULATION AND RESULTS 6. To recognize the plasma particle type electron or ion (negative or positive), it must compare the probability with another random number R2. 7. The charge of the dust grain would be changed after each electron or ion (negative or positive) collection, and it is increased or decreased by one charge. 3.3 The Simulation Our simulation converts the physical discrete charging model to program which simulates the charging process of a dust grain immersed in plasma with negative ion. At first the dust grain would be uncharged so the experiment starts with a zero charge at a time step equal zero where j refers to plasma particle electron, negative ion or positive ion, then the two steps will be repeated for plasma particles which will fall on the grain. A. First Step: Choose a Random Time Interval This step is based on the physical discrete charging model, which assumes that the plasma particles arrive at random time intervals, there will be one time step per particle that is collected and it corresponds to: ………………………………….. (3-1) The currents must be calculated from equations (2-5, 2-6, and 2-7) that are predicted by the OML theory to find the probabilities. 40 CHAPTER THREE SIMULATION AND RESULTS The random time step collecting a plasma particle depends on the probability per unit time of , , and the total probability is given in equation (2-15). The probability of collecting a plasma particle is [19]: ……………………….. (3-2) To calculate the random time interval one must generate a random number R1 where and equate it to the previous equation of probability to yield [19]: ……………………….. (3-3) B. Second Step: Choose Electron, Negative ion or Positive ion The plasma particle arrives in a random sequence. Generate a random number R2 to determine whether the next collected particle is an electron or an ion (negative or positive), where . Probability that the next particle is electron, negative ion or positive ion will be i. If and compared with R2 as follows: then, the charge will be process is electron collection. However, at state that means the that means process isn’t electron collection. The probability of other particle must be examined. ii. If then, the charge will be the process is negative ion collection. 41 that means CHAPTER THREE iii. If SIMULATION AND RESULTS then, the charge will be that means the process is positive ion collection. 3.4 The program of model The model was translated to a numerical calculation by using computer programs. The program has been written with FORTRAN programming language to simulate computer experiment of the charging process for a dust grain in negative ion plasma. the discrete charging model is employed in this simulation to calculate statistical fluctuations such as the time distribution of a dust charge, number charge equilibrium and charging time for different value of (ratio of number density of electron to number density of positive ion) and different grains size, and also the phase velocity negative ion dust acoustic wave has been calculated for different value of (ratio of number density of negative ion to number density of positive ion). The flow chart of program is illustrated in figure (3.1) 42 CHAPTER THREE SIMULATION AND RESULTS Start tj=0,Qj=0 Calculate j, Random no.R1, Calculate p, Calculate ∆tj, Calculate Ie, I-, I+ Random no.R2 Kind of particle Electron Negative ion No Done for enough time Positive ion Yes Calculate fluctuations Q(t) Calculate fluctuations statistics Calculate the phase speed DNIA wave Stop Figure (3.1): Flow chart of the program 43 CHAPTER THREE SIMULATION AND RESULTS 3.4.1 The Program Input Data The results of program are computed from the electron, positive ion and negative ion currents from the orbital motion limited theory from equations (2.5), (2.6) and (2.7) in chapter two, and electric potential of dust particle from equation (2.4). For all these calculations the input data are: 1. Positive ions (K+ potassium ions) mass m+= 39 amu, negative ions ( sulfur hexafluoride ions) mass m-= 146 amu. 2. The electron temperature (Te), negative ion temperature (T-), and positive ion temperature (T+) equal to 0.2 eV. 3. The number density of the plasma n=1016 m-3. 4. The number density of the grain nd=103 m-3. 5. The ratio of number density of negative ion to number density of positive ion (ηn) can be changed from 0 to 10-1. 6. A spherical dust grain is assumed with diameter d that can be changed from 0.1-10 µm. 7. The charging process starts with an isolated and uncharged grain so initially the charge number N=0 on the grain surface. 8. The time required to calculate the charge from zero to the suitable time that we choose, called the experiment time. 9. Some of a well-known physical constants are: =9.109*10-31 Kg. a. The electron mass is b. The electron charge=1.602*10-19C. c. The permittivity constant for space d. Boltzmann constant KB=1.38*10-23 J/Ko. 44 =8.854*10-12 farad/m. CHAPTER THREE SIMULATION AND RESULTS 3.4.2 The Program Calculations The results of program are a sequence of the calculations process which is done according to the following steps (subroutines): a. The Charge Fluctuations on Dust Grain The first output data of program give a picture about the charge fluctuation on dust grain when it is immersed in plasma with negative ion. The data represented that charge on the grain is an integer multiple of the electron charge at random times b. The fluctuations statistics 1. The Histogram It indicates the fraction of dust particle having a certain charge at limited time, by using the output data of the first subroutine, it can determine the charge distributions from the time series by making a histogram of the time spent at each charge level, and the peak is called level balance. 2. The Equilibrium Charge Number The charge Q on a dust grain is related to its surface (or floating) potential . (relative to the plasma potential) by , where a is the radius of the (spherical) grain. The surface potential of a dust particle in a negative ion plasma is determined by balancing the currents due to positive ions, negative ions, and electrons. The charge number (N=Q/e) on a dust particle at balance level is called the charge number equilibrium. It can be determined by using the output data of the histogram subroutine. 45 CHAPTER THREE SIMULATION AND RESULTS 3. The charging time The particle has no charge and is suddenly immersed in a plasma with conditions that remain steady, so that the particle’s charge gradually varies from zero toward its equilibrium value; in this case the charging time has been defined as the time required for a particle’s charge to reach to equilibrium value. The charging time can be determined by using the output data of the first and the Equilibrium charge number subroutines. 4. RMS Fluctuation Level The root mean square level calculates the amplitude of the fluctuations. By using the time series N(t) from first subroutine, we can get Q(t) then find ∆Q and normalized it by the equilibrium charge 〈 〉,to find the root mean square level 〈 〉 .RMS reveals simple power law relation[19]. 〈 〉 |〈 〉| ⁄ ………. (3-4) c. The Phase velocity Dust-Negative Ion Acoustic Wave We can calculate the phase velocity dust-negative ion acoustic wave is given in equation (2-18) by using the output data of the charge number equilibrium subroutine and studying the different parameters effect on the phase speed. 46 CHAPTER THREE 3.5 SIMULATION AND RESULTS The Results The results of the simulation to study the charging of dust grain immersed in plasma with negative ion and dust-ion acoustic wave, the results presented as the same sequence of the subroutines with grouping them according to the effect of parameters such as number density of negative ion and grain size. 3.5.1 The charge dust grain fluctuations For the comparison purpose, our simulation employed to show the charging process in an electron grain in this plasma (e- ion plasma. The presence of the dust ion) leads to charging the dust negatively because the mobility of electrons larger than the mobility of ions .The charge on the grain will reach the equilibrium state in which the charge Q will fluctuate around the equilibrium charge<Q>. Figure(3.1) showes the chraging process for a dust grain by collecting electrons, and positive ions from plasma with out negative ion, notes that the range of the charge fluctutions between -35 and -20. Calculations show the chraging process for a dust grain with dimeter = 0.1µm immersed in K+ plasma if a significant fraction of the electrons are attached to negative ions; the magnitude of the charge on the dust particles is reduced. If the ratio ηe= ne/n+ of the electron density to positive ion density is sufficiently small and the positive ions are lighter than the negative ions, then the dust charge can be positive. The ions and electrons have equal temperatures T+ = Te =T-= 0.2 eV. 47 CHAPTER THREE SIMULATION AND RESULTS Negative ion plasma is formed by attachment of electrons on the highly electronegative sulfur hexafluoride SF6 molecule by the reaction When the SF6 density is added into K+ plasma, some electrons become attached to form ions and there is a corresponding reduction in the negative current due to the fact that the ions are considerably less mobile than the electrons, as Figure (3.2) shows that the range of the charge fluctutions is between -25 and -5 and the range drifts towards the positive comparison with Figure (3.1). When the SF6 density is increased in K+ plasma, more electrons become attached to form ions and there is a corresponding reduction in the negative current of electrons. Therefore, the negativity of charge number on dust grain decreases gradually to positive charge number. Figures (3.3), (3.4), (3.5), and (3.6) show that the range of the charge fluctuations is about (-8 –4), (-6 – 6), (-2 – 8), and (-2–10) respectivly. 48 CHAPTER THREE SIMULATION AND RESULTS 0 D=0.1µm Charge Number(N=Q/e) -5 ηe =1 -10 -15 -20 -25 -30 -35 -40 0.0E+0 1.0E-3 2.0E-3 3.0E-3 Time(Sec) 4.0E-3 5.0E-3 6.0E-3 Figure (3. 1): Charge number on surface grain as a function of time when D=0.1µm, ηe =1 (no negative ion) 0 D=0.1µm ηe=10-1 Charge Number(N=Q/e) -5 -10 -15 -20 -25 -30 0.0E+0 1.0E-3 2.0E-3 3.0E-3 Time(Sec) 4.0E-3 5.0E-3 6.0E-3 Figure (3.2): Charge number on surface grain as a function of time when D=0.1µm, ηe=10-1 49 CHAPTER THREE SIMULATION AND RESULTS 10 D=0.1µm 8 ηe=10-2 Charge Number(Sec) 6 4 2 0 -2 -4 -6 -8 -10 0.0E+0 1.0E-3 2.0E-3 3.0E-3 Time(Sec) 4.0E-3 5.0E-3 6.0E-3 Figure (3.3): Charge number on surface grain as a function of time when D=0.1µm, ηe=10-2 8 D=0.1µm ηe=10-3 6 Charge Number(N=Q/e) 4 2 0 -2 -4 -6 -8 0.0E+0 1.0E-3 2.0E-3 3.0E-3 Time(Sec) 4.0E-3 5.0E-3 6.0E-3 Figure (3.4): Charge number on surface grain as a function of time when D=0.1µm, ηe=10-3 50 CHAPTER THREE SIMULATION AND RESULTS 14 D=0.1µm 12 ηe=10-4 Charge Number(N=Q/e) 10 8 6 4 2 0 -2 -4 0.0E+0 1.0E-3 2.0E-3 3.0E-3 Time(Sec) 4.0E-3 5.0E-3 6.0E-3 Figure (3.5): Charge number on surface grain as a function of time when D=0.1µm, ηe=10-4 12 D=0.1µm ηe=10-5 10 Charge Number(N=Q/e) 8 6 4 2 0 -2 -4 0.0E+0 1.0E-3 2.0E-3 3.0E-3 Time(Sec) 4.0E-3 5.0E-3 6.0E-3 Figure (3.6): Charge number on surface grain as a function of time when D=0.1µm, ηe=10-5 51 CHAPTER THREE SIMULATION AND RESULTS 3.5.2 The Time Distribution of The grain Charge After the collection of charges by dust grain, these charges will approach the equilibrium value <Q> and the probabilities for collecting electrons, negative ions, and positive ions are less unequal so the charge will always fluctuate around the equilibrium value. The charge distributions are determined from the time series by making histogram of time spent at each charge level to calculate charge equilibrium value, the equilibrium charge number takes larger time from the computer experiment time. Figures (3.7), (3.8), (3.9), (3.10), (3.11), and (3.12) show distribution functions for each case in section 3.5.1. In figure (3.7) the chraging process for a dust grain by collecting electrons and positive ions (K+) from plasma. Ions are much heavier than electrons. Therefore, the dust grain becomes negatively charged. The equilibrium charge number is -29 because this level takes longer time compared with the other levels. When the SF6 density is added into K+ plasma, some electrons become attached to form ions and ηe=10-1, the negativity of charge number on dust grain decreases and The equilibrium charge number becomes -12. See figure (3.8). If the SF6 density is increased in K+ plasma so as to ηe=10-2, the equilibrium charge number becomes -1 as in the figure (3.9). 52 CHAPTER THREE SIMULATION AND RESULTS 8.0E-4 D=0.1µm 7.0E-4 ηe=1 Charge Distribution(Sec) 6.0E-4 5.0E-4 4.0E-4 3.0E-4 2.0E-4 1.0E-4 0.0E+0 -20 -21 -22 -23 -24 -25 -26 -27 -28 -29 -30 -31 -32 -33 -34 -35 -36 Charge Number Figure (3.7): Charge distribution function for grain of D=0.1µm, ηe=1 (no negative ion). The equilibrium charge number is=-29 1.4E-3 D=0.1µm ηe=10-1 Charge DIistribution 1.2E-3 1.0E-3 8.0E-4 6.0E-4 4.0E-4 2.0E-4 0.0E+0 -6 -7 -8 -6 -9 -10 -11 -12 -13 -14 -15 -16 -17 -18 -19 -20 -21 -22 -23 -24 Charge Number Figure (3.8): Charge distribution function for grain of D=0.1µm, ηe=10-1.The equilibrium charge number is=-12. 53 CHAPTER THREE SIMULATION AND RESULTS 2.5E-3 D=0.1µm ηe=10-2 Charge Distribution(Sec) 2.0E-3 1.5E-3 1.0E-3 5.0E-4 0.0E+0 0 -1 -2 1 2 -3 -4 -5 -6 -7 3 4 5 -8 -9 6 7 Charge Number Figure (3.9): Charge distribution function for grain of D=0.1µm, ηe =10-2.The equilibrium charge number is=-1. In this state, the ratio of number density of electrons to number density of positive ions equals 10-3, the charge number on dust grain becomes positive and equals one that is to say the positive current dominates on charging process of dust grain because the positive ions are lighter than the negative ions and number density of electrons is sufficiently small. See figure (3.10). The positively of charge on dust grain is increased .Whenever, the ratio of number density of electron to number density of positive ion is decreased as figure (3.11) shows the charge number equilibrium becomes three when the ratio of number density of electron to number density of positive ion (ηe) equals 10-4. But figure (3.12) shows the charge number equilibrium remains constant when the ratio of number density of electron to number density of positive ion (ηe) equals 10-5 because the main effect of electron is neglected. 54 CHAPTER THREE SIMULATION AND RESULTS 4.5E-3 D=0.1µm 4.0E-3 ηe=10-3 Charge Distribution(Sec) 3.5E-3 3.0E-3 2.5E-3 2.0E-3 1.5E-3 1.0E-3 5.0E-4 0.0E+0 0 1 2 -1 -2 -3 -4 3 4 5 -5 -6 6 Charge Number Figure (3.10): Charge distribution function for grain of D=0.1µm, ηe =10-3.The equilibrium charge number is=1 2.5E-3 D=0.1µm ηe=10-4 Charge DIistribution(Sec) 2.0E-3 1.5E-3 1.0E-3 5.0E-4 0.0E+0 0 -1 1 2 3 4 5 6 -2 -3 7 8 9 10 11 Charge Number Figure (3.11): Charge distribution function for grain of D=0.1µm, ηe =10-4.The equilibrium charge number is=3 55 CHAPTER THREE SIMULATION AND RESULTS 2.5E-3 D=0.1µm ηe=10-5 Charge Distribution(N=Q/e) 2.0E-3 1.5E-3 1.0E-3 5.0E-4 0.0E+0 0 -1 1 2 3 4 5 6 -2 -3 7 8 9 10 Charge Number Figure (3.12): Charge distribution function for grain of D=0.1µm, ηe =10-5.The equilibrium charge number is=3. 3.5.3 The Equilibrium Charge Number The charges on grain approach the equilibrium value 〈 〉, after the collection of charges by dust grain, The charge on a grain will fluctuate in discrete steps (and at random times) about the steady-state value〈 〉 ,but the continues model neglects the fact that the electron and ion currents collected by the grain that actually consists of individual electrons and ions. a. Effect of Parameter ηe on the equilibrium charge number A plot of the equilibrium charge number on dust ( for the parameter ) as a function for the case in which the positive ion is potassium and the negative ion is as shown in figure (3.13) for dust grain diameter equals 0.1µm. Notice that the charge on the dust is reduced as the parameter ηe increased, and the dust surface charge can be positive. 56 CHAPTER THREE SIMULATION AND RESULTS 4 Charge Number Equilibrium 2 0 1.0E-5 -2 1.0E-4 1.0E-3 1.0E-2 1.0E-1 1.0E+0 -4 -6 -8 -10 -12 -14 ηe=ne/n+ Figure (3.13): the equilibrium charge Number grain as a function the parameter ηe when D=0.1µm. When the relation between equilibrium charge number and parameter is plotted for different dust grain diameters, this relation takes same behavior (as in figures (3.14) and (3.15)) but the charge number equilibrium increases when grain size increases. 57 CHAPTER THREE SIMULATION AND RESULTS 40 Charge Number Equilibrium 20 0 1.0E-5 -20 1.0E-4 1.0E-3 1.0E-2 1.0E-1 1.0E+0 -40 -60 -80 -100 -120 -140 -160 ηe=ne/n+ Figure (3.14): the equilibrium charge number grain as a function of the parameter ηe when D=1µm. 400 Charge Number Equilibrium 200 0 1.0E-5 -200 1.0E-4 1.0E-3 1.0E-2 1.0E-1 1.0E+0 -400 -600 -800 -1000 -1200 -1400 -1600 ηe=ne/n+ Figure (3.15): the equilibrium charge number grain as a function of the parameter ηe when D=10µm. 58 CHAPTER THREE SIMULATION AND RESULTS b. The Effect of Grain Size on the equilibrium charge number The grain size is an important parameter that effects on the charge collected by dust grain. Figure (3.16) shows the equilibrium charge number as a function of grain size for different value of parameter ηe and = = =0.2eV. The surface charge has been determined by the computer simulation for various diameter of spherical grains that lead to increase dust surface area exposed to plasma, so the collection of electrons, negative ions, and positive ions currents become large and equilibrium charge number on the dust grain are also large. These results are in agreement with the equation (2.4) in chapter two, the relation between the grain charge and radius is linear. This figure notes that the change of equilibrium charge number is slowly as a function grain size when ηe =10-3,10-4, and 10-5 because the positive and the negative currents dominate on charging process of dust grain and both the negative and positive ions is heavier than electron while the electron and positive ions currents dominate on charging process of dust grain when ηe =10-1, and 10-2 .Therefore, the change of equilibrium charge number is rapidly as a function grain size. 59 CHAPTER THREE SIMULATION AND RESULTS ηe=1.00E-1 ηe=1.00E-2 ηe=1.00E-3 ηe=1.00E-4 ηe=1.00E-5 400 200 Charge Number Equilibrium 0 -200 0 2 4 6 8 10 12 -400 -600 -800 -1000 -1200 -1400 -1600 diameter (µm) Figure (3.16): The charge number equilibrium as a function of grain diameter when ηe -1 =10 , 10-2,10-3,10-4,and 10-5 respectively. 3.5.4 The dust surface potential When the dust is charged by the collection of the plasma particles flowing onto it surface, it acquires surface potential, this potential depends on the charge that acquired by grain surface according to equation (2.4). The dust surface potential ( parameter ) is plotted as a function for the for the case in which the positive ion is potassium the negative ion is and for different size of grins as in Fig. (3.17). Notice that the positive ion is the lighter species. Thus, in the presence of a heavy (compared to the positive ion) negative ion, the charge on the dust is reduced, and the dust surface potential can be positive. Where the positive ion, negative ion, and electron are at the same temperatures and equal to 0.2 eV. 60 CHAPTER THREE SIMULATION AND RESULTS These results are in agreement with the experimental results of Robert Merlino et al (2006) [17]. D=0.1µm D=1µm D=10µm 0.1 potential on Dust Grian (V) 0.05 0 1.0E-5 -0.05 1.0E-4 1.0E-3 1.0E-2 1.0E-1 1.0E+0 -0.1 -0.15 -0.2 -0.25 -0.3 -0.35 -0.4 -0.45 -0.5 Figure (3.17): The dust surface potential of electrons in the plasma. T+ = Te = T-. ηe=n-/n+ as a function for the fractional concentration Figure (3.18): Difference between the probe floating potential and plasma space potential, . for various SF6 pressures (the experimental results of Robert Merlino et al (2006))[17]. 61 CHAPTER THREE SIMULATION AND RESULTS 3.5.5 The Charging Time a. The effect of Parameter ηe on the charging time From the results of computer simulation, the effect of negative ions can be studied when added to plasma on charging time of grain. Figure (3.19) shows the charging time of grain as a function of parameter ηe. Notice that the charging time decreases when the number density of electrons reduces from ηe= 10-1 to 10-2 because the negativity of equilibrium charge on dust grain decreases gradually. Therefore, the time is needed to reach the equilibrium charge number decreases to equilibrium charge become-1. Hence, the charging time is trivial when the parameter ηe equals 10-2. When the parameter ηe equals 10-3 , the positive ions current dominates on charging process of dust grain .Therefor, the equilibrium charge becomes positive but has a little value and equals one. Hence, the charging time is trivial. Whenever the positivity of equilibrium charge on dust grain increases gradually, the charging time also increases when the value ηe changes from10-3 to 10-4. But, when ηe changes from 10-4 to 10-5, the charging time becomes constant because the equilibrium charge number is constant. From this figure, it can be concluded the charging time is proportional with the absolute value of equilibrium charge number. 62 CHAPTER THREE SIMULATION AND RESULTS 6.E-5 Charging Time (Sec) 5.E-5 4.E-5 3.E-5 2.E-5 1.E-5 0.E+0 1.0E-5 1.0E-4 1.0E-3 ηe= ne /n+ 1.0E-2 1.0E-1 Figure (3.19): The charging time as a function of the parameter ηe when D=0.1µm. Figure (3.20) shows the charging time of lager grain (D=1µm) as a function parameter ηe. It can be seen from this figure that the charging time decreases for all the values of parameter ηe. 2.E-5 2.E-5 Charging Time (Sec) 1.E-5 1.E-5 1.E-5 8.E-6 6.E-6 4.E-6 2.E-6 0.E+0 1.0E-5 1.0E-4 1.0E-3 ηe =ne /n+ 1.0E-2 Figure (3.20): The charging time as a function of the parameter ηn when D=1µm. 63 1.0E-1 CHAPTER THREE SIMULATION AND RESULTS Whenever the grain size increases, the charging time decreases for all value of parameter ηe and also the difference in the charging time becomes very simple.as in figure (3.21). 1.6E-6 Charging Time (Sec) 1.4E-6 1.2E-6 1.0E-6 8.0E-7 6.0E-7 4.0E-7 2.0E-7 0.0E+0 1.0E-5 1.0E-4 1.0E-3 ηe=ne/n+ 1.0E-2 1.0E-1 Figure (3.21): The charging time as a function of the parameter ηe when D=10µm. b. The Grain Size Effect on the charging time The charging time is the time required for a grain’s charge to reach its equilibrium value that is inversely proportional with dust grain size as in equation (2.13). Figure (3.22) reveals that the charging time as a function of grain diameter for different value of parameter ηe and Te=T-=T+=0.2eV.Notce in this figure, the relation between the charging time and dust grain size is inversely proportional when ηe = 10-1, 10-4, and 10-5 because the dust surface area exposed to plasma increases, so that the collection of electrons and ions currents become large. But the value of ηe = 10-2 and behavior of diameter =0.1 µm is irregular behavior because the grain reaches equilibrium state at the first electron collects on the grain. Therefore, the charging time is trivial, 64 CHAPTER THREE SIMULATION AND RESULTS also the value of ηe = 10-3 and diameter =0.1 µm is irregular behavior, when the first positive ion collects on the grain, the grain reaches equilibrium state and charge equilibrium of this grain equals 1. 5.0E-5 1.00E-01 1.00E-02 4.5E-5 1.00E-03 1.00E-04 4.0E-5 1.00E-05 Charging Time (Sec) 3.5E-5 3.0E-5 2.5E-5 2.0E-5 1.5E-5 1.0E-5 5.0E-6 0.0E+0 0.1 1 diameter (µm) 10 Figure (3.22): The charging time as a function of grain diameter at ηe = 10-1, 10-2, 10-3, 10-4, and 10-5. 3.5.6 RMS Level of Charge Fluctuation RMS of charge fluctuations is inversely proportional to the square root of equilibrium charge number. Small dust grain collects few charges and the fluctuation around the equilibrium charge value are slow with high amplitude,but increasing particle size leads to collect more electrons and ions on its surface and the charge number equilibrium increases, so the fluctuation amplitude will be decreased. 65 CHAPTER THREE SIMULATION AND RESULTS Figure (3.23) represents the RMS fluctuations as a function of equilibrium charge number for different value of parameter ηe and Te=T=T+=0.2eV. This figure shows no affect turning charge on dust grain between positive and negative charges because the RMS fluctuations depends on absolute value of equilibrium charge number. 0.5 1.00E-01 1.00E-02 1.00E-03 1.00E-04 1.00E-05 0.45 0.4 0.35 0.3 RMS 0.25 0.2 0.15 0.1 0.05 0 1 10 100 equilibrium Charge Number (N) 1000 10000 Figure (3.23): RMS level of fluctuation as a function the equilibrium charge number on dust grain when ηn = 10-1, 10-2, 10-3, 10-4, and 10-5. 66 CHAPTER THREE SIMULATION AND RESULTS 3.5.7 The Dust-Negative Ion Acoustic Wave According to equation (2.18), it represents that the relation between the phase velocity dust-negative ion acoustic wave and the negative ion temperature is linear; this velocity is calculated by using the equilibrium charge from computer simulation. The phase speed of these wave increases as the negative ion temperature increases because dynamics of negative ions increase. Figure (3.24) shows the phase velocity dust-negative ion acoustic wave as a function of the negative ion temperature for ηe =10-1, D=10µm and Te =T+=0.2eV. 450 440 430 vo(m/Sec) 420 410 400 390 380 370 360 350 0.1 0.12 0.14 0.16 0.18 0.2 0.22 Negtive Ion Temperature (eV) Figure (3.24): The phase velocity dust-negative ion acoustic wave as a function of the negative ion temperature (eV) for D=10µm. It implies that for no dust ηd=0 cold negative ion T-=0 limits, the phase velocity of this wave is equal to √ ⁄ . This means that the Dust- Negative Ion Acoustic (DNIA) waves are associated with dynamics of negative ions, where the inertia comes from the mass of the negative ions and restoring force is provided by the thermal pressures of electrons and light 67 CHAPTER THREE SIMULATION AND RESULTS ions. It is also clear that for fixed light ion number density, i.e., n+=constant, the phase speed of these wave increases (decreases) as the negative ion (electron) number density increases. Figure (3.25) shows the phase speed dust-negative ion acoustic wave as a function ηn (ratio of the number density of negative ion to number density of positive ion). These results are agreement with the experiment results of I. Goertz et al (2007) [31]. 350 vo(m/Sec) 300 250 200 150 100 50 0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9 1 ηn=n-/n+ Figure (3.25): The phase velocity dust-negative ion acoustic wave as a function of the parameter ηn with T- =0 and no dust Figure (3.26): Full circles: phase velocity ofthe ion acoustic wave as function of the SF6 admixture (ne =5×1015 m−3,Te = 2 eV). 68 CHAPTER THREE SIMULATION AND RESULTS The connection between the phase velocity dust-negative ion acoustic waves and the parameter ηn (ratio of the number density of negative ion to number density of positive ion) for Te=T+=0.2, Tn=0.125Te is provided by the calculation of the phase velocity waves at state presence and absence dust, as a function of ηn, shown in Fig.( 3.27). For absence dust, the phase speed increases as the parameter ηn increases. For presence dust, the dust particles remain at rest and influence the wave propagation only by their effect on the overall charge balance. The presence of large dust particles leads to a reduction of plasma density; therefore, it leads generally to slow the phase velocity dust-negative ion acoustic waves as the parameter ηn increases. 390 without Dust 340 vo(m/Sec) 290 With Dust 240 190 140 0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9 1 ηn=n-/n+ Figure (3.27): The phase velocity dust-negative ion acoustic waves as a function of the parameter ηn with dust and no dust. 69 CHAPTER THREE 3.6 SIMULATION AND RESULTS Conclusions 1. The charging of dust grains in negative ion plasma can be controlled by varying the relative fraction of negative ions in the plasma. As the negative ion density increases, the magnitude of the negative dust charge is reduced and a transition to positively charged dust. 2. The charge distribution function has peak at the equilibrium charge value. 3. The increasing in the surface area of dust grain leads to increase the charges that fall on the grain surface. 4. The increasing of dust grain size leads to decrease the charging time so larger dust particle charges so fast and collects more positive ions and electrons than smaller one. 5. RMS of charge fluctuations is inversely proportional to the dust grain size. 6. The phase velocity dust-negative ion acoustic waves increase as the negative ion temperature increases. 7. The phase velocity DNIA waves increase as the number density of negative ion increases. 8. The phase velocity DNIA waves for absence dust are larger than the phase velocity DNIA waves for presence dust in the same circumstances. 70 CHAPTER THREE 3.7 SIMULATION AND RESULTS Future works According to the results obtained from this study, it can be suggested: 1. 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Schwabe, “Microparticles as Probes in a Highly Magnetized Dusty Plasma”, ph.D Thesis in Technische Universität München (2006). 76 اخلالصة هذا انبحث يقدو حماكات حاسوبيه ندراسة عًهيهه حهحٍ ايبيبهات انرباريهة اررًهورال م ب سيها(انكهونٌ-ايهوٌ انبوجاسهيوو حتحهو ايوَات سانبه (ايوَات سداسي فهوريد انكربيهث باالعحًها عههم يو يهم ريايهي ي هًم يو يهم انحهحٍ ارصل هم بتهد جههويز نيححو جأثري االيوٌ ان انب م عًهيه ححٍ ايبيبات انربارية. نهذا ارو يم مت حتويهه اىل ح ابات عد يه باسحخداو انربايج اياسهوبية نانربَهايج اياسهوبي ار هحخدو م ههذا انتًهم مت كحابحهه بهرهة انلههورجزاٌ نبيههاٌ عًهيههه انحههحٍ ن سيههٍ جوسيههس انحههحصات نح ههاز حههحصه ايبيبيههة نسيههٍ انحههحٍ نقههيى لحهلههة يههٍ َ( ηeههبه كفافههه االنكونَههههات اىل كحافههههه االيوَههههات ارو بههههة = 10-5,10-4,10-3,10-2,10-1,كهه هذنا ح ههههاز سههههزعه ههههور ارو ههههات (. negative ion-dust acoustic نَحائج انبحث انيحث ايكاَيه انححكى م عًهيه ححٍ ايبيبة يٍ خ ل جرري َ به اإلنكونَات م انب سيا حبيث عصهد سيها َ هبه االيوَات ان انبة م انب سيا يتظى االنكونَات سوف جزجبط باأليوٌ ان انب مما ي بب قهه جيار االنكونَات ان انبة نان هًا نييوَهات ارو بة بايزكة حنو ايبيبة انربارية نذنا جححول ححصه ايبيبة يٍ ان انب اىل ارو ب جدرجييا. نكهذنا ا نصحهائج انيهحث جهأثري جزكيهش االيهوٌ ان هانب ن ر هه حزارجهه عههم سهزعه هور ارو هات( negative ion-dust . acoustic