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Reading out Charge Qubits with a Radio Frequency Single Electron Transistor K. Bladh, D. Gunnarsson, G. Johansson, A. Käck, G. Wendin, P. Delsing Microtechnology Center at Chalmers MC2, Department of Microelectronics and Nanoscience, Chalmers University of Technology and Göteborg University, S-412 96, Göteborg, Sweden A. Aassime Service de Physique de l’Etat Condensé, CEA-Saclay, F-91191 Gif-sur-Yvette,France M. Taslakov Swedish National Testing and Research Institute, SP Box 857, SE-501 15, Borås, Sweden and Institute of Electronics Bulgarian Academy of Sciences, Sofia, Bulgaria (Dated: April 19, 2002) We describe fabrication and measurements of Single Electron Transistors operated in the Radio Frequency mode (RF-SET). We demonstrate very high sensitivity for RF-SETs and we evaluate the back-action from an RF-SET, when used as a read-out device for charge qubits. We conclude that single-shot read-out is possible with a signal to noise ratio greater than one, and that niobium qubits would substantially improve the signal to noise ratio. Furthermore we describe how the RF-SET could be used to read out a differential qubit in a gradiometer coupling. PACS numbers: 03.67.Lx, 73.23.Hk, 85.25.Na INTRODUCTION Quantum computers are predicted to perform certain computational tasks much faster than ordinary classical computers [1, 2]. Even though the difficulties in realizing a quantum computer are tremendous, the distant goal of quantum computers has focused a lot of attention on quantum state engineering and quantum measurement, areas where substantial progress has been made. A large number of qubit systems have been suggested, but so far only relatively primitive systems with a limited number of qubits have been tested. The most advanced demonstration so far is a seven qubit implementation [3] of Shor’s algorithm [1]. The different types of qubit systems can be divided into two categories: i) those which are based on microscopic systems such as molecules, trapped atoms, or photons [3–8], and ii) those which are based on solid state systems [9–13]. Both categories have advantages and disadvantages, especially the microscopic systems have long coherence times, but are hard to integrate into systems with a larger number of qubits. For the solid state systems the situation is the opposite. The system that we will discuss in this paper is the Single Cooper-pair Box (SCB)[14]. It is a solid state system, which is based on a small superconducting island connected to a charge reservoir via a Josephson junction. The Karlsruhe group has, in a series of papers, described theoretically how this system can be used as a qubit [9, 15, 16]. Quantum coherence in a SCB was first demonstrated by Nakamura et al. [17, 18], however the coherence times were quite short, of the order of 10 ns. In a very recent experiment [19] coherence times of the order of 1 µs have been observed. The read-out of a SCB with a single electron transistor (SET) [20, 21] has been discussed in a number of papers [16, 22–24]. The radio-frequency version of the SET (the RF-SET) [24–27] is especially interesting since it combines very high sensitivity with high speed. An alternative read-out scheme which uses the switching current of a large Josephson junction has been developed by the Saclay group [19]. In both cases it seems that single-shot read-out should be possible, even if it has not yet been demonstrated. In this paper we discuss the read-out of a SCB qubit with a Radio Frequency Single Electron Transistor. We also analyze the back-action of the RF-SET on the qubit based on measurements on two different SETs. In section 2 we describe the fabrication of the SETs and the qubits. We then describe the measurement setup, and in section 4 we discuss the measured data. In section 5 we discuss the back-action, and in section 6 we suggest a new type of differential qubit which can be read out in a gradiometer configuration. SAMPLE FABRICATION Choosing the right parameters and chemicals is essential to have sample fabrication working well. For shadow evaporation of metals, different systems have been developed to have certain characteristics in combination with the materials being used. P. Dubos et al. [28] have demonstrated the use of a trilayer resist based on polyethersolfone(PES)/germanium/PMMA for use with niobium evaporation. The thermostable PES can withstand the elevated temperatures during niobium evaporation so that the typical problems with out-gassing from the resist does not degrade the superconducting properties of the strips being fabricated. A calixarene derivative 2 FIG. 1: An example of one of the structures fabricated with the method described in the text. It shows an SET with a gate and some nearby ground planes fabricated by evaporation of 250+400 Å aluminum at two different angles. The smallest line width is 70 nm. e-beam resist has been developed by J. Fujita et al. [29] to have extremely high resolution, higher than PMMA, so that sub 10 nm lines can be fabricated. Some of the samples presented in this paper were made using a bilayer resist consisting of PMGI in the bottom layer and ZEP520A in the top layer. However, this bottom layer created a number of problems, and we are now fabricating samples with a bilayer resist system that has very high yield and quality. The new resist system consists of a top layer of ZEP520A:Anisole (supplied by Nippon Zeon Co Ltd) diluted 1:2, spun to a suitable thickness and baked 10 min at 170 ◦ C. The bottom layer is 8%wt P(MMA-MAA) copolymer in ethyl lactate baked 5 min at 170 ◦ C. After e-beam exposure the top layer is developed 40 sec in oxylene, rinsed 30 sec in IPA and dried in N2 . The bottom layer is developed in IPA:H2 O 5:1 until enough undercut is produced, rinsed 30 sec in IPA and dried in N2 . Rinsing of the samples is important to get the best results. After evaporation of 250+400 Å aluminum, excess metal is lifted off in n-methyl pyrrolidone. An example of a device fabricated with this new resist is shown in Fig. 1 The main advantage of this bilayer is the reproducibility and the high sample yield. In total 46 SETs (92 junctions) in different geometries have been fabricated resulting in 45 usable devices with resistances in the kΩ range and only one SET not working. The spread in resistance of the sample was such that 80% of the devices were within ±15 kΩ of the target resistance of 40 kΩ. We think that this spread in resistance is not due to differences in the bilayer but rather the irreproducibility of the conditions in the vacuum chamber during evaporation. With an evaporation system working in a controlled cli- FIG. 2: The layout for the integrated qubit and SET, The Qubit on the left is made in a SQUID geometry such that the Josephson coupling energy can be tuned with a magnetic field. mate we think this bilayer could produce tunnel junctions with near 100% yield and reduce the current spread in resistance so that most fabricated circuits have the same resistance within a few kΩ. Compared to numerous other resist systems we have tested, none came close to having the same performance. The system also shows excellent stability against changes in external parameters such as humidity and ageing, which is good for the long-term reproducibility of these results. In Fig. 2 we show the layout for a qubit-SET sample. The qubit on the left is made in a SQUID geometry such that the Josephson coupling energy can be tuned with an external magnetic field, and the charge on the box can be controlled via the gate lead which couples to the qubit from the left via the gate capacitance CgQ . The SET is coupled to the qubit via the coupling capacitance CC , and the working point of the SET can be adjusted with the SET-gate which is coupled via the capacitance CgS . The sum capacitance of the SET is CΣ = CSET + CC + CgS . MEASUREMENT SET-UP The measurements were performed in a dilution refrigerator with a base temperature of about 20 mK. A block TABLE I: SET-Sample 1 2 3 R [kΩ] 44.1 41.0 48.0 CΣ [aF] 370 270 600 √ δQ [µe/ Hz] 6.3 3.2 60 δ[h̄] 13 4.8 730 3 30 P (nW) 20 10 0 250 300 350 400 Frequency (MHz) FIG. 4: The power spectrum of the shot noise of the SET when a current of 1µA is sent through the SET (Sample #1) and after the amplifier noise has been subtracted. The noise is coupled out to the amplifiers via the tank circuit, and thus gives important information about the tank circuit. The dotted line is a fit to the data using a simple LRC-model. FIG. 3: A block scheme of the RF-SET measurement system. scheme of the measurement set-up is shown in Fig. 3. A weak RF-signal (the carrier) is launched towards the tank circuit via a directional coupler and a bias tee. The reflected signal is amplified by a cold amplifier and two warm amplifiers. We have used carrier frequencies in the range of 300-500 MHz. The reflected signal can be analyzed either in the frequency domain or in the time domain. The tank circuit consists of a capacitance which is just the stray capacitance of the contact pad of the sample substrate and an inductor. We have used two different types of inductors, a commercial chip inductor, which was flip chipped onto the substrate, and a circuit board inductor which was bonded to the substrate [30]. Both types of inductors give similar results, but the circuit board inductor is easier to connect, and has a higher self resonance frequency. The tank circuit is analyzed by applying a relatively large current trough the SET and detecting the shot noise which is coupled out to the amplifiers via the tank circuit. In Fig. 4, the noise spectrum of such a measurement is shown. In this measurement the noise spectrum at zero current was subtracted from the spectrum taken at 1 µA to remove the noise contribution coming from the amplifier. The form of the noise spectrum can be easily fitted to a simple circuit model from which we can extract the parameters of the tank circuit. For the typical case shown in Fig. 4 we get a resonant frequency of 331 MHz and a Q value of 18. This corresponds to an inductor value of 710 nH and a capacitance of 330 fF. To analyze the signal in the frequency domain we used an Advantest spectrum analyzer. A typical frequency spectrum can be seen in Fig. 5. Here a small gate signal with a frequency of 2 MHz and an amplitude of 0.035 erms was applied to the gate. This modulation generates the side peaks which can be seen in Fig. 5. Just as in an AM-radio, there are two different methods to retrieve the modulating signal and study it in the time domain. Either one can rectify and low pass filter the amplitude modulated carrier, or one can mix the reflected signal with another RF-source, which is phase FIG. 5: The frequency domain response of the RF-SET (Sample # 2) when a 2 MHz signal with an amplitude corresponding to 0.035 erms is applied to the gate. 4 20 15 10 I (nA) 5 0 -5 Pure RF-Mode -10 RF-Amplitude -15 -20 -1.5 -1.0 -0.5 0.0 0.5 1.0 1.5 V (mV) 30 FIG. 6: The time response from an RF-SET using the rectifying method. The input is a step function corresponding to a 0.2 e charge change on the gate capacitance. The bandwidth of this measurement is limited to 1 MHz. A single trace is shown with no averaging. 10 I (nA) locked to the carrier. By adjusting the phase between the two sources, the output amplitude from the mixer can be optimized. The two methods give similar results, but the mixing method normally gives somewhat higher signal to noise ratio. A typical time domain response to a 0.2e gate signal using the rectifying method is shown in Fig. 6. 20 0 RF+DC-Mode -10 RF-Amplitude -20 DC-bias -30 -2 -1.5 -1 -0.5 0 0.5 1 1.5 2 V (mV) PERFORMANCE OF THE RF-SET In the following we will discuss and compare the results obtained in three different SETs, samples #1 and #2 were optimized for best sensitivity, whereas sample #3 was integrated with a qubit. The parameters for the different samples, are summarized in Table I. The current voltage (IV) characteristics of Sample #1 and #2 are shown in Fig. 7 a and b respectively. The IVcharacteristic of the SETs could be modulated with a gate voltage as shown for sample #1 and #2 in Fig. 7. The gate voltage period was ∆Vg =10 mV corresponding to a gate capacitance CgS =16 aF for both samples. We have worked with two different modes of RF-excitation, as indicated in Fig. 7. Either we used a relatively large RF-amplitude and no dc-voltage (pure RF-mode), or we used a dc-voltage and a small RF-amplitude (RF+DCmode). Generally one can say that the RF+DC-mode normally gave better sensitivity. For a given gate voltage, the IV-characteristic is asymmetric due to the asymmetric bias. As the bias voltage is increased an additional charge is induced on the gate capacitance. For a negative bias this induced charge is of the opposite sign, and thus the effective gate charge is FIG. 7: Current voltage characteristics for a) sample #1 and b) sample #2. Curves are given for four different gate voltages. The two different modes of operation, pure RF mode and RF+DC-mode are also indicated in the a) and b) figures, respectively. different as can be seen in Fig. 7a. To evaluate the sensitivity performance of an SET, we measure the signal to noise ratio of one of the side peaks in the frequency spectrum when a small ac signal is applied to the gate. One of the side peaks is shown in detail In Fig. 8 for a gate amplitude corresponding to 0.0095 erms and a gate frequency of 2 MHz. The charge sensitivity of the SET can be calculated as δQ = √ ∆Q RBW × 10SNR[dB]/20 (1) where ∆Q is the value of the gate signal measured in electrons (rms), RBW is the resolution bandwidth used for the spectrum analyzer, and SNR is the signal to noise ratio for the side peak, measured in dB. From the data √ in Fig. 8 we can deduce a charge sensitivity of 3.2 µe/ Hz. 5 FIG. 8: One of the side peaks in the frequency spectrum for sample 2, with the gate frequency of 2 MHz and a gate amplitude corresponding to 0.0095 erms . The resolution bandwidth was 10 kHz. FIG. 10: The signal to noise ratio as a function of RFamplitude for a fixed bias voltage of 0.72 mV i.e at the Josephson Quasi Particle (JQP) peak, cf Fig. 9. The resolution bandwidth was 10 kHz. Just as for SQUIDs one can convert this charge sensitivity to an (uncoupled) energy sensitivity. as a function of the bias voltage when a relatively small RF-amplitude is applied. One can see that there are a number of maxima which are due to modulation of different features in the IV-curve. Note also that the SNR curve is not symmetric, which is again due to the gate charge induced due to the asymmetric bias voltage. The signal to noise ratio also varies with rf amplitude, as can be seen in Fig. 10. Here the RF+DC mode is used, and it can be seen that the SNR does not vary strongly with the RF-amplitude, the maximum being relatively flat. δ = δQ2 2CΣ (2) In this case we find an (uncoupled) energy sensitivity δ = 4.8 h̄, which is approaching the shot noise limit. The shot noise in an ordinary SET should give a lower limit around δ ≈ 0.7 h̄ [22], and for an RF-SET the noise is predicted to be slightly higher [31] so that we could expect to reach δ ≈ 1 h̄ at best. The SNR is of course dependent on a large number of parameters, such as carrier frequency and amplitude, gate frequency, dc-bias etc. In Fig. 9 we show the SNR BACK-ACTION When performing a measurement on a qubit, the measurement necessarily dephases the qubit. However, there can also be a mixing of the two qubit states which destroys the information that the read-out system tries to measure. The mixing occurs due to voltage fluctuations of the SET island SV (ω) and the characteristic time for this process is the mixing time tmix , which can be expressed in a simple form [16, 22] as Γ1 = FIG. 9: The signal to noise ratio as a function of bias voltage. IV-characteristics for several values of gate charge are also shown. Data is taken from Sample #3 with a resolution bandwidth of 3kHz, 0.1 erms applied at the gate and an RF-amplitude of -97 dBm 1 tmix = e2 2 EJ2 κ SV (∆E/h̄), h̄2 ∆E 2 (3) where we define the coupling coefficient as κ = Cc /Cqb and where the Josephson energy of the box EJ is assumed to be small compared to ∆E. As can be seen in Eq.(3), the mixing caused by backaction depends strongly on ∆E, and on the spectral density of the voltage fluctuations at the frequency corresponding to the energy difference between the two qubit states ∆E/h̄. These fluctuations can be thought of in terms of two contributions, one from the shot noise, 6 / FIG. 11: Comparison of the calculations of the spectral density of the voltage fluctuations of the SET island using the full quantum mechanical calculation (full line), the classical shot noise (dashed line), and the quantum fluctuations assuming a linear SET impedance (dotted line). Parameters for sample #1 are used in all calculations and one from the quantum fluctuations in the SET. At low frequency, the shot noise will dominate, while the quantum fluctuations will dominate at high frequencies. At high frequencies the impedance of the SET can be thought of as a linear resistance in parallel with the junction capacitances and the quantum fluctuations of the SET can be expressed as SV (ω) = 2h̄ωRe [ZSET (ω)] (4) To obtain the spectrum of fluctuations in the intermediate regime it is necessary to solve the full quantum problem, which was done in [23]. The result of this calculation and the comparison to the shot noise and quantum fluctuation results in the two limits, are shown in Fig. 11 for sample # 1. As can be seen the result of the full calculation coincides with the shot noise and the quantum noise in the low and high frequency limits respectively. In addition to this spectrum, the RF excitation gives a component at fRF , and the non-linearity of the IVcharacteristics gives an additional component at 3fRF . However these frequencies are much lower than the relevant mixing frequency ∆E/h̄ To resolve the two states of the qubit, which differ by two electron charges, we need a measuring time tm which can be expressed as [16]: FIG. 12: Calculated SV (f ) for samples #1(full line) and #2(dashed line). The arrows show the energy separations of the two qubit states for an aluminum and a niobium qubit, respectively. tmix /tm . The spectral densities SV (f) for the two samples at the optimum charge sensitivity, at a current of 6.7 and 8.0 nA for samples #1 and #2, respectively, are displayed in Fig. 12. As can be seen both from Eq. 3 and in Fig. 12, the mixing time increases strongly with increasing ∆E. In our case ∆E is limited by the superconducting energy gap ∆, which for aluminum films corresponds to about 2.5 K. Using niobium as the qubit material would substantially increase the mixing time. If we assume that EC and thus also ∆E can be scaled with ∆ and that the coupling coefficient κ is kept constant, mixing times of several ms can be reached. In that case, other sources would most probably dominate the mixing. The results for the samples #1 and #2 are summarized in Table II, where a coupling κ = 0.01 is assumed. A DIFFERENTIAL QUBIT Although the results above show that a Single Cooperpair Box may be measured in a single-shot measurement with a reasonable signal-to-noise ratio, the present design suffers from a number of problems. In an attempt to improve the present system we here suggest an alternative qubit layout. TABLE II: tm = δQ κe 2 . (5) Now we can use the measured data for samples #1 and #2 to calculate both tm and tmix , and thus we can also get the expected signal-to-noise ratio for a singleshot measurement, which is simply given by SN RSS = SET Qubit δQ √ Sample material e/ Hz 1 Al 6.3 1 Nb 6.3 Al 3.2 2 2 Nb 3.2 ∆E SV (ω) [K] [nV2 /Hz] 2.4 0.29 15.5 0.056 2.4 0.39 15.5 0.080 tm [µs] 0.40 0.40 0.10 0.10 tmix SNR [µs] 8.6 4.6 1860 68 6.4 8.0 1300 114 7 but with increased bandwidth. Furthermore, the 1/f charge noise, which is possibly the worst source of decoherence [33], can be divided into two different parts: the noise coming from long and short distances. The noise sources which are far away from the qubit will couple similarly to both islands and thus the effect of this noise will act as a common mode signal and thus be reduced. However, this is probably not a major improvement, since the noise sources located close to the SET-island are believed to dominate. L C CJ CC Cgs CJ CC CQB Cgs VS1 VS2 CJ Cg Cg CJ CONCLUSIONS -Vg/2 Vg/2 FIG. 13: A differential qubit read out by a gradiometer coupled RF-SET. The two SETs are tuned in anti-phase such that when a charge moves from left to right on the qubit, the current increases in both SETs. A problem with the ordinary SCB is that it sometimes shows e-periodicity instead of 2e-periodicity. The origin of this problem is not yet fully understood, but one source is that quasi particles, generated in the reservoir, diffuse to the junction and tunnel onto the island. Using a twoisland box (or if you like, an unconnected junction) would drastically decrease this problem since the islands are no longer coupled to a large reservoir. In fact this was the system that was originally suggested by Shnirman et al. [15]. Apart from the parity improvement there are also a number of other advantages with the two island box. One advantage is that one can make the read-out system in the form of a gradiometer, where two SETs read out one island each, as shown in Fig. 13. In such a configuration the two SETs can be tuned into opposite points of their transfer functions, so that the current would increase in both SETs when charge increases on the gate of the left SET and decreases on the gate of the right SET. The sensitivity and back-action from the SETs will be similar to the case described above (i.e. in Fig. 3), however this differential set-up will improve the system in two different ways. First, the noise from the cold amplifier which is coupled to the qubit via the tank circuit and the two SETs will be a common mode signal, and will thus not be coupled into the box. The amount to which this noise source can be reduced depends on how well the two SETs and the coupling capacitances can be matched. Just as in the case of the Saclay qubit [19] and the new Delft qubit [32] a symmetric layout improves the system. Secondly, this configuration also lowers the impedance of the two parallel coupled SETs, and thus one can use a tank circuit with a lower Q-value with maintained sensitivity, In summary we have demonstrated a very high charge sensitivity for Radio Frequency Single Electron Transistors,√at best we achieve a charge sensitivity of δQ=3.2 µe/ Hz and an uncoupled energy sensitivity of δ =4.8 h̄. We have also calculated the back-action which we would get in reading out a qubit, using the experimental results for two of the samples. We conclude that a single-shot measurement should be possible, and that the use of niobium qubits would substantially improve the signal to noise ratio of such a measurement. Furthermore, we also suggest a new type of differential qubit and show how such a qubit could be read out with a differentially coupled RF-SET. 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