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Sustain. Environ. Res., 25(3), 131-139 (2015) 131 Investigation of the environmental indicators at the main library of Sultan Qaboos University (SQU) in the Sultanate of Oman Sabah Abdul-Wahab,1,* Nahed Salem2 and Sappurd Ali3 1 Department of Mechanical and Industrial Engineering Sultan Qaboos University Muscat 123, Sultanate of Oman 2 Department of Library and Information Sultan Qaboos University Muscat 123, Sultanate of Oman 3 National Engineering and Scientific Commission (NESCOM) Islamabad 44000, Pakistan Key Words: Sick building syndrome, indoor air quality, thermal environment, library building, Oman ABSTRACT An investigation of the status of the indoor air quality and thermal environment of the new library building at Sultan Qaboos University was the primary objective of the current study. The secondary objective was to discover the extent to which users of the library suffered from symptoms of sick building syndrome (SBS) due to a poor indoor environment. In order to fulfill these objectives, the concentrations of indoor air pollutants and ranges of thermal comfort parameters were recorded at five different locations in the building. The results of the study indicated that the occupants of the library were being affected by SBS due to raised levels of carbon dioxide, total volatile organic compounds, and relative humidity (RH) along with an overly cool indoor environment. Increased levels of RH and CO2 indicated inadequate ventilation in the building. Short-term exposure to the polluted indoor environment of the library impacts the productivity, comfort level, and health of its library patrons. It is hoped that this study will contribute to the literature associated with quality of life in public indoor environments. INTRODUCTION Many studies have been conducted in recent years to investigate indicators of sick building syndrome (SBS) in various types of buildings, but SBS in libraries has garnered the attention of only a few researchers [1-19]. Furthermore, researchers who have conducted their work on libraries have focused their attention primarily on describing their architectural elements and the developments and improvements made to libraries over time. Most studies on libraries have dealt with the implications of these developments on libraries and the services they offer. Some researchers have focused upon the stages of development that library buildings go through over time and studying the impact of modern technical developments on their functions. Other researchers have described libraries’ safety and security systems, while yet others have focused upon *Corresponding author Email: [email protected] the architectural design of libraries [15]. At the same time, only a very limited number of studies focus on the environmental dimension of libraries and the effect on SBS, despite its importance to and impact on the quality of the performance of libraries’ information specialists. Hence, the relevant studies published internationally remain limited; further, Arab studies related to the topic are a rarity. The researchers of this study did not find any studies focusing adequately on this topic. No light was shed on the extent to which indoor air quality (IAQ) impacts the health of librarians and the extent to which this is reflected in their performance. This is what drew the attention of Abdul-Wahab and Salem [15] to the IAQ inside libraries and the necessity of determining the extent to which the occupants develop SBS. This determination was achieved by focusing on the main library of Sultan 132 Abdul-Wahab et al., Sustain. Environ. Res., 25(3), 131-139 (2015) Qaboos University (SQU) in the Sultanate of Oman as their case study, examining the interior environment of the building along with the extent to which the occupants are exposed to contaminants that cause SBS. Their study aimed at throwing light on SBS in libraries, and the extent to which it is influenced by the indoor environment. This was conducted through a study of the main library, which is located between an old and new building at SQU. To achieve this objective, the study adopted a descriptive survey methodology for the collection and description of the data, as well as a case-study methodology applied to the library building of SQU. The study relied upon a questionnaire to monitor SBS symptoms. The most important findings of the study showed that people in SQU’s old and new buildings suffer from SBS. In particular, sinusitis, dryness of the throat, and eye inflammation were some of the most prominent SBS problems from which SQU librarians suffer. SBS symptoms were influencing the efficiency of the library workers, and the rate of absenteeism increased. The degree of control over thermal levels was reduced in the new building while the level of noise was raised. Inadequate ventilation was also observed in SQU’s library. The study concluded with the recommendation that it is essential to observe environmental dimensions when designing libraries, taking into consideration the expected impact of SBS on librarians. Also, the study offered some recommendations for improving the environmental conditions of SQU’s new library and the amelioration of SBS in libraries in general. Keeping in mind the important findings of the study of Abdul-Wahab and Salem [15], the current work was designed by the same authors with the objective of investigating the status of IAQ and the thermal environment in SQU’s new library. The other objective of the current study is to determine the extent to which the users of the library suffer from symptoms of SBS due to exposure to indoor air pollutants and variations in the thermal environment. In order to achieve these objectives, the real time measurements of various physical and chemical components of IAQ, including air speed, temperature, relative humidity (RH), particulates, carbon dioxide, carbon monoxide, ammonia, nitric oxide (NO), nitrogen dioxide (NO2), ozone, and total volatile organic compounds (TVOCs), were taken. Due to the unavailability of any Omani standard or guideline for IAQ, the measured levels of indoor environmental parameters were compared with the permitted values defined in various international standards or guidelines, including the American S o c i e t y o f H e a t i n g , R e f r i g e r a t i n g , a n d A i rConditioning Engineers (ASHRAE) [20,21], World Health Organization (WHO) [22-24], National Institute for Occupational Safety and Health (NIOSH) [25], Environmental Protection Agency (EPA) [26] and Federal Republic of Germany (DFG/(MAK) [27], as well as previous studies such as those by Mølhave [28] and Brown [29]. MATERIALS AND METHODS In order to record the concentrations of indoor air pollutants and ranges of thermal comfort factors, five locations were selected in the new SQU library: the basement, the main reception and female study areas of the ground floor, the first floor’s Omani Studies Center Library, and the male study area on the third floor. The sampling of IAQ indicators was carried out for a period of 24 h at all locations except in the basement, where the duration of measurement was 48 h. The data measurements were conducted by means of environmental monitoring equipment using a WolfPack Modular Area Monitor (Gray Wolf Sensing Solutions, Shelton, Connecticut, USA) [30-33], which has integrated IAQ and toxic gases probes. In the present study, it was used to measure CO2, CO, RH, temperature, NH3, NO, NO2, SO2, H2S, O3, and TVOCs for an average period of 15 min. The indoor air speed was measured with the help of an AS-202A thermo anemometer probe (GrayWolf Sensing Solutions). The size distribution and number concentration of airborne particles were recorded using a six-channel GW3016 particle counter (Enviro Technology Services, Gloucestershire, UK). Calibration of the equipment was accomplished by comparison with standards maintained by Lighthouse Worldwide Solutions and the size calibrations were accomplished in accordance with the International Organization for Standardization 21501-4 Standard. More details about the specifications of the sensors of the Gray Wolf equipment can be found in the company’s manual. The WolfSense PC and Advanced Report Generator package was used to download the measured data. All the parameters were sampled for an average period of 15 min. The evaluation of IAQ in the building was carried out by comparing the measured levels of chemical pollutants and factors of thermal comfort with that of international standards or guidelines for average periods of 15 min and 1 h. The basis of the standard/ guideline values was of the effects on human health. The comparison between measured and permitted values was made on the basis of highest levels measured for each average period at each selected location. It is worth mentioning here that the measured concentrations of NH3, NO, SO2 and H2S, were either zero or < 0.3 ppm for each average interval, so their Abdul-Wahab et al., Sustain. Environ. Res., 25(3), 131-139 (2015) magnitudes are not available in the tables. RESULTS AND DISCUSSION 1.Evaluation of IAQ for an Average 15-min Period Table 1 illustrates the highest 15-min average levels/ranges of on-site measured parameters of IAQ along with the relevant standards/guidelines at the selected locations of library buildings. Table 1 shows that the measured levels of NO2, O3, and CO in SQU’s library were well within the limits described by the ASHRAE [20] and WHO [24]; hence, these pollutants were not contributing to the deterioration of IAQ in the SQU libraries. However, as illustrated in Table 1, the measured concentrations of CO2, TVOCs, and the ranges of temperature, RH, and air velocity were not within the threshold values as specified in international standards/guidelines. 133 1.1.CO2 The recorded concentrations of CO 2 at all of the selected locations in the SQU library were lower than the NIOSH acceptable limit of 30,000 ppm [25]; however, it was at an unacceptable level as determined by ASHRAE [20] standards. This suggests the necessity of maintaining a steady-state CO 2 level which, to remove human generated pollutants, is defined within an occupied space as < 700 ppm above the outdoor air concentrations. If the concentration of CO2 remains under this limit, then 95% of the building‘s occupants will find the IAQ acceptable, and no additional ventilation will be required to dilute the building’s pollutants introduced by copiers, laser printers, etc. [34]. Table 1 shows that three of the library’s locations - the main reception area, and the female and male study areas - were not meeting ASHRAE standards for IAQ [20]. The peak values logged at the main reception area, and female and male study areas were 858, 832, Table 1. Peak levels/ranges of parameters of IAQ for 15-min averaging period Parameter Location Peak level/range Standard/Guideline Ozone (ppm) Basement 0.04 Main reception 0.05 Female study area 0.05 Male study area 0.05 Omani studies centre 0.05 Nitrogen Dioxide (ppm) Basement 0.01 1 Main reception 0.01 ASHRAE [20] Female study area 0.01 Male study area 0.01 Omani studies centre 0.02 Carbon Monoxide (ppm) Basement 0.5 90 Main reception 0.7 WHO [24] Female study area 0.5 Male study area 0.7 Omani studies centre 0.2 Carbon Dioxide (ppm) Basement 426 30,000 NIOSH [25] Main reception 858 700 (continuous exposure) Female study area 832 ASHRAE [20] Male study area 1077 Omani studies centre 474 TVOC (µg m-3) Basement 389 < 200 (comfort range) Main reception 367 200-3000 (multifactorial exposure range) Female study area 594 Mølhave [28] Male study area 452 Omani studies centre 514 Air speed (m s-1) Basement 0.01-0.22 0.05-0.3 Main reception 0.03-0.83 ASHRAE [21] Female study area 0.32-0.46 Male study area 0.08-0.2 Omani studies centre 0.06-0.09 Temperature (°C ) Basement 21.3-23.6 22.5-26.0 (Summer) Main reception 21.5-23.4 20.0-23.5 (Winter) Female study area 18.7-23.4 ASHRAE [21] Male study area 21.3-25.5 Omani studies centre 20.4-22.0 Relative Humidity (%) Basement 51-63 30-60 Main reception 48-59 ASHRAE [21] Female study area 57-68 Male study area 42-61 Omani studies centre 66-79 134 Abdul-Wahab et al., Sustain. Environ. Res., 25(3), 131-139 (2015) and 1077 ppm, respectively. The measured values at the main reception area, and female and male study areas exceeded the suggested standard threshold by 23, 19, and 54%, respectively. The CO2 measurement trends at these locations indicated that the peak concentrations of CO2 exceeded the standard values during the library’s periods of higher occupancy, which is a clear sign of poor dilution and dispersion of human- and buildinggenerated pollutants in the absence of any specific outdoor pollutant source. The circulation of fresh air not only plays a vital role in the dispersion and dilution of the indoor pollutants but also is a prime indicator of ventilation adequacy in a building. These elevated levels of indoor CO2 reflect the meager ventilation in SQU’s library. This result is in agreement with what has been found in previous studies [35-40]. Elevated levels of CO 2 are associated with symptoms of SBS, and insufficient ventilation can cause discomfort, stuffiness, burning eyes, fatigue, dizziness, headaches, and reduced productivity in a building’s occupants due to the buildup of human-and building-generated pollutants [16]. These symptoms can be caused by a combination of CO 2 and many other pollutants in a poorly ventilated space [41]. Several studies have demonstrated that there is a positive correlation between the occurrences of SBS symptoms and elevated indoor CO2 levels [5,16,42-44]. The risk of SBS continued to decrease significantly with decreasing CO2 concentrations (< 800 ppm). The increase in ventilation rates can be associated with a significant decrease in the prevalence of SBS symptoms or with further significant improvements in perceived air quality [37]. Based on the above results, it can be concluded that CO2 was contributing to SBS in SQU’s library. 1.2.TVOCs Due to the unavailability of occupational and environmental standards for indoor exposure to TVOCs, the four exposure ranges proposed by Mølhave [28] are used in the present study to define acceptable levels of TVOCs: comfort range (< 200 µg m -3 ), multifactorial range (200-3,000 µg m-3), discomfort range (3,000-25,000 µg m -3 ), and toxic range (> 25,000 µg m-3). Table 1 shows that people in SQU’s library were exposed to TVOCs at the multifactorial level. The maximum concentrations of TVOCs were observed in the female study area (594 µg m-3) and the Omani Studies Center Library (514 µg m-3). TVOC concentrations > 500 µg m-3 are considered indicative of the presence of complicated VOC mixtures which may result in irritation of the eyes, nasal membranes, throat, and respiratory tract, and in general discomfort. Reports of such symptoms were mentioned in a previous study conducted by Abdul-Wahab and Salem [15] for the same building, as well as in other studies [45-47]. High indoor levels of TVOCs may be caused by the emission of pollutants by new furniture or carpets, aerosol sprays, cleaning agents, or paints. Also possible are outdoor sources of TVOCs which become indoor air pollutants. In the current study, vehicle parking areas were located on two sides of the library and the vehicle exhaust may become trapped in the library. Such a phenomenon has been reported in other studies, too [48,49]. Many studies have linked people’s exposure to TVOCs to symptoms of SBS [1,16,17,40,44]. It can be concluded from the above discussion that TVOCs also play a role in making the SQU library building “sick”; further investigation of VOCs in the library is recommended. 1.3.Thermal comfort Table 1 illustrates that the recorded values of thermal comfort are not meeting the standards for IAQ as specified by ASHRAE [21]. The thermal comfort level of the air at most selected locations in the library was on the low side of acceptable values (0.05-0.30 m s-1). Maximum air speeds with magnitudes of 0.83 and 0.46 m s-1 were recorded at the library’s main reception area and the female study area, respectively. The minimum measured values of air speed were 0.06-0.09 m s-1 at the Omani Studies Center Library. This is a clear indication of the inadequacy of the ventilation in the building. Air speed of less than 0.1 m s-1 can cause stuffiness while more than 0.3 m s-1 causes draughts. For air speed higher than 0.1 m s -1, an increase in air temperature is required to take into account air movement [50]. The optimum air speed which is suitable to achieve a pleasant feeling inside a building in the summer is 0.9 m s-1 and in winter is 0.15 m s-1 [51]. The measured values of temperature and RH inside the building at the selected locations were in the range of 18.7-25.5 °C and 42-79%, respectively, which again deviated from the ranges specified by ASHRAE’s [21] standards (temperature: 22.5-26.5 °C and RH: 3060%). It can be inferred from the data shown in Table 1 that the temperature in the SQU library was much lower than the ASHRAE’s acceptable thermal comfort zone in major parts of the building while the range of RH was higher than the standards’ objectives. This is in agreement with the results of a study conducted by Yau et al. [17] of university buildings. In the current study, low temperature values (20.4-22.0 °C) and elevated values of RH (66-79%) were recorded in the Omani Studies Center Library. As mentioned earlier, the circulation of fresh air inside the library was very low (air speed: 0.06-0.09 m s -1) which can affect Abdul-Wahab et al., Sustain. Environ. Res., 25(3), 131-139 (2015) the temperature and RH values inside the building. Similar results were also reported in previous studies [44,52]. Among all indoor air environmental factors, occupant discomfort is most commonly associated with raised RH levels. Excess RH in indoor air can cause fatigue, and increased reports of stuffiness, headaches, and dizziness. Furthermore, high humidity can cause increased pollutant emission from a building’s construction materials, especially in the case of formaldehyde and other VOCs, which can result in inferior air quality [34]. Moreover, elevated levels of RH can lead to interior conditions favorable for the growth of molds and microbials. The existence of such biological contaminants in indoor environments is associated with serious health problems [29]. As soon as the temperature of the hands falls below thermal neutrality, the lower temperatures can have a strong effect on manual tasks due to the effect on blood flow [37]. The change in temperature can significantly affect the intensity of headaches, concentration, and general well-being. In the light of the above discussion, it can be inferred that temperature, RH, and air speed levels are not suitable for the thermal comfort zone in the SQU library, and its occupants have very little control over these parameters, which is in accord with the findings of a previous study [15]. Raised thermal levels above those of acceptable thermal comfort may increase complaints of SBS and has also been found in various previous studies [6,15,44,52]. 1.4.Particulate matter (PM) Data on PM were not recorded for a full 24-h period due to the unavailability of sufficient couplings. Only two measuring probes were available with the WolfPack area monitor at the time of the study. Measured concentrations of PM with a diameter < 10 µm (PM10) for a 15-min average period are represented in Table 2. Although a comparison of short-term onsite measurements is not possible due to the lack of any standard or guideline for this average period, it is possible to get some idea about the PM levels in the building. The highest concentrations of PM10 and total PM (TPM) were observed at the library’s main reception area, with magnitudes of 36-71 and 55-136 µg m-3 (Table 2). These levels indicate the presence of internal and external sources of PM in the building, which can affect the health of occupants. 2.Evaluation of IAQ for an Average 1-h Period The peak levels/ranges of the physical environment and chemical contaminants for an average 1-h period are displayed in Table 3 which shows that 135 levels of CO2, TVOCs, temperature, and RH are not within the allowable limits determined by international standards. The measured levels of CO2 were within the acceptable values determined by NIOSH, but exceeded ASHRAE’s acceptable levels [20]. The highest concentrations of CO 2 were observed in the male study area (1,070 ppm) which exceeds the maximum acceptable value of 700 ppm by 53%. The levels of CO2 also exceeded the allowable limits in the female study area and the main reception area by 18 and 22%, respectively, indicating the inadequacy of ventilation in the building. The occupants may experience health effects in buildings where CO2 levels are elevated. At high levels, CO2, along with exposure to other indoor Table 2. Measured concentrations of particulate matter with diameter less than 10 µm for 15-min averaging period Parameter Location Range PM 0.3 (µg m-3) Basement Main reception Female study area Male study area Omani studies centre Basement Main reception Female study area Male study area Omani studies centre Basement Main reception Female study area Male study area Omani studies centre Basement Main reception Female study area Male study area Omani studies centre Basement Main reception Female study area Male study area Omani studies centre Basement Main reception Female study area Male study area Omani studies centre Basement Main reception Female study area Male study area Omani studies centre 0.0 0.0 0.0 0.0 0.0 PM 0.5 (µg m-3) PM 1.0 (µg m-3) PM 2.5 (µg m-3) PM 5.0 (µg m-3) PM 10.0 (µg m-3) TPM (µg m-3) Standard/ Guideline - <1 <1 <1 <1 4-8 - <1 <1 <1 <1 5-10 - 1-2 2-3 1-2 1-3 5-11 35 (24-h average) EPA [26] 3-10 15-26 6-10 9-27 8-16 - 4-21 36-71 14-24 21-58 8-17 150 (24-h average) EPA [26] 9-49 55-136 23-35 44-103 17-39 150-230 (24-h average) WHO [23] 136 Abdul-Wahab et al., Sustain. Environ. Res., 25(3), 131-139 (2015) pollutants, can cause headaches, dizziness, nausea, and other symptoms. Additionally, high CO2 concentrations can be associated with an increased prevalence of certain SBS-associated symptoms such as mucous membrane and lower respiratory issues, even when peak concentrations are below 1,000 ppm [5,16,43,44]. The measured TVOC values in the SQU library also fell in the multifactorial acceptable exposure range as defined by Mølhave [28] but exceeded the guideline value of 500 ppm for an average 1-h period as determined by Brown [29]. These levels were exceeded by only 2% in the female study area and the Omani Studies Center Library. The possibility of affecting the health of a building’s occupants and increasing the possibility of an occurrence of SBS exists within this range of exposure. Temperature and RH ranges in the building were not in accordance with the standard ranges set by ASHRAE either [21]. The temperature in most of the selected locations was lower than that determined acceptable by ASHRAE limits while the RH exceeded the stipulated range of 60% [21]. This is an obvious indication of a cooler and more humid indoor environment within a building than has been determined acceptable by international guidelines, which may be hazardous to occupants’ health. A high RH can foster the proliferation of molds and dust mites along with a release of pollutants from building materials which can have a direct effect on people’s comfort and productivity [34]. When the occupants of the building are exposed to higher levels of humidity, the occurrence of SBS symptoms like fatigue, headache, and difficulty in thinking is not out of the question [52]. CONCLUSIONS The current study was suggested based on the findings of a previous study carried out by same authors which set out to determine the extent to which the new SQU library enjoys a better interior environment and to what extent the occupants of the building suffer from SBS. The objective of the study was achieved through a battery of tools, most important of which were questionnaires and interviews. The results of this study showed that the SQU library is suffering from an environment that encourages SBS. Keeping in Table 3. Peak levels/ranges of parameters of IAQ for 1- hour averaging period Parameter Location Peak level/range Ozone (ppm) Basement 0.04 Main reception 0.05 Female study area 0.09 Male study area 0.01 Omani studies centre 0.10 Nitrogen Dioxide (ppm) Basement 0.01 Main reception 0.01 Female study area 0.01 Male study area 0.01 Omani studies centre 0.02 Carbon Monoxide (ppm) Basement 0.60 Main reception 0.68 Female study area 0.50 Male study area 0.70 Omani studies centre 0.20 Carbon Dioxide (ppm) Basement 436 Main reception 850 Female study area 829 Male study area 1070 Omani studies centre 469 TVOC (µg m-3) Basement 372 Main reception 364 Female study area 510 Male study area 452 Omani studies centre 510 Temperature (°C) Basement 22.8-23.6 Main reception 21.6-23.4 Female study area 19.9-22.9 Male study area 20.7-25.4 Omani studies centre 20.2-21.9 Relative Humidity (%) Basement 45-62 Main reception 43-58 Female study area 58-64 Male study area 42-60 Omani studies centre 66-78 Standard/Guideline 0.12 ASHRAE [20] 0.1 WHO [24] 25 WHO [22] 10,000 MAK [27] 700 (continuous exposure) ASHRAE [20] 500 Brown [29] 22.5-26.0 (Summer) 20.0-23.5 (Winter) ASHRAE [21] 30-60 ASHRAE [21] Abdul-Wahab et al., Sustain. Environ. Res., 25(3), 131-139 (2015) mind the findings of previous study, the present work was designed to evaluate the indoor environmental conditions of the new SQU library by determining the indoor levels of physical and chemical irritants. The results of the current study confirmed the previously observed health impacts of IAQ as related to SBS. It is apparent from the findings of the present study that the occupants of SQU’s new library were affected as a result of exposure to chemical contaminants along with uncomfortable thermal levels. The elevated levels of CO2 were indicative of insufficient building ventilation. The observed concentrations of TVOCs and PM10 indicated the presence of strong indoor and outdoor contaminant sources, and there is a need to pay attention not only to these pollutants but also to biological contaminants in order to complete an investigation of IAQ. The physical environment of the library was also not appropriate for the occupants due to low temperature and high RH. The elevated levels of each of these parameters were possibly worsening the IAQ. Pathological symptoms such as headaches, membrane irritation, inflammation, fatigue, dizziness, stuffiness, etc. may have been due to the manifestation of elevated IAQ levels. The current study was essential in order to investigate the extent to which the indoor environment of the new SQU library was contaminated due to the existence of indoor air pollutants and to what extent the occupants of the building enjoyed an acceptable thermal environment. The other objective of this work was to know whether library users suffered from SBS as a result of chemical contamination and thermal discomfort. In order to fulfill these objectives, the ground level concentrations of indoor air pollutants and ranges of thermal comfort parameters were recorded at five different locations in the building. The measured levels of IAQ parameters were compared with international standards and guidelines. The results indicated that that the occupants of the building were affected as a result of exposure of to excessive levels of CO2, PM, and TVOCs and discomfort caused by physical environmental indicators like air velocity, temperature, and RH. The elevated levels of CO 2 reflected the insufficiency of the building’s ventilation. The observed concentrations of TVOCs and PM were evidenced by strong indoor and outdoor pollution sources. The temperature of the building was also found to be cooler than the thermal comfort zone. Exposure to the polluted indoor environment was impacting the productivity, comfort level, and wellbeing of the workers in the library. Complaints of symptoms associated with SBS, such as headaches, irritation, fatigue, dizziness, etc. have been common due to elevated levels of indoor air pollutants. 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