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Remote Observations of the Electric Field within Thundercloud: New LIDAR - Based Techniques The real time measurement of spatial and temporal distribution of the electric field in and around thunderclouds is important for understanding the formation mechanisms of thunderclouds, for predicting the appearance of lightning strokes and for understanding the processes of the cosmic ray electrons acceleration and the bremsstrahlung photons generation caused by the electric field of clouds. Now the electric field meters, used for this purpose, are set on Earth surfaces or installed on balloons. These techniques are limited as they typically provide a single sample at discrete altitudes at one time. LIDAR systems are the main instrument which allows to realize real time remote measurement of the electric field strength and direction with high spatial and temporal resolution. LIDAR systems are based on the absorption and/or scattering of light by the gas, liquid or solid state. Atomic and molecular spectra can be measured very accurately and sensitively using spectroscopy techniques. Scattering of Electromagnetic Waves Geometric Mie Elastic Reyleigh Back Raman Non Elastic Fluorescence EM wave induced dipole moment P ~ χ (1)E + χ (2)E1E2 + χ (3)E1E2E3 + … Linear Nonlinear Four Wave Mixing P ~ χ (3)E1E2E3exp{ i [ΔKr – Δωt ]} ω = ω1 – ω2 + ω3 K = K 1 – K2 + K3 I ~ │χ(3)│2 I1I2I3 Four Wave Mixing & Electric Field 1. Difference Frequency Generation P ~ χ (3)E1E2E ωE = ω3 = 0 => ω = ω1 – ω2 K = K1 – K2 I ~ │χ(3)│2 I1I2E2 Experimentally realized (laboratory)!!! V. N. Ochkin et all. 1995 1atm, 532nm, 683nm H2 – 2.4 μm => 20V/cm 2. Sum Frequency Generation P ~ χ (3)E1E3E ωE = ω2 = 0 => ω = ω1 + ω3 K = K1 + K3 I ~ │χ(3)│2 I1I3E2 Experimentally realized (laboratory)!!! Second and Third Harmonic Generation & Electric Field Electric Field Induced Second harmonic generation (EFISH) P ~ χ (3)(2ω) E12E ωE = ω2 = 0 ω1 = ω3 I2ω ~ │χ(3)(2ω)│2 I12E2 Third harmonic generation P ~ χ (3)(3ω) E13 I3ω ~ │χ(3)(3ω)│2 I13 Electric Field E2 ~ │χ(3)(2ω)/χ(3)(3ω)│2 I1 I2ω ̸ I3ω Proposed!!! N2 – ω1 = 4.2 μm O2 – ω1 = 6.3 μm CO2 – ω1 = 7.5 μm H2O – ω1 = 2.7 μm CARS & Electric Field Infrared Wave Generation ω3 = ωE = 0 ω1 – ω2 = Ω = ωir Iir ~ │χir(3)│2 I1 I2 E2 Coherent Antistokes Raman Scattering (CARS) ω3 = ω1 2ω1 – ω2 = ωas Ias ~ │χCARS(3)│2 I12 I2 Electric Field E2 ~ │χCARS (3) / χir (3) │2 I1 Iir / Ias Experimentally realized (laboratory)!!! P. Bohm et all. 2013 1000 mbar H2 – 2.4 μm => 20V/cm N2 – 4.29μm => 300V/cm Comparison of Linear and Nonlinear techniques Nonlinear spectroscopy Advantages: Direct measurement of the electric field. High spectral resolution (Limited by laser line-widths). Disadvantages: Required two laser sources. Registration of IR signal (required fast IR detector for spatial and temporal resolution). Strong absorption of the IR radiation by water (required additional investigations). Development for other molecules, atoms, charged molecules, ions, isotopes etc. Development of Nonlinear spectroscopy techniques for remote sensing in situ. Linear Spectroscopy Advantages: One laser source Disadvantages: Electric field measurement via its influence on the spectrum of gases (not direct). Required high resolution spectrometer, including IR. Required large aperture receiving optics. Required (in some cases) high power IR laser. The electric field remote sensing methodology in thunderclouds need additional investigations and development !!! Development of Atmospheric Polarization LIDAR System Laser Emitter (a+b) Receiving Telescope (c), Polarization Separator (d). Laser Emitter Laser Emitter output beam parameters Pulse Energy 1064nm 300-500 mJ 532nm 100-200 mJ Beam Divergence <10-4 rad Polarization linearity <10-3 Pulse duration 10 ns Repetition rate 10-20 Hz Output beam diameter 112 mm 1 - Convex mirror, 2 – Electro optical Q-Switch, 3 – Diaphragm, 4 – Output polarizer, 5 – laser oscillator pump chamber, 6 – Quarter wave-plate, 7 – Concave mirror, 8 and 16 – Two wavelength mirrors, 9 – Glan prism polarizer, 10 – Flash- lamp driver cables, 11 – mirror, 12 – Cooling system pipes, 13 – Laser amplifier pump chamber, 14 – Flash-lamps, 15 – Second harmonic generator, 17 – Hole for the output beam. Polarization Separator The green points are the separated cross-polarized beams. Laser Emitter and Receiving Optical System Alignment Alignment Laboratory Stand By means of the laboratory stand was aligned: The Laser, including, laser oscillator and laser amplifier. The Laser with Beam Expander (14X). Diode Laser beam with its beam expander (200X). Diode Laser beam optical axis with RT housing tube axis. Receiving Telescope (RT) mirror optical axis with Diode Laser beam optical axis and RT housing axis. Polarization Separator (PS) optical axis with RT Mirror optical axis. PS with cross-polarized beams outputs and RT mirror focus. Signal transportation fibers with cross-polarized beams. Adjustment of PMTs for registration of GLD beam. The YerPhI LIDAR System System Triggering Photodiode PMTs Laser Beam Expander The Laser Aiming Optics Q-Switch Driver Cables Laser Cooling Pipes Laser Emitter Alignment Receiving Telescope Flash-lamp Supply Cables Signal and Supply Cables LIDAR System Registration System Triggering Fiber Laser Beam Expander Laser Emitter Output Energy Control Fibers The Laser Laser Emitter Alignment Mount Receiving Telescope Polarization Separator Alignment Mount Polarization Separator Aiming Optics Registration System Triggering Photodiode Laser Emitter Alignment PMTs Optical Filter Boxes Receiving Mirror Focus Finder Optical Signal Outputs Stepper Motor end Switch Optical Signal Transportation Fibers to PMTs Play-free Gear Stepper Motor The LIDAR Registration and Control System LIDAR Controllable Parameters LE beam 1064nm output energy. LE beam 532nm output energy. LE beam repetition rate. LE Q-Switch driver pulse delay. LE beam polarization finder. PS – LE beam polarization angle. Registration delay. LE – RT angle. PMT supply voltage. LIDAR azimuth and elevation. LE cooling temperature. System Triggering PD and its electronics PMT Power Supplies NI USB DAQ NI DAQ BNC Inputs and Outputs Triggering Pulse (5nsec/div). PD and PMT Amplifier Power Supplies Stepper Motor Driver Oscilloscope 500MHz PMT with voltage divider and Signal Amplifier The YerPhI LIDAR System Sorry for quality. First Backscattered Signal Observations Laser flash-lamp background and Reflected from a wall signal (250m). Horizontal - 30m/div; Vertical signals - 0.1V/div; Vertical trigger - 2V/div; PMT - 0.5kV. Backscattering from the Atmosphere. Horizontal - 750m/div; Vertical - 20mV/div; Laser - 100mJ; PMT - 2kV; PS ~ 90deg. First Backscattered Signal Observations Scattering from Atmosphere and Clouds. (Hor.-750m/div; Ver.-20mV/div; PMT-2kV; PS-90deg). First Backscattered Signal Observations Scattering from Atmosphere and Clouds. Horizontal - 750m/div; Vertical - 50mV/div; PMT - 2kV; PS ~ 45deg). Planned Investigations in Nearest Future 1. Reyleigh and Mie backscattering: – Depolarization ratio profile. 2. Raman backscattering N2 (607nm), O2 (580nm), H2O (645nm): – Depolarization ratio of spectral bands. 3. Electric field under and inside the clouds. Linear P ~ χ (1)E1 exp{ i [ K1r – ω1t ]} 1. Power 2. Wavelength 3. Line-width 4. Polarization - Absorption, etc. - Raman, Fluorescence, Stark, Doppler, etc. - Stark, Doppler, etc. - Kerr, Pockels, Faraday, etc. Polarization φ = 2π (no - ne) L / λ = 2π B L E12 Bwater = 5.2 10-12 cm/V2 For 1000 V/cm and 500m =>φ = π /2 --> λ/4 plate Cloud Type LWC (g/m3) Atmosphere Cirrus .03 Fog .05 Stratus .25-.30 Cumulus .25-.30 Stratocumulus .45 Cumulonimbus 1.0-3.0 0.1-5.0 LIDARs for CTA Germany France Argentina Spain France Max Plank U Montpellier2 Buenos Aires U Barcelona U Montpellier I (Munich) LUPM Elastic 1064 Elastic 532 Elastic 355 Raman 387(N2) Raman 607(N2) Raman 408(H2O) Raman 645(H2O) Elastic Polar. Distance Laser Rep. Rate 1064nm Energy 532nm 355nm Pulse width for MAGIC for HESS X X X 0.5 - 18 20 Soliton Quantel GmbH Brilliant 30 2000 20 0.005 180 65 0.5 5 Polarization Beam Dia. (Expander) Divergence Receiving Mirror Dia. HPD Detector Readout Hamamatsu R9792U-40 IFAE/UAB X X X X - LUPM X X X X - Armenia U Torino U Naples YERPHI ARCADE X X X X X X X 0.25 - 10 0.1 - 15 Quantel Custom Centurion made 100 10 - 20 40 300-500 18 100-200 6 8 10 Continuum Inlite II-50 50 125 60 20 10 Quantel Brilliant 20 360 180 100 5 Quantel CFR400 20 400 230 90 7 Polar. Polar. Polar. Polar. Depolar. 600 PMT 6 0.75 6x400 PMT/HPD 6 0.5 1800 PMT/HPD 7 3.5 1800 PMT 20 (10x) (3) 0.3 250 PMT Photonis XP2012B 51mm Hamamatsu H10721-110 25mm Hamamatsu H10721-100 38mm GAGE 8265 LICEL LICEL (10x) 600 CEILAP X X X X X X - Italy Hamamatsu Hamamatsu R329P R1332Q 50mm 50mm LICEL CAEN km Hz mJ ns Polar. 110 (14x) mm (1) <0.1 mrad 250 mm PMT FEU-83 FEU-100 25mm NI DAQ