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QUANTUM TRANSPORT IN THE TUNNELING AND COTUNNELING REGIMENS Javier F. Nossa M. Goal •I want to show you an animation that I have been working with!!! •Why? •Because I like animations!!! •Quantum transport. 25 Nov 2010 Quantum transport in the Tunneling and Cotunneling regimens J.F. Nossa Sequential Regimen System Fermi Level of Source is lower than first unoccupied level of dot L unoccupied energy levels R E EF source D occupied energy levels quantized energy levels gate drain E k T B Energy spacing must be greater E ( N 1) ( N ) than thermal smearing 25 Nov 2010 Quantum transport in the Tunneling and Cotunneling regimens addition energy J.F. Nossa Sequential Regimen Applying a potential, the dot energy levels are shifted. An electron can now occupy the dot Fermi energy of source is higher than first dot unoccupied energy level Coulomb blockade prevents others. L electrons R EF source 25 Nov 2010 gate drain Quantum transport in the Tunneling and Cotunneling regimens J.F. Nossa Sequential Regimen Ground state energy levels Constant interaction model: U ( N ) EC N 2 eVg N U ( N 1) EC ( N 1) 2 eVg ( N 1) EC Charging energy ( N 1) U ( N 2) U ( N 1) L tunneling in R tunneling out This cycle is known as single electron tunneling ( N ) U ( N 1) U ( N ) source gate drain We fix VG and vary VDS VL VR 25 Nov 2010 Quantum transport in the Tunneling and Cotunneling regimens J.F. Nossa Sequential Regimen ( N 1) Current (N ) Current Step 25 Nov 2010 Quantum transport in the Tunneling and Cotunneling regimens J.F. Nossa Sequential Regimen Energy levels Constant interaction model: U ( N ) EC N 2 eVg N U ( N 1) EC ( N 1) 2 eVg ( N 1) L EC Charging energy ( N 1) U ( N 2) U ( N 1) R ( N ) U ( N 1) U ( N ) Source§ gate drain We fix VDS VL VR and vary VG 25 Nov 2010 Quantum transport in the Tunneling and Cotunneling regimens J.F. Nossa Sequential Regimen 25 Nov 2010 Quantum transport in the Tunneling and Cotunneling regimens J.F. Nossa Sequential Regimen Energy levels Constant interaction model: U ( N ) EC N 2 eVg N U ( N 1) EC ( N 1) 2 eVg ( N 1) EC Charging energy ( N 1) U ( N 2) U ( N 1) L R ( N ) U ( N 1) U ( N ) Source gate drain We change both VDS VL VR and VG 25 Nov 2010 Quantum transport in the Tunneling and Cotunneling regimens J.F. Nossa Sequential Regimen Coulomb diamonds, differential conductance Current Steps Current Oscillations 25 Nov 2010 Quantum transport in the Tunneling and Cotunneling regimens J.F. Nossa Anderson Model H n Un n Two level system , Coulomb diamond E (0) 0 E () 0 E () 0 E (2) 2 0 U 25 Nov 2010 N=0 Quantum transport in the Tunneling and Cotunneling regimens N=1 N=2 J.F. Nossa Sequential Regimen So far we have taken into account only ground states... ... what if we included excited states? 25 Nov 2010 Quantum transport in the Tunneling and Cotunneling regimens J.F. Nossa Sequential Regimen N N+1 If a line terminates at the N-electron Coulomb blockade region, the transition necessarily involves an N-electron excited state 25 Nov 2010 Quantum transport in the Tunneling and Cotunneling regimens J.F. Nossa Anderson Model H n Un n B S Two level system , Coulomb diamond E (0) 0 E () 0 B N=0 E () 0 B N=1 N=2 E (2) 2 0 U 25 Nov 2010 Quantum transport in the Tunneling and Cotunneling regimens J.F. Nossa Cotunneling Regimen So far, only single-particle processes have been considered. First order processes in the tunneling Hamiltonian. Two-particle processes. Higher order tunneling process Cotunneling One electron occupies the dot while, at the same time, another electron leaves the dot L ( N 1) U ( N 2) U ( N 1) R ( N ) U ( N 1) U ( N ) Source§ Because EIS Ei 25 Nov 2010 Intermediated state gate drain Virtual process Quantum transport in the Tunneling and Cotunneling regimens J.F. Nossa Cotunneling Regimen Elastic Cotunneling D (N ) 0 D ( N 1) 0 L R 0 Initial state Intermediate state Final state Spin Effects in Single-Electron Transistors, Ghislain Granger, MIT 2005 25 Nov 2010 Quantum transport in the Tunneling and Cotunneling regimens J.F. Nossa Cotunneling Regimen Inelastic Cotunneling E f Ei D (N ) 0 D ( N 1) 0 L 0 R 0 L Initial state Intermediate state Final state The dot is left in an excited state L E f Ei 25 Nov 2010 Quantum transport in the Tunneling and Cotunneling regimens J.F. Nossa Cotunneling Regimen Cotunneling in the differential conductance dI / dV V Sequential tunneling: current inside the diamond is not allowed 25 Nov 2010 Two regimes: one consisting of elastic processes only, and one including both elastic and inelastic contributions S. De Franceschi et.al., Phys. Rev. Lett. 86, 878 Quantum transport in the Tunneling and Cotunneling regimens J.F. Nossa Anderson Model H n Un n B S Two level system , Coulomb diamond E (0) 0 E () 0 B N=0 E () 0 B N=1 N=2 E (2) 2 0 U E () E () 0 B ( 0 B) 2 B 25 Nov 2010 Quantum transport in the Tunneling and Cotunneling regimens J.F. Nossa Anderson Model H n Un n B S Two level system , Coulomb diamond E (0) 0 E () 0 B N=0 E () 0 B N=1 N=2 E (2) 2 0 U E () E () 0 B ( 0 B) 2 B 25 Nov 2010 Quantum transport in the Tunneling and Cotunneling regimens J.F. Nossa Anderson Model dI / dV Step instead of peak N=0 E (N ) 25 Nov 2010 N=1 N=2 V Quantum transport in the Tunneling and Cotunneling regimens J.F. Nossa TUNNELING AND COTUNNELING PHENOMENA IN SET THANK YOU !!! Javier F. Nossa M.