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Quantum Information Processing with 1010 Electrons ? René Stock IQIS Seminar, October 2005 People: • Barry Sanders • Peter Marzlin • Jeremie Choquette Motivation Quantum information processing realizations Ions Solid State systems Photons NMR Need for hybridization and interfacing of different technologies Neutral Atoms Superconductors Surface Plasmons ? coherent charge density oscillations involving 1010 electrons Outline • What are surface plasmons: Introduction • Excitation of surface plasmons at surfaces • Entanglement and surface plasmons • Surface plasmons in quantum information implementations Outline • What are surface plasmons: Introduction • Excitation of surface plasmons at surfaces • Entanglement and surface plasmons • Surface plasmons in quantum information implementations What are surface plasmons ? • Electric field propagating at surface r E z metal x − − − + + + − − − + + + − − − dielectric ε1 ε2 € Hy • • Maxwell Equations and continuity D = ε0E + P = ε E (linear medium) € divD = 0 € € E x1 E1 = 0 exp[i( kx1 x − k z1z − ωt )] E z1 0 H1 = E y1 exp[i( kx1 x − k z1z − ωt )] 0 1 ∂D =0 → c ∂t divB =€ 0 rot H − € E x1 = E x 2 → ε1 E z1 = ε2 E z 2 H y1 kz1 H y1 ε1 Ex2 E 2 = 0 exp[i( kx 2 x + k z2 z − ωt )] Ez2 0 H 2 = E y 2 exp[i( kx 2 x + k z2 z − ωt )] 0 SP Dispersion relation kx = Hy 2 k = − z 2 Hy 2 ε2 = € ω ε1ε2 c ε1 + ε2 2 ω kx2 + kzi2 = εi 2 c What are surface plasmons ? • Evanescent electric field propagating at surface z r E z metal x − − − + + + − − − + + + − − − dielectric Ez ∝ e−kz z ε1 ε2 Hy • Surface Plasmon: Longitudinal charge € density oscillations involving 1010 electrons€ Ez ω ε1ε2 ksp = c ε1 + ε2 Surface Plasmon Polariton: Polaritons are quasiparticles resulting from € strong coupling of electromagnetic waves with an electric or magnetic dipolecarrying excitation, in this case plasmons. € What are surface plasmons ? • Evanescent electric field propagating at surface z r E z metal x − − − + + + − − − + + + − − − dielectric Ez ∝ e−kz z ε1 ε2 Ez Hy • € € ε1 = ε1′ + i ε1′′ ε2 is real ω ε1ε2 kx = c ε1 + ε2 ω ε1′ε2 kx′ = c ε1′ + ε2 3 2 ω ε1′ε2 ε1′′ kx′′ = c ε1′ + ε2 2(ε1′) 2 ε1′′ < ε1′ € e.g. Ag ε = −22.4 − 0.91i Au ε = −23.0 € − 0.77i 1 2 [also ε(ω )] € What are surface plasmons ? • Evanescent electric field propagating at surface z r E z metal x − − − + + + − − − + + + − − − dielectric ε1 ε2 Hy • Ez ∝ e−kz z δm Ez δd € € 3 2 [Figures courtesy of Barnes et al., Nature 424, p824 (2003)] ω ε1′ε2 ε1′′ δsp ⇔ k x′′ = c ε1′ + ε2 2(ε1′) 2 Extremely short lifetimes for surface plasmons ( 10-15 s to 10-12 s) € Outline • What are surface plasmons: Introduction • Excitation of surface plasmons at surfaces • Entanglement and surface plasmons • Surface plasmons in quantum information implementations Excitation of Surface Plasmons • Attenuated total reflection ksp = ω ε1ε2 ω < c ε1 + ε2 c [Figures courtesy of Barnes et al., Nature 424, p824 (2003)] ω €kx = sin θ ε0 c r klight θres r kx r metal film ksp attenuated total reflection at surface plasmon resonance € € [other figures courtesy of R. Stock, Thesis, UNM (2001)] Excitation of Surface Plasmons • 0.4 Attenuated total reflection prism gold air 0.3 ksp = ω ε1ε2 ω < c ε1 + ε2 c 2 normal incidence E (z ) 0.2 E0 0.1 ω €kx = sin θ ε0 c 0 -200 0 r klight 6 5 2 θres E (z ) 4 E0 400 600 distance (Å) 8 7 200 prism gold air surface plasmon resonance angle 3 r 2 kx 1 r metal film 0 -200 0 200 400 600 ksp strong field enhancement effect due to surface plasmons € € [Figures courtesy of R. Stock, Thesis, UNM (2001)] Excitation of Surface Plasmons • Periodic structure r r r r ksp = k x ± m Gx ± n Gy → € • ε1ε2 m +n λ=D ε1 + ε2 2 2 Periodic sub wavelength hole array € versatile wavevector matching using periodic structures [Figures courtesy of Ghaemi et al., PRB 58, p6779 (1998) and Altewischer et al., Nature 418, p304 (2002)] Excitation of Surface Plasmons • Periodic sub wavelength hole array 700 nm ksp 200 nm 200 nm ksp Enhanced optical transmission through array of sub wavelength holes (compared to diffraction theory) [Figures courtesy of Ghaemi et al., PRB 58, p6779 (1998) and Altewischer et al., Nature 418, p304 (2002)] Outline • What are surface plasmons: Introduction • Excitation of surface plasmons at surfaces • Entanglement and surface plasmons • Surface plasmons in quantum information implementations Implementations using Surface Plasmons • Field enhancement effect – Surface enhanced spectroscopy – Strong coupling to waveguides – Biophotonics: Biological and chemical detectors (sensitivity to ε2 at the surface) • Nanoscale technology – Nano-optics and nano-circuitry on surfaces: • Mirrors (reflectivity> 90%) • Nanowires (waveguides) for plasmons – “Plasmonic” computer chips and other nanoscale technology – Data storage • Quantum nature of surface plasmons – SPASERS (surface plasmon amplification by spontaneous emission of radiation) – Single photon light sources – Quantum information processing Seidel et al., PRL 94, 177401 (2005) Surface Plasmons and Entanglement • Polarization entangled photons ψ = • 1 X1Y2 + e iφ Y1 X 2 ( 2 ) Experimental setup € Nature 418, p304 (2002) Coincidence detection after transmission through hole array Surface Plasmons and Entanglement • Experiment Reduced visibility due “which-path” information in solid? Surface Plasmons and Entanglement • Which-path information: include state of solid E. Moreno, F.J. Garcia-Vidal, D. Erni, J. I. Cirac, L. Martin-Moreno PRL 92, 236801(2004) • € € Interaction models? a) all Sab are orthogonal: solid and biphoton entangled → trace over solid: mixed state for biphoton, “which-polarization” information b) all Sab are equal: no entanglement between solid and photon states → trace over solid: biphoton entangled depending on tab • Choose b): no which-path labels introduced in solid • Observed visibilities can be explained by polarization dependent transmission of hole array Surface Plasmons and Entanglement • Energy-time entanglement S. Fasel, N. Gisin, H. Zbinden, D. Erni, E. Moreno, F. Robin PRL 94, 110501(2005) ψ = € 1 ( 1,0;1,0 2 AB + e iφ 0,1;0,1 AB ) → energy-time entanglement especially robust against environmental disturbance → telecom wavelength particularly interesting for quantum communication Surface Plasmons and Entanglement • Energy-time entanglement S. Fasel, N. Gisin, H. Zbinden, D. Erni, E. Moreno, F. Robin PRL 94, 110501(2005) → macroscopic cat states (surface plasmons) living at different “epochs” that differ by more than the cats (surface plasmon) lifetime Outline • What are surface plasmons: Introduction • Excitation of surface plasmons at surfaces • Entanglement and surface plasmons • Surface plasmons in quantum information implementations Surface Plasmons in Quantum Information • Proposal: Cavity QED with Surface Plasmons D. E. Chang, A. S. Sorensen, P. R. Hemmer, and M. D. Lukin quant-ph/0506117 • efficient coupling of emitter (quantum • plasmon cavity created by plasmon dot, atom) to plasmon mode of nanowire mirrors (2k|| grating on surface) with reflectivity > 0.9 • evanescent coupling of nanowire to dielectric waveguide → single photon source • field enhancement: stronger coupling and faster interaction times • one photon sources Surface Plasmons in Quantum Information • Proposal: Cavity QED with Surface Plasmons D. E. Chang, A. S. Sorensen, P. R. Hemmer, and M. D. Lukin quant-ph/0506117 → calculation of plasmons modes → efficiency of single photon generation P • fractional power emitted into fundamental plasmon mode • one photon source efficiency: 0.7 (coupling to wire), 0.9 coupling to cavity Summary Summary • Entanglement survives excitation and deexcitation of surface plasmons • Applications for hybridization of different QIP implementations • Problems: – Short Coherence time (usually < 10-12 s) – Limited spatial propagation (usually < 1 mm) References • General review: • Surface Plasmons: • Entanglement experiments – Theoretical analysis – Time-energy entanglement • Hybrid proposal J. Opt. A 5, S16-S50 (2003) H. Raether: Surface Plasmons, Springer 1988 Nature 418, 304 (2002) PRL 92, 236801(2004) PRL 94, 110501(2005) quant-ph/0506117