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Transcript
MAX-BORN-INSTITUT FÜR NICHTLINEARE OPTIK UND KURZZEITSPEKTROSKOPIE IM FVB E.V.
Institutskolloquium
Am Mittwoch, 9. Juli 2008 um 16:00 Uhr spricht
Prof. Dr. Jonathan P. Marangos
Imperial College London, Quantum Optics & Laser Science
Group (QOLS)
“Controlling and Measuring Structure with
Sub-Optical Cycle Electron Dynamics in a
Strong Field”
Abstract: It is well known that strong field processes, such as high order harmonic generation (HHG), depend
upon the sub-optical cycle dynamics of the strongly driven electrons. We will discuss some of our recent work
where the sub-optical cycle dynamics of the driven electrons are examined using both theoretical and
experimental approaches. Techniques for making sub-optical cycle temporal resolution measurements are
identified and control methods that may soon be used in practice are treated theoretically.
We will discuss the probing of proton rearrangements within laser field ionised molecules via HHG using the
chirp encoded property of the electron recollisions. The initial experimental confirmation of this technique in
H2 and CH4 are presented and discussed. New observations of transient two-centre interference in the H2
molecule are obtained via the same method. In this case the two-centre destructive interference condition is
briefly satisfied as the internuclear separation expands through the appropriate value around ~1.4fs after field
ionization; this offers a new way to directly measure extremely fast intra-molecular structural change.
Next we discuss the optimal electric field waveform for maximising the electron recollision energy. This was
found, to be a simple saw-tooth form with a DC off-set. We briefly discuss practical routes for approaching this
ideal. We also examine the control of an electron wavepacket when strong fields of different frequency and
perpendicular polarisation are employed.
Ort:
Max-Born-Saal, MBI, Max-Born-Str. 2a
Prof. Dr. W. Sandner
Direktor Bereich A
Direktor Bereich B
Direktor Bereich C
Bereich Z
Prof. Dr. Ingolf V. Hertel
Prof. Dr. Wolfgang Sandner
Prof. Dr. Thomas Elsässer
Dr. Jörn Kändler
Max-Born-Institut, Max-Born-Straße 2A, D-12489 Berlin, Tel.: 030/6392 1505, Fax: 030/6392 1519