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Validation of the FSCK Radiation Model for Oxycoal Combustion *A. G. Clements1, K. J. Hughes1, M. Pourkashanian1, M. E. de Tejada2, S. Grathwohl2, J. Maier2, G. Sheffknecht2 Energy2050, University of Sheffield, Sheffield, United Kingdom, S10 2JT Institute of Combustion and Power Plant Technology (IFK), University of Stuttgart, Pfaffenwaldring 23, 70569 Stuttgart, Germany 1 2 Abstract for oral presentation: One of the key challenges in the deployment of oxyfuel and carbon capture technologies is associated with the cost and efficiency penalty that these regimes will impose over conventional processes. Modelling can provide a means to optimise the combustion process, and appropriate use of modelling techniques will help in the design of economically feasible carbon capture technology. Thermal radiation is the most significant mode of heat transfer at combustion temperatures, however modelling the spectral variation in the radiative properties of combustion gasses is challenging. The increased concentrations of radiatively participating species under oxyfuel conditions, principally H2O and CO2, increases the role of gas-phase absorption and emission of thermal radiation. The full-spectrum correlated k (FSCK) model has been previously shown to achieve high accuracy evaluations of radiative quantities within a time-frame suitable for CFD calculations. Pilot scale facilities provide much needed validation data for modelling. This study compares CFD predictions against experimental measurements carried out at IFK’s semi industrial scale 500 kWth furnace, which was operated under air-fired and oxyfuel conditions. The down fired test furnace is fitted with a flue gas recycle line so that the oxyfuel combustion regime can be employed with a real flue gas recycle. In-flame species and temperature profiles were measured for both firing conditions, alongside radiative heat fluxes to the furnace wall. The modelling approach to radiative transfer in this study combines the FSCK model with Mie theory calculations of particle radiative properties. CFD calculations of air-fired and oxyfuel combustion within the pilot-scale furnace are compared against the measurements of radiative heat flux and in-flame temperature and species profiles. The results demonstrate improved agreement with measured values for the radiative heat flux in both air-fired and oxyfuel combustion when compared against the standard grey WSGG radiation model. Keywords: oxyfuel combustion, radiation, CFD, FSCK Acknowledgement: The research leading to these results has received funding from the European Community's Seventh Framework Programme (FP7/2007-2013) under grant agreement n° 268191. * Corresponding author: e-mail: [email protected] Tel: +44 114 21 57277