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Prom. Nr. 2100 Investigations Isotopes Ga64, Ga66, on the Odd-odd Ga68 and the Odd-even Isotope Ga67 THESIS presented to THE SWISS FEDERAL INSTITUTE OF TECHNOLOGY, ZURICH for the Degree of DOCTOR OF NATURAL SCIENCE by AMBUJ MUKERJI M. Sc. of Calcutta, India Accepted on the recommendation of Prof. Dr. P. Scherrer and Prof. Dr. W. Pauli Basle E. Birkhauser & 1952 Co., Ltd. Investigations the odd-odd on and the odd-even isotopes Ga64, Ga66, Ga68 isotope Ga67 by Ambuj Mukerji. Summary. Disintegrations of the odd-odd isotopes Ga64, Ga66 and Ga68 have investigated by spectrometer and coincidence measurements. The positron activity assigned in literature to Ga64 has to be attributed to some impurities. Disintegration schemes for Ga66 and Ga68 have been established. Spin assignments been ground to states of Ga66 and Ga68 have been Nordheim's rules regarding odd-odd compared to those predicted by nuclei. new y-radiations observed during the course of disintegration of Ga67 reported in the supplement and a disintegration scheme proposed. The findings difficult to reconcile with the predictions from shell model in its simplest form. Some are are 1. Introduction. It is well known that all the odd-odd nuclei with the of 1H2, 3Li6, 5B10 and 7N14 are unstable. grate into the corresponding stable exception They, therefore, disinte¬ even-even numbers isobars. The nuclear predicted with the spins its in shell of the nuclear model1-4) simplest form of single help nuclei the odd-odd For Nordheim5) has formul¬ particle picture. ated an empirical rule about the manner in which the odd proton and the odd neutron combine together to give the total spin of a nucleus of this type in its ground state. But till now only relatively few instances are known to verify the validity of this rule and it of the nuclei with odd seems to also, it mass can be be too premature to draw conclusions from it. Otherwise important to know more about the combinations of seems nuclei, as it is hoped that valuable informa¬ properties of bound states of nuclei may be obtained from such studies. The precise investigation of the disintegration schemes of radioactive isotopes is a good method for assigning spins of the nuclear energy levels. The work reported here is a part of a bigger programme of in¬ vestigations that is being carried out in this laboratory to study the modes of decay of odd-odd nuclei and consequently, the excited spins of the odd-odd tions about the states of the even-even nuclei.