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Quantum Optical Measurement: A Tutorial Michael G. Raymer Oregon Center for Optics, University of Oregon [email protected] I review experimental work on the measurement of the quantum state of optical fields, and the relevant theoretical background. The basic technique of optical homodyne tomography is described, with particular attention paid to the role played by balanced homodyne detection in this process. I discuss some of the original single-mode squeezedstate measurements as well as recent developments. I also discuss applications of state measurement techniques to an area of scientific and technological importance–the ultrafast sampling of time-resolved photon statistics. Quantum mechanics is a theory of information, and the state of a system is the means of describing the statistical information about that system. How can the quantum state of a physical system be completely determined by measurements? Following Leonhardt, we affirm that “knowing the state means knowing the maximally available statistical information about all physical quantities of a physical object.” Typically by “maximally available statistical information” we mean probability distributions. Hence, knowing the state of a system means knowing the probability distributions corresponding to measurements of any possible observable pertaining to that system. For multiparticle (or multimode) systems, this means knowing joint probability distributions corresponding to joint measurement of multiple particles (or modes). The state of an individual system cannot, even in principle, be measured. However, the state of an ensemble of identically prepared systems can be measured. Each member of an ensemble of systems is prepared by the same state-preparation procedure. Each member is measured only once, and then discarded. Thus, multiple measurements can be performed on systems all in the same state, without worrying about the measurement apparatus disturbing the system. A mathematical transformation is applied to the data in order to reconstruct, or infer, the state. The relevant interpretation of the measured state in this case is that it is the state of the ensemble. M.G.Raymer_TTRL2a_V2_2005 1 of 42 PART 1 : Quantum Optical Measurement Michael G. Raymer Oregon Center for Optics, University of Oregon [email protected] ----------------------------We review the measurement of optical fields, including direct detection and balanced homodyne detection. We discuss single-mode squeezed-state measurements as well as recent developments including: other field states, multimode measurements, and other new homodyne schemes. We also discuss applications of homodyne measurement techniques to an area of scientific and technological importance–the ultrafast sampling of time-resolved photon statistics. M.G.Raymer_TTRL2a_V2_2005 2 of 42 OUTLINE PART 1 1. Noise Properties of Photodetectors 2. Quantization of Light 3. Direct Photodetection and Photon Counting PART 2 4. Balanced Homodyne Detection 5. Ultrafast Photon Number Sampling PART 3 6. Quantum State Tomography M.G.Raymer_TTRL2a_V2_2005 3 of 42 REFERENCES CITED 1. RB - RW Boyd, “Radiometry and the Detection of Radiation” 2. RL - R Loudon, “The Quantum Theory of Light” 3. MW - L Mandel, E Wolf, “Optical Coherence and Quantum Optics” 4. VR - “Low Noise Techniques in Detectors,” Ann Rev Nucl Part Sci 38, 217 (1988) 5. MR - M Raymer et al, "Ultrafast measurement of opticalfield statistics by dc-balanced homodyne detection," JOSA B 12, 1801 (1995). M.G.Raymer_TTRL2a_V2_2005 4 of 42 NOISE PROPERTIES OF DETECTORS DIRECT PHOTODETECTION (MW Ch9, RB Ch8-11, RL Ch6) • PHOTOEMISSIVE DETECTORS -- Photoelectric Effect Assume no detector noise, and independent events T light current ei(t) V t mean rate = r (constant) mean current <i>= e r Number of events in time T is n. Mean <n>=n=r T Photoelectron Number Probability=Poisson M.G.Raymer_TTRL2a_V2_2005 5 of 42 NOISE PROPERTIES OF DETECTORS mean rate = r (constant) Number of events in time T is n. Mean (ensemble average) <n>=n=r T Photoelectron Number Probability=P(n) Variance of n: var(n) = <(n -<n>)2> = <n 2> -<n>2 Standard Deviation: std(n)=var(n)1/2 P(n) std(n) O <n > n M.G.Raymer_TTRL2a_V2_2005 6 of 42 Photoelectron Number Probability=Poisson T n −n n e p(n) = n! Variance: var(n) = Δn 2 = n = rT Standard Deviation: std(n) = Δn = n t Shot Noise Level (SNL) <n>=0.1 mean rate = r (constant) p(n) <n>=1 <n>=5 <n>=10 n M.G.Raymer_TTRL2a_V2_2005 7 of 42 Photoelectron Number Probability (Semiclassical Theory) If the mean rate r(t) is not constant. T Define Integrated rate: W = 1 ∫ r(t) dt (η=QE) η 0 T T t Probability for Integrated rate to equal W: P(W). Probability to count n photoelectrons in time T: p(n) = Variance: ∫ ∞ 0 (ηW ) n e−η W P(W ) dW n! var(n) = η 2 var(W ) + wave noise (Mandel’s formula) n particle noise M.G.Raymer_TTRL2a_V2_2005 8 of 42 Photoelectron Number Probability -- Example Classical Blackbody Light in Single Mode (frequency, direction) T 1 Short-time integration, T<<1/Δω W = ∫ r(t) dt (η=QE) η 0 T filter, Δω ∫ 0 I dt n T T P(W ) = < W >−1 e−W /<W > t mean number of counts: n = η W = η r T Probability to count n photoelectrons in time T: p(n) = ∫ ∞ 0 1 ⎛ n ⎞ (ηW ) n e−η W P(W ) dW = ⎜ ⎟ n + 1⎝ n + 1⎠ n! n Bose-Einstein Distribution (derived here semiclassically) M.G.Raymer_TTRL2a_V2_2005 9 of 42 Photoelectron Number Probability=Bose-Einstein 1 ⎛ n ⎞ p(n) = ⎜ ⎟ n + 1⎝ n + 1⎠ Mean: Variance: T n n =ηrT var(n) = n 2 + n t Thermal-like Noise <n>=0.1 mean rate = r (non-constant) p(n) <n>=1 <n>=5 <n>=10 n M.G.Raymer_TTRL2a_V2_2005 10 of 42 Breakdown of the Semiclassical Photodetection Theory p(n) = ∫ ∞ 0 (ηW ) n e−η W P(W ) dW n! 1 W = η Variance: var(n) = η 2 var(W ) + wave noise 0 r(t) dt (η=QE) n particle noise There exist light sources for which var(n) < T ∫ T n T t M.G.Raymer_TTRL2a_V2_2005 11 of 42 QUANTIZATION OF THE OPTICAL FIELD I ω j ˆ (+ ) ˆ E (r,t) = i ∑ b j u j (r) exp(−iω j t) 2 ε0 j monochromatic planewave modes: u j (r) = V −1/ 2 ε j exp(i k j ⋅ r) photon annilation and creation operators: commutator: † ˆ ˆ [b j , bk ]= δ j k n-photon state: (ωj > 0) polarization † bˆ j , bˆk one-photon state: † 1ω = bˆω vac † nω = (bˆω ) n vac M.G.Raymer_TTRL2a_V2_2005 12 of 42 QUANTIZATION OF THE OPTICAL FIELD II Field Uncertainty and Squeezing ω j ˆ (+ ) ˆ A single monochromatic mode: E = i b u 0 (z)exp(−iω 0 t) 2 ε0 Hermitean operators: qˆ = (bˆ + bˆ † ) / 21/2 pˆ = (bˆ − bˆ † ) / i21/2 t Eˆ (+ ) (z,t) ∝ qˆ cos(ω 0 t − k0 z) + pˆ sin(ω 0 t − k0 z) q, p = quadrature operators [qˆ, pˆ ] = i They obey: p Uncertainty relation: std(q) std( p) ≥ 1 / 2 q M.G.Raymer_TTRL2a_V2_2005 13 of 42 QUANTIZATION OF THE OPTICAL FIELD III Coherent State - ideal laser output Eˆ (+ ) (z,t) ∝ qˆ cos(ω 0 t − k0 z) + pˆ sin(ω 0 t − k0 z) quadrature operators: qˆ = (bˆ + bˆ † ) / 21/2 pˆ = (bˆ − bˆ † ) / i21/2 t p Equal Uncertainties: std(q) = std( p) = 1 / 2 std(p) std(q) q M.G.Raymer_TTRL2a_V2_2005 14 of 42 QUANTIZATION OF THE OPTICAL FIELD IV Field Uncertainty and Squeezing Eˆ (+ ) (z,t) ∝ qˆ cos(ω 0 t − k0 z) + pˆ sin(ω 0 t − k0 z) quadraturesqueezed light: qˆ = (bˆ + bˆ † ) / 21/2 pˆ = (bˆ − bˆ † ) / i21/2 t q noise reduced p noise increased p std(p) std(q) q M.G.Raymer_TTRL2a_V2_2005 15 of 42 Coherent and Squeezed States Eˆ (+ ) (z,t) ∝ qˆ cos(ω 0 t − k0 z) + pˆ sin(ω 0 t − k0 z) p p p0 std(p) p0 std(p) std(q) q0 q [ std(q) q0 ] ψ(q) = exp −(q − q0 ) / 2 − i p0 q 2 photon number probability: Poisson n n e−n p(n) = n ψ = n! q0 + ip0 2 n=α ,α= 2 q β 2 = (1 / 2)e−2 s ψ(q) = [ ] exp −(q − q0 ) / (2β 2 ) − i p0 q 2 2 photon number probability? M.G.Raymer_TTRL2a_V2_2005 16 of 42 Quadrature-Squeezed Vacuum States vacuum Eˆ (+ ) (z,t) ∝ qˆ cos(ω 0 t − k0 z) + pˆ sin(ω 0 t − k0 z) p p q ψ(q) = exp[−q 2 / 2 q β 2 = (1 / 2)e−2 s ] ψ(q) = exp[−q 2 / (2β 2 ) s=2 p(n) podd (n) = 0 ] (pair creation) peven (n) = n ψ 2 = n n ⎛ ⎞ 1 ⎛1 ⎞ ⎜⎝ n / 2 ⎟⎠ cosh(s) ⎜⎝ 2 tanh(s)⎟⎠ M.G.Raymer_TTRL2a_V2_2005 17 of 42 Two-Mode Squeezed States by Second-order Nonlinearity: Optical Parametric Amplification: pump (ωp) --> signal (ω1) + idler (ω2) coherent seed fields (amplifier, OPA) signal(ω1) signal(ω1) idler (ω2) χ(2) idler (ω2) pump (ωp) z=O z=L ∂ g ˆ ˆ ˆ† ˆ † ˆ ˆ ψ = − i H ψ , H = i (b1 b2 − b1 b2 ) ∂z 2 photon difference number ND is a constant of the motion: † † Nˆ = (nˆ − nˆ ) = (bˆ bˆ − bˆ bˆ ) D 1 2 1 [Nˆ D , Hˆ ] = 0 1 2 2 Equal numbers of photons added to signal and idler beams M.G.Raymer_TTRL2a_V2_2005 18 of 42 Difference-Number Squeezing: Classical Particle Model Case 1. Independent coherent-state fields (equal means) photon difference number n1 n2 (ω1) (ω2) N D = n1 - n2 variances add: var(ND)= var(n1)+ var(n2) =<n1>+<n2>=2<n1>=<nTOT> SHOT-NOISE LEVEL (SNL) Case 2. Coherent seeds (OPA) n1 signal(ω1) n2 idler (ω2) χ(2) pump (ωp) j1 =n1 +m j2 =n2 +m j1 j2 ND= j1 - j2= n1 - n2 (output noise = same as input noise) M.G.Raymer_TTRL2a_V2_2005 19 of 42 Difference-Number Squeezing: Classical Particle Model II Coherent seeds signal(ω1) idler (ω2) n1 n2 (OPA) j1 =n1 +m χ(2) m>> n1 , n2 j1 j2 j2 =n2 +m ND= j1 - j2= n1 - n2 (output noise = same as input noise) input: var(ND)=<n1>+<n2> = <nTOT> (input SNL) output: var(ND)=<n1>+<n2> << <jTOT> (output SNL) p(N D ) output input ND <jTOT>= <n1>+<n2> +2m Gain= <jTOT>/<nTOT> M.G.Raymer_TTRL2a_V2_2005 20 of 42 300ps, 1064nm (η=0.8) KTP M.G.Raymer_TTRL2a_V2_2005 21 of 42 p(ND), (seeds) p(ND), amplified ND ND var(ND) theory <n1>= <n2>=106 69% below SNL M.G.Raymer_TTRL2a_V2_2005 22 of 42 WIGNER DISTRIBUTION visualize state of a single mode in (q, p) phase space. Eˆ (+ ) (z,t) ∝ qˆ cos(ω 0 t − k0 z) + pˆ sin(ω 0 t − k0 z) projected distributions: Pr(q), Pr(p) p p q q Underlying Joint Distribution? M.G.Raymer_TTRL2a_V2_2005 23 of 42 WIGNER DISTRIBUTION in (q, p) phase space. p W(q,p) W(q,p) p q 1 W (q, p) = 2π Pr(q) = ∫ ∞ −∞ ∫ ∞ −∞ q ψ (q + q '/ 2) ψ * (q − q '/ 2) exp(−i q ' p) dq ' W (q, p) dp , Pr( p) = ∫ ∞ −∞ W (q, p) dq W(q,p) acts like a joint probability distribution. But it can be negative. M.G.Raymer_TTRL2a_V2_2005 24 of 42 WIGNER DISTRIBUTION for one-photon state | 1 > ψ(q) = q exp[−q / 2 2 ] p W(q,p) q negative q 2q 2 + 2 p 2 −1 W (q, p) = exp(−q 2 − p 2 ) π M.G.Raymer_TTRL2a_V2_2005 25 of 42 WIGNER DISTRIBUTION for vacuum state | O > ψvac (q) = exp[−q / 2 2 ] p Wvac(q,p) q positive q 1 W (q, p) = exp(−q 2 − p 2 ) π M.G.Raymer_TTRL2a_V2_2005 26 of 42 Impact of Losses or Detector Inefficiency on the WIGNER DISTRIBUTION convolve with a smoothing function: W after (q, p) = ∫ ∞ exp[−(q − x) 2 /ε 2 − ( p − y) 2 /ε 2 ] πε −∞ ε2 = 1 / η − 1 2 W (x, y) dx dy η = Quantum Efficiency Example: η = 0.5 --> convolve with vacuum-state Wigner distribution: W after (q, p) = ∫ ∞ −∞ exp[−(q − x) 2 − ( p − y) 2 ] π W (x, y) dx dy M.G.Raymer_TTRL2a_V2_2005 27 of 42 QUANTIZATION OF THE OPTICAL FIELD V Multimode Fields Photon-flux amplitude operator: (+ ) ˆ Φ (r,t) = i c ∑ bˆ j u j (r) exp(−iω j t) j monochromatic planewave modes: u j (r) = V −1/ 2 ε j exp(i k j ⋅ r) Photon flux through a plane at z=O: Iˆ (t) = ∫ (− ) (+) 2 ˆ (x,0,t) ⋅ Φ ˆ (x,0,t) d x Φ Det x z Integrated photon number in time T: Nˆ = ∫ T 0 Iˆ (t) dt M.G.Raymer_TTRL2a_V2_2005 28 of 42 QUANTIZATION OF THE OPTICAL FIELD VI Wave-packet Modes (+ ) ˆ Φ (r,t) = i c ∑ j change of mode basis: bˆ j u j (r) exp(−iω j t) u j (r) = V −1/ 2 ε j exp(i k j ⋅ r) (+ ) ˆ Φ (r,t) = i c ∑ aˆ k v k (r,t) k Non-mon0chromatic Wave-Packet Modes: Unitary Transformation orthogonality: v k (r,t) = ∑ Ck j u j (r) exp(−iω j t) j ∫ (temporal modes) v k * (r,t) ⋅v j (r,t) d 3 r = δ k j new annihilation operators: aˆ k = ∑ Ck* m bˆm m [aˆ j , aˆ k ] = δ j k † M.G.Raymer_TTRL2a_V2_2005 29 of 42 QUANTIZATION OF THE OPTICAL FIELD Wave-packet Modes (+ ) ˆ Φ (r,t) = i c ∑ aˆ k v k (r,t) k Non-mon0chromatic (temporal) Wave-Packet Modes: k=O: = + v 0 (r,t) = ∑ C0 j u j (r) exp(−iω j t) j + + M.G.Raymer_TTRL2a_V2_2005 30 of 42 QUANTIZATION OF THE OPTICAL FIELD VII (+ ) ˆ Φ (r,t) = i c ∑ Non-monchromatic WavePacket Modes aˆ k v k (r,t) k † aˆ k operator creates one photon in the v k (r,t) wave packet ˆak † vac = 0, 0,...1k , 0, 0... v k (r,t) z detector array one click M.G.Raymer_TTRL2a_V2_2005 31 of 42 Summary: 1. Field can be quantized in monochromatic modes (Dirac), or non-monochromatic wave packets (Glauber) 2. A single wave packet can be created in onephoton states, coherent states, or squeezed states. 3. Measurement techniques are needed that can determine the properties of these wave-packet states. next sections: A. importance of high quantum efficiency (Q.E.) and temporal selectivity B. properties of detectors C. balanced homodyne detection M.G.Raymer_TTRL2a_V2_2005 32 of 42 1. Importance of high quantum efficiency (Q.E.) and fast time response for quantum-state characterization model Q.E. as a loss, such as from a beam splitter: example: n-photon number state |n> ideal detector m counts |n> TBS= transmission loss j probability(m) = binomial distribution n! m pr(m) = TBS (1− TBS ) n−m m!(n − m)! quantum state is changed by losses, or by low Q.E. M.G.Raymer_TTRL2a_V2_2005 33 of 42 2. Importance of temporal selectivity: Multimode Fields (+ ) ˆ Φ (r,t) = i c ∑ aˆ k v k (r,t) k Non-mon0chromatic Wave-Packet Modes: = + Want to measure the light in just one of these packets. + How to select? + M.G.Raymer_TTRL2a_V2_2005 34 of 42 PROPERTIES OF DETECTORS 1. Photo-Cathodes (photomultiplier, PMT) sensitivity single photon quantum efficiency 10-20% gain noise 10-20% dark current 10-14 amp time response 10ps-10ns Good Bad Bad Good Good gain ~ 106 light e- current i(t) t V M.G.Raymer_TTRL2a_V2_2005 35 of 42 2. Avalanche Semiconductor (Silicon) Photodiode sensitivity quantum efficiency gain noise dark current time response - single photon 80% 100% large 10ps Good Good Bad Bad Fair electron-hole pair created n-type + p-type --> avalanche gain~106 current meter large reverse bias V M.G.Raymer_TTRL2a_V2_2005 36 of 42 3. Linear -Response Semiconductor (Silicon) Photodiode quantum efficiency read-out noise gain noise dark current time response - 99% 100-300 photons small 10-9 amp 10ns Excellent Bad Good Bad Bad electron-hole pair created n-type + p-type (no gain) current meter small reverse bias V M.G.Raymer_TTRL2a_V2_2005 37 of 42 Origin of Read-out Noise in Linear -Response Semiconductor (Silicon) Photodiode Integrate current for a time T =RcCf= 2 µs 1. Dark Current iD=10-9A --> mean number of counts = iDT/e std(nD)=(iDT/e)1/2 =110 counts Rc Cf V Rf Cd 2. Read-out Noise: FET A. Thermal Noise - mean counts = O std(nTh) = std( iTh)T/e ; var( iTh)=2 kB Temp/ (T Rf) std(nTh) = 80 counts (room temp) M.G.Raymer_TTRL2a_V2_2005 38 of 42 2. Read-out Noise (cont’d): B. Series resistance Noise - mean counts = O Tf= carrier transit time through FET channel = 10-8s Cd = detector capacitance = 10 pF var(nS)=(4 kB Temp/e2)(Tf/T) Cd std(nS) = 250 counts (room temp) Cf V Rc Rf Cd FET M.G.Raymer_TTRL2a_V2_2005 39 of 42 Summary: Linear -Response Silicon Photodiode var(nDARK)~ var(nTHERMAL)~ T ; var(nSERIES)~1/ T Optimum Integration Time, T ~ 1-10 µs Electronic Noise ~ 200 electrons per pulse Can detect ~ 300 photoelectrons per pulse using a linearresponse photodiode. Quantum Efficiency is high ~ 99% Example: <n> = 4 106 --> SNL = 2 103 = 10 x Electronic Noise Smithey, Beck, Belsley, M.R., Phys. Rev. Lett. 69, 2650 (1992) M.G.Raymer_TTRL2a_V2_2005 40 of 42 1. Would like to use the Linear-Response Silicon Photodiode’s high Quantum Efficiency 2. Would like to find a technique to select a single wave-packet mode 3. Would like to measure quadrature amplitudes of selected single wave-packet mode Eˆ (+ ) (z,t) ∝ qˆ cos(ω 0 t − k0 z) + pˆ sin(ω 0 t − k0 z) qˆ = ( aˆ + aˆ † ) / 21/2 pˆ = (aˆ − aˆ † ) / i21/2 M.G.Raymer_TTRL2a_V2_2005 41 of 42 end of PART 1 M.G.Raymer_TTRL2a_V2_2005 42 of 42