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Status of the polarized source at MAMI Kurt Aulenbacher, Valeri Tioukine, Markus Wiessner, Konrad Winkler Institutfur Kernphysik der Universitdt Mainz, 55118 Mainz, Germany Abstract. This talks addresses the operation of the polarized source at the Mainz Microtron MAMI. The source is operating with selected photocathodes of modulation doped, uniaxially strained layer photocathodes, which results in an average spin polarization of 80% and a quantum efficiency of typically 2fj,A/mW. The operative lifetime has been improved by employing a novel activation technique which reduces transmission losses in the vicinity of the cathode. In addition a considerable simplification of the laser system has become possible by improving the power output of laser diode seed lasers so that it is not necessary to employ power amplifier units. It was shown that the potential for increasing the laser power is limited in our setup because of the thermal resistance between cathode and the surrounding electrode. PHOTOCATHODE PROPERTIES AND LIFETIME IMPROVEMENT This talk deals with some results and observations concerning the attempt to improve the operative stability for operation with optimized polarization in our setup operating at the MAinz Microtron MAMI. The photocathode that is employed at MAMI is a 150nm thick strained layer cathode [1], with an active region that consists of uniaxially strained GaAsQ 95PQ 05. In recent years the fabrication at Joffe institute in St. Petersburg/Russia has been optimized, so that ever higher polarizations and quantum efficiencies are available for production runs at MAMI. The latest samples achieve typical quantum efficiencies (q.e.'s) of 2 jiA/mW in the maximum of the polarization spectrum. At this maximum the exciting photon energy is 1.50 eV corresponding to 826 nm wavelength. The available average polarization is about 80%. An increase of polarization is frequently observed during the quantum efficiency decay, a drop of a factor two may increase the polarization by 6% (absolute). This was also observed by Mamaev et al. with the same type of cathodes [2]. The decrease of q.e. is believed to be caused by contamination of the Cesium/Oxygen (Cs/O) activation layer and is undesirable because of the need for stable operating conditions. It has been long guessed that very small transmission losses in the vicinity of the anode of the source lead to this contamination, and that the losses are generated by photoemission from the edge area of the cathode. It is not possible to suppress edge emission by mechanical masks because of unwanted focussing effects. The attempts to create a non mechanical mask have lead to the anodization technique [3] which was successfully applied at JLAB, where the cathode is oxidized outside a small area around the main laser spot, so that the quantum efficiency is close to zero on the outer parts of the cathode. Even though we have demonstrated that this method indeed leads to reduced transmission losses and to an increased photocathode lifetime [4] CP675, Spin 2002:15th Int'l. Spin Physics Symposium and Workshop on Polarized Electron Sources and Polarimeters, edited by Y. L Makdisi, A. U. Luccio, and W. W. MacKay © 2003 American Institute of Physics 0-7354-0136-5/03/$20.00 1088 we decided to make a further modification to the process. We have applied the Cs/O evaporation through an aperture of 3 mm ('mask'). This method has the advantage that no chemical treatment of the sensitive cathodes is necessary, and that it is possible to do a comparative measurement of lifetimes with the same cathode. The mask activation suppresses all photoemission outside the 3 mm diameter activation area. Even after several weeks of observation we have not been able to detect photoemission outside this area, what indicates that the activation layer does not spread laterally on the semiconductor surface. In order to implement this technique we make use of the possibility to move the cathode holder in vacuum by manipulators, so that the cathode is activated in the mask and then removed from the mask and transferred to its operational position in the source. In figure 1 a comparison is presented, it shows the behavior of the same cathode operated at 200 Mikroamperes, once activated 'nude' and then masked. 16- yude cathode ^-catnode reactivated with mask 14- Nude cathode 12- Cs:0 Layer 10- 8- Anodized cathode Oxide layer ^^^^^^^^^^ B WW™ ^*W$^~~~----~~^__ 0 ^d^ <S^H • - 2 0 2 4 6 8 10 12 14 16 Mask activated cathode 18 extracted charge in Coulomb FIGURE 1. Right: Illustration of the Cs/O coverage of 'nude', 'anodized' and 'mask activated' photocathodes. Left: Comparison q.e.-decay during beam current production. It is evident that the decrease of q.e. is much smaller in the mask activated case. The mask activation allows therefore to extract more charge. A measure for the available charge in practical operation is given by Q = I • i where i (the 'lifetime') is defined as the time for a 1/e decrease of q.e. from its initial value. We observe a local q.e.-decrease which is restricted to the vicinity of the emission spot: The local extractable charge from one beamspot of the laser (of the area At) is restricted to Q/At = 3 • 104C/cm2 or about 20 Coulomb per beamspot. This has negligible effect on availability, since the beam spot position can be changed remotely during operation with a minimum impact on the injection parameters. For the total charge that can be extracted from the cathode (for one activation) we observe differences if operated on long time scale (moderate average current of 10-30 juA, typical for operation with strained layer cathodes) and on short time scale (test experiments with bulk GaAs cathodes of high q.e. and high average currents of 200 juA). In the first case we found Q=40 and in the second case Q>100 Coulomb. Even in the first regime it was possible to operate all experiments in the last year continuously with high polarization over their scheduled runtime. 1089 LASER STUDIES FOR 2.5 GHZ PULSED OPERATION The Master oscillator power amplifier (MOPA) system was first described with 0.5 GHz operation for accelerator injection by Poelker [5] and transferred to 2.5 GHz for our purposes later on [6]. It was considered as a mature system which allows to produce sufficient optical power at a high stability. However an unforeseen problem occurred when the vendor of the power amplifier elements stopped production in 1999, whereas the master oscillator laser diodes remain available. Our last amplifier burnt out in Spring 2002 after about 4000 hours of operation. Even though power amplifiers are available from a new manufacturer1, we found favorable circumstances to omit the power amplifier and hence to obtain a considerable simplification of the system. Presently our laser system consists out of the master oscillator laser alone. The reason for this possibility is found in the ever higher quantum efficiencies (and good lifetimes) that can be achieved with strained layer cathodes. The master oscillator is a high power single mode laser diode which is capable of producing 200 mW of average power in c.w. operation. With the typical initial efficiency of 2/j.A/mW the diode can in principle deliver enough power to drive the accelerator to the limit of its capabilities (100 jUA) and still have a considerable reserve for optical transmission losses and decreasing q.e.. Plaser>150mW BF=2,3W t/ps t/ps Double-stub tuner Master Diode 7 =o 2.5 Ghz optical power out 60 80 100 120 140 160 180 200 Average laser power / mW FIGURE 2. Upper part: Pulse distortion at high average powers. Lower left: schematic of diode r.f.drive. Lower right: transmission as a function of average output power for different r.f. power levels. The remaining problem for high power output is the requirement for 2.5 GHz pulse operation which is essential to achieve good transmission through the accelerator. The Toptica AG, Munich, Germany, model Toptica TA100 1090 typical operation consists of driving the diode with a d.c.-current and superimposing r.f.-power by a bias-t (see figure 2). Improved r.f.-coupling to the diode is achieved with the help of a double stub tuner. We found that increasing the average power of the diode resulted in severe pulse distortion and pulse lengthening (see upper part of figure 2). Consequently the accelerator transmission decreases with increasing power. However we found that this can be compensated to some extent by increasing the r.f.-power at the diode. The lower right part of figure 2 shows the dependence on the r.f. power level. We find that more than lOOmW of output power can be realized at > 90% transmission. Since the total charge from the source is limited a high transmission leads to an optimized continuous operation of the cathode. Presently all running experiments at MAMI can be supplied by this simple system. However, in order to be prepared for future eventualities (e.g. cathodes with smaller q.e.'s) we will install a MOPA system in parallel to the existing system. An additional problem that must be solved before the high power capabilities of the MOPA can be employed, is discussed in the next section. TEMPERATURE EFFECTS IN CATHODES We investigated the temperature increase that is generated by the operation at average laser powers which would be typical for operation of MAMI at the limits of its capabilities (lOOjuA). In order to do this under realistic conditions we have employed a non invasive technique. The luminescence radiation generated by the laser absorption in the semiconductor was observed and spectrally resolved (see figure 3). For a bulk-GaAs cathode - which is assumed to behave thermally identical to a strained layer cathode the position of the luminescence spectrum is related to the temperature by the Varshni equation [7]. photocathode Thermal contact between cathode and holder Pump laser luminescence radiation to spectrometer 780 800 820 840 860 880 900 920 940 Wavelength [nm] FIGURE 3. Left part: schematic situation for the laser-heating experiment, Right side: Observed spectral shift with average power The thermal conditions in this experiment where chosen in a way that they are similar to the operation in the polarized source: We used the same photocathode holder, and the 1091 holder was coupled to room temperature by a good thermal conductance. The limiting thermal resistance should therefore be the thermal contact between cathode and holder. Figure 3 shows the spectral shift that is observed when the optical power is increased. From the spectral shift we conclude that the temperature increase is about 40 degree per 100 mW. Under this circumstances it seems not appropriate to use higher average powers than 100 mW because it is believed that the lifetime of the Cs/O surface layer will be reduced drastically at temperatures higher than 50°C. From this we conclude that the operation of strained GaAs at average currents of 100 juA will possibly suffer from the increased temperature. We will therefore start work to decrease the thermal resistance of the cathode/holder interface in the near future. ACKNOWLEDGMENTS This work was supported by the Deutsche Forschungsgemeinschaft (DFG) through the SFB 443 and by the European Union through INTAS grant 9900125. Further we want to thank Dima Orlov and Uli Waigel from MPI Heidelberg for productive discussions concerning photoluminescence spectroscopy. REFERENCES 1. Drescher, P., Andresen, H. G., Aulenbacher, K., Bermuth, J., Dombo, T., Euteneuer, H., Faleev, N. N., Fischer, H., Galaktionov, M. S., v. Harrach, D., Hartmann, P., Hoffmann, J., Jennewein, P., Kaiser, K.H., Kobis, S., Kovalenkov, O. V., Kreidel, H. J., Langbein, J., Mamaev, Y. A., Nachtigall, C, Petri, M., Pliitzer, S., Reichert, E., Schemies, M., Steffens, K.-H., Steigerwald, M., Subashiev, A. V., Trautner, H., Vinokurov, D. A., Yashin, Y. P., and Yavich, B. S., Appl, Phys, A, 63, 203-206 (1996). 2. Mamaev, Y. A., Yashin, Y. P., Subashev, A. V., Ambrajei, A. N., and Rochansky, A. V., "Temperature dependence of electron spin dynamics," in Spin 2000, 14th international spin physics symposium, AIP proceedings, Vol. 570, edited by K. Hatanaka, T. Nakano, K. Imai, and H. Ejiri, AlP-publishing, Melville, New York, 2001, pp. 920-925. 3. Sinclair., C., "Performance of the Jefferson Laboratory polarized electron source at high average current," in International workshop on polarized sources and targets, (PST99), edited by A. Gute, S. Lorenz, and E. Steffens, University of Erlangen, D-91058 Erlangen, 1999, pp. 222-230. 4. Aulenbacher, K., Euteneuer, H., Jennewein, P., Kaiser, K.-H., Kreidel, H. J., v. Harrach, D., Reichert, E., Schuler, J., Tioukine, V., Wiessner, M., and Winkler, K., "New results from the Mainz polarized electron facilities," in Spin 2000,14th international spin physics symposium, AIP proceedings, Vol. 570, edited by K. Hatanaka, T. Nakano, K. Imai, and H. Ejiri, AlP-publishing, Melville, New York, 2001, pp. 949-954. 5. Poelker, M., Appl. Phys. Lett., 67, 2762-2764 (1995). 6. Aulenbacher, K., Euteneuer, H., v. Harrach, D., Hartmann, P., Hoffmann, J., Jennewein, P., Kaiser, K.-H., Kreidel, H. J., Leberig, M., Nachtigall, C., Reichert, E., Schemies, M., Schuler, J., Steigerwald, M., and Zalto, C., "High capture efficiency for the polarized beam at MAMI by r.f. synchronized photoemission," in Proceedings sixth European accelerator conference (EPAC98), edited by S. Myers, L. Lilijeby, C. Petit-Jean-Genaz, J. Poole, and K.-G. Rensfeldt, Institute of physics publishing, Bristol andPhiladalphia, 1998, pp. 1388-1390. 7. Varshni, Y. 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