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Bernard Fernandez Unravelling the Mystery of the Atomic Nucleus A Sixty Year Journey 1896— 1956 English ^ version by Springer Georges Ripka Contents 1 Radioactivity: The First Puzzles The "Uranic Rays" of Henri Becquerel The Is It 1 : 2 Discovery Really Phosphorescence? 4 5 What Is the Nature of the Radiation? A Limited Why Was Impact on 6 Scientists and the Public 7 1896? Radioactivity Discovered by 7 Chance? 9 Polonium and Radium 9 Marya Sktodowska 10 Pierre Curie Polonium and Radium: Pierre and Marie Curie Invent Radiochemistry.. 14 Enigmas 17 Emanation from Thorium 17 Ernest Rutherford Rutherford Studies /}-Rays 11 Radioactivity: a-and 18 /3-Rays 19 Are Electrons Rutherford in Montreal: The Radiation of Thorium, the Exponential "Induced" and "Excited" Elster and Geitel: The A Third 19 Decrease 20 Radioactivity Radioactivity 24 Type of Ray: y-Rays The Emanation of Thorium Is a Gas Belonging to the Argon Family Enigma, a Deeply Astonishing Subject" Puzzle Is Disentangled "An a-Rays Revisited Radioactivity Is an Atomic Decay The Energy of Radioactivity Conjecture of Rutherford 24 26 27 29 30 The Puzzle Is Unravelled: Radioactive Families Where Does the .... 25 A Proliferation of "X" Radiations The 22 of the Air and of the Earth 30 Come from? 32 xi xii Contents Experimental Radioactivity Evidence of Transmutation 35 is Understood. Radioactive Families 35 Consecrations and Mourning: The End of an Era 1903: Henri 37 Shares the Nobel Prize Becquerel with Pierre and Marie Curie 37 The Death of Pierre Curie 39 1908: Rutherford is Awarded the Nobel Prize 40 The Death of Henri 40 Becquerel References 41 A Nucleus at the Heart of the Atom 47 Prehistory of the Atom Eighteenth Century: 48 Beginning 47 The Abbot Nollet of the Nineteenth Century: Dalton, William John Prout, Gay-Lussac, Avogadro, and Ampere Do Atoms Really 50 1865: Loschmidt Estimates Spectral 49 Exist? the Size of Air Lines: A First Indication of Jean Perrin Advocates the Reality an Molecules 51 Internal Structure of Atoms of Atoms 52 1897: The Electrons Are in the Atom 55 Electric Discharges in Gases, Cathode Rays "Dynamids": The Atoms of Philipp Lenard Numeric Attempts to Describe and the Electron Balmer and Rydberg a 57 of Jean Perrin: The Atom Is Like Small Scale Solar System 57 The "Saturn" Model of Hantaro Nagaoka The "Plum-Pudding" 58 Atom of J. J. Thomson 59 Charles Barkla Measures the Number of Electrons in The Scattering of a Particles Makes It Possible to "See" a an Atom 60 Nucleus in the Atom 63 An Observation of Marie Curie 63 William The 56 Consisting Entirely of Electrons Speculation 55 55 Spectral Rays: J. J. Thomson's First Model: An Atom A 52 Henry Bragg: The Slowing "Scattering" of a-Particles Down of a-Particles in Matter 63 65 The Nature of the a-Particle: An Unresolved Question 66 The First Geiger Counter 67 The Nature of the a-Particle 69 Another Way 70 Back to the The to Count a-Particles: Scintillations Scattering of a-Particles Experiments of Geiger and 71 Marsden Are the Large Deviations Caused by 72 Multiple Small Deviations? Rutherford Invents the Nucleus A Last Ingredient: Moseley Measures the in the Atom Barkla Creates 73 74 Charge of the Nucleus 77 X-ray Spectroscopy 77 xiii Contents The Diffraction of Max X-rays: and William Lawrence Henry Moseley Measures the Laue, William Henry von 78 Bragg Charge of Nuclei 79 81 A Paradox 83 References Quantum Mechanics: The Unavoidable Branching Off An Improbable Beginning Path 89 89 91 91 The Peak of Classical Mechanics 92 A Persistent Problem 1900: Max Planck Invents the Quantum 94 of the Action A Quantum of Action 96 Einstein and Light Quanta 96 The Heat of Solids 99 Specific Solvay Council and the Theory of Quanta Bohr: The Quanta Are in the Atom Bohr Introduces Quanta in the Theory of the Atom 103 99 "On the Constitution of Atoms and Molecules" 105 The First Niels Two Other Papers in Bohr's 1913 103 108 Trilogy 109 1913-1923: Victories and Setbacks Skepticism, Enthusiasm and Adhesion Confirmation: The Experiment 110 Lines: The Zeeman and Stark Effects A Proliferation of Arnold 109 of Franck and Hertz Optical Sommerfeld: Elliptic Orbits and New Quantum Numbers 110 Ill Relativistic Corrections and the Fine Structure Constant 112 A Hoax! 113 A Further Contribution of Einstein: The Interaction 113 Between Radiation and Matter The Stark Effect: A of the Theory of 114 Quanta The "Correspondence Principle" Kossel, Bohr and the Mendeleev Table 115 The Rare Earths 118 1918, 1925: Victory Spin 1921 and 1922: Three Nobel Prizes Attributed to and the Pauli Wolfgang Principle 118 121 122 The Stern and Gerlach A Quanta 121 Pauli Max Born The 116 Compton Experiment Effect Strange Explanation of the Zeeman Effect Principle 123 124 125 Pauli's Exclusion 126 The 127 "Spin" of the Electron Quantum Mechanics Louis de Broglie Heisenberg and Matrix Mechanics 131 131 133 xiv Conlents New Physics 135 Pauli Applies the New Mechanics The Schrodinger Equation and Heisenberg to the Spectrum 136 Hydrogen 136 of the Same Coin Schrodinger, Two Sides The Probabilistic of 139 of Max Born Interpretation and the End of Determinism 139 The Pauli Matrices 141 Indistinguishable Particles: Bose-Einstein "Statistics" 141 Enrico Fermi: A New "Statistics" 143 Paul Adrien Maurice Dirac 144 "Bosons" and "Fermions" The Uncertainty Relations 147 of Heisenberg 148 Nobel Acknowledgments The Fifth The German A Brief 152 Council: An Assessment of the New Mechanics Solvay Language, Bibliography the Language of Quantum 153 Mechanics 154 155 References 157 A Timid 163 Infancy The Atomic Nucleus in 1913 163 The 165 Discovery The of Isotopes Chemistry of Frederick and the Measurement of Masses of Nuclei Radioactive Products 165 Soddy 166 Isotopes 166 The Revival of The First Positively Charged "Canal Rays" 168 Physical Measurements of Atomic Masses 168 Francis Aston and the First Mass The "Whole Number Law" and The Exceptional Mass of the Spectrometer the Old Hypothesis of William Hydrogen 169 Prout... Atom 173 A Nobel Prize for the "Whole-Number Rule" The Atomic Masses Known in 1932: The An Enquiry Full of Surprises: fi The Velocity of the fi Binding Energy Radioactivity Electrons 171 175 of Nuclei .... 176 179 180 Otto Hahn 180 Lise Meitner 182 Hahn, Meitner and fi Radioactivity The First "/? Spectrometer" 184 The Kaiser Wilhelm Institut 186 Clouds Are Gathering 186 James Chadwick: A Continuous Is It 185 fi Spectrum! 187 Continuous Spectrum? In Berlin: The War 189 Lise Meitner Returns 190 Really a The Decisive A Scandal: fi Radioactivity Experiment of Charles Ellis to Energy May Not Be Conserved! 190 191 193 xv Contents Geigerand Bothe: A "Coincidence" Experiment The Idea of Wolfgang Pauli But Why Are So Many Spectral Lines Observed? The Key to the Mystery Cavendish Professor of Physics Between Vienna and Controversy 203 Cambridge 205 How Do the Transmutations Occur? According The Nucleus in 1920 207 to Rutherford 208 The Size of the Nucleus The Constitution of the Nucleus and of Rutherford the Visionary: 208 Isotopes 209 The Neutron 210 Chadwick Hunts for New Forces The Rapid Expansion of 213 Means Experimental Scintillation Methods 213 The Point Counter 214 The Geiger-Muller 215 Counter Development Digression: The Electronically Amplified Ionization Chamber 216 Coincidence Measurements 219 The Birth and A The Measurement of the A Unique of Wireless Radio Energy 217 220 of y Radiation 222 Detector: Wilson's Cloud Chamber 227 The Atomic Nucleus in 1930 Some Certainties and One At the Beginning 228 Enigma of 1932, the 231 Enigma Remains 233 References 241 1930-1940: A Dazzling Development The Nucleus: A New Quantum 241 Boundary Mechanics Acting 242 in the Nucleus Salomon Rosenblum and the Fine Structure of a Radioactivity 1931: The First International The The 202 202 New Nuclear Reactions A 196 200 The First Nuclear Reaction Rutherford, 194 199 The First Nuclear Reactions Sir Ernest 193 Discovery Discovery of an of Nuclear Congress Exceptional Isotope: Physics Deuterium of the Neutron 244 246 249 253 Frederic and Irene Joliot-Curie 254 Protons Are Ejected 256 The Neutron Is Revealed 257 Lighter or Heavier than the Proton? Nuclear Theory After the Discovery of the Neutron Is the Neutron Werner Ettore Heisenberg Majorana Eugene P. Wigner 258 263 263 267 270 xvi Contents Do the Protons and Neutrons form Shells as Electrons Do in the Atom? 271 A New Particle: The Positron Cosmic 279 Rays 279 Blackett and Occhialini 280 Carl Anderson Discovers a Positive Electron 282 The Positive Electron of Anderson and that of Dirac 283 Irene and Frederic Joliot-Curie 286 The Birth of Particle Accelerators Direct Acceleration: A 289 High-Voltage Race 290 Acceleration in 295 Steps "Charge Independence" of the Nuclear Force The Discovery of Artificial Radioactivity The Joliot-Curies After the "A New Kind of Solvay Radioactivity" 303 305 Council 307 308 The Chemical Proof It Spreads like 309 310 Importance of the Discovery 311 The Wildfire New Perspectives for Radioactive Indicators 312 The Death of Marie Curie 313 The 1935 Nobel Prizes Are Attributed to Chadwick and the Joliot-Curies to 314 The School of Rome The Theory Neutron of 315 jS Decay Physics 316 in Rome 318 "Slow" Neutrons 321 A New Field in Nuclear Physics 323 Resonances 324 Fermi Is Awarded the Nobel Prize. The End of the Rome Team 326 The Great Exodus of Jewish Scientists Under Nazism A Proliferation of Theories: Yukawa, Breit and Wigner, 327 Bohr Hideki Yukawa 331 331 The First Theories of Nuclear Reactions The Structure of the Nucleus According 335 to Bohr in 1937 338 The Death of a Giant: Ernest Rutherford 341 Hans Bethe Sums 343 Up the Situation in 1936-1937 Hans Albrecht Bethe 343 The Structure of Nuclei 344 Nuclear Reactions 348 The Fission of Uranium 349 A Fragile Discovery: The Transuranic Elements 349 Loads of "Transuranic" Elements 352 At the Institut du Radium 354 Lise Meitner Flees Nazi Germany Otto Hahn and Fritz Strassmann Set 358 Again to Work 359 Contents xvii More and More Disconcerting Results 360 The Word Is Finally Uttered 363 The News 364 Spreads to the United States Confirmations 365 Niels Bohr: The Theory of Fission, Uranium 235 368 The Number of Emitted Neutrons 370 Leo Szilard 371 Is 372 a Chain Reaction Possible? The Last Publications Before the War 375 Francis Perrin and the Critical Mass 377 French Patents 378 References The A 381 Upheavals of the Second World War 395 Chronology 395 The New Face of Physics After the War Big Science: Physics on a Large 401 Scale 402 Team Work 402 The H-Bomb: Political and The American Military Implications 403 Supremacy and 404 After the War Europe Japan Is "Big Science" Really the 405 Result of the War? 409 References The Time of New 411 Maturity Experimental 413 Means 413 New Accelerators Have Ever New Detectors, New Increasing Energies Measuring 414 Instruments 419 Data Accumulate The 425 of Bethe Papers 425 Real Transuranic Nuclei 425 The Lifetime of the Neutron Electron 429 Scattering and the Electric Charge Distribution in Nuclei The "Shell" Structure of Nuclei 433 A Model of The Particles? Quasi-independent Symmetries and Supermultiplets Put Forth 430 Maria Arguments by Spin-Orbit Interaction of Wigner Goeppert-Mayer The 434 et Feenberg 434 435 436 Johannes Hans Daniel Jensen 437 A Paradoxical Model 438 Elastic Scattering and the The Nucleus Is Like "Optical Model" a Cloudy Crystal "Optical" Attempts The Woods-Saxon The Computer: 441 Ball 442 442 Potential 443 A Decisive Instrument 444 "Optical" Contents xviii 447 Direct Nuclear Reactions The Stripping of a 448 Deuteron Direct Reactions and Reactions Which Proceed the Formation of a Compound Though 452 Nucleus 455 A Collective Behavior Photonuclear Reactions 455 Giant Resonances 456 Are All Nuclei 457 The Spherical? Quadrupole Moment: An Indicator of Nuclear Deformation James Rainwater and Aage 458 Bohr 460 Aage Bohr, the Resolution of a Paradox 463 A Unified Model of the Nucleus 463 Ben Mottelson 464 New Data, New Confirmations Bohr and Mottelson: The The Birth of Nuclear Nuclear Key Spectroscopy to 465 Spectra 467 468 Nobel Awards 469 The Nuclear Force of the Discovery The it0 Completes the Pion n 469 Meson The 470 Trio 471 The Hard Core 473 Nuclear Matter The 473 Challenge Keith Brueckner, Jeffrey Goldstone, Hans Bethe, and And What About Niels Bohr's an a Few Others 474 475 Solid Foundations The End of 458 Original Objection? Era 476 476 References 479 Where the Narrative Ends 487 Glossary 491 Bibliography of cited books 521 Index The Periodic Law 513 or Mendeleev table 530